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Polarization-dependent photoinduced metal–insulator transitions in manganites

Science Bulletin 2024年第2期69卷 183-189页

作者： Lina Deng Weiye Zhang Hanxuan Lin Lifen Xiang Ying Xu Yadi Wang Qiang Li Yinyan Zhu Xiaodong Zhou Wenbin Wang Lifeng Yin Hangwen Guo Chuanshan Tian Jian Shen State Key Laboratory of Surface Physics Institute for Nanoelectronic Devices and Quantum Computingand Department of PhysicsFudan UniversityShanghai 200433China Shanghai research center for Quantum Sciences Shanghai 201315China Zhangjiang Fudan International innovation center Fudan UniversityShanghai 201210China Collaborative innovation center of Advanced Microstructures Nanjing 210093China Shanghai Branch CAS Center for Excellence and Synergetic Innovation Center in Quantum Information and Quantum PhysicsShanghai 201315China

In correlated oxides,collaborative manipulation on light intensity,wavelength,pulse duration and polarization has yielded many exotic discoveries,such as phase transitions and novel quantum *** view of potential optoelectronic applications,tailoring long-lived static properties by light-induced effects is highly *** far,the polarization state of light has rarely been reported as a control parameter for this ***,we report polarization-dependent metal-to-insulator transition(MIT)in phaseseparated manganite thin films,introducing a new degree of freedom to control static ***,we observed giant photoinduced resistance jumps with striking features:(1)a single resistance jump occurs upon a linearly polarized light incident with a chosen polarization angle,and a second resistance jump occurs when the polarization angle changes;(2)the amplitude of the second resistance jump depends sensitively on the actual change of the polarization *** transmittance measurements reveal that the origin of the above phenomena is closely related to the coexistence of anisotropic *** results represent a first step to utilize light polarization as an active knob to manipulate static phase transitions,pointing towards new pathways for nonvolatile optoelectronic devices and sensors.

关键词： Metal-insulator phase transitions Polarization of light Electronic phase separation Selective domain controllability

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Multi-performance evaluation of high-throughput accelerated corrosion test for high-strength low-alloy 921A steel

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Journal of Iron and Steel research International 2024年第5期31卷 1260-1278页

作者： Cong-cong Du Ming-hua Qin Zhan-fang Wu Dong-ling Li Lei Zhao Xiang-yang Li Hai-zhou Wang Beijing Advanced innovation center for Materials Genome Engineering National Center for Materials Service SafetyUniversity of Science and Technology BeijingBeijing100083China China Iron and Steel research Institute Group Co. Ltd.Beijing100081China Beijing Advanced innovation center for Materials Genome Engineering Central Iron and Steel Research InstituteBeijing100081China

The corrosion behavior of high-strength low-alloy 921A steel in a simulated marine atmospheric environment was studied using a high-throughput experimental *** corrosion behavior,corrosion morphology,and corrosion products of 921A steels were analyzed using various techniques,including corrosion mass loss method,polarization curve,white-light interferometry,scanning electron microscopy,energy-dispersive spectrometry,microbeam X-ray fluorescence spectrometry,X-ray diffraction technique,and X-ray photoelectron *** test results indicated that 921A steel exhibits better corrosion resistance than Q450NQR1 steel in simulated harsh atmospheric environments,as evidenced by a lower corrosion mass loss rate throughout the corrosion *** corrosion products of both steels consisted ofα-FeOOH,Fe_(3)O_(4),andγ-FeOOH,withα-FeOOH being more prevalent in the rust layer of 921A steel than in Q450NQR1 *** inner rust layer of 921A steel also exhibited an appositional enrichment region of Cr,Ni,Mo,and V,leading to its superior corrosion resistance compared to that of Q450NQR1 *** efficacy of high-throughput accelerated corrosion experimental methods was highlighted for evaluating the corrosion resistance of steel materials in harsh environmental *** findings suggest that 921A steel exhibits better corrosion resistance compared to Q450NQR1 steel and has the potential to be more suitable in harsh marine atmospheric *** characterization of the rust layer structures and composition reveals the parallel enrichment of certain elements in the inner rust layer of 921A steel,which enhances its corrosion resistance.

关键词： Atmospheric corrosion High-throughput experimental method High-strength low-alloy steel Corrosion characteristics Rust layer Element enrichment

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Higher-order properties and extensions for indirect MRAC and APPC of linear systems

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Science China(Information Sciences) 2024年第4期67卷 218-238页

作者： Yanjun ZHANG Zhipeng ZHANG Jian SUN Lei WANG Kangkang ZHANG National Key Lab of Autonomous Intelligent Unmanned Systems Beijing Institute of Technology Beijing Institute of Technology Chongqing innovation center College of Control Science and Engineering Zhejiang University Department of Electrical and Electronic Engineering Imperial College London KIOS research and innovation center of Excellence University of Cyprus

Recently, a reference derived some new higher-order output tracking properties for direct model reference adaptive control(MRAC) of linear time-invariant(LTI) systems: limt→∞ e~((i))(t) = 0, i = 1,..., n~*-1, where n~* and e~((i))(t) denote the relative degree of the system and the i-th derivative of the output tracking error, respectively. However, a naturally arising question involves whether indirect adaptive control(including indirect MRAC and indirect adaptive pole placement control) of LTI systems still has higher-order tracking properties. Such properties have not been reported in the literature. Therefore, this paper provides an affirmative answer to this question. Such higher-order tracking properties are new discoveries since they hold without any additional design conditions and, in particular, without the persistent excitation condition. Given the higher-order properties, a new adaptive control system is developed with stronger tracking features.(1) It can track a reference signal with any order derivatives being unknown.(2) It has higher-order exponential or practical output tracking properties.(3) Finally, it is different from the usual MRAC system, whose reference signal’s derivatives up to the n~* order are assumed to be known. Finally, two simulation examples are provided to verify the theoretical results obtained in this paper.

关键词： higher-order tracking indirect adaptive control model reference adaptive control adaptive pole placement control

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Photophysical Properties and Photovoltaic Performance of Sensitizers with a Bipyrimidine Acceptor

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Transactions of Tianjin University 2024年第5期30卷 406-418页

作者： Shiling Liu Kun Gong Wei Li Dongzhi Liu Xueqin Zhou School of Chemical Engineering and Technology Collaborative Innovation Center of Chemical Science and Engineering Tianjin Engineering Research Center of Functional Fine Chemicals Tianjin University

Molecular engineering is a crucial strategy for improving the photovoltaic performance of dye-sensitized solar cells（DSSCs）. Despite the common use of the donor–π bridge–acceptor architecture in designing sensitizers, the underlying structure–performance relationship remains not fully understood. In this study, we synthesized and characterized three sensitizers: MOTP-Pyc, MOS2P-Pyc, and MOTS2P-Pyc, all featuring a bipyrimidine acceptor. Absorption spectra, cyclic voltammetry, and transient photoluminescence spectra reveal a photo-induced electron transfer（PET） process in the excited sensitizers. Electron spin resonance spectroscopy confirmed the presence of charge-separated states. The varying donor and π-bridge structures among the three sensitizers led to differences in their conjugation effect, influencing light absorption abilities and PET processes and ultimately impacting the photovoltaic performance. Among the synthesized sensitizers, MOTP-Pyc demonstrated a DSSC efficiency of 3.04%. Introducing an additional thienothiophene block into the π-bridge improved the DSSC efficiency to 4.47% for MOTS2P-Pyc. Conversely, replacing the phenyl group with a thienothiophene block reduced DSSC efficiency to 2.14% for MOS2P-Pyc. Given the proton-accepting ability of the bipyrimidine module, we treated the dye-sensitized TiO2photoanodes with hydroiodic acid（HI）, significantly broadening the light absorption range. This treatment greatly enhanced the short-circuit current density of DSSCs owing to the enhanced electron-withdrawing ability of the acceptor. Consequently, the HI-treated MOTS2P-Pyc-based DSSCs achieved the highest power conversion efficiency of 7.12%, comparable to that of the N719 dye at 7.09%. This work reveals the positive role of bipyrimidine in the design of organic sensitizers for DSSC applications.

关键词： Acidichromic property Bipyrimidine acceptor Charge separation Dye-sensitized solar cells Molecular engineering Photophysical processes

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Optimizing Sorghum Productivity Using Balanced Fertilizers on Dryland

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Phyton-International Journal of Experimental Botany 2024年第7期93卷 1403-1420页

作者： Samijan Samijan Endah Nurwahyuni Sri Minarsih Agus Supriyo Sodiq Jauhari Yulis Hindarwati Meinarti Norma Setiapermas Raden Heru Praptana Endah Winarni Vina Eka Aristya research center for Food Crops Research Organization for Agriculture and FoodNational Research and Innovation Agency(BRIN)Cibinong Science CenterJl.Raya Jakarta-Bogor Km.46Bogor16911Indonesia

Sorghum is theﬁfth most required cereal crop *** bicolor has the advantage of being adaptive to both lowland and dryland,with drought-tolerant and wide *** low nutrient availability in dryland requires additional effective fertilizers to increase sorghum *** research aimed to assess the appli-cation of organic,inorganic,and biofertilizers for sorghum productivity on *** in Central Java,Indonesia as dryland sorghum areas,from November 2022 to February *** experiment cooperates with the farmers in a split-plot design,the main plot was two varieties and subplots of four *** enhanced sorghum yield(21.38%–36.06%)with combined fertilizer was greater than the existing *** con-trol does not rely on inorganic fertilizers but also on applying *** sorghum farming economic value farming indicated that combinations of fertilizer treatments and varieties provide beneﬁts of USD 929.81–1955.81 with a revenue-cost ratio(R/C)value>*** is an essential food commodity that faces the threat of the global crisis and an unfavorable *** study indicated balanced fertilizers could provide sufﬁ-cient nutrients to the soil and increase nutrient absorption availability for sorghum growth and *** fertilization increases the uptake of N,P,and K nutrients correlates with an increase in yield of 21.38%–36.06%.

关键词： Biofertilizer dryland adaptability economic value sorghum potential yield

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OSDA-free synthesis of FeZSM-22 zeolite from natural minerals for n-octane hydroisomerization

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Chinese Journal of Chemical Engineering 2024年第2期66卷 51-59页

作者： Tiesen Li Ting Chen Yinghui Ye Peng Dong TinghaiWang Qingyan Cui Chan Wang Yuanyuan Yue National Engineering research center of Chemical Fertilizer Catalyst College of Chemical EngineeringFuzhou UniversityFuzhou 350002China Qingyuan innovation Laboratory Quanzhou 362801China

A seed-directed approach to synthesizing Fe ZSM-22 zeolite without organic structure directing agent(OSDA)was developed by using Fe-rich diatomite as all aluminum and iron *** Fe ZSM-22zeolite with optimal crystallinity and purity can be obtained by systematically adjusting feed composition and synthesis *** show that Fe ZSM-22 zeolite synthesized with OSDA-free owns high crystallinity,obvious thin needle-shaped morphology and high Bronsted/Lewis acid ***,when used for n-octane hydroisomerization reaction,its derived catalyst exhibits the best catalytic performance reflected by the highest selectivity to C_(8)isomers compared to the two reference catalysts prepared based on a Fe-containing and a Fe-free ZSM-22 synthesized through an OSDA-directed route from natural diatomite and conventional chemicals,*** work provides an alternative route to sustainably synthesizing heteroatomic zeolites with high performance.

关键词： FeZSM-22 zeolite OSDA-free synthesis Natural minerals n-octane hydroisomerization

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Assessment of corrected time-step method for nominal ionospheric gradient calculation: A comparative analysis with spatial approaches

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Earth and Planetary Physics 2024年第4期8卷 641-649页

作者： Slamet Supriadi Prayitno Abadi Susumu Saito Harry Bangkit Dwiko Unggul Prabowo Adi Purwono Ginaldi Ari Nugroho research center for Smart Mechatronics National Research and Innovation Agency(BRIN)BandungIndonesia research center for Climate and Atmosphere BRINBandungIndonesia School of Electrical Engineering Telkom UniversityKab.BandungIndonesia Electronic Navigation research Institute National Institute of MaritimePort and Aviation TechnologyTokyoJapan research center for Space BRINBandungIndonesia

The effect of ionospheric delay on the ground-based augmentation system under normal conditions can be mitigated by determining the value of the nominal ionospheric gradient(σvig).The nominal ionospheric gradient is generally obtained from Continuously Operating Reference Stations data by using the spatial single-difference method(mixed-pair,station-pair,or satellite-pair)or the temporal single-difference method(time-step).The time-step method uses only a single receiver,but it still contains ionospheric temporal *** introduce a corrected time-step method using a fixed-ionospheric pierce point from the geostationary equatorial orbit satellite and test it through simulations based on the global ionospheric *** also investigate the effect of satellite paths on the corrected time-step method in the region of the equator,which tends to be in a more north–south direction and to have less coverage for the east–west ionospheric *** study also addresses the limitations of temporal variation correction coverage and recommends using only the correction from *** processes are developed under simulations because observational data are still difficult to *** findings demonstrate that the corrected time-step method yieldsσvig values consistent with other approaches.

关键词： ground-based augmentation system nominal ionospheric gradient time-step correction global ionospheric model

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Inhibition of protein degradation increases the Bt protein concentration in Bt cotton

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Journal of Integrative Agriculture 2024年第6期23卷 1897-1909页

作者： Yuting Liu Hanjia Li Yuan Chen Tambel Leila.I.M Zhenyu Liu Shujuan Wu Siqi Sun Xiang Zhang Dehua Chen Jiangsu Key Laboratory of Crop Genetics and Physiology/Co-innovation center for Modern Production Technology of Grain Crops Yangzhou UniversityYangzhou 225009China Agricultural research Cooperation Biotechnology and Biosafety Research CenterKhartoum 13314Sudan

Bacillus thuringiensis(Bt)cotton production is challenged by two main problems,i.e.,the low concentration of Bt protein at the boll setting stage and the lowest insect resistance in bolls among all the cotton plant’s ***,increasing the Bt protein concentration at the boll stage,especially in bolls,has become the main goal for increasing insect resistance in *** this study,two protein degradation inhibitors(ethylene diamine tetra acetic acid(EDTA)and leupeptin)were sprayed on the bolls,subtending leaves,and whole cotton plants at the peak flowering stage of two Bt cultivars(medium maturation Sikang 1(SK1))and early maturation Zhongmian 425(ZM425)in 2019 and *** Bt protein content and protein degradation metabolism were *** results showed that the Bt protein concentrations were enhanced by 21.3 to 38.8%and 25.0 to 38.6%in the treated bolls of SK1 and ZM425 respectively,while they were decreased in the subtending leaves of these treated *** the treated leaves,the Bt protein concentrations increased by 7.6 to 23.5%and 11.2 to 14.9%in SK1 and ZM425,*** combined application of EDTA and leupeptin to the whole cotton plant increased the Bt protein concentrations in both bolls and subtending *** Bt protein concentrations in bolls were higher,increasing by 22.5 to 31.0%and 19.6 to 32.5%for SK1 and ZM425,*** organs treated with EDTA or/and leupeptin showed reduced free amino acid contents,protease and peptidase activities and significant enhancements in soluble protein *** results indicated that inhibiting protein degradation could improve the protein content,thus increasing the Bt protein concentrations in the bolls or/and leaves of cotton ***,the increase in the Bt protein concentration without yield reduction suggested that these two protein degradation inhibitors may be applicable for improving insect resistance in cotton production.

关键词： Bt cotton Bt protein inhibition of protein degradation protein degradation metabolism

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EBSD analysis of grain boundary evolution and dynamic recrystallization of Inconel 625 superalloy at various hot spinning feed rates

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Progress in Natural Science:Materials International 2024年第1期34卷 56-65页

作者： Zhanjie Jing Jiangkun Fan Xudong Liu Yuelin Song Zixiao Wang Kai Cao Yuetan Chen Heng Fu Jianing Zhang Jinshan Li State Key Laboratory of Solidification Processing Northwestern Polytechnical University Chongqing innovation center Northwestern Polytechnical University National&Local Joint Engineering research center for Precision Thermoforming Technology of Advanced Metal Materials

Hot spinning can make the material withstand shear stress, so that the shape of the material has a great change,which is one of the main processing methods of nickel-based alloy plate members. Inconel 625 alloy, which has excellent high temperature mechanical properties and can be used as the main candidate material for aerospace applications, needs further study on its hot spinning deformation behavior and deformation mechanism. In this paper, the effect of feed rate on the microstructure evolution of Inconel 625 superalloy was studied by the electron backscattered diffraction technology. The microstructure with necklace-like structures composed of dynamic recrystallization(DRX) grains was observed after hot spinning. It was found that at the low feed rate, the promotion of DRX degree and grain refinement happened, where the grain size reached the trough of 10.99 μm under a feed rate of 300 mm/min. However, with the further feed rate rising, the degree of DRX was suppressed to a certain extent and grain size increased to 14.26 μm. On balance, the feed rate of 300 mm/min was the most efficient condition for grain refinement. Besides, it was revealed that both discontinuous dynamic recrystallization(DDRX) and continuous dynamic recrystallization(CDRX) occurred during hot spinning. DDRX includes the initial grain boundary nucleation by bulging and the annealing twin boundary assisted nucleation, while the CDRX mechanism is related to the continuous subgrain rotation within the deformed grain. DDRX is the main DRX mechanism.

关键词： Inconel 625 superalloy Hot spinning Grain boundary evolution DRX mechanism

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Effects of prebiotics on the fermentation of traditional suancai of Northeast China

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Food Science and Human Wellness 2024年第3期13卷 1358-1367页

作者： Mingwei Zhao Xinying Cao Yuzheng Wu Sibo Zou Zhigao Li Xinping Lin Chaofan Ji Liang Dong Sufang Zhang Chenxu Yu Huipeng Liang National Engineering research center of Seafood Collaborative Innovation Center of Provincial and Ministerial Co-construction for Deep ProcessingCollaborative Innovation Center of Seafood Deep ProcessingSchool of Food Science and TechnologyDalian Polytechnic UniversityDalian 116034China Department of Agricultural and Biosystems Engineering Iowa State UniversityIA 50011USA

Suancai is a traditional fermented vegetable widely consumed in Northeast *** this study,different prebiotics were used to improve the quality of *** prebiotics(inulin(INU),xylooligosaccharide(XO S),galactooligosaccharide(GOS),and stachyose(STA))were shown to reduce the pH value and increase the content of total titratable acidity(TTA)in suancai,while the contents of most organic acids were also *** addition of prebiotics had significant effects on the bacterial microbiota during the suancai fermentation *** prebiotics were shown to contribute to the growth of *** suancai sample with fructooligosaccharides(FOS)had the highest relative abundance of ***,INU and XOS could increase the abundance of *** evaluate the quality of suancai fermented with prebiotics,profiles of volatile flavor compounds(VOCs)and free amino acids(FAA)were *** prebiotics affected the VOCs and FAA profiles via transforming the bacterial *** addition,the addition of prebiotics also changed the taste profiles of the suancai *** study is among the first attempts to reveal the effects of different prebiotics on suancai fermentation,and the findings provide a foundation to develop new ways for improving the quality of suancai.

关键词： Bacterial microbiota Lactic acid bacteria Flavor Amino acid Taste

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