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Innovative Mn3-xO4-y@NCA design:Leveraging Mn/O vacancies and amorphous architecture for enhanced sodium-ion storage

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Journal of Energy Chemistry 2024年第10期97卷 747-756页

作者： Kaijun Xie Xin Liu Kai Xia Lipeng Diao Ping Lu Mengmeng Wang Long Fang Yihui Zou Dongjiang Yang Xiaodong Zhang College of Chemistry and Chemical Engineering College of Environmental Science and Engineering State Key Laboratory of Bio-fibers and Eco-textiles Shandong Collaborative Innovation Center of Marine Biobased Fibers and Ecological Textiles Institute of Marine Biobased Materials Qingdao University Institute of Micro/Nano Materials and Devices Ningbo University of Technology

Manganese-based oxide electrode materials suffer from severe Jahn-Teller（J-T） distortion,leading to severe cycle instability in sodium ion ***,it is difficult to adjust the electron at d orbitals exactly to a low spin state to eliminate orbital degeneracy and suppress J-T distortion *** article constructed concentration-controllable Mn/O coupled vacancy and amorphous network in Mn3O4and coated it with nitrogen-doped carbon aerogel(Mn3-xO4-y@NCA).The existence of Mn/O vacancies has been confirmed by scanning transmission electron microscopy（STEM） and positron annihilation lifetime spectroscopy（PALS）.Atomic absorption spectroscopy（AAS） and X-ray photoelectron spectroscopy（XPS） determine the most optimal ratio of Mn/O vacancies for sodium ion storage is 1:*** functional theory（DFT） calculations prove that Mn/O coupled vacancies with the ratio of 1:2could exactly induce a low spin states and a d4electron configuration of Mn,suppressing the J-T distortion *** abundant amorphous regions can shorten the transport distance of sodium ions,increase the electrochemically active sites and improve the pseudocapacitance *** the synergetic effect of Mn/O coupled vacancies and amorphous regions,Mn3-xO4-y@NCA exhibits an energy density of 37.5 W h kg-1and an ultra-high power density of 563 W kg-1in an asymmetric *** sodium-ion batteries,it demonstrates high reversible capacity and exceptional cycling *** research presents a new method to improve the Na+storage performance in manganese-based oxide,which is expected to be generalized to other structural distortion.

关键词： Amorphous network Concentration-controllable Mn/O coupled vacancies Manganese-based metal oxide Sodium ion battery Sodium ion supercapacitor

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Assessment of Seasonal Rainfall Prediction in Ethiopia: Evaluating a Dynamic Recurrent Neural Network to Downscale ECMWF-SEAS5 Rainfall

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Advances in Atmospheric Sciences 2024年第11期 2230-2244页

作者： Abebe KEBEDE Kirsten WARRACH-SAGI Thomas SCHWITALLA Volker WULFMEYER Tesfaye ABEBE Markos WARE Hawassa University College of Agriculture Arba Minch University Water Institute of Technology Faculty of Meteorology and Hydrology Institute of Physics and meteorology University of Hohenheim

Seasonal rainfall plays a vital role in both environmental dynamics and decision-making for rainfed agriculture in Ethiopia, a country often impacted by extreme climate events such as drought and flooding. Predicting the onset of the rainy season and providing localized rainfall forecasts for Ethiopia is challenging due to the changing spatiotemporal patterns and the country's rugged topography. The Climate Hazards Group Infra Red Precipitation with Station Data(CHIRPS), ERA5-Land total precipitation and temperature data are used from 1981–2022 to predict spatial rainfall by applying an artificial neural network(ANN). The recurrent neural network(RNN) is a nonlinear autoregressive network with exogenous input(NARX), which includes feed-forward connections and multiple network layers, employing the Levenberg Marquart algorithm. This method is applied to downscale data from the European Centre for Medium-range Weather Forecasts fifth-generation seasonal forecast system(ECMWF-SEAS5) and the Euro-Mediterranean Centre for Climate Change(CMCC) to the specific locations of rainfall stations in Ethiopia for the period 1980–2020. Across the stations, the results of NARX exhibit strong associations and reduced errors. The statistical results indicate that, except for the southwestern Ethiopian highlands, the downscaled monthly precipitation data exhibits high skill scores compared to the station records, demonstrating the effectiveness of the NARX approach for predicting local seasonal rainfall in Ethiopia's complex terrain. In addition to this spatial ANN of the summer season precipitation, temperature, as well as the combination of these two variables, show promising results.

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Experimental clearance rate and intraguild predation of jellyfish Cyanea nozakii

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Journal of Oceanology and Limnology 2024年第1期42卷 128-140页

作者： Pengpeng WANG Fang ZHANG Song SUN Shuguo LÜ CAS Key Laboratory of marine Ecology and Environmental Sciences Institute of OceanologyChinese Academy of SciencesQingdao 266071China Laboratory for marine Ecology and Environmental Sciences Pilot National Laboratory for Marine Science and Technology(Qingdao)Qingdao 266237China University of Chinese Academy of Sciences Beijing 100049China Jiaozhou Bay marine Ecosystem Research Station Chinese Academy of SciencesQingdao 266071China center for Ocean Mega-Science Chinese Academy of SciencesQingdao 266071China Institute of marine Ecology and Environment Hainan Academy of Environmental SciencesHaikou 570100China

Cyanea nozakii,a common jellyfish distributed in offshore China,has a complex trophic relationship with other zooplankton ***,few studies have reported the predation rates and prey selection patterns of *** medusae on different prey *** is also lacking on the intraguild predation of Aurelia coerulea(another common bloom jellyfish in offshore China)by *** address the knowledge gaps,the clearance rates of *** for different prey items,including copepods(small1000μm),fish larvae,and gelatinous prey(hydromedusae,*** ephyrae,and chaetognaths),were *** influence of predator size on the clearance rate was also ***,we examined the intraguild predation of *** on *** *** clearance rates of *** varied widely with prey organisms,being independent of prey *** organisms,except for chaetognaths,were captured with considerably high efficiency,followed by fish larvae and copepods,indicating the preferential prey selection of gelatinous organisms by *** clearance rate increased linearly with the cross-sectional area of *** size in medusae may,to some extents,underpin their capacity to capture more prey by increasing the encounter rate and capture success through *** preyed voraciously on *** in high feeding efficiency,but the clearance rate decreased with increasing ***(as prey)*** phenomenon of intraguild predation suggests a speculative hypothesis of potential population regulation of *** by *** information regarding the feeding ecology of *** reported in this study is important for understanding plankton dynamics in marine ecosystems with extensive occurrences of this jellyfish.

关键词： Scyphomedusae predation rate gelatinous organisms prey selection feeding mechanism

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Photoelectrocatalytic hydrogen evolution and synchronous degradation of organic pollutants by pg-C_(3)N_(4)/β-FeOOH S-scheme heterojunction

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Science China(Technological Sciences) 2024年第4期67卷 1238-1252页

作者： LI XiBao HAN Tao ZHOU YingTang XIE Yu LUO YiDan HUANG JunTong CHEN Zhi DENG Fang School of Materials Science and Engineering Nanchang Hangkong UniversityNanchang 330063China National-Local Joint Engineering Research center of Heavy Metal Pollutants Control and Resource Utilization Nanchang Hangkong UniversityNanchang 330063China Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316022China

Crafting photoelectrocatalytic materials with robust oxidation-reduction properties for simultaneous hydrogen evolution and pollutant degradation poses a formidable *** this study,a pg-C_(3)N_(4)/β-FeOOH S-scheme heterostructure with a special energy band structure was developed by anchoring porous pg-C_(3)N_(4)on needle shapedβ-*** as a hole extraction layer,needle-leaf-likeβ-FeOOH can facilitate efficient hole migration and enhance charge ***,the optimized 0.2-pg-C_(3)N_(4)/β-FeOOH could degrade 78%of ofloxacin(OFLO)in 90 *** organic pollutants could absorb a large number of holes,which prompted a greater proportion of photogenerated electrons to actively participate in the hydrogen evolution reaction at the ***,the hydrogen production of 0.2-pg-C_(3)N_(4)/β-FeOOH reached 1452.88μmol cm^(-2)h^(-1),exhibiting a notable increase of 61.81-165.12μmol cm^(-2)h^(-1)compared with that in the absence of *** and theoretical calculation results underscore that this investigation is grounded in a distinctive electron and hole dual channel transfer *** findings offer novel insights for the future development of S-scheme heterojunction photoelectrocatalytic materials capable of concurrently degrading pollutants and promoting hydrogen evolution.

关键词： photoelectrocatalysis hydrogen evolution degradation synchronous S-scheme heterojunction

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First-Arrival Picking Method for Active Source Data with Ocean Bottom Seismometers Based on Spatial Waveform Variation Characteristics

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Journal of Ocean University of China 2024年第4期23卷 970-980页

作者： LIU Hongwei XING Lei ZHU Henghua ZHANG Jin ZHANG Jing LIU Huaishan Key Laboratory of Submarine Geosciences and Prospecting Techniques Ministry of EducationCollege of Marine GeosciencesOcean University of ChinaQingdao 266100China Laboratory for marine Mineral Resources Qingdao Marine Science and Technology CenterQingdao 266071China College of Underwater Acoustic Engineering Harbin Engineering UniversityHarbin 150001China Shandong Institute of Geological Survey Jinan 250014China

The precision and reliability of first-arrival picking are crucial for determining the accuracy of geological structure inversion using active source ocean bottom seismometer(OBS)refraction *** methods for first-arrival picking based on sample points are characterized by theoretical errors,especially in low-sampling-frequency OBS data because the travel time of seismic waves is not an integer multiple of the sampling *** this paper,a first-arrival picking method that utilizes the spatial waveform variation characteristics of active source OBS data is ***,the distribution law of theoretical error is examined;adjacent traces exhibit variation characteristics in their ***,a label cross-correlation superposition method for extracting highfrequency signals is presented to enhance the first-arrival picking *** from synthetic and field data verify that the proposed approach is robust,successfully overcomes the limitations of low sampling frequency,and achieves precise outcomes that are comparable with those of high-sampling-frequency data.

关键词： first-arrival picking spatial waveform variation label cross-correlation superposition method

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Compound events of heatwave and dust storm in the Taklamakan Desert

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Science China Earth Sciences 2024年第7期67卷 2073-2083页

作者： Yuzhi LIU Jianping HUANG Ziyuan TAN Chenglong ZHOU Dan LI Yongkun XIE Key Laboratory for Semi-Arid Climate Change of the Ministry of Education Lanzhou UniversityLanzhou 730000China Collaborative Innovation center for Western Ecological Safety Lanzhou UniversityLanzhou 730000China Taklamakan National Station of Observation and Research for Desert meteorology in Xinjiang Urumqi 830002China

Taklamakan Desert(TD)has been characterized by numerous heatwaves and dust storms,leading to negative effects on societies and ecosystems at regional and global ***,the association between heatwaves and dust storms is poorly *** this study,we describe the association between heatwaves and dust events and propose a mechanism for such compound events in the *** results show that,from 1993 to 2022,the frequency and intensity of heatwaves in the TD have increased at a rate of 0.21 days year^(-1)and 0.02℃ year^(-1),*** than 40% of heatwaves existed with dust events,which significantly lagged behind ***,the higher the air temperature,the hotter and drier the soil,leading to more dust emissions in the *** high-occurrence heatwave years,a large-scale wave train of“cyclone-anticyclone-cyclone”in the northwest-southeast direction was found,with the anticyclone of which hovered over the TD *** anomalous anticyclones favored the formation and maintenance of heatwaves,and subsequent anomalous cyclones in the wave train triggered strong dust events followed by *** climate warming,the compound events of heatwave and dust storm are becoming bigger hazards threatening the socioeconomic and ecological security in the TD,the profound study of which is critical to understanding regional extreme responses.

关键词： Heatwave Dust storm Compound events Taklamakan Desert

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Acoustic Velocity-Based Inversion of the Physical Properties of Sea Ice in the Central Arctic Region

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Journal of Ocean University of China 2024年第5期23卷 1213-1220页

作者： KONG Yadong XING Junhui XU Haowei XU Chong Key Laboratory of Submarine Geosciences and Prospecting Techniques Ministry of Education (MOE) and College of Marine Geosciences Ocean University of China Laboratory for marine Mineral Resources Qingdao Marine Science and Technology Center

Studying the Arctic sea ice contributes to a comprehensive understanding of the climate system in polar regions and offers valuable insights into the interplay between polar climate change and the global climate and environment. One of the key research aspects is the investigation of the temperature, salinity, and density parameters of sea ice to obtain essential insights. During the 11th Chinese National Arctic Research Expedition, acoustic velocity was measured on an ice core at a short-term ice station, however, temperature, salinity, and density were not measured. In the present work, we utilized a genetic algorithm to invert these obtained acoustic velocity data to sea ice temperature, salinity, and density parameters on the basis of the relationship between acoustic velocity and the physical properties of Arctic summer sea ice. We validated the effectiveness of this inversion procedure by comparing its findings with those of other researchers. The results indicate that within the normalized depth range of 0.43 – 0.94, the ranges for temperature, salinity, and density are-0.48 –-0.29℃, 1.63 – 3.35, and 793.1 – 904.1 kg m-3, respectively.

关键词： acoustic velocity Arctic sea ice genetic algorithm inversion of sea ice properties

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Influence of preheating treatments on cyanide content， nutritional composition， physicochemical properties， color and oxidative stability of flaxseed meal

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中国油脂 2024年

作者： ZHOU Junzhuo CHU Pengfei DONG Guimei PEI Xuechen HUANG Jiaqian ZHENG Rui YIN Fawen ZHOU Dayong SKL of marine Food Processing & Safety Control， National Engineering Research center of Seafood， Collaborative Innovation center of Seafood Deep Processing， Liaoning Province Key Laboratory for marine Food Science and Technology， School of Food Science and Technology， Dalian Polytechnic University

This study aimed to investigate the effects of different preheating treatments （steaming， roasting and microwave） of flaxseed on cyanide content， nutritional composition， physicochemical properties， color and oxidative stability of flaxseed meal. The three preheating methods of flaxseed all significantly decreased the hydrocyanic acid （HCN） contents. By contrast， microwave was the most effective detoxification method. After 5 min of microwave treatment， the HCN content in flaxseed was reduced from 94.65 ± 1.68 mg/kg to 7.80 ± 0.57 mg/kg. In addition， the three preheating methods all significantly increased the polyphenol content， thiobarbituric acid reactive substances （TBARS）， peroxide value （POV）， and a*value， and slightly decreased polyunsaturated fatty acid （PUFA） contents， but significantly decreased total amino acid contents as well as L*， W*and b*values. Interestingly， the three preheating methods all improved the oxidative stability and color stability of flaxseed upon accelerated storage under 40 °C. Compared with steaming （120 ℃ for 20 min） and roasting （100 ℃ for 40 min）， microwave （560 W for 4 min） is recommended for decreasing cyanide content， as well as enhancing the flaxseed' stability and qualitative attributes.

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Storage and redistribution of anthropogenic CO_(2) in the western North Pacific:The role of subtropical mode water transportation

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Fundamental Research 2024年第1期4卷 103-112页

作者： Cheng-long Li Lei Han Wei-dong Zhai Di Qi Xu-chen Wang Hong-mei Lin Li-wen Zheng Institute of marine Science and Technology Shandong UniversityQingdao 266237China China-ASEAN College of marine Science and Technology Xiamen University MalaysiaSelangorMalaysia Southern marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai 519080China Polar and marine Research Institute Jimei UniversityXiamen 361021China Key Laboratory of marine Chemistry Theory and Technology and Frontiers Science Center for Deep Ocean Multispheres and Earth SystemMinistry of EducationOcean University of ChinaQingdao 266100China center for Isotope Geochemistry and Geochronology Pilot National Laboratory for Marine Science and Technology(Qingdao)Qingdao 266237China Weihai Institute of marine Ecology and Economy Research Weihai 264400China

Oceanic uptake and storage of anthropogenic CO_(2)(CANT)are regulated by ocean circulation and *** decipher the storage and redistribution of CANT in the western North Pacific,where a major CANT sink develops,we investigated the water column carbonate system,dissolved inorganic radiocarbon and ancillary parameters in May and August 2018,spanning the Kuroshio Extension(KE,35-39°N),Kuroshio Recirculation(KR,27-35°N)and subtropical(21-27°N)*** column CANT inventories were estimated to be 40.5±1.1 mol m^(-2) in the KR zone and 37.2±0.9 mol m^(-2) in the subtropical *** comparison with historical data obtained in 2005,relatively high rates of increase of the CANT inventory of 1.05±0.20 and 1.03±0.12 mol m^(-2) yr^(-1) in the recent decade were obtained in the KR and subtropical zones,*** water-mass-based analyses suggest that formation and transport of subtropical mode water dominate the deep penetration,storage,and redistribution of CANT in those two *** the KE zone,however,both the water column CANT inventory and the decadal CANT accumulation rate were small and uncertain owing to the dynamic hydrology,where the naturally uplifting isopycnal surfaces make CANT penetration relatively *** findings of this study improve the understanding of the spatiotemporal variations of CANT distribution,storage,and transport in the western North Pacific.

关键词： Oceanic CO_(2)uptake Anthropogenic CO_(2)storage Subtropical mode water Kuroshio extension Kuroshio recirculation Western North Pacific

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Proteomic response of Phaeocystis globosa to nitrogen limitation

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Journal of Oceanology and Limnology 2024年第1期42卷 141-149页

作者： Haisu LIU Ruiwang WEI Qiangyong LEI Lei CUI Songhui LÜ Key Laboratory of Eutrophication and Red Tide Prevention Research Center for Harmful Algae and Marine BiologyJinan UniversityGuangzhou 510632China Southern marine Science and Engineering Guangdong Laboratory Zhuhai 519082China National Engineering Laboratory of Electronic and Information Standardization Shenzhen 518057China

Phaeocystis globosa is an important unicellular eukaryotic alga that can also form *** can cause massive harmful algal blooms and plays an important role in the global carbon or sulfur *** far,the ecophysiology of *** has been investigated by numerous ***,the proteomic response of *** to nitrogen depletion remains largely *** compared four protein preparation methods of *** for two-dimensional electrophoresis(2-DE)(Urea/Triton X-100 with trichloroacetic acid(TCA)/acetone precipitation;TCA/acetone precipitation;Radio Immuno Precipitation Assay(RIPA)with TCA/acetone precipitation;and Tris buffer).Results show that the combination of RIPA with TCA/acetone precipitation had a clear gel background and showed the best protein spot separation effect,based on which the proteomic response to nitrogen depletion was studied using *** addition,we identified six differentially expressed proteins whose relative abundance increased or decreased more than 1.5-fold(Pmarine microalgae.

关键词： Phaeocystis globosa nitrogen limitation proteomic response two-dimensional electrophoresis

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