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Journal of energy Chemistry 2025年第1期100卷 621-627页

作者： Fei Lv Longjie Liu Jiazhe Wu Pengfei Wang Lixia Pan Dengwei Jing Yubin Chen International Research Center for renewable energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Combining water electrolysis and rechargeable battery technologies into a single system holds great promise for the co-production of hydrogen （H2） and ***,the design and development of such systems is still in its ***,an integrated hydrogen-oxygen （O2）-electricity co-production system featuring a bipolar membrane-assisted decoupled electrolyzer and a Na-Zn ion battery was established with sodium nickelhexacyanoferrate （NaNiHCF） and Zn2+/Zn as dual redox *** decoupled electrolyzer enables to produce H2and O2in different time and space with almost 100%Faradaic efficiency at 100 mA ***,the charged NaNiHCF and Zn electrodes after the electrolysis processes formed a Na-Zn ion battery,which can generate electricity with an average cell voltage of 1.75 V at 10 m A *** connecting Si photovoltaics with the modular electrochemical device,a well-matched solar driven system was built to convert the intermittent solar energy into hydrogen and electric energy with a solar to hydrogen-electricity efficiency of 16.7%,demonstrating the flexible storage and conversion of renewables.

关键词： Hydrogen Electricity Decoupled water electrolyzer Na-Zn ion battery Solar energy

Bimetallic Single‑Atom Catalysts for water Splitting

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Nano-Micro Letters 2025年第1期17卷 1-45页

作者： Megha A.Deshmukh Aristides Bakandritsos Radek Zbořil Nanotechnology centre Centre for Energy and Environmental TechnologiesVŠB–Technical University of Ostrava17.listopadu 2172/1570800 Ostrava‑PorubaCzech Republic Regional centre of Advanced Technologies and Materials Czech Advanced Technology and Research Institute(CATRIN)Palacky University OlomoucŠlechtitelů241/2778371 Olomouc–HoliceCzech Republic

Green hydrogen from water splitting has emerged as a critical energy vector with the potential to spearhead the global transition to a fossil fuel-independent *** field of catalysis has been revolutionized by single-atom catalysts(SACs),which exhibit unique and intricate interactions between atomically dispersed metal atoms and their ***,bimetallic SACs(bimSACs)have garnered significant attention for leveraging the synergistic functions of two metal ions coordinated on appropriately designed *** offer an avenue for rich metal–metal and metal–support cooperativity,potentially addressing current limitations of SACs in effectively furnishing transformations which involve synchronous proton–electron exchanges,substrate activation with reversible redox cycles,simultaneous multi-electron transfer,regulation of spin states,tuning of electronic properties,and cyclic transition states with low activation *** review aims to encapsulate the growing advancements in bimSACs,with an emphasis on their pivotal role in hydrogen generation via water *** subsequently delve into advanced experimental methodologies for the elaborate characterization of SACs,elucidate their electronic properties,and discuss their local coordination ***,we present comprehensive discussion on the deployment of bimSACs in both hydrogen evolution reaction and oxygen evolution reaction,the two half-reactions of the water electrolysis process.

关键词： Single-atom catalysts Single-atom dimers Hydrogen evolution Oxygen evolution water splitting

Flexible molecules dedicate to release strain of inverted inorganic perovskite solar cell

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Journal of energy Chemistry 2025年第1期100卷 87-93页

作者： Hongrui Sun Sanlong Wang Pengyang Wang Yali Liu Shanshan Qi Biao Shi Ying Zhao Xiaodan Zhang Institute of Photoelectronic Thin Film Devices and Technology Renewable Energy Conversion and Storage Center State Key Laboratory of Photovoltaic Materials and CellsNankai University Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin Haihe Laboratory of Sustainable Chemical Transformations Engineering Research Center of Thin Film Photoelectronic Technology of Ministry of Education Collaborative Innovation Center of Chemical Science and Engineering (Tianjin)

The tensile strain in inorganic perovskite films induced by thermal annealing is one of the primary factors contributing to the inefficiency and instability of inorganic perovskite solar cells （IPSCs）,which reduces the defect formation ***,a flexible molecule 5-maleimidovaleric acid （5-MVA） was introduced as a strain buffer to release the residual strain of *** anhydride and carboxyl groups in 5-MVA interact strongly with the uncoordinated Pb2+through Lewis acid-base reaction,thus tightly“pull”the perovskite *** in-between soft carbon chain increased the structural flexibility of CsPbI2.85Br0.15perovskite materials,which effectively relieved the intrinsic internal strain of CsPbI2.85Br0.15,resisted the corrosion of external strain,and also reduced the formation of defects such as VIand *** addition,the introduction of 5-MVA improved crystal quality,passivated residual defects,and narrowed energy level ***,power conversion efficiency （PCE） of NiOxbased inverted IPSCs increased from 19.25% to 20.82% with the open-circuit voltage enhanced from 1.164 V to 1.230 *** release of strain also improved the stability of CsPbI2.85Br0.15perovskite films and devices.

关键词： Perovskite solar cells

揭示钙钛矿前驱体溶液的胶体组成及其对成膜的影响（英文）

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Science China Materials 2025年第1期 156-164页

作者：娄甜甜陈乐添杨桂春陈鹏赵文燕李红时李国然 School of Materials Science and Engineering Institute of New Energy Material Chemistry Renewable Energy Conversion and Storage Center Nankai University School of Mechanical and Electronic Engineering Jingdezhen Ceramic University

胶体是钙钛矿前驱体溶液的重要组成部分,对钙钛矿的成膜质量有重大影响.在这项工作中,我们探索了两种不同类型前驱体的胶体成分:原料单体混合溶解(MMD)和预合成的钙钛矿单晶再溶解(SCR).我们发现了一种新的溶解化学平衡机制,即从混合单...

胶体是钙钛矿前驱体溶液的重要组成部分,对钙钛矿的成膜质量有重大影响.在这项工作中,我们探索了两种不同类型前驱体的胶体成分:原料单体混合溶解(MMD)和预合成的钙钛矿单晶再溶解(SCR).我们发现了一种新的溶解化学平衡机制,即从混合单体到3C立方相(α相)的转变涉及一个可逆的转变过程. MMD的方法产生了多聚Pb-I溶剂化胶束,而SCR方法产生的则是六方卤化铅基的钙钛矿胶体,这种胶体组成的差别显著影响了成膜质量.值得注意的是,六方相胶体是有利的成核位点,可促进形成晶粒更大、相更均匀、缺陷更少的α相钙钛矿薄膜.这项工作证明了调控胶体成分的重要性,并从理论上深入探讨了以粉末、微晶和单晶等形式重新溶解钙钛矿的有利影响.

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New Linkage with Linear Actuator for Tracking PV Systems with Large Angular Stroke

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Chinese Journal of Mechanical Engineering 2011年第5期24卷 744-751页

作者： VISA Ion DIACONESCU Dorin SAULESCU Radu VATASESCU Monica BURDUHOS Bogdan renewable energy Systems and Recycling Research centre Transilvania University of Brasov

This paper focuses on the development of an optimized photovoltaic tracking system involving low-cost, relative simple mechanisms, with linear actuators able to insure strokes comparable with those resulted when using gear rotary actuators. Starting with a rhombus linkage, with a linear actuator on the diagonal used for the elevation motion till 90°, a new performance solution is generated. This new linkage allows large angular strokes by using an asymmetric rhombus and an eccentrically positioned linear actuator. The paper can be divided in three main parts. Firstly the kinematical modeling of the new linkage is addressed, which permits the establishing of the linkage dimensions according to two adjustable parameters （k2, k5）. Using the resulted correlations, in the second part the linkage synthesis algorithm is developed; the steps followed in this algorithm are presented in a numerical application considering a tracked PV platform, where the azimuthal vertical movement is obtained with the new proposed rhomboidal linkage. In the last part of the paper an analysis is done with the aim of determining the PV platform tracking efficiency （which represents the ratio between the received and the available beam solar energy） using the new linkage, in the meteorological conditions of Brasov, Romania implementation site.

关键词： solar tracking linkage linear actuator angular stroke transmission angle

Toward the Design of Multi Asymmetric Surface Dielectric Barrier Discharge (ASDBD) Actuators

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Plasma Science and Technology 2015年第1期17卷 56-63页

作者： Massiel ZADEH V.ROHANI F.CAUNEAU F.FABRY L.FULCHERI centre for Processes Renewable Energies and Energy Systems-PERSEE- MINES ParisTech

This paper investigates the electrical and mechanical behaviors of a single-ASDBD actuator and a two-ASDBD one supplied in sinusoidal mode（1-10 kHz）.The main objective of our research is to determine the optimum frequency values for the function of these actuators with a given power *** this purpose,we determine the electrical power density input to the actuators versus frequency through two methods：i） a semi-theoretical method,based on an impedance calculation,and ii） an experimental method,based on direct electrical *** methods show that the addition of a second ASDBD changes the resonance frequency value of the actuator by moving it towards low *** characterizing the aerodynamic mobile layer structure induced by the single-ASDBD actuator,we analyze experimentally the mechanical response of a two-ASDBD actuator as a function of the inter-ASDBD *** experiments demonstrate that the induced electric wind velocity and the electro-mechanical yield of a twoASDBD actuator reach a maximum value for an optimum inter-ASDBD distance,which is a useful value for the design of highly efficient multi-ASDBD actuators.

关键词： ASDBD actuator resonance frequency electro-mechanical yield

A sustainable integration of removing CO_(2)/NO_(x) and producing biomass with high content of lipid/protein by microalgae

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Journal of energy Chemistry 2022年第10期31卷 13-25,I0002页

作者： Junying Zhu Baowen Guo Fengxiang Qie Xu Li Xikang Zhao Junfeng Rong Baoning Zong Research centre of renewable energy Research Institute of Petroleum ProcessingSINOPECBeijing 100083China

Due to the boost of CO_(2)/NO_(x)emissions which cause environmental pollution,processes that remove such pollutants from flue gas have attracted increasing attention in recent *** these technologies,biological CO_(2)/NO_(x)emission reduction has received more ***,a kind of photosynthetic microorganism,offer great promise to convert CO_(2)/NO_(x)to biomass with high content of lipid and protein,which can be used as feedstock for various products such as biodiesel,health products,feedstuff and *** this paper,biological CO_(2)/NO_(x)removing technologies by microalgae,together with the products(such as biofuel and protein)and their economic viability are *** commercial applications of microalgae for biodiesel and protein products are hampered by the high production cost of biomass,the use of CO_(2)/NO_(x)from flue gas as carbon and nitrogen sources can reduce the cost of biomass production,which makes these technologies more competent for real-life ***,it is projected that the increasing in CO_(2)allowances will lead to further reduction in the cost of biomass production,which especially favors related products with lower values such as ***,by combining various process optimization and integration,biorefinery is proposed and considered as the crucial component for the sustainable and economically feasible bulk applications of microalgae biomass.

关键词： Microalgae Greenhouse gas NO_(x) Biodiesel Protein

Electrode/Electrolyte Optimization‑Induced Double‑Layered Architecture for High‑Performance Aqueous Zinc‑(Dual)Halogen Batteries

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Nano-Micro Letters 2025年第3期17卷 121-137页

作者： Chengwang Zhou Zhezheng Ding Shengzhe Ying Hao Jiang Yan Wang Timing Fang You Zhang Bing Sun Xiao Tang Xiaomin Liu School of Textiles and Clothing School of Chemistry and Chemical EngineeringQingdao UniversityQingdao 266071ShandongPeople’s Republic of China centre for Clean energy Technology School of Mathematical and Physical SciencesFaculty of ScienceUniversity of Technology SydneyUltimoNSW 2007Australia School of Chemistry and Chemical Engineering Henan Normal UniversityXinxiang 453007HenanPeople’s Republic of China

Aqueous zinc-halogen batteries are promising candidates for large-scale energy storage due to their abundant resources,intrinsic safety,and high theoretical ***,the uncontrollable zinc dendrite growth and spontaneous shuttle effect of active species have prohibited their practical ***,a double-layered protective film based on zinc-ethylenediamine tetramethylene phosphonic acid(ZEA)artificial film and ZnF2-rich solid electrolyte interphase(SEI)layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic *** ZEA-based artificial film shows strong affinity for the ZnF2-rich SEI layer,therefore effectively suppressing the SEI breakage and facilitating the construction of double-layered protective film on the zinc metal *** double-layered architecture not only modulates Zn2+flux and suppresses the zinc dendrite growth,but also blocks the direct contact between the metal anode and electrolyte,thus mitigating the corrosion from the active *** employing optimized metal anodes and electrolytes,the as-developed zinc-(dual)halogen batteries present high areal capacity and satisfactory cycling *** work provides a new avenue for developing aqueous zinc-(dual)halogen batteries.

关键词： Zn metal anodes Double-layered protective film Electrode/electrolyte optimization Aqueous zinc-(dual)halogen batteries

water quality, agriculture and food safety in China:Current situation, trends, interdependencies, and management

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Journal of Integrative Agriculture 2015年第11期14卷 2365-2379页

作者： ZHANG Xiao-nan GUO Qiu-ping SHEN Xiao-xue YU Sheng-wen QIU Guo-yu Shenzhen Engineering Laboratory for water Desalinization with renewable energy School of Environment and EnergyPeking University Chinese Academy for Environmental Planning

water quality in China is becoming a severe challenge for agriculture and food safety, and it might also impact health of population via agriculture and food. Thus, it is causing widespread concern. Based on extensive literatures review and data mining, current situation of water pollution in China and its effects on food safety were analyzed. The 2nd National water Resource Survey in China show that the surface water all over the country was under slight pollution and about 60% of groundwater is polluted. Drinking water quality is basically guaranteed in urban area but it is worrisome in rural areas. In addition, China is the largest consumer of fertilizer and pesticide in the world and the amounts of application still show increasing trends. Fertilizers and pesticides are the most important sources of pollution, which affect human health as persistent organic pollutants and environmental endocrine disruptors. Eutrophication of surface water and nitrate pollution of groundwater are serious threats to drinking water safety. Sewage irrigation is becoming a pollution source to China＇s water and land because of lacking of effective regulations. Although, with the advance in technology and management level, control of nitrogen and phosphorus emissions and reducing water pollution is still a major challenge for China.

关键词： agriculture drinking water eutrophication fertilizer food safety groundwater heavy metals microcystin nitrate pesticide pollution water quality

Applying chemical engineering concepts to non-thermal plasma reactors

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Plasma Science and Technology 2018年第6期20卷 161-171页

作者： Pedro AFFONSO NOBREGA Alain GAUNAND VANDad ROHANI Fran?ois CAUNEAU Laurent FULCHERI MINES ParisTech PSL Research UniversityPERSEE-Centre for ProcessesRenewable Energy and Energy Systems MINES ParisTech PSL Research UniversityCTP-Centre for Thermodynamics of p Processes

Process scale-up remains a considerable challenge for environmental applications of non-thermal *** the impact of reactor hydrodynamics in the performance of the process is a key step to overcome this *** this work,we apply chemical engineering concepts to analyse the impact that different non-thermal plasma reactor configurations and regimes,such as laminar or plug flow,may have on the reactor *** do this in the particular context of the removal of pollutants by non-thermal plasmas,for which a simplified model is *** generalise this model to different reactor configurations and,under certain hypotheses,we show that a reactor in the laminar regime may have a behaviour significantly different from one in the plug flow regime,often assumed in the non-thermal plasma *** the other hand,we show that a packed-bed reactor behaves very similarly to one in the plug flow *** those results,the reader will find in this work a quick introduction to chemical reaction engineering concepts.

关键词： non-thermal plasma chemical engineering dielectric barrier discharge(DBD) corona discharge plug flow reactor volatile organic compounds