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China Foundry 2024年第1期21卷 11-19页

作者： Wen-ning Liu Wei Zhang Peng-yue Wang Yi-xian Liu Xiang-yi Jiao Ao-xiang Wan Cheng-gang Wang Guo-dong Tong Shou-mei Xiong School of Materials Science and Engineering Tsinghua UniversityBeijing 100084China Key Laboratory for Advanced Materials Processing technology Tsinghua UniversityBeijing 100084Beijing China FAW Group co. Ltd.Changchun 130013China China FAW Foundry co. Ltd.Changchun 130013China

The effect of slow shot speed on externally solidified crystal(ESC),porosity and tensile property in a newly developed high-pressure die-cast Al-Si alloy was investigated by optical microsco.y(OM),scanning electron microsco.y(SEM)and laboratory co.puted tomography(CT).Results showed that the newly developed AlSi9MnMoV alloy exhibited improved mechanical properties when co.pared to the AlSi10MnMg *** AlSi9MnMoV alloy,which was designed with trace multico.ponent additions,displays a notable grain refining effect in co.parison to the AlSi10MnMg *** elements Ti,Zr,V,Nb,B promote heterogeneous nucleation and reduce the grain size of primaryα-*** a lower slow shot speed,the large ESCs are easier to form and gather,developing into the dendrite net and *** an increase in slow shot speed,the size and number of ESCs and porosities significantly *** addition,the distribution of ESCs is more dispersed and the net-shrinkage *** tensile property is greatly improved by adopting a higher slow shot *** ultimate tensile strength is enhanced from 260.31 MPa to 290.31 MPa(increased by 11.52%),and the elongation is enhanced from 3.72%to 6.34%(increased by 70.52%).

关键词： hypoeutectic Al-Si alloy high pressure die casting porosity externally solidified crystal tensile property

Multidimensional regulation of Ti-Zr-Cr-Mn hydrogen storage alloys via Y partial substitution

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Nano Research 2024年第5期17卷 4211-4220页

作者： Haixiang Xiu Wanqiang Liu Dongming Yin Nan Ding Wenfeng Qiao Shaolei Zhao Long Liang co.g Liu Shaohua Wang Qingshuang Wang Bingbing Chen Limin Wang Yong Cheng School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resources Utilization Changchun Institute of Applied ChemistryChinese Academy of Sciences(CAS)Changchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China Department of Energy Science and Engineering Nanjing Tech UniversityNanjing 211816China National Engineering Research Center of Nonferrous Metals Materials and Products for New Energy GRINM Group Co.Ltd.Beijing 100088China GRIMAT Engineering Institute co. Ltd.Beijing 101407China co.lege of Life Science and technology Changchun University of Science and TechnologyChangchun 130022China

High density and safe storage of hydrogen are the preco.ditions for the large-scale application of hydrogen ***,the hydrogen storage properties of Ti_(0.6)Zr_(0.4)Cr_(0.6)Mn_(1.4) alloys are systematically studied by introducing Y element instead of Ti element through vacuum arc *** the partial substitution of Y,a seco.d phase of rare earth oxide is added in addition to the main suction hydrogen phase,C14 Laves *** to the unique properties of rare earth elements,the partial substitution of Y can not only improve the activation properties and plateau pressure of the alloys,but also increase the effective hydrogen storage capacity of the *** co.prehensive properties of hydrogen storage alloys are improved by multidimensional regulation of rare earth *** them,Ti_(0.552)Y_(0.048)Zr_(0.4)Cr_(0.6)Mn_(1.4) has the best co.prehensive *** alloy can absorb hydrogen without activation at room temperature and 5 MPa,with a maximum hydrogen storage capacity of 1.98 wt.%.At the same time,it reduces the stability of the hydride and the enthalpy change value,making it easier to release *** theoretical analysis and first-principle simulation,the results show that the substitution of Y element reduces the migration energy barrier of hydrogen and the structural stability of the system,which is co.ducive to hydrogen *** alloy has superior durability co.pared to the original alloy,and the capacity retention rate was 96.79%after 100 hydrogen absorption/desorption cycles.

关键词： AB_(2)-type hydrogen storage alloy rare earth element first-principles simulation multidimensional regulation

Exploring the Interplay between Local Chain Structure and Stress Distribution in Polymer Networks

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Chinese Journal of Polymer Science 2024年第6期42卷 874-885页

作者： Jin-Tong Xue Yang Bai Li Peng Xian-Bo Huang Zhao-Yan Sun School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei230026China State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun130022China National-certified Enterprise technology Center Kingfa Science and Technology Co.Ltd.Guangzhou510663China

The mechanical behavior of polymer networks is intrinsically co.related with the local chain topology and chain *** this study,we delve into this relationship through the lens of co.rse-grained molecular dynamics(CG-MD)*** aim is to illuminate the intricate interplay between local topology and stress distribution within polymer monomers,cross-linkers,and various co.ponents with distinct cross-link co.nections,thereby elucidating their co.lective impact on the mechanical properties of polymer *** mainly focus on how specific local structures co.tribute to the overall mechanical response of the *** particular,we employ local stress analysis to unravel the mechanics of these *** findings reveal the diverse responses of individual co.ponents,such as junctions,strands,cross-linkers between junctions,and dangling chain ends,when subjected to ***,we observe that these co.ponents exhibit varying degrees of deformation tolerance,undersco.ing the significance of their roles in determining the mechanical characteristics of the *** investigations highlight junctions as primary co.tributors to stress accumulation,and particles with higher local stress showing a stronger co.relation between stress and Voronoi ***,our results indicate that both strands and cross-linkers between junctions exhibit heightened stress levels as strand lengths *** study enhances our understanding of the multifaceted factors governing the mechanical attributes of cross-linked polymer systems at the microstructural level.

关键词： Local chain structure Local stress Molecular dynamics simulation

High-pressure study on calcium azide(Ca(N_(3))_(2)):Bending of azide ions stabilizes the structure

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Chinese Physics B 2024年第5期33卷 542-548页

作者：武晓鑫王颖健李思琪吕俊呈王婧姝杨丽华张旗刘艳清张俊凯贾洪声 Key Laboratory of Functional Materials Physics and Chemistry (Ministry of Education) College of PhysicsJilin Normal UniversityChangchun 130103China The Joint Laboratory of MXene Materials Jilin Normal University & Jilin 11 Technology Co.Ltd.Changchun 130103China

The high-pressure structure and elastic properties of calcium azide(Ca(N_(3))_(2))were investigated using in-situ highpressure x-ray diffraction and Raman scattering up to 54 GPa and 19 GPa,*** co.pressibility of Ca(N_(3))_(2)changed as the pressure increased,and no phase transition occurred within the pressure from ambient pressure up to 54 *** measured zero-pressure bulk modulus of Ca(N_(3))_(2)is higher than that of other alkali metal azides,due to differences in the ionic character of their metal-azide *** CASTEP,all vibration modes of Ca(N_(3))_(2)were accurately identified in the vibrational spectrum at ambient *** the high-pressure vibration study,several external modes(ext.)and internal bending modes(ν_(2))of azide anions(N_(3)^(-))softened up to~7 GPa and then hardened beyond that *** evidence is co.sistent with the variation observed in the F_(E)–f_(E)data analyzed from the XRD result,where the slope of the curve changes at 7.1 *** main behaviors under pressure are the alternating co.pression,rotation,and bending of N_(3)^(-)*** bending behavior makes the structure of Ca(N_(3))_(2)more stable under pressure.

关键词： high pressure calcium azide azide anions

Role of texture before rolling: a research based on texture and magnetic properties of 4.5 wt.% Si non-oriented electrical steel

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Journal of Iron and Steel Research International 2024年第8期31卷 1973-1986页

作者： Yu-fan Wang Guo-qing Zu Shi-cheng Sun Ying Han Wei-wei Zhu Hui Wu Yu Zhao Xu Ran Key Laboratory of Advanced Structural Materials of Ministry of Education Changchun University of TechnologyChangchun 130012JilinChina CRRC changchun Railway Vehicles co. Ltd.Changchun 130000JilinChina School of Metallurgy Northeastern UniversityShenyang 110819LiaoningChina School of Mechanical MaterialsMechatronic and Biomedical EngineeringUniversity of WollongongWollongongNSW 2522Australia

The evolution of microstructure,texture,and magnetic properties with random texture,near-co.per texture,weak near-cube texture,and strong λ fiber(/ND(normal direction))before rolling of non-oriented electrical steel was *** recrystallized hot bands with different textures but similar grain sizes were prepared by pre-annealing at low-temperature and high-temperature normalization *** was observed that the final annealed products exhibited similar recrystallized *** co.trast,the final annealed product with more 2 fiber before rolling exhibited a stronger cube *** the fiber before rolling beco.ing stronger,the proportion of(111)deformed matrices became larger,which co.ld be observed in the early recrystallization *** overwhelmingly dominant 2 orientation nuclei are formed in the(111)deformed matrix and beco.e the dominant ***,the best magnetic properties are obtained in the products with strong 2 fiber before rolling,co.responding to the strong cube texture and low anisotropyparameter.

关键词： Texture before rolling Non-oriented electrical steel-Nucleation Grain growth Magnetic property

Hollow structured Fe@C nanorods for boosting dehydrogenation properties of α-AlH_(3)

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Nano Research 2024年第9期17卷 8184-8191页

作者： Yuan Zhao Qingshuang Wang Dongming Yin Xiaoli Wang Shouliang Li Chunli Wang Long Liang Shaolei Zhao Limin Wang Yong Cheng School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Shandong Provincial Key Laboratory of Monocrystalline Silico. Semico.ductor Materials and technology College of Chemistry and Chemical EngineeringDezhou UniversityDezhou 253023China Henan Nayu New Material co. Ltd.Xinxiang 453000China

α-AlH_(3)is regarded as one of the most promising hydrogen storage materials due to its high hydrogen storage capacity(10.1 wt.%,148 kg·m^(-3)).However,in practical applications,the associated hydrogen release temperature remains relatively *** effectively address this issue,hollow structured Fe@C nanorods derived from Fe-MOF are introduced as highly efficient catalyst to optimize the dehydrogenation properties ofα-AlH_(3).co.paratively,the initial hydrogen release temperature ofα-AlH_(3)+3 wt.%Fe@C is reduced to 94.2℃,which is significantly lower than that of pureα-AlH_(3)(137.8℃).At 100 and 120℃,it exhibits hydrogen capacities of 5.38 wt.%and 7.47 wt.%,respectively,whereas pureα-AlH_(3)only delivers hydrogen capacities of 0.24 wt.%and 5.94 wt.%under the same *** density functional theory(DFT)calculations further indicate that the existence of Fe@C catalyst can make the length of Al-H bond increase,which is more co.ducive to the release of *** results show that the synergistic effect of Fe and porous carbon in Fe@C nanorods can improve the hydrogen desorption kinetics ofα-AlH_(3),providing a good prospect for the application ofα-AlH_(3)in hydrogen storage fields.

关键词： Fe@C α-AlH_(3) dehydrogenation catalyst

Activity regulation and applications of metal-organic framework-based nanozymes

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Rare Metals 2024年第3期43卷 900-914页

作者： Ge Fang Shou-Xin Bao Gen-Xiu Zhou Cui-Cui Ge State Key Laboratory of radiation Medicine and Protection School of Radiation Medicine and ProtectionSchool for Radiological and Interdisciplinary Sciences(RAD-X)Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education InstitutionsSoochow UniversitySuzhou 215123China Suzhou Nanomicro technology co. LtdSuzhou 215000China

As a new generation of artificial enzymes,nanozymes show outstanding advantages such as high stability,low co.t,and facile synthesis,which endow them with promising applications in biomedical and environmental *** the various reported nanozymes,metal-organic frameworks(MOFs)co.ld mimic the active center of natural enzymes and provide a hydrophobic environment,which makes MOFs attractive alternatives to natural *** to the highly structural diversity and tailorability of MOFs,rational design will co.tribute to improve the activity of MOF-based nanozymes and promote their potential applications in both biomedical and environmental ***,a co.prehensiye suminary of activity regulatory strategies of MOF-based nanozymes is urgently ***,we summarized the activity regulatory strategies of MOFs with intrinsic enzyme-like activities via modulation of metal nodes,ligands,structures and *** the applications of MOF-based nanozymes in biosensing,hazardous degradation,antibacterial,and cancer therapy were also ***,the current challenges and future perspectives were discussed in *** is highly expected that this review will provide a better understanding on the rational design of novel high-performance MOF-based nanozymes.

关键词： Metal-organic frameworks(MOF)-based nanozymes Activity regulation Biosensing Cancer therapy Hazardous degradation Antibacterial

Carbon efficiency modeling and optimization of solar-powered cellular networks

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Science China(Information Sciences) 2024年第5期67卷 228-243页

作者： Yuxi ZHAO Xiaohu GE Wen YAN Tao HAN Yi ZHONG School of Electronic Information and co.munications Huazhong University of Science and Technology Huawei technology co. Ltd.

As wireless co.munication traffic experiences rapid growth, the carbon emissions caused by the co.munication industry are also on the rise. To achieve “carbon neutrality”, researchers are co.sidering the use of renewable energy sources to power cellular networks, thereby reducing carbon emissions. However, a challenge arises when using renewable energy, specifically owing to the unpredictable nature of both the energy co.sumption of the cellular network and the power generation from renewable sources. This inco.sistency results in low renewable energy utilization and reduced carbon efficiency. Herein, we co.struct a carbon efficiency model of solar-powered cellular networks using practical data from solar radiation. We propose a mechanism that alternately optimizes the performance of the renewable energy network and the cellular network. This approach is based on co.vex optimization theory and the Dinkelback algorithm, and it leads to the design of a carbon efficiency optimization algorithm. This algorithm aims to improve the carbon efficiency of cellular networks and reduce their carbon emissions. Simulation results demonstrate that our optimization scheme yields a maximum improvement of 2.56 × 108bps/g in the carbon efficiency of the cellular network as co.pared to co.ventional power allocation schemes such as the traditional water filling method and heuristic energy sharing and charge/discharge algorithms.

关键词： cellular networks renewable energy carbon efficiency co.vex optimization theory dinkelbach

Current-co.lapse suppression and leakage-current decrease in AlGaN/GaN HEMT by sputter-TaN gate-dielectric layer

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Journal of Semico.ductors 2024年第7期45卷 70-75页

作者： Bosen Liu Guohao Yu Huimin Jia Jingyuan Zhu Jiaan Zhou Yu Li Bingliang Zhang Zhongkai Du Bohan Guo Lu Wang Qizhi Huang Leifeng Jiang Zhongming Zeng Zhipeng Wei Baoshun Zhang State Key Laboratory of High-Power Semico.ductor Laser School of PhysicsChangchun University of Science and TechnologyChangchun 130022China Nanofabrication facility Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China Suzhou Powerhouse Electronics technology co. Ltd.Suzhou 215123China

In this paper, we explore the electrical characteristics of high-electron-mobility transistors(HEMTs) using a TaN/AlGaN/GaN metal insulating semico.ductor(MIS) structure. The high-resistance tantalum nitride(TaN) film prepared by magnetron sputtering as the gate dielectric layer of the device achieved an effective reduction of electronic states at the TaN/AlGaN interface, and reducing the gate leakage current of the MIS HEMT, its performance was enhanced. The HEMT exhibited a low gate leakage current of 2.15 × 10^(-7) mA/mm and a breakdown voltage of 1180 V. Furthermore, the MIS HEMT displayed exceptional operational stability during dynamic tests, with dynamic resistance remaining only 1.39 times even under 400 V stress.

关键词： AlGaN/GaN MIS HEMTs gate dielectric layer depletion-mode gate reliability I_(on)/I_(off)ratio

Current status and development of CMOS SiPM for scintillator-based radiation detectors toward all-digital sensors[Invited]

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Chinese Optics Letters 2024年第2期22卷 17-27页

作者： Nico.a D'Ascenzo 胡文韬劳慧华越轩张博房磊奚道明郑睿邱奥 Emanuele Antonecchia 凌怡清刘雨晴李琰俞航肖鹏谢庆国 Wuhan National Laboratory for Optoelectronics Wuhan 430074China Biomedical Engineering Department Huazhong University of Science and TechnologyWuhan 430074China RAYQUANT technology co. Ltd.Ezhou 436044China RAYSOLUTION Healthcare co. Ltd.Hefei 230000China RAYMEASURE technology co. Ltd.Suzhou 215000China RAYCAN technology co. Ltd.Suzhou 215000China co.lege of co.puter Science and Software Engineering Shenzhen UniversityShenzhen 518060China

Modern scintillator-based radiation detectors require silico. photomultipliers(Si PMs)with photon detection efficiency higher than 40%at 420 nm,possibly extended to the vacuum ultraviolet(VUV)region,single-photon time resolution(SPTR)co.nt rate(DCR)co.centrations at low CMOS scales,deep-level carrier generation in shallow trench isolation fabrication,and power co.sumption,among *** advances at 350 and 110 nm CMOS nodes are benchmarked against available Si PMs obtained in CMOS and co.mercial customized *** co.cept of digital multithreshold Si PMs with a single microcell readout is finally reported,proposing a possible direction toward fully digital scintillator-based radiation detectors.

关键词： silico. photomultiplier co.plementary metal-oxide semico.ductor digital SiPM