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Cu nanowire array with designed interphases enabling high performance Si anode toward flexible lithium-ion battery

Nano Research 2024年第3期17卷 1516-1524页

作者： Pengfei Su Ziqi Zhang Linshan Luo Zhiyong Zhang Chaofei Lan Yahui Li Shaowen Xu Shanpeng Pei Guangyang Lin Cheng Li Xiang Han Wei Huang Songyan Chen Fujian Provincial Key Laboratory of Semiconductors and Applications Collaborative Innovation Center for Optoelectronic Semiconductors and Efficient DevicesDepartment of PhysicsXiamen UniversityXiamen 361005China College of Materials science and Engineering Nanjing Forestry UniversityNanjing 210037China science and Technology on Analog Integrated Circuit Laboratory Chongqing 400060China Shandong Electric Power Engineering Consulting Institute Co. Ltd.Jinan 250013China

To meet the growing demand for wearable smart electronic devices,the development of flexible lithium-ion batteries(LIBs)is *** is an ideal candidate for the anode material of flexible lithium-ion batteries due to its high specific capacity,low working potential,and earth *** largest challenge in developing a flexible silicon anode is how to maintain structural integrity and ensure stable electrochemical reactions during external *** this work,we propose a novel design for fabricating core–shell electrodes based on a copper nanowire(CuNW)array core and magnetron sputtered Si/C *** nanowire array structure has characteristics of bending under longitudinal stress and twisting under transverse stress,which helps to maintain the mechanical stability of the structure during electrode bending and *** low-temperature annealing generates a small amount of Cu3Si alloy,which enhances the connection strength between Si and the conductive network and solves the poor conductivity problem of Si,which is known as a semiconductor *** unique configuration design of CuNW@Si@C-400℃ leads to stable long cycle performance of 1109 mAh∙g^(-1) after 1000 cycles and excellent rate performance of 500 mAh∙g^(-1) at a current density of 10 A∙g^(-1).Furthermore,the CuNW@Si@C-400℃||LiFePO_(4)(LFP)full battery demonstrates excellent flexibility,with a capacity retention of more than 96%after 100 *** study provides a promising strategy for the development of flexible lithium-ion batteries.

关键词： flexible lithium-ion battery silicon anode magnetron sputtering core–shell electrode Cu nanowire array

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A review of ^(17)O isotopic labeling techniques for solid-state NMR structural studies of metal oxides in lithium-ion batteries

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Magnetic Resonance Letters 2024年第2期4卷 46-53页

作者： Xiaoli Xia Lei Zhu Weiping Tang Luming Peng Junchao Chen School of Chemistry and Chemical Engineering Shanghai Jiao Tong University800 Dongchuan RoadShanghai200240China Key Laboratory of Mesoscopic Chemistry of Ministry of Education and collaborative innovation center of Chemistry for Life sciences School of Chemistry and Chemical EngineeringNanjing University163 Xianlin RoadNanjing210023China State Key Laboratory of space Power-Sources Technology Shanghai Institute of Space Power-SourcesShanghai200245China

Recent advances in utilizing ^(17)O isotopic labeling methods for solid-state nuclear magnetic resonance(NMR)investigations of metal oxides for lithium-ion batteries have yielded extensive insights into their structural and dynamic ***,we commence with a brief introduction to recent research on lithium-ion battery oxide materials studied using ^(17)O solid-state NMR *** we delve into a review of ^(17)O isotopic labeling methods for tagging oxygen sites in both the bulk and surfaces of metal *** last,the unresolved problems and the future research directions for advancing the ^(17)O labeling technique are discussed.

关键词： ^(17)O solid-state NMR ^(17)O isotopic labeling methods Bulk and surfaces of metal oxides DFT calculation

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Reconciling East Asia’s mid-Holocene temperature discrepancy through vegetation-climate feedback

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science Bulletin 2024年第15期69卷 2420-2429页

作者： Jie Chen Qiong Zhang Zhengyao Lu Yanwu Duan Xianyong Cao Jianping Huang Fahu Chen Key Laboratory of Western China’s Environmental Systems(Ministry of Education) College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China Department of Physical Geography and Bolin Centre for Climate Research Stockholm UniversityStockholm 10691Sweden Department of Physical Geography and Ecosystem science Lund UniversityLund 22100Sweden Group of Alpine Paleoecology and Human Adaptation(ALPHA) State Key Laboratory of Tibetan Plateau Earth SystemEnvironment and Resources(TPESER)Institute of Tibetan Plateau Research(ITPCAS)Chinese Academy of Sciences(CAS)Beijing 100101China collaborative innovation center for Western Ecological Safety Lanzhou UniversityLanzhou 730000China

The term“Holocene temperature conundrum”refers to the inconsistencies between proxy-based reconstructions and transient model simulations,and it challenges our understanding of global temperature evolution during the *** reconstructions indicate a cooling trend following the Holocene Thermal Maximum,while model simulations indicate a consistent warming trend due to icesheet retreat and rising greenhouse gas *** factors,such as seasonal biases and overlooked feedback processes,have been proposed as potential causes for this *** this study,we examined the impact of vegetation-climate feedback on the temperature anomaly patterns in East Asia during the mid-Holocene(~6 ka).By utilizing the fully coupled earth system model EC-earth and performing simulations with and without coupled dynamic vegetation,our objective was to isolate the influence of vegetation changes on regional temperature *** findings reveal that vegetation-climate feedback contributed to warming across most of East Asia,resulting in spatially diverse temperature changes during the mid-Holocene and significantly improved model-data *** results high-light the crucial role of vegetation-climate feedback in addressing the Holocene temperature conundrum and emphasize its importance for simulating accurate climate scenarios.

关键词： Holocene temperature conundrum Holocene Thermal Maximum Vegetation-climate feedback East Asia Paleoclimate simulations

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Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou,China

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Journal of Environmental sciences 2024年第4期138卷 62-73页

作者： Lijun Yun Chunlei Cheng Suxia Yang Zaihua Wang Mei Li Qi En Zhong LiyuanMao Sulin Liu Xiaoya Cheng Duanying Chen Fan Yang Zhen Zhou Institute of Mass Spectrometry and Atmospheric Environment Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollutionJinan UniversityGuangzhou 510632China Guangdong-Hongkong-Macao Joint Laboratory of collaborative innovation for Environmental Quality Guangzhou 510632China State Key Laboratory of Loess and Quaternary Geology Institute of Earth EnvironmentChinese Academy ScienceXi’an 710061China Institute for Environment and Climate Research Jinan UniversityGuangzhou 510632China Guangdong Academy of sciences Institute of Resources Utilization and Rare Earth DevelopmentGuangzhou 510650China Environmental Monitoring Station of Pudong New District Shanghai 201200China

Organic nitrogen(ON)compounds play a significant role in the light absorption of brown carbon and the formation of organic aerosols,however,the mixing state,secondary formation processes,and influencing factors of ON compounds are still *** paper reports on the mixing state of ON-containing particles based on measurements obtained using a highperformance single particle aerosol mass spectrometer in January 2020 in *** ON-containing particles accounted for 21% of the total detected single particles,and the particle count and number fraction of the ON-containing particles were two times higher at night than during the *** prominent increase in the content of ON-containing particles with the enhancement of NO_xmainly occurred at night,and accompanied by high relative humidity and nitrate,which were associated with heterogeneous reactions between organics and gaseous NO_(x)and/or NO_(3)*** synchronous decreases in ON-containing particles and the mass absorption coefficient of water-soluble extracts at 365 nm in the afternoon may be associated with photo-bleaching of the ON species in the *** addition,the positive matrix factorization analysis found five factors dominated the formation processes of ON particles,and the nitrate factor(33%)mainly contributed to the production of ON particles at *** results of this study provide unique insights into the mixing states and secondary formation processes of the ON-containing particles.

关键词： Organic nitrogen compounds Single particles Mixing state Secondary formation Nighttime chemistry

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Synergistic Impacts of Indian Ocean SST and Indo-China Peninsula Soil Moisture on the 2020 Record-breaking Mei-yu

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Advances in Atmospheric sciences 2024年第9期41卷 1735-1750页

作者： Yinshuo DONG Haishan CHEN Xuan DONG Wenjian HUA Wenjun ZHANG Key Laboratory of Meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environment Change/Collaborative Innovation Center on Forecast and Evaluation of Meteorological DisastersNanjing University of Information Science and TechnologyNanjing 210044China School of Atmospheric sciences Nanjing University of Information Science and TechnologyNanjing 210044China Bureau of Hydrology ChangJiang Water Resources CommissionWuhan 430010China

The Yangtze River basin(YRB)experienced a record-breaking mei-yu season in June‒July *** unique long-lasting extreme event and its origin have attracted considerable *** studies have suggested that the Indian Ocean(IO)SST forcing and soil moisture anomaly over the Indochina Peninsula(ICP)were responsible for this unexpected ***,the relative contributions of IO SST and ICP soil moisture to the 2020 mei-yu rainfall event,especially their linkage with atmospheric circulation changes,remain *** using observations and numerical simulations,this study examines the synergistic impacts of IO SST and ICP soil moisture on the extreme mei-yu in *** show that the prolonged dry soil moisture led to a warmer surface over the ICP in May under strong IO SST *** intensification of the warm condition further magnified the land thermal effects,which in turn facilitated the westward extension of the western North Pacific subtropical high(WNPSH)in June‒*** intensified WNPSH amplified the water vapor convergence and ascending motion over the YRB,thereby contributing to the 2020 *** contrast,the land thermal anomalies diminish during normal IO SST backgrounds due to the limited persistence of soil *** roles of IO SST and ICP soil moisture are verified and quantified using the Community earth System *** synergistic impacts yield a notable 32%increase in YRB *** findings provide evidence for the combined influences of IO SST forcing and ICP soil moisture variability on the occurrence of the 2020 super mei-yu.

关键词： super mei-yu Indian Ocean SST soil moisture Indochina Peninsula

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Individual dynamics and local heterogeneity provide a microscopic view of the epidemic spreading

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Chinese Physics B 2024年第5期33卷 656-663页

作者：朱友源沈瑞哲董昊王炜 Kuang Yaming Honors School Nanjing UniversityNanjing 210023China collaborative innovation center of Advanced Microstructures National Laboratory of Solid State MicrostructureSchool of PhysicsNanjing UniversityNanjing 210093China Institute for Brain sciences Nanjing UniversityNanjing 210023China State Key Laboratory of Analytical Chemistry for Life science Nanjing UniversityNanjing 210023China

The COVID-19 pandemic has caused severe global disasters,highlighting the importance of understanding the details and trends of epidemic transmission in order to introduce efficient intervention *** the widely used deterministic compartmental models have qualitatively presented continuous “analytical” insight and captured some transmission features,their treatment usually lacks spatiotemporal ***,we propose a stochastic individual dynamical(SID)model to mimic the random and heterogeneous nature of epidemic *** SID model provides a unifying framework for representing the spatiotemporal variations of epidemic development by tracking the movements of each *** this model,we reproduce the infection curves for COVID-19 cases in different areas globally and find the local dynamics and heterogeneity at the individual level that affect the disease *** macroscopic trend of virus spreading is clearly illustrated from the microscopic perspective,enabling a quantitative assessment of different ***,this model is also applicable to studying stochastic processes at the “meter scale”,e.g.,human society’s collective dynamics.

关键词： Brownian motion epidemic spreading heterogeneity

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Gate Tunable Labyrinth Domain Structures in a van der Waals Itinerant Ferromagnet Cr7Te8

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Chinese Physics Letters 2024年第9期 85-91页

作者：孟奎李泽亚申艺成毕翔宇饶俊豪钱玉婷高战胜陈朋邱彩玉秦峰吴金雄罗锋黄俊伟袁洪涛 National Laboratory of Solid State Microstructures Jiangsu Key Laboratory of Artificial Functional MaterialsCollege of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced MicrostructuresNanjing University center for the Physics of Low-Dimensional Materials Henan Joint International Research Laboratory of New Energy Materials and Devices School of Physics and Electronics Henan University Tianjin Key Lab for Rare earth Materials and Applications Center for Rare Earth and Inorganic Functional Materials Smart Sensor Interdisciplinary Science Center School of Materials Science and EngineeringNankai University

Manipulating magnetic domain structure plays a key role in advanced spintronics devices. Theoretical rationale is that the labyrinthine domain structure, normally appearing in ferromagnetic thin films with strong magnetic anisotropy, shows a great potential to increase data storage density for designing magnetic nonvolatile memory and logic devices. However, an electrical control of labyrinthine domain structure remains elusive.

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Compound events of heatwave and dust storm in the Taklamakan Desert

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science China earth sciences 2024年第7期67卷 2073-2083页

作者： Yuzhi LIU Jianping HUANG Ziyuan TAN Chenglong ZHOU Dan LI Yongkun XIE Key Laboratory for Semi-Arid Climate Change of the Ministry of Education Lanzhou UniversityLanzhou 730000China collaborative innovation center for Western Ecological Safety Lanzhou UniversityLanzhou 730000China Taklamakan National Station of Observation and Research for Desert Meteorology in Xinjiang Urumqi 830002China

Taklamakan Desert(TD)has been characterized by numerous heatwaves and dust storms,leading to negative effects on societies and ecosystems at regional and global ***,the association between heatwaves and dust storms is poorly *** this study,we describe the association between heatwaves and dust events and propose a mechanism for such compound events in the *** results show that,from 1993 to 2022,the frequency and intensity of heatwaves in the TD have increased at a rate of 0.21 days year^(-1)and 0.02℃ year^(-1),*** than 40% of heatwaves existed with dust events,which significantly lagged behind ***,the higher the air temperature,the hotter and drier the soil,leading to more dust emissions in the *** high-occurrence heatwave years,a large-scale wave train of“cyclone-anticyclone-cyclone”in the northwest-southeast direction was found,with the anticyclone of which hovered over the TD *** anomalous anticyclones favored the formation and maintenance of heatwaves,and subsequent anomalous cyclones in the wave train triggered strong dust events followed by *** climate warming,the compound events of heatwave and dust storm are becoming bigger hazards threatening the socioeconomic and ecological security in the TD,the profound study of which is critical to understanding regional extreme responses.

关键词： Heatwave Dust storm Compound events Taklamakan Desert

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Imaging momentum-space Cooper pair formation and its competition with the charge density wave gap in a kagome superconductor

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science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 142-150页

作者： Yiming Sun Yubing Tu Yang Luo Shuikang Yu Hongyu Li Yunmei Zhang Ping Wu Zhuying Wang Fan Zhang Wanru Ma Zuowei Liang Jianjun Ying Tao Wu Ziji Xiang Junfeng He Lei Shan Zhenyu Wang Xianhui Chen Department of Physics CAS Key Laboratory of Strongly Coupled Quantum Matter Physicsand Hefei National LaboratoryUniversity of Science and Technology of ChinaHefei 230026China Information Materials and Intelligent Sensing Laboratory of Anhui Province Institutes of Physical Science and Information TechnologyAnhui UniversityHefei 230601China collaborative innovation center of Advanced Microstructures Nanjing 210093China

The superconducting ground state of kagome metals AV_(3)Sb_(5)(where A stands for K,Rb,or Cs)emerges from an exotic charge density wave(CDW)state that potentially breaks both rotational and time reversal ***,the specifics of the Cooper pairing mechanism,and the nature of the interplay between these two states remain elusive,largely due to the lack of momentum-space(k-space)superconducting energy gap *** implementing Bogoliubov quasiparticle interference(B QPI)imaging,we obtain k-space information on the multiband superconducting gap structureΔ_(SC)^(i)(k)in pristine CsV_(3)Sb_(5).We show that the estimated energy gap on the vanadium d_(xy/x^(2)-y^(2))orbital is anisotropic but nodeless,with a minimal value located near the M ***,a comparison ofΔ_(SC)^(i)(k)with the CDW gapΔ_(CDW)^(i)(k)obtained by angle-re solved photoemission spectro scopy(ARPES)reveals direct k-space competition between the se two order parameters,i.e.,the opening of a large(small)CDW gap at a given momentum corresponds to a small(large)superconducting *** the long-range CDW order is suppressed by replacing vanadium with titanium,we find a nearly isotropic energy gap on both the V and Sb *** information will be critical for identifying the microscopic pairing mechanism and its interplay with intertwined electro nic orders in this kagome superconductor family.

关键词： kagome lattice charge density wave superconducting energy gap scanning tunneling microscopy

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Predictability of the 7·20 extreme rainstorm in Zhengzhou in stochastic kinetic-energy backscatter ensembles

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science China earth sciences 2024年第7期67卷 2226-2241页

作者： Min YANG Peilong YU Lifeng ZHANG Xiaobing PAN Quanjia ZHONG Yunying LI College of Meteorology and Oceanography National University of Defense TechnologyChangsha 410073China Key Laboratory of High Impact Weather(Special) China Meteorological AdministrationChangsha 410073China collaborative innovation center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environment ChangeNanjing University of Information Science and TechnologyNanjing 210044China Department of Ocean science Hong Kong University of Science and TechnologyHong Kong 999077China

The scale-dependent predictability of the devastating 7·20 extreme rainstorm in Zhengzhou,China in 2021 was investigated via ensemble experiments,which were perturbed on different scales using the stochastic kinetic-energy backscatter(SKEB)scheme in the WRF model,with the innermost domain having a 3-km grid *** daily rainfall(RAIN24h)and the cloudburst during 1600-1700 LST(RAIN1h)were *** demonstrated that with larger perturbation scales,the ensemble spread for the rainfall maximum widens and rainfall forecasts become closer to the *** ensembles with mesoscale or convective-scale perturbations,RAIN1h loses predictability at scales smaller than 20 km and RAIN24h is predictable for all *** in ensembles with synoptic-scale perturbations,the largest scale of predictability loss extends to 60 km for both RAIN1h and ***,the average positional error in forecasting the heaviest rainfall for RAIN24h(RAIN1h)was 400 km(50-60)*** southerly low-level jet near Zhengzhou was assumed to be directly responsible for the forecast uncertainty of *** rapid intensification in low-level cyclonic vorticity,mid-level divergence,and upward motion concomitant with the jet dynamically facilitated the *** analysis of the divergent,rotational and vertical kinetic spectra and the corresponding error spectra showed that the error kinetic energy at smaller scales grows faster than that at larger scales and saturates more quickly in all ***-scale perturbations not only boost larger-scale error growth but are also conducive to error growth at all scales through a downscale cascade,which indicates that improving the accuracy of larger-scale flow forecast may discernibly contributes to the forecast of cloudburst intensity and position.

关键词： Stochastic kinetic-energy backscatter(SKEB) Extreme rainfall Ensemble forecast Predictability

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