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Dynamically enhanced Autler–Townes splitting by orthogonal XUV fields

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Chinese Physics B 2024年第7期33卷 344-350页

作者：吴立龙姜维超彭良友 Institute of Quantum Precision Measurement College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics School of PhysicsPeking UniversityBeijing 100871China

Based on numerical solutions of the time-dependent Schr ¨odinger equation, we theoretically investigate the photoelectron spectrum of hydrogen atoms ionized by a pair of ultrashort, intense, and orthogonally polarized laser pulses with a relative time delay in a pump–probe configuration. The pump pulse resonantly excites electrons from the 1s and 2p levels,inducing Rabi oscillations. The resulting dynamically enhanced Autler–Townes(AT) splitting is observed in the photoelectron energy spectrum upon interaction with the second probe pulse. In contrast to the previous parallel-polarization scheme, the proposed orthogonal-polarization configuration enables the resolution of dynamically enhanced AT splitting over a considerably wider range of probe photon energies.

关键词： Autler–Townes splitting orthogonal XUV fields photoelectron spectra Rabi frequency

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High-efficiency Brillouin lasing in a planar GeSbS spiral-ring resonator

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Chinese Optics Letters 2024年第7期22卷 71-76页

作者： Jingcui Song Yuhang Wei Chunxu Wang Shuixian Yang Yan Li Tianhua Feng Xiaojie Guo Zhaohui Li Guangdong Provincial Key Laboratory of optoelectronic Information Processing Chips and Systems and School of Electronics and Information Technology Sun Yat-sen UniversityGuangzhou 510006China Peng Cheng Laboratory Shenzhen 518000China Department of Electronic engineering College of Information Science and TechnologyJinan UniversityGuangzhou 510632China Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications Institute of Photonics TechnologyJinan UniversityGuangzhou 510632China college of Physics and optoelectronic engineering Jinan UniversityGuangzhou 510632China Southern Marine Science and engineering Guangdong Laboratory(Zhuhai) Zhuhai 519000China

Stimulated Brillouin scattering in planar integrated circuits promises to realize compact and highly coherent *** we report efficient Brillouin lasing at telecommunication wavelength from a planar Ge_(25)Sb_(10)S_(65) chalcogenide(ChG)resonator with a high quality factor above 106.A low lasing threshold of 24.8 mW is achieved with a slope efficiency of 8.3%.An 8-kHz linewidth is measured for 1.56-mW on-chip output *** work offers a good opportunity to enrich the versatility and functionality of the ChG photonics on account of their intrinsic advantages of low loss,high third-order nonlinearity,and potential capacity for wafer-scale fabrication.

关键词： Brillouin lasing chalcogenide photonics planar integrated circuit high-Q resonator

Ultracompact silicon on-chip polarization controller

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Photonics Research 2024年第2期12卷 183-193页

作者： WEIKE ZHAO YINGYING PENG MINGYU ZHU RUORAN LIU XIAOLONG HU YAOCHENG SHI DAOXIN DAI State Key Laboratory for Modern Optical Instrumentation Center for Optical&Electromagnetic ResearchCollege of Optical Science and EngineeringInternational Research Center for Advanced PhotonicsZhejiang UniversityZijingang CampusHangzhou 310058China School of Precision Instrument and optoelectronic engineering Tianjin UniversityTianjin 300072China Key Laboratory of optoelectronic Information Science and Technology Ministry of EducationTianjin 300072China Ningbo Research Institute Zhejiang UniversityNingbo 315100China

On-chip polarization controllers are extremely important for various optical *** this paper,a compact and robust silicon-based on-chip polarization controller is proposed and demonstrated by integrating a special polarization converter and phase *** special polarization converter consists of a 1×1 Mach–Zehnder interferometer with two polarization-dependent mode converters at the input/output *** light with an arbitrary state of polarization(SOP)is launched into the chip,the TE_(0)and TM_(0)modes are simultaneously *** polarization extinction ratio(PER)and the phase difference for the TE_(0)∕TM_(0)modes are tuned by controlling the first phase shifter,the polarization converter,and the second phase *** a result,one can reconstruct the light SOP at the output *** fabricated polarization controller,as compact as~150μm×700μm,exhibits an excess loss of less than 1 dB and a record PER range of>54 dB for arbitrary input light beams in the wavelength range of 1530–1620 nm.

关键词： polarization SOP interferometer

In situ protonation in a locally flexible porous coordination polymer for enhancing proton-carrier loading and proton conductivity

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Science China Chemistry 2024年第10期67卷 3432-3437页

作者： Xianzhe Wei Jincheng Liu Yan Su Weitao Wang Guixiang Wang Gen Zhang Ping Wang Cheng Gu State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSouth China University of Technology college of Polymer Science and engineering State Key Laboratory of Polymer Materials EngineeringSichuan University Key Laboratory for Soft Chemistry and Functional Materials of Ministry of Education School of Chemistry and Chemical EngineeringNanjing University of Science and Technology

Designing efficient proton-conductive materials is crucial in fuel cells. Yet, it remains a substantial challenge because of the issues in proton mobility, proton-carrier amount, and orientation of proton host materials. Herein, we report an in-situ protonation strategy to produce a locally flexible porous coordination polymer(PCP) to enhance the proton-carrier loading and proton conductivity. The local dipole flipping of the ligand allows effective proton exchange with low activation energy, promoting interpore proton transport through the pore apertures and pore walls. The protonation induces substantial charges to the frameworks and enhances the interaction with proton carriers, thereby increasing the loading of the proton carriers. By this design strategy, the resulting PCP exhibits enhanced phosphoric acid loading and extraordinary proton conductivities under both aqueous and anhydrous conditions compared to its isoreticular analog that features rigidity without proton-exchange *** work provides a new avenue for designing proton-conductive materials that combine structural dynamics with performance merits.

关键词： porous coordination polymers in-situ protonation local flexibility proton-exchange mechanism proton conduction

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Superhydrophobic melamine sponge prepared by radiation-induced grafting technology for efficient oil–water separation

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Nuclear Science and Techniques 2024年第09期 18-29页

作者： Ying Sun Wen-Rui Wang Dan-Yi Li Si-Yi Xu Lin Lin Man-Li Lu Kai Fan Chen-Yang Xing Lin-Fan Li Ji-Hao Li Shanghai Institute of Applied Physics Chinese Academy of Sciences University of Chinese Academy of Sciences School of Architecture and Materials Chongqing College of Electronic Engineering Center for Stretchable Electronics and NanoSensors Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education College of Physics and Optoelectronic Engineering Shenzhen University

This paper presents a superhydrophobic melamine(ME) sponge(ME-g-PLMA) prepared via high-energy radiation-induced in situ covalent grafting of long-alkyl-chain dodecyl methacrylate(LMA) onto an ME sponge for efficient oil–water separation. The obtained ME-g-PLMA sponge had an excellent pore structure with superhydrophobic(water contact angle of 154?)and superoleophilic properties. It can absorb various types of oils up to 66–168 times its mass. The ME-g-PLMA sponge can continuously separate oil slicks in water by connecting a pump or separating oil underwater with a gravity-driven *** addition, it maintained its highly hydrophobic properties even after long-term immersion in different corrosive solutions and repeated oil adsorption. The modified ME-g-PLMA sponge exhibited excellent separation properties and potential for oil spill cleanup.

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Progress and prospects of graphene-based materials in lithium batteries

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Rare Metals 2024年第5期43卷 1886-1905页

作者： Shen Lai Tao Huang Pei Liu Hong-Bin Wang Shi-Chun Yang Xin-Hua Liu Kai Yang Qian-Ling Zhang Jian-Hong Liu Jiang-Tao Hu Graphene Composite Research Center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060China college of Physics and optoelectronic engineering Shenzhen UniversityShenzhen 518060China Shenzhen Eigen-Equation Graphene Technology Co.Ltd Shenzhen518060China School of Transportation Science and engineering Beihang UniversityBeijing 100191China Department of Electrical and Electronic engineering Advanced Technology InstituteUniversity of SurreyGuildfordSurrey GU27XHUK

Reasonable design and applications of graphene-based materials are supposed to be promising ways to tackle many fundamental problems emerging in lithium batteries,including suppression of electrode/electrolyte side reactions,stabilization of electrode architecture,and improvement of conductive ***,extensive fundamental research on this aspect has been performed so ***,when it comes to large-scale industrial applications,the utilization of graphene-based materials progresses at a very slow ***,there presents a severe technological decoupling between academic research and industrial application,and there is an urgent need to link ***,in order to address current issues of graphene-based materials used in lithium batteries,we present their latest advancements with stateof-the-art *** applications of graphenebased materials in practical lithium batteries are highlighted and predicted to bridge the gap between the academic progress and industrial manufacture,thereby paving the way for accelerating the development of graphenebased material as well as lithium battery industry.

关键词： Lithium batteries Graphene-based materials Academic research Industrial application Development direction

Highly efficient tunable photodetector with a bipolar response in van der Waals heterojunctions

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Science China(Technological Sciences) 2024年第2期67卷 639-646页

作者： SHI ChaoFan ZHANG Shi XIAO KeNing ZHANG LiBo HAN Li ZHU YuLin TANG WeiWei LIU ChangLong LI GuanHai CHEN XiaoShuang college of Physics and optoelectronic engineering Hangzhou Institute for Advanced StudyUniversity of Chinese Academy of Sciences Hangzhou310024China State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China

The heterojunction integration of two-dimensional(2D)materials via van der Waals(vdW)forces,unencumbered by lattice and processing constraints,constitutes an efficacious approach to enhance the overall optoelectronic performance of photodetectors,due to an assortment of distinctive light-matter ***,vdW heterojunction photodetectors based on transition metal dichalcogenides(TMDs)face an inevitable trade-off between low dark currents and high responsivity,curtailing the application potential of myriad novel optoelectronic components in sensing,spectral,and communication *** this study,we present the successful actualization of a highly sensitive,self-powered,and gate-tunable bipolar response *** mechanisms underlying photocurrent generation were scrutinized via bias-,power-,and position-dependent mapping photoresponse measurements,identifying the photovoltaic effect,which is attributable to the Schottky junction’s built-in electric field,as the predominant *** prototype Au-WS2-graphene photodetector exhibits a remarkable light on/off ratio of 1.2×10^(6),a specific detectivity of 6.12×10^(11)cm H^(z1/2)W^(-1)with 20μs response time at 638 *** wide gate-tunable responsivity provides an adjustability scope,ranging from 0.9 to 3.1 A W^(-1).Notably,the device demonstrates an exceptional linear photocurrent response,with a linear dynamic range(LDR)value approximating 130 dB,which significantly surpasses that of other photodetectors based on TMDs.

关键词： WS2/graphene van der Waals heterojunction gate-tunable bipolar response

Asymmetric frequency multiplexing topological devices based on a floating edge band

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Photonics Research 2024年第6期12卷 1201-1212页

作者： JIAJUN MA CHUNMEI OUYANG YUTING YANG DONGYANG WANG HONGYI LI LI NIU YI LIU QUAN XU YANFENG LI ZHEN TIAN JIAGUANG HAN WEILI ZHANG Center for Terahertz Waves and college of Precision Instrument and optoelectronics engineering and Key Laboratory of Optoelectronics Information and TechnologyTianjin UniversityTianjin 300072China School of Materials Science and Physics China University of Mining and TechnologyXuzhou 221116China optoelectronics Research Centre University of SouthamptonSouthampton SO171BJUK Guangxi Key Laboratory of optoelectronic Information Processing School of Optoelectronic EngineeringGuilin University of Electronic TechnologyGuilin 541004China School of Electrical and Computer engineering Oklahoma State UniversityStillwaterOklahoma 74078USA

Topological photonics provides a platform for robust energy transport regardless of sharp corners and ***,the frequency multiplexing topological devices have attracted much attention due to the ability to separate optical signals by wavelength and hence the potential application in optical communication *** frequency multiplexing topological devices are generally based on the slow light ***,the resulting static local spatial mode or finely tuned flat band has zero-group velocity,making it difficult for both experimental excitation and channel ***,we propose and experimentally demonstrate an alternative prototype of asymmetric frequency multiplexing devices including a topological rainbow and frequency router based on floating topological edge mode(instead of localized ones);hence the multiple wavelength channels can be collectively excited with a point source and efficiently routed to separate output *** channel separation in our design is achieved by gradually tuning the band gap truncation on a topological edge band over a wide range of frequencies.A crucial feature lies in that the topological edge band is detached from bulk states and floating within the upper and lower photonic band *** interestingly,due to the sandwiched morphology of the edge band,the top and bottom band gaps will each truncate into transport channels that support topological propagation towards opposite directions,and the asymmetrical transportation is realized for the frequency multiplexing topological devices.

关键词： tuning floating hence

Metal-organic framework-based single-atom electro-/ photocatalysts: Synthesis, energy applications, and opportunities

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Carbon Energy 2024年第1期6卷 1-43页

作者： Munir Ahmad Jiahui Chen Jianwen Liu Yan Zhang Zhongxin Song Shahzad Afzal Waseem Raza Liaqat Zeb Andleeb Mehmood Arshad Hussain Jiujun Zhang Xian-Zhu Fu Jing-Li Luo Shenzhen Key Laboratory of Energy Electrocatalytic Materials Guangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Materials Science and EngineeringShenzhen UniversityShenzhenGuangdongChina college of Physics and optoelectronic engineering Shenzhen UniversityShenzhenGuangdongChina college of Chemistry and Environmental engineering Shenzhen UniversityShenzhenGuangdongChina Department of Environmental engineering China Jiliang UniversityHangzhouZhejiangChina Institute for Advanced Study Shenzhen UniversityShenzhenGuangdongChina School of Bioengineering Dalian University of TechnologyDalianLiaoningChina college of Materials Science and engineering Fuzhou UniversityFuzhouFujianChina Institute for Sustainable Energy Shanghai UniversityShanghaiChina

Single-atom catalysts(SACs)have gained substantial attention because of their exceptional catalytic ***,the high surface energy limits their synthesis,thus creating significant challenges for further *** the last few years,metal–organic frameworks(MOFs)have received significant consideration as ideal candidates for synthesizing SACs due to their tailorable chemistry,tunable morphologies,high porosity,and chemical/thermal *** this perspective,this review thoroughly summarizes the previously reported methods and possible future approaches for constructing MOF-based(MOF-derived-supported and MOF-supported)***,MOF-based SAC's identification techniques are briefly assessed to understand their coordination environments,local electronic structures,spatial distributions,and catalytic/electrochemical reaction *** review systematically highlights several photocatalytic and electrocatalytic applications of MOF-based SACs for energy conversion and storage,including hydrogen evolution reactions,oxygen evolution reactions,O_(2)/CO_(2)/N_(2) reduction reactions,fuel cells,and rechargeable *** light is also shed on the future development of this highly exciting field by highlighting the advantages and limitations of MOF-based SACs.

关键词： carbon energy generation MOF-derived-supported MOF-supported single atoms