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Plasmonic tandem heterojunctions enable high-efficiency charge transfer for broad spectrum photocatalytic hydrogen production

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Journal of Energy Chemistry 2025年第1期100卷 710-720页

作者： Wenxuan Chen Xiu-Qing Qiao Guo Hui Bojing Sun Dongfang Hou Meidi Wang Xueqian Wu Tao Wu Dong-Sheng Li College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials China Three Gorges University Hubei three gorges Laboratory College of Chemistry and Materials Science and Guangdong Provincial Key Laboratory of Supramolecular Coordination Chemistry Jinan University

Rational engineering of semiconductor photocatalysts for efficient hydrogen production is of great significance but still challenging,primarily due to the limitations in charge transfer ***,a fascinating plasmonic tandem heterojunction with the hc-CdS/Mo2C@C heterostructure is aimfully prepared for effectively promoting the charge separation kinetics of the CdS photocatalyst via the synergistic strategy of phase junction,Schottky junction,and photothermal *** difference in atomic configuration between cubic-CdS （c-CdS） and hexagonal-CdS （h-CdS） leads to effective charge separation through a typical Ⅱ charge transfer mechanism,and plasmonic Schottky junction further extracts the electrons in the hc-CdS phase junction to realize gradient charge ***,the photothermal effect of Mo2C@C helps to expand the light absorption,accelerate charge transfer kinetics,and reduce the hydrogen evolution energy *** carbon layer provides a fast channel for charge transfer and protects the photocatalyst from *** a result,the optimized hc-CMC photocatalyst exhibits a significantly high photocatalytic H2production activity of 28.63 mmol/g/h and apparent quantum efficiency of 61.8%,surpassing most of the reported *** study provides a feasible strategy to enhance the charge transfer kinetics and photocatalytic activity of CdS by constructing plasmonic tandem heterogeneous junctions.

关键词： Cadmium sulfide

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A Novel Model for Describing Rail Weld Irregularities and Predicting Wheel-Rail Forces Using a Machine Learning Approach

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Computer Modeling in Engineering & Sciences 2025年第1期142卷 555-577页

作者： Linlin Sun Zihui Wang Shukun Cui Ziquan Yan Weiping Hu Qingchun Meng State Key Laboratory of High-Speed Railway Track System China Academy of Railway Sciences Corporation LimitedBeijing100081China Railway Engineering Research Institute China Academy of Railway Sciences Corporation LimitedBeijing100081China School of Aeronautic Science and Engineering Beihang UniversityBeijing100191China

Rail weld irregularities are one of the primary excitation sources for vehicle-track interaction dynamics in modern high-speed *** can cause significant wheel-rail dynamic interactions,leading to wheel-rail noise,component damage,and *** researchers have employed the vehicle-track interaction dynamic model to study the dynamic interactions between wheel and rail induced by rail weld geometry ***,the cosine wave model used to simulate rail weld irregularities mainly focuses on the maximum value and neglects the geometric *** this study,novel theoretical models were developed for three categories of rail weld irregularities,based on measurements of the high-speed railway from Beijing to *** vertical dynamic forces in the time and frequency domains were compared under different running *** forces generated by the rail weld irregularities that were measured and modeled,respectively,were compared to validate the accuracy of the proposed ***,based on the numerical study,the impact force due to rail weld irrregularity is modeled using an Artificial Neural Network(ANN),and the optimum combination of parameters for this model is *** results showed that the proposed model provided a more accurate wheel/rail dynamic evaluation caused by rail weld irregularities than that established in the *** ANN model used in this paper can effectively predict the impact force due to rail weld irrregularity while reducing the computation time.

关键词： Rail weld irregularity high-speed railway vehicle-track coupled dynamics wheel/rail dynamic vertical force artificial neural networks

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In situ polymerization of poly(3,4-ethylenedioxythiophene)protective layer towards stable zinc anode

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Nano Research 2025年第1期18卷 382-394页

作者： Debin Luo Peng Zhou Xiaowei Lv Panpan Sun Xiaohua Sun Hewei Zhao College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion MaterialsChina Three Gorges UniversityYichang 443002China Hubei three gorges Laboratory Yichang 443007China School of Chemistry Beihang UniversityBeijing 100191China

Aqueous zinc-ion devices are considered promising candidates for energy storage due to their high safety,low cost and relatively high energy ***,the dendrite growth,hydrogen evolution reaction(HER)and corrosion of the zinc anode significantly limit the development of Zn-ion ***,an inexpensive poly(3,4-ethylenedioxythiophene)(PEDOT)protective layer was constructed in situ on the Zn surface using electropolymerization to suppress dendrite growth and side reactions,thereby enhancing the reversibility of *** and theoretical calculations revealed that this hydrophilic protective layer promotes the desolvation process of hydrated Zn^(2+)and facilitates the transport of zinc ions,thus improving the thermodynamic and kinetic properties of Zn^(2+)deposition and inhibiting interfacial side ***,the optimized PEDOT@Zn symmetric battery exhibited a cycling stability exceeding 1250 h at 0.5 mA·cm^(-2)and 0.25 mAh·cm^(-2),with a significantly reduced overpotential(from 91.8 to 35 mV).With the assistance of the PEDOT protective layer,the PEDOT@Zn//Cu battery maintained approximately 99.5%Coulombic efficiency after 450 ***-situ scanning electron microscopy(SEM)and in situ optical microscopy characterizations further confirmed that the PEDOT protective layer can effectively suppress the growth of zinc ***,the Zn-ion capacitors assembled by the PEDOT@Zn and activated carbon also demonstrated outstanding cycling stability.

关键词： zinc-ion devices zinc anode poly(3 4-ethylenedioxythiophene)(PEDOT) dendrite desolvation process

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Operation Risk Analysis of Electric Vehicle With Ultra-fast Charging Integrated to Distribution Network Considering the Bearing Capacity of Power System

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Dianwang Jishu/Power System Technology 2025年第1期49卷 187-197页

作者： Xu, Yanchun Li, Sijia Zhang, Tao Mi, Lu Hubei Provincial Key Laboratory for Operation and Control of Cascaded Hydropower Station China Three Gorges University Hubei Province Yichang 443002 China Department of Electrical and Computer Engineering Texas A & M University TX 77840 United States

At present, the access of distributed generation and electric vehicles with ultra-fast charging to the distribution network will increase the operational risk of the system. Aiming at the problem that the existing risk assessment indicators fail to consider the system capacity effectively, this paper proposed a comprehensive index of risk assessment of distribution networks considering the power system's capacity. The distributed generation output model and the electric vehicle load model with ultra-fast charging were first constructed. Then, the index based on the distribution entropy theory was used to measure the risk caused by the over-limit of state variables such as voltage and power and the uncertainty of their distribution. The index based on the Theil entropy theory was introduced to measure the risk caused by the equilibrium degree of the incremental distribution of state variables after the load impacted the system. The weight analysis method combining the order relationship method and the objective weighting method was used to evaluate the system risk comprehensively. Finally, the rationality of the comprehensive index was calculated and analyzed by testing the IEEE 33-node system. The results show that the comprehensive index proposed can effectively evaluate the potential risk when the system does not exceed the limit and consider that the ultra-fast charging of electric vehicles will change the time series distribution characteristics of comprehensive risk. The research in this paper can provide theoretical guidance for the safe operation of electric vehicles. with ultra-fast charging connected to the distribution network. © 2025 Power System Technology Press. All rights reserved.

关键词： Risk analysis

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Multi-powder dam concrete with high performance and low adiabatic temperature rise

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中国有色金属学会会刊：英文版 2009年第S3期19卷 727-733页

作者：李新宇陈文耀陈炜旻 Hydrochina Huadong Engineering Corporartion china three gorges Project corporation

Based on the fluidity, strength, heat of hydration and loop crack resistance experiment of multi-powder paste, the components and proportion of multi-powder were optimized and the concrete properties were studied. The multi-powder consists of limestone powder, slag, fly ash and moderate heat Portland cement (PMH cement). The results show that the compressive strength of the multi-powder paste and mortar is close to those of PMH cement, fly ash paste and mortar currently used in dam concrete, yet the flexural strength is relatively higher. The multi-powder paste is featured by larger fluidity, lower heat of hydration and delayed cracking time. In comparison, less unit water consumption and cement is used in multi-powder concrete, and under premise of equal mechanical performance, deformation, thermal performance and durability, the adiabatic temperature rise at 28 d is reduced by 2 ℃. In this way, the crack resistance is improved and it is feasible both technically and economically to produce HPC for dam concrete.

关键词： multi-powder paste dam concrete high performance concrete crack resistance adiabatic temperature rise

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Optimization design of foundation excavation for Xiluodu super-high arch dam in china

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Journal of Rock Mechanics and Geotechnical Engineering 2015年第2期7卷 120-135页

作者： Qixiang Fan Shaowu Zhou Ning Yang china three gorges corporation

With better understanding of the quality and physico-mechanical properties of rocks of dam foundation,and the physico-mechanical properties and structure design of arch dam in association with the foundation excavation of Xiluodu arch dam,the excavation optimization design was proposed for the foundation surface on the basis of feasibility *** analysis and numerical analysis results demonstrated the feasibility of using the weakly weathered rocks III1and III2as the foundation surface of super-high arch *** view of changes in the geological conditions at the dam foundation along the riverbed direction,the design of extending foundation surface excavation area and using consolidating grouting and optimizing structure of dam bottom was introduced,allowing for harmonization of the arch dam and ***-dimensional(3D)geomechanics model test and fi nite element analysis results indicated that the dam body and foundation have good overload stability and high bearing *** monitoring data showed that the behaviors of dam and foundation correspond with the designed patterns in the construction period and the initial operation period.

关键词： Super-high arch dam Foundation surface Optimization design Stability analysis

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Monitoring result analyses of high slope of five-step ship lock in the three gorges Project

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Journal of Rock Mechanics and Geotechnical Engineering 2015年第2期7卷 199-206页

作者： Qixiang Fan Hongbing Zhu Jun Gen china three gorges corporation

The construction of the double-lane five-step ship lock of the three gorges Project （TGP） wascommenced in 1994, the excavation of the ship lock was completed by the end of 1999, and the ship lockwas put in operation in June 2003. The side slopes of the ship lock are characterized by great height（170 m）, steepness （70 m in height of upright slope）, and great length （over 7000 m in total length）. Inassociation with the ship lock, the surrounding rocks in slope have a high potential to deform, withwhich the magnitude of deformation is restricted. Monitoring results show that the deformation of thefive-step ship lock high slopes of the TGP primarily occurred in excavation period, and deformationtended to be stable and convergent during operation period, suggesting the allowable ranges of *** present, the slopes and lock chambers are stable, and the ship lock works well under normaloperation condition, enabling the social and economic benefits of the TGP. 2015 Institute of Rock and Soil Mechanics, Chinese Academy of Sciences. Production and hosting byElsevier B.V. All rights reserved.

关键词： three gorges Project(TGP) Five-step ship lock Slope Monitoring analysis

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Numerical simulation of two droplets impacting upon a dynamic liquid film

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Chinese Physics B 2022年第4期31卷 562-573页

作者： Quan-Yuan Zeng Xiao-Hua Zhang Dao-Bin Ji three gorges Mathematical Research Center China Three Gorges UniversityYichang 443002China College of Science China Three Gorges UniversityYichang 443002China Engineering Research Center of Eco-environment in three gorges Reservoir Region Ministry of EducationChina Three Gorges UniversityYichang 443002China

The impact of droplets on the liquid film is widely involved in industrial and agricultural *** recent years,plenty of works are limited to dry walls or stationary liquid films,and the research of multi-droplet impact dynamic films is not *** on this,this paper employs a coupled level set and volume of fluid(CLSVOF) method to numerically simulate two-droplet impingement on a dynamic liquid *** our work,the dynamic film thickness,horizontal central distance between the droplets,droplets’ initial impact speed,and simultaneously the flow velocity of the moving film are *** evolution phenomenon and mechanism caused by the collision are analyzed in *** find that within a certain period of time,the droplet spacing does not affect the peripheral crown height;when the droplet spacing decreases or the initial impact velocity increases,the height of the peripheral crown increases at the beginning,and then,because the crown splashed under Rayleigh-Plateau instability,this results in the reduction of the crown *** the same time,it is found that when the initial impact velocity increases,the angle between the upstream peripheral jet and the dynamic film becomes *** more obvious the horizontal movement characteristics,the more restrained the crown height;the spread length increases with the increase of the dynamic film speed,droplet spacing and the initial impact *** the liquid film is thicker,more fluid enters the crown,due to the crown being unstable,the surface tension is not enough to overcome the weight of the rim at the end of the crown,resulting in droplets falling off.

关键词： two droplets moving liquid film CLSVOF mechanism analysis

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Load transfer laws of tensile anchors in rock masses with weak interlayers based on a shear-slipping updating model

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Journal of Mountain Science 2022年第3期19卷 812-825页

作者： WANG Yan XIANG Xin LI Chang-dong ZHU Guo-qiang SONG Cheng-bin XIAN Jin-ye ZHANG Jia-jun Faculty of Engineering China University of GeosciencesWuhan 430074China china three gorges corporation limited Beijing 100038China three gorges Research Center for Geo-hazards Ministry of Education China University of GeosciencesWuhan 430074China

The load transfer characteristics of a tensile anchor in the rock mass with weak interlayers were investigated,considering the nonuniform stress of the horizontally layered rock mass along *** improved shear-slipping model was proposed to describe the stress evolution characteristics of the bolt-rock *** on the improved model,analytical solutions of the axial force,shear stress distribution and load-displacement relationship considering the residual stress stage were *** effects of the stratigraphic sequence,pulling force and bolt diameter on the stress distribution of the anchorage interface were evaluated by using analytical *** results were verified by applying the finite difference numerical simulation *** sensitivity of each parameter to the axial force and shear stress of the rock bolt was determined based on calculation of the sensitivity *** study results show that the axial force and shear stress tend to decrease nonuniformly along the rock bolt towards the anchorage *** to the existence of weak interlayers,the shear stress mutates at the weak and hard rock interface,and the axial force appears to“rebound”at the bottom of the anchored *** has more significant effects on the axial force and shear stress at the bottom of the anchor than at the top of the *** pulling force is more sensitive to the anchor stress than stratigraphic sequence when the bolt diameter is *** study provides a theoretical framework for the fundamental problem of tensile bolts in horizontally or vertically laminated rock masses,providing a theoretical basis for anchor design.

关键词： Weak interlayer Tensile anchor Residual stress Shear-slipping updating model Sensitivity

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ELLIPTIC EQUATIONS IN DIVERGENCE FORM WITH DISCONTINUOUS COEFFICIENTS IN DOMAINS WITH CORNERS

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Acta Mathematica Scientia 2024年第5期44卷 1903-1915页

作者： Jun CHEN Xuemei DENG three gorges Mathematical Research Center China Three Gorges UniversityYichang443002China

We study equations in divergence form with piecewise Cα*** domains contain corners and the discontinuity surfaces are attached to the edges of the *** obtain piecewise C^(1,α) estimates across the discontinuity surf... 详细信息

关键词： elliptic equations divergence form discontinuous coefficients corner regularity

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