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Electrochemical conversion of methane to bridge the gap in the artificial carbon cycle

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Journal of Energy Chemistry 2025年第1期100卷 286-308页

作者： Yuhao Peng Yuefeng Song Ihar Razanau Juanxiu Xiao Wei Xiao Di Hu Guoxiong Wang College of Chemistry and Molecular Sciences Hubei Key Laboratory of Electrochemical Power Sources Wuhan University State Key Laboratory of Catalysis Dalian National Laboratory for Clean Energy iChEM (Collaborative Innovation Center of Chemistry for Energy Materials) Dalian Institute of Chemical Physics Chinese Academy of Sciences Laboratory of Physical-Chemical Technologies SSPA Scientific and Practical Materials Research Centre of NAS of Belarus State Key Laboratory of Marine Resources Utilization in South China Sea Collaborative Innovation Center of Marine Science and Technology School of Marine Science and Engineering Hainan University Department of Chemical and Environmental Engineering University of Nottingham Ningbo China

Methane, an abundant one-carbon（C1） resource, is extensively used in the industrial production of vital fuels and value-added chemicals. However, current industrial methane conversion technologies are energy-and carbon-intensive, mainly due to the high activation energy required to break the inert C–H bond, low selectivity, and problematic side reactions, including CO2emissions and coke deposition. Electrochemical conversion of methane（ECM） using intermittent renewable energy offers an attractive solution, due to its modular reactor design and operational flexibility across a broad spectrum of temperatures and pressures. This review emphasizes conversion pathways of methane in various reaction systems, highlighting the significance and advantages of ECM in facilitating a sustainable artificial carbon cycle. This work provides a comprehensive overview of conventional methane activation mechanisms and delineates the complete pathways of methane conversion in electrolysis contexts. Based on surface/interface chemistry, this work systematically analyzes proposed reaction pathways and corresponding strategies to enhance ECM efficiency towards various target products, including syngas, hydrocarbons, oxygenates, and advanced carbon materials. The discussion also encompasses opportunities and challenges for the ECM process, including insights into ECM pathways, rational electrocatalyst design, establishment of benchmarking protocols, electrolyte engineering, enhancement of CH4conversion rates, and minimization of CO2emission.

关键词： Methane Electrochemical conversion Reaction mechanism Catalyst design Electrode Electrocatalysis

A Comprehensive Survey on Federated Learning Applications in Computational Mental Healthcare

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Computer Modeling in Engineering & Sciences 2025年第1期142卷 49-90页

作者： Vajratiya Vajrobol Geetika Jain Saxena Amit Pundir Sanjeev Singh Akshat Gaurav Savi Bansal Razaz Waheeb Attar Mosiur Rahman Brij B.Gupta Institute of Informatics and Communication University of DelhiDelhi110021India Maharaja Agrasen College University of DelhiDelhi110096India Computer Engineering Ronin InstituteMontclairNJ 07043USA Department of Research and innovation Insights2TechinfoJaipur302001India University centre for Research and Development(UCRD) Chandigarh UniversityChandigarh140413India Management Department College of Business AdministrationPrincess Nourah bint Abdulrahman UniversityRiyadh11671Saudi Arabia CCRI&Department of Computer Science and Information Engineering Asia UniversityTaichung413Taiwan Symbiosis centre for Information Technology(SCIT) Symbiosis International UniversityPune411057India Center for Interdisciplinary Research University of Petroleum and Energy Studies(UPES)Dehradun248007India

Mental health is a significant issue worldwide,and the utilization of technology to assist mental health has seen a growing *** aims to alleviate the workload on healthcare professionals and aid *** applications have been developed to support the challenges in intelligent healthcare ***,because mental health data is sensitive,privacy concerns have *** learning has gotten some *** research reviews the studies on federated learning and mental health related to solving the issue of intelligent healthcare *** explores various dimensions of federated learning in mental health,such as datasets(their types and sources),applications categorized based on mental health symptoms,federated mental health frameworks,federated machine learning,federated deep learning,and the benefits of federated learning in mental health *** research conducts surveys to evaluate the current state of mental health applications,mainly focusing on the role of Federated Learning(FL)and related privacy and data security *** survey provides valuable insights into how these applications are emerging and evolving,specifically emphasizing FL’s impact.

关键词： Depression emotional recognition intelligent healthcare systems mental health federated learning stress detection sleep behaviour

Image reconstruction for cone-beam computed tomography using total p-variation plus Kullback-Leibler data divergence

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Chinese Physics B 2017年第7期26卷 461-473页

作者：蔡爱龙李磊王林元闫镔郑治中张瀚铭胡国恩 National digital Switching System Engineering & Technological Research centre

Accurate reconstruction from a reduced data set is highly essential for computed tomography in fast and/or low dose imaging applications. Conventional total variation（TV）-based algorithms apply the L1 norm-based penalties, which are not as efficient as Lp（0〈p〈1） quasi-norm-based penalties. TV with a p-th power-based norm can serve as a feasible alternative of the conventional TV, which is referred to as total p-variation（TpV）. This paper proposes a TpV-based reconstruction model and develops an efficient algorithm. The total p-variation and Kullback-Leibler（KL） data divergence, which has better noise suppression capability compared with the often-used quadratic term, are combined to build the reconstruction model. The proposed algorithm is derived by the alternating direction method（ADM） which offers a stable, efficient, and easily coded implementation. We apply the proposed method in the reconstructions from very few views of projections（7 views evenly acquired within 180°）. The images reconstructed by the new method show clearer edges and higher numerical accuracy than the conventional TV method. Both the simulations and real CT data experiments indicate that the proposed method may be promising for practical applications.

关键词： image reconstruction total p-variation minimization Kullback-Leibler data divergence p-shrinkage mapping

An experimental and numerical study of packing, compression, and caking behaviour of detergent powders

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Particuology 2014年第1期12卷 2-12页

作者： Subhash C.Thakur Hossein Ahmadian Jin Sun Jin Y.Ooi School of Engineering University of Edinburgh Newcastle innovation centre Procter and Gamble Technical Centre Ltd

This paper presents an experimental and numerical study of the packing, compression, and caking behaviour of spray dried detergent （SDD） powders with a two-fold aim： an experimental process of observation and evaluation of the packing, compression and caking behaviour of SDD powders, and a numerical approach based on discrete element modelling （DEM）. The mechanical properties, including the stress-strain response and the corresponding porosity change as a function of consolidation stress in a confined cylinder, the stress-strain response during unconfined shearing and the cake strength as a func- tion of consolidation stress, were evaluated and compared for different SDD powders using an extended uniaxial tester （Edinburgh Powder Tester - EPT）. The experiments using EPT showed excellent repro- ducibility in the measurement of packing, compression and caking behaviour and were therefore very useful for describing the handling characteristics of these powdered products including screening new products and different formulations. It was found that the sample with higher moisture had lower bulk porosity but higher compressibility and cake strength. The porosity, compressibility and cake strength were found to vary across different size fractions of the same sample. The larger sieve-cut samples had higher initial bulk porosity, compressibility and cake strength. It is revealed that moisture plays a sig- nificant role in packing, compression, and shearing behaviour of the powder. Three-dimensional DEM modelling using a recently developed elasto-plastic adhesive-frictional contact model showed that the contact model is able to capture the detergent behaviour reasonably well and can be used to model complex processes involving these powders.

关键词： Discrete element methodPowder flowCohesive materialUniaxial testPlasticityContact model

Green Plant Leaf-inspired Smart Camouflage Fabrics for Visible Light and Near-infrared Stealth

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Journal of Bionic Engineering 2022年第3期19卷 788-798页

作者： Qixin Lu Min Li Anli Tian Shaohai Fu Jiangsu Engineering Research centre for digital Textile Inkjet Printing Key Laboratory of Eco-TextileMinistry of EducationJiangnan UniversityWuxi214122China National Manufacturing innovation centre of Advanced Dyeing and Finishing Technology Ministry of EducationJiangnan UniversityWuxi214122China

Due to Visible light and Near-Infrared(Vis–NIR)stealth play an important role in the commercial,military,and scientific fields,camouflage materials related to it attracted increasing attention in *** plant leaves,as the most extensive background materials on the earth,were widely simulated in the camouflage ***,difficult full-spectrum simulation(380–2500 nm),low-similarity simulation and the complex preparation have been great challenges for Vis–NIR Camouflage Materials(Vis–NIR-CMs).Herein,basing on the color-matching principle,two novel Vis–NIR-CMs including Dark Green Materials and Light Green Materials(DGM and LGM)were facilely fabricated by simple printing organic disperse dyes including *** Blue 291,*** Yellow 114,and *** Orange 30(B-291,Y-114 and O-30),and titanium dioxide(TiO_(2))on the viscose *** on the excellent red edge property of B-291 and high scattering ability of TiO2,DGM and LGM exhibited generally high spectral correlation coefficients r_(m)(>0.95)with green plant ***,with the great color performance,excellent objects covering performance,low areal density(7.7 MPa),high softness(>81.27),high air permeability(>45.848 mm s^(−1)),DGM and LGM showed good simulation performance and wearing comfort to satisfy the application *** work presents a high-similarity Vis–NIR-CMs as a reference for full-spectrum camouflage materials,as well as low-cost and efficient preparation method is beneficial to the development of camouflage field.

关键词： Vis-NIR Camouflage materials Plant leaves Organic dyes Viscose fabrics

Recycling of magnesium drive train components

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Science China(Technological Sciences) 2009年第1期52卷 148-154页

作者： Daniel FECHNER Carsten BLAWERT Norbert HORT Karl Ulrich KAINER MagIC-Magnesium innovation centre GKSS Research Centre Max-Planck-Straβe 1

With the development of new heat resistant magnesium alloys, the automotive industry has introduced several parts to the drive train. The rising number of large magnesium components will result in a higher quantity of automotive post consumer scrap. It was the aim of this work to find a reasonable alloy system for the recycling of these magnesium drive train components. A matrix of potential recy-cling alloys based on the magnesium alloy AM50 was prepared via permanent mould casting. The materials were investigated via tensile testing, creep tests and salt spray tests. Three alloys were selected for processing via high pressure die casting and the tests were repeated on the new materials. A promising system for recycling has been isolated and will be investigated more deeply for the influence of impurities.

关键词： magnesium recycling end-of-life vehicles recycling alloy post consumer scrap

High precision and efficiency robotic milling of complex parts:Challenges,approaches and trends

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Chinese Journal of Aeronautics 2022年第2期35卷 22-46页

作者： Zerun ZHU Xiaowei TANG Chen CHEN Fangyu PENG Rong YAN Lin ZHOU Zepeng LI Jiawei WU School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of digital Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan 430074China Wuhan digital Design and Manufacturing innovation centre Co. Ltd.Wuhan 430074China

Due to the advantages of large workspace,low cost and the integrated vision/force sensing,robotic milling has become an important way for machining of complex *** recent years,many scholars have studied the problems existing in the applications of robotic milling,and lots of results have been made in the dynamics,pose planning,deformation control etc.,which provides theoretical guidance for high precision and high efficiency of robotic *** the perspective of complex parts robotic milling,this paper focuses on machining process planning and control techniques including the analysis of the robot-workspace,robot trajectory planning,vibration monitoring and control,deformation monitoring and *** well as the principles of these technologies such as robot stiffness characteristics,dynamic characteristics,chatter mechanisms,and deformation *** methods and characteristics related to the theory and technology of robotic milling of complex parts are summarized *** latest research progress and achievements in the relevant fields are *** is hoped that the challenges,strategies and development related to robotic milling could be clarified through the carding work in this paper,so as to promote the application of related theories and technologies in high efficiency and precision intelligent milling with robot for complex parts.

关键词： Complex parts Deformation Dynamics Robotic milling Stiffness Vibration control

Coherent and tunable radiation with power enhancement from surface plasmon polaritons

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Chinese Physics B 2015年第7期24卷 435-440页

作者：龚森钟任斌胡旻陈晓行张平赵陶刘盛纲 Cooperative innovation centre of THz Science University of Electronic Science and Technology of China

Surface plasmon polaritons excited by an electron beam can be transformed into coherent and tunable light radiation waves with power enhancement in the simple structure of a metal film with a dielectric medium loading. In this paper, the process of the radiation transformation of this radiation, and the dependencies of the radiation characteristics on the parameters of the structure and the electron beam are studied in detail. The radiation power enhancement is greatly influenced by the beam energy and the film thickness in the infrared to ultraviolet frequency region. Up to 122 times radiation power enhancement and 6.5% radiation frequency tuning band can be obtained by optimizing the beam energy and the parameters of the film.

关键词： surface plasmon polaritons electron beam radiation power enhancement

Recent advances in wheel–rail RCF and wear testing

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Friction 2023年第12期11卷 2181-2203页

作者： Sundar SHRESTHA Maksym SPIRYAGIN Esteban BERNAL Qing WU Colin COLE centre for Railway Engineering Central Queensland UniversityRockhampton 4701Australia Australasian centre for Rail innovation Canberra 2601Australia

The wear and rolling contact fatigue (RCF) testing approaches for wheels and rails have been reviewedand evaluated in this study. The study points out the advantages and limitations of the existing approaches. Thebroad analysis revealed that scaled laboratory-based wear testing is widely applied. However, it is necessary topredetermine the input parameters and observing parameters for scaled wear testing for three reasons: first, toemulate the real-world scenarios as closely as possible;second, to postprocess the results received from the scaledtesting and transfer them into real practice at full scale;third, to present the results in a legible/appropriate ***, most of the important parameters required for wear testing have been discussed with fundamental andsystematic explanations provided. Additionally, the transition of the parameters from the real-world into the testdomain is explained. This study also elaborates on the challenges of the RCF and wear testing processes andconcludes by providing major considerations toward successful testing.

关键词： wear testing rolling contact fatigue(RCF)testing wheel-rail