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Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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Journal of Energy Chemistry 2025年第1期100卷 730-738页

作者： Peng Zheng Wang Zhou Ying Mo Biao Zheng Miaomiao Han Qin Zhong Wenwen Yang Peng Gao Lezhi Yang Jilei Liu College of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean EnergyHunan Province Key Laboratory for Advanced Carbon Materials and Applied TechnologyHunan UniversityChangsha 410082HunanChina Greater Bay Area institute for innovation Hunan UniversityGuangzhou 511300GuangdongChina changsha research institute of Mining&Metallurgy Co. LTD.Changsha 410017HunanChina

Hard carbon (HC) has been considered as promising anode material for sodium-ion batteries (SIBs).The optimization of hard carbon’s microstructure and solid electrolyte interface (SEI) property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectroscopy/electrochemical impedance spectroscopy (FTIR/EIS) and X-ray photoelectron spectroscopy (XPS) analysis demonstrate the presence of more BC3and less B–C–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping content exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： Hard carbon Sodium-ion batteries Boron doping Pore structure Electrode/electrolyte interphases

Recent progress on elemental tellurium and its devices

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Journal of Semiconductors 2025年第1期46卷 91-106页

作者： Jiachi Liao Zhengxun Lai You Meng Johnny C.Ho Department of Materials Science and Engineering City University of Hong KongKowloonHong Kong 999077China changsha Semiconductor Technology and Application innovation research institute College of Semiconductors(College of IntegratedC ircuits)Hunan UniversityChangsha 410082China institute for Materials Chemistry and Engineering Kyushu UniversityFukuoka 8168580Japan State Key Laboratory of Terahertz and Millimeter Waves City University of Hong KongKowloonHong Kong 999077China

The rapid advancement of information technology has heightened interest in complementary devices and *** p-type semiconductors often lack sufficient electrical performance,thus prompting the search for new materials with high hole mobility and long-term *** tellurium(Te),featuring a one-dimensional chiral atomic structure,has emerged as a promising candidate due to its narrow bandgap,high hole mobility,and versatility in industrial applications,particularly in electronics and renewable *** review highlights recent progress in Te nanostructures and related devices,focusing on synthesis methods,including vapor deposition and hydrothermal synthesis,which produce Te nanowires,nanorods,and other *** applications in photodetectors,gas sensors,and energy harvesting devices are discussed,with a special emphasis on their role within the internet of things(IoT)framework,a rapidly growing field that is reshaping our technological *** prospects and potential applications of Te-based technologies are also highlighted.

关键词： elemental tellurium photodetector field-effect transistor gas sensor energy harvesting device

Mechanism of cryorolling and aging treatment for enhancing corrosion properties of 2195 Al−Li alloy

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Transactions of Nonferrous Metals Society of China 2025年第1期35卷 13-29页

作者： Yue XIAO Wen-shuai WANG Waqas FARID Li-hua ZHANG Charlie KONG Hai-liang YU State Key Laboratory of Precision Manufacturing for Extreme Service Performance Central South UniversityChangsha 410083China Light Alloy research institute Central South UniversityChangsha 410083China Mark Wainwright Analytical Centre University of New South WalesSydneyNSW 2052Australia

The impact of cryorolling(CR)and room temperature rolling(RTR)followed by artificial aging on the corrosion characteristics of 2195 Al−Li alloy(AA2195)was *** electron microscope,scanning electron microscope,optical microscope,intergranular corrosion experiment,and electrochemical experiment were *** different stages of aging treatment,the corrosion behavior of both CR and RTR samples exhibited a sequential progression of pitting corrosion,followed by intergranular corrosion,and then pitting corrosion *** corrosion rates of both samples initially showed an increase,followed by a gradual stabilization over *** size and density of T1 phase significantly influenced the corrosion performance of the *** the peak aging and over-aging stages,the CR sample exhibited superior corrosion resistance to the RTR sample,attributed to its finer T1 phase.

关键词： 2195 Al−Li alloy cryorolling aging treatment corrosion performance

Reduced graphene oxide-mediated electron-hole separation using titanium dioxide increases the photocatalytic antibacterial activity of bone scaffolds

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Bio-Design and Manufacturing 2025年第1期8卷 100-115,I0044页

作者： Pei Feng Haifeng Tian Feng Yang Shuping Peng Hao Pan Cijun Shuai State Key Laboratory of Precision Manufacturing for Extreme Service Performance College of Mechanical and Electrical EngineeringCentral South UniversityChangsha 410083China NHC Key Laboratory of Carcinogenesis of Hunan Cancer Hospital and the Affiliated Cancer Hospital of Xiangya School of Medicine Cancer Research InstituteSchool of Basic Medical ScienceCentral South UniversityChangsha 410013China RESEARCH ARTICLE The Key Laboratory of Carcinogenesis and Cancer Invasion of the Chinese Ministry of Education of Xiangya Hospital and School of Basic Medical Science Central South UniversityChangsha 410013China Department of Periodontics&Oral Mucosal Section Xiangya Stomatological Hospital&Xiangya School of StomatologyCentral South UniversityChangsha 410013China institute of Additive Manufacturing Jiangxi University of Science and TechnologyNanchang 330013China College of Mechanical Engineering Xinjiang UniversityUrumqi 830017China

Fast electron-hole recombination issues during titanium dioxide(TiO_(2))photocatalysis limit its application in preventing bacterial infection during bone defect *** this study,TiO_(2)@reduced graphene oxide(rGO)composites were synthesized using a hydrothermal method in which rGO,which possesses very high electrical conductivity,promotes the separation of photoelectron-hole pairs of TiO_(2),thus improving the efficiency of photocatalytic production of reactive oxygen species(ROS).Subsequently,TiO_(2)@rGO composites were introduced into poly-L-lactic acid(PLLA)to prepare bone scaffolds with photocatalytic antibacterial function via selective laser *** results showed that TiO_(2)grew on the surface of rGO and formed a covalent bond connection(Ti-O-C)with rGO.A decreased electrochemical impedance of TiO_(2)@rGO composites was observed,and the transient photocurrent intensity increased from 0.05 to 0.5μA/cm^(2).Analysis of electron spin resonance found that the photocatalytic products of TiO_(2)were·OH and·O^(2-),two kinds of ROS capable of killing bacteria via disrupting the structure of the bacterial membrane in *** experiments showed that the PLLA/TiO_(2)@rGO scaffolds had good antibacterial properties against Escherichia coli and Staphylococcus ***,we report that these scaffolds exhibited both enhanced mechanical properties due to the addition of TiO_(2)@rGO as a reinforcement material and good biocompatibility during cell proliferation.

关键词： Reduced graphene oxide Photocatalysis Reactive oxygen species Antibacterial properties Bone scaffold

Impacts of emission reduction and meteorological conditions on air quality improvement from 2016 to 2020 in the Northeast Plain,China

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Journal of Environmental Sciences 2025年第5期151卷 484-496页

作者： Xueling Yang Qiyuan Wang Lang Liu Jie Tian Hailing Xie Luyao Wang Yue Cao Steven Sai Hang Ho Key Laboratory of Aerosol Chemistry and Physics State Key Laboratory of Loess and Quaternary GeologyInstitute of Earth EnvironmentChinese Academy of SciencesXi’an 710061China Xi’an institute for Innovative Earth Environment research Xi’an 710061China National Observation and research Station of Regional Ecological Environment Change and Comprehensive Management in the Guanzhong Plain Xi’an 710061China College of Meteorology and Oceanography National University of Defense TechnologyChangsha 410073China Division of Atmospheric Sciences Desert Research InstituteRenoNV 89512USA

The Northeast Plain in China ranks among the top five regions that have been significantly impacted by haze *** effectively control pollution,it is crucial to accurately assess the effects of emission reduction *** this study,we analyzed surveillance data and found substantial decreases(ranging from 19.0%to 50.1%)in average annual mass concentrations of key pollutants(such as CO,SO_(2),NO_(2),and PM_(2.5))in the Northeast Plain from 2016 to *** precisely determine the contributions of meteorological conditions and emission reductions to the improvement of air quality in the Northeast Plain,we conducted three scenario *** comparing source emissions in December 2016 and 2020 using the WRF-Chem model(except for SO_(2)),we observed significant reductions of 21.3%,8.8%,and 9.8%in mass concentrations of PM_(2.5),NO_(2),and CO,respectively,from 2016 to *** highlights the essential role that meteorological conditions play in determining air quality in the Northeast ***,further reducing source emissions by 30%in December 2016 resulted in subsequent reductions of 25.3%,29.0%,4.5%,and 30.3%in mass concentrations of PM_(2.5),SO_(2),NO_(2),and CO,respectively,under the same meteorological ***,source emission reduction was effective for PM_(2.5),SO_(2),and CO,but not for NO_(2).The improvement in air quality in the Northeast Plain from 2016 to 2020 can be attributed to the combined effects of improved meteorological conditions and reduced pollution sources.

关键词： Air quality Emission reduction Meteorological conditions The Northeast Plain WRF-Chem

Thermal stress concentration points and stress mutations in nano-multilayer film structures

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Communications in Theoretical Physics 2025年第1期77卷 179-189页

作者： Ying Zheng Zhi You Wang Qianju Song Zao Yi Shubo Cheng Can Ma Chaojun Tang Qingdong Zeng Sohail Ahmad School of Mathematics and Science Joint Laboratory for Extreme Conditions Matter PropertiesThe State Key Laboratory of Environment-friendly Energy MaterialsTianfu Institute of Research and InnovationSouthwest University of Science and TechnologyMianyang 621010China School of Electronic Information and Electric Engineering Changsha UniversityChangsha 410022China School of Physics and Optoelectronic Engineering Yangtze UniversityJingzhouHubei 434023China School of Chemistry and Chemical Engineering Jishou UniversityJishou 416000China Department of Oncology Sichuan Science City HospitalMianyangSichuan Province 621000China College of Science Zhejiang University of TechnologyHangzhou 310023China School of Physics and Electronic-information Engineering Hubei Engineering UniversityXiaogan 432000China institute of Physics Bahauddin Zakariya UniversityMultan66000Pakistan

In the multilayer film-substrate system,thermal stress concentration and stress mutations cause film buckling,delamination and cracking,leading to device *** this paper,we investigated a multilayer film system composed of a substrate and three film *** thermal stress distribution inside the structure was calculated by the finite element method,revealing significant thermal stress differences between the *** is mainly due to the mismatch of the coefficient of thermal expansion between *** materials respond differently to changes in external temperature,leading to compression between *** are obvious thermal stress concentration points at the corners of the base layer and the transition layer,which is due to the sudden change of the shape at the geometric section of the structure,resulting in a sudden increase in local *** address this issue,we chamfered the substrate and added an intermediate layer between the substrate and the transition layer to assess whether these modifications could reduce or eliminate the thermal stress concentration points and extend the service life of the multilayer *** results indicate that chamfering and adding the intermediate layer effectively reduce stress discontinuities and mitigate thermal stress concentration points,thereby improving interlayer bonding strength.

关键词： multilayer structure thermal stress concentration point stress mutation chamfer intermediate layer

Direct Photolithography of WO_(x) Nanoparticles for High‑Resolution Non‑Emissive Displays

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Nano-Micro Letters 2025年第3期17卷 297-309页

作者： Chang Gu Guojian Yang Wenxuan Wang Aiyan Shi Wenjuan Fang Lei Qian Xiaofei Hu Ting Zhang Chaoyu Xiang Yu‑Mo Zhang Laboratory of Optoelectronic Information Technology and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China Hangzhou Bay Laboratory of Advanced Nano‑Optoelectronic Materials and Devices Qianwan Institute of CNITECHNingbo 315336People’s Republic of China Smart Materials for Architecture research Lab Innovation Center of Yangtze River DeltaZhejiang UniversityJiaxing 314100People’s Republic of China university of Science and Technology of China Hefei 230026People’s Republic of China State Key Lab of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun 130012People’s Republic of China

High-resolution non-emissive displays based on electrochromic tungsten oxides(WOx)are crucial for future near-eye virtual/augmented reality interactions,given their impressive attributes such as high environmental stability,ideal outdoor readability,and low energy ***,the limited intrinsic structure of inorganic materials has presented a significant challenge in achieving precise patterning/pixelation at the micron ***,we successfully developed the direct photolithography for WOx nanoparticles based on in situ photo-induced ligand *** strategy enabled us to achieve ultra-high resolution efficiently(line width3600 cycles),as well as promising applications in electronic logos,pixelated displays,flexible electronics,*** success and advancements presented here are expected to inspire and accelerate research and development(R&D)in high-resolution non-emissive displays and other ultra-fine micro-electronics.

关键词： Electrochromic Direct photolithography WOx nanoparticles In situ photo-induced ligand exchange High-resolution displays

Effects of Lignite Humic Acid and Lignite Humic Acid-based Combined Amendment on Soil Quality in Saline-sodic Farmlands in the West Liaohe Plain, China

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Chinese Geographical Science 2025年第2期 401-414页

作者： NIE Zhaoyang ZHANG Lu ZHANG Tieyi GUO Liangliang ZHOU Jie AN Fenghua MA Hongyuan WANG Zhichun YANG Fan Northeast institute of Geography and Agroecology Chinese Academy of Sciences university of Chinese Academy of Sciences jilin Agricultural university

Water scarcity and soil salinization pose significant challenges to agriculture in the West Liaohe Plain, eastern Inner Mongolia, China. Shallow-buried drip irrigation can improve soil water use efficiency to alleviate water shortage in agriculture and the application of lignite humic acid reduces the adverse effects of soil salinization. However, further research is needed to investigate the effects of different application rates of lignite humic acid and humic acid-based combined amendment on soil physicochemical properties, nutrient contents, and crop yield in saline-sodic farmlands under shallow-buried drip irrigation. A two-year field experiment was conducted with control without any amendment(CK), three treatments amended with 3 t/ha(H1), 6 t/ha(H2), and 12 t/ha(H3) lignite humic acid,and three application rates with 15 t/ha(T1), 22.5 t/ha(T2), and 30 t/ha(T3) lignite humic acid-based combined amendment in 2021 and2022. The results showed that H3 reduced soil bulk density, p H, electrical conductivity, and total alkalinity, while increasing the contents of soil organic matter, total nitrogen, and available potassium in the two-year experiment. Moreover, the maize yield in H3 increased by an average of 35.5%. T2 decreased soil bulk density, p H, total alkalinity, and increased maize yield by 16.2%, compared to the first year. These results suggest that T2 consistently improved both soil quality and crop yield. Correlation analyses showed that lignite humic acid and its complexes promote maize growth and increase yield by increasing soil organic matter and total nitrogen while reducing soil salinity and total alkalinity. Based on the comprehensive analysis of the field data and the results of the comprehensive evaluation of soil quality, it was determined that the appropriate improvement measures for saline-sodic farmlands under shallow-buried drip irrigation are the application of 12 t/ha of lignite humic acid and 22.5 t/ha of lignite humic acid-based combined

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A robust multi-VSGs coordinated control strategy for distributed secondary frequency regulation in islanded microgrids

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Science China Technological Sciences 2025年第3期68卷 335-352页

作者： Jing ZHANG Yong LI Jinjie LIN Sijia HU Yijia CAO Fang LIU Mingmin ZHANG Li HE College of Electrical and Information Engineering Hunan University Greater Bay Area institute for innovation Hunan University College of Information Science and Engineering Central South University College of Electronic Information and Electrical Engineering Changsha University College of Information and Electrical Engineering Hunan University of Science and Technology

Islanded microgrids(IMGs) offer a viable and efficient energy self-sustaining solution for distributed resources in remote areas. While without utility grid support, the frequency of IMG is susceptible to mismatches between demand and generation. Moreover, IMGs encounter uncertain and nonlinear load disturbances together with system parameter perturbation,which further compromises frequency stability. To this aim, this paper proposes a robust multi-virtual synchronous generators(multi-VSGs) coordinated control strategy for distributed secondary frequency regulation(DSFR) in IMGs, which exhibits minimal model dependency and avoids reliance on global information. Two critical methods are developed:(1) a robust VSG control framework that incorporates the linear active disturbance rejection control(LADRC) technique, which enables the estimation and effective elimination of uncertain load disturbances and system's parameter perturbations;(2) a novel secondorder consensus algorithm-based control law for robust secondary frequency regulation, which is featured with proper power sharing among different participants, suppressed power oscillation caused by response disparities, and reduced reliance on complex communication system. Building on methods(1) and(2), a novel multi-VSGs coordinated control strategy is proposed, providing a robust solution for IMG's frequency restoration, and its dynamic characteristics are explored in detail. The correctness and effectiveness of the proposal are verified by both simulation and the hardware-in-the-loop(HIL) experiment results across typical scenarios.

关键词： islanded microgrid (IMG) distributed secondary frequency regulation (DSFR) robust multi-VSGs coordinated control linear active disturbance rejection control (LADRC)