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Superhydrophobic melamine sponge prepared by radiation-induced grafting technology for efficient oil-water separation

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Nuclear Science and Techniques 2024年第9期35卷 103-114页

作者： Ying Sun Wen-Rui Wang Dan-Yi Li Si-Yi Xu Lin Lin Man-Li Lu Kai Fan Chen-Yang Xing Lin-Fan Li Ji-Hao Li Shanghai Institute of Applied physics Chinese Academy of SciencesShanghai 201800China University of Chinese Academy of Sciences Beijing 100049China School of Architecture and Materials Chongqing College of Electronic EngineeringChongqing 401331China Center for Stretchable electronics and NanoSensors Key Laboratory of Optoelectronic Devices and Systems of Ministry of EducationCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China

This paper presents a superhydrophobic melamine(ME)sponge(ME-g-PLMA)prepared via high-energy radiation-induced in situ covalent grafting of long-alkyl-chain dodecyl methacrylate(LMA)onto an ME sponge for efficient oil–water *** obtained ME-g-PLMA sponge had an excellent pore structure with superhydrophobic(water contact angle of 154°)and superoleophilic *** can absorb various types of oils up to 66–168 times its *** ME-g-PLMA sponge can continuously separate oil slicks in water by connecting a pump or separating oil underwater with a gravity-driven *** addition,it maintained its highly hydrophobic properties even after long-term immersion in different corrosive solutions and repeated oil *** modified ME-g-PLMA sponge exhibited excellent separation properties and potential for oil spill cleanup.

关键词： Radiation-induced graft polymerization Oil–water separation Sponge Superhydrophobic

Tunable hexagonal boron nitride topological optical delay line in the visible region

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Chinese Optics Letters 2024年第5期22卷 124-130页

作者：费宏明武敏林瀚杨毅彪肖连团 college of physics Taiyuan University of TechnologyTaiyuan 030024China college of Information engineering Shanxi Vocational University of Engineering Science and TechnologyJinzhong 030619China college of Science RMIT UniversityMelbourneVictoria 3000Australia college of Electronic Information and Optical engineering Taiyuan University of TechnologyTaiyuan 030024China

Tunability,ultracompact design,high group index,low loss,and broad bandwidth are desired properties for integrated optical delay lines(ODLs).However,those properties are challenging to achieve simultaneously in the visible *** paper proposes a tunable hexagonal boron nitride topological optical delay line(ODL)in the visible region based on valley photonic *** topological edge state from the beard-type boundary allows the achievement of an ultralow group velocity close to zero,which results in a large group index of 629 at 645 ***,we demonstrate tuning of the slow-light wavelength and optical delay times with electrically tunable liquid crystals by applying external *** device has an ultracompact size of 5μm×2.7μm with an optical delay distance of 25a(a is the lattice constant)and a delay time of 12 *** design can provide a new possibility for designing ODLs working in the visible region for optical communication and quantum computing systems.

关键词： valley photonic crystal topological edge states optical delay lines

A novel thermally-stable single-phase phosphor Ca2InTaO6:Dy3+ for NUV-excited white LEDs

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Journal of Rare Earths 2024年第10期42卷 1855-1864页

作者： Jian Hu Ruirui Cui Jun Zhang Peng Linghu Youzhen Shi Xiang Guo Key Laboratory of Micro-Nano-electronics and Software Technology of Guizhou Province College of Big Data and Information EngineeringGuizhou University college of Computer and Information engineering Guizhou University of Commerce

The work focuses on the utilization of the conventional solid-state sintering procedure to synthesize white phosphors Ca2InTaO6:xDy3+（0.02≤x≤0.12）.Utilizing X-ray diffraction,the phase structure of samples was examined,and the crystal structure was refined using the Rietveld method.A scanning electron microscope was used to analyze the microstructure of ***-principles calculations confirm that the indirect bandgap of Ca2InTaO6is 3.786 eV,The luminous properties and energy transfer mechanism of Ca2InTaO6:xDy3+were studied using photoluminescence ***4F9/2→6H13/2transition of Dy3+ions is responsible for the greatest emission peak,which was measured at 575 *** to research,the lifespan falls as the concentration of Dy3+doping amount rises because of frequent interaction and ene rgy transfer between Dy3+*** correlated color temperature of the WLEDs packaged with Ca2InTaO6:0.08Dy3+is 4677 K and CIE 1931 chromaticity coordinates are（0.3578,0.3831）.Meantime,the phosphor also shows outstanding te mperature stability property,which maintains 83.8% of its initial emission intensity at 450 K（activation energy of 0.1467 eV）.The W-LEDs retain their performance for 100 min when powered at 3.4 V voltage and 600 mA current,demonstrating the packed W-LEDs' sustaine d operation at high temperatures.

关键词： Ca2InTaO6:Dy3+ phosphors Photoluminescence Rare earths Thermal imaging Thermal stability W-LEDs

95 GeV light Higgs in the top-pair-associated diphoton channel at the LHC in the minimal dilaton model

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Chinese physics C 2024年第7期48卷 75-83页

作者：王坤朱经亚 college of Science University of Shanghai for Science and TechnologyShanghai 200093China School of physics and electronics Henan UniversityKaifeng 475004China

Motivated by experimental hints and theoretical frameworks indicating the existence of an extended Higgs sector,we explore the feasibility of detecting a 95 GeV light Higgs boson decaying into a diphoton within the minimal dilaton model at the 14 TeV ***,we identify the correlations between the production cross section,decay branching ratios,and model parameters,e.g.,the scalar mixing angle■Subsequently,we utilize Monte Carlo simulations to generate the signal of the light Higgs boson via the■process,along with the corresponding *** effectively separate the signal from the dominant backgrounds■,we employ a meticulous cut-based selection ***,we find that with an integrated luminosity of L=3000fb^(-1),the regions of■can be covered over the3σlevel.

关键词： 95 GeV light Higgs minimal dilaton model Monte Carlo simulations LHC diphoton decay channel

Thermogalvanic hydrogel-based e-skin for self-powered on-body dual-modal temperature and strain sensing

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Microsystems & Nanoengineering 2024年第2期10卷 293-302页

作者： Zhaosu Wang Ning Li Xinru Yang Zhiyi Zhang Hulin Zhang Xiaojing Cui college of Electronic Information and Optical engineering Taiyuan University of TechnologyTaiyuan030024China college of Materials Science and engineering Taiyuan University of TechnologyTaiyuan030024China School of physics and Information engineering Shanxi Normal UniversityTaiyuan030031China

Sensing of both temperature and strain is crucial for various diagnostic and therapeutic ***,we present a novel hydrogel-based electronic skin(e-skin)capable of dual-mode sensing of temperature and *** thermocouple ion selected for this study is the iodine/triiodide(I−/I3−)redox couple,which is a common component in everyday *** leveraging the thermoelectric conversion in conjunction with the inherent piezoresistive effect of a gel electrolyte,self-powered sensing is achieved by utilizing the temperature difference between the human body and the external *** composite hydrogels synthesized from polyvinyl alcohol(PVA)monomers using a simple freeze‒thaw method exhibit remarkable flexibility,extensibility,and adaptability to human *** incorporation of zwitterions further augments the resistance of the hydrogel to dehydration and low temperatures,allowing maintenance of more than 90%of its weight after 48 h in the *** its robust thermal current response,the hydrogel was encapsulated and then integrated onto various areas of the human body,including the cheeks,fingers,and ***,the detection of the head-down state and the monitoring of foot movements demonstrate the promising application of the hydrogel in supervising the neck posture of sedentary office workers and the activity *** successful demonstration of self-powered on-body temperature and strain sensing opens up new possibilities for wearable intelligent electronics and robotics.

关键词： hydrogel modal utilizing

Effective strategies to promote Z(S)-scheme photocatalytic water splitting

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Chinese Chemical Letters 2024年第3期35卷 27-39页

作者： Ye Yuan Junan Pan Weinan Yin Haoxuan Yu Fengshun Wang Weifeng Hu Longlu Wang Dafeng Yan college of Electronic and Optical engineering&college of Flexible electronics(Future Technology) Nanjing University of Posts&Telecommunications(NUPT)Nanjing 210023China college of Chemistry and Chemical engineering Hubei UniversityWuhan 430062China

Artificial Z(S)-scheme photocatalytic water splitting systems have attracted extensive attention due to their advantages such as wide light absorption range,high charge separation efficiency and strong carrier redox ***,it is still challenging to design and prepare Z(S)-scheme photocatalysts with low-cost and highly stability for efficiently photocatalytic overall water splitting using solar *** review mainly introduces various strategies to improve the photocatalytic water splitting performance of Z(S)-scheme *** strategies mainly focus on enhancing or extending the range of light absorption,promoting charge separation,and enhancing surface redox reaction in Z(S)-scheme ***,the main challenges of Z(S)-scheme photocatalytic water splitting systems and their future development directions are pointed *** review would be beneficial to understanding the challenges and opportunities faced by the research field of Z(S)-scheme photocatalytic systems,and has important guiding significance for the development and utilization of high-performance Z(S)-scheme photocatalytic reaction system in the future.

关键词： Z(S)-scheme Overall water splitting Light absorption Charge separation Loading co-catalyst

Non-adiabatic holonomic quantum operations in continuous variable systems

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Science China(physics,Mechanics & Astronomy) 2024年第6期67卷 12-19页

作者： Hao-Long Zhang Yi-Hao Kang Fan Wu Zhen-Biao Yang Shi-Biao Zheng Fujian Key Laboratory of Quantum Information and Quantum Optics College of Physics and Information EngineeringFuzhou UniversityFuzhou 350116China

Quantum operations by utilizing the underlying geometric phases produced in physical systems are favoured due to their potential *** a system in a non-degenerate eigenstate undergoes an adiabatically cyclic evolution dominated by its Hamiltonian,it will get a geometric phase,referred to as the Berry *** a non-adiabatically cyclic evolution produces an Aharonov-Anandan geometric *** two types of Abelian geometric phases are extended to the non-Abelian cases,where the phase factors become matrix-valued and the transformations associated with different loops are *** and non-Abelian(holonomic)operations are prevalent in discrete variable systems,whose limited(say,two)energy levels,form the *** their developments in continuous systems have also been investigated,mainly due to that,bosonic modes(in,such as,cat states)with large Hilbert spaces,provide potential advantages in fault-tolerant quantum *** we propose a feasible scheme to realize non-adiabatic holonomic quantum logic operations in continuous variable systems with cat *** construct arbitrary single-qubit(two-qubit)gates with the combination of single-and two-photon drivings applied to a Kerr Parametric Oscillator(KPO)(the coupled KPOs).Our scheme relaxes the requirements of the previously proposed quantum geometric operation strategies in continuous variable systems,providing an effective way for quantum control.

关键词： cat qubit continuous variable systems non-Abelian

Versatile oxidized variants derived from TMDs by various oxidation strategies and their applications

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Chinese Chemical Letters 2024年第6期35卷 14-25页

作者： Gu Gong Mengzhu Li Ning Sun Ting Zhi Yuhao He Junan Pan Yuntao Cai Longlu Wang college of Electronic and Optical engineering&college of Flexible electronics(Future Technology) Nanjing University of Posts&Telecommunications(NUPT)Nanjing 210023China

The physicochemical properties of transition metal dichalcogenides(TMDs)are highly related to their structures and usually stable in ***,under certain conditions they could be transformed into different structures due to *** this,various materials with fascinating structures have been explored by oxidation strategies,which possess novel properties and great potential in various applications such as solar batteries,hydrogen evolution reaction(HER)catalysts,and field effect transistors(FET).In this review,we systematically summarize the atomic structures of TMD oxidized variants and the corresponding fabrication *** various characterization methods,the chemical components of TMD oxidized variants are ***,we expound the promising applications of the oxidized *** review is expected to provide a new insight for preparing precise materials at the atomic level through corresponding oxidation strategies.

关键词： Transition metal dichalcogenides Oxidation strategies Oxidized variants Hydrogen evolution reaction Physicochemical properties

Radiation build-up and dissipation in Raman random fiber laser

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Science China(Information Sciences) 2024年第1期67卷 254-260页

作者： Shengtao LIN Zinan WANG Jiaojiao ZHANG Pan WANG Han WU Yifei QI Key Laboratory of Optical Fiber Sensing and Communications University of Electronic Science and Technology of China college of electronics and Information engineering Sichuan University

Raman random fiber laser(RRFL) is a complex physical system that arises from the distributed Raman amplification and the intrinsic stochasticity of fiber *** analysis of the underlying lightwave kinetics at steady state has been the focus of considerable ***,the transient state,such as the RRFL build-up and dissipation,is particularly important for revealing the lightwave interaction ***,we investigate for the first time the RRFL dynamics at the transient state and track the RRFL temporal and spectral evolution theoretically and ***,with the contribution of random distributed feedback,RRFL build-up exhibits continuous Verhulst logistic growth curves without cavity-related features,which is significantly different from the step-like growth curve of conventional fiber ***,the radiation build-up duration is inversely related to the pump power,and the spectral evolution of the RRFL undergoes two phases,i.e.,from spectral density increase to spectral *** the steady state to the pump switch-off state,the RRFL output power dissipates immediately,and the remaining Stokes lightwave from the Rayleigh scattering will gradually disappear after one round *** work provides new insights into the transient dynamic features of the RRFL.

关键词： random fiber laser stimulated Raman scattering transient phenomenon nonlinear optics łinebreak biological growth dynamics