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Atomization characteristics of pyrolysis oil derived from waste tires

Waste Disposal and Sustainable energy 2024年第1期6卷 39-52页

作者： Hong Feng Zhitong Yin Qin Hong Yiming Hu Lintao Liu Jun Wang Qunxing Huang Yonggang Zhou ZJMI environmental energy Co. LtdHangzhou310003China Tongxiang Taiaisi environmental protection energy Co. Ltd.Jiaxing314500China State Key Laboratory of Clean energy Utilization Zhejiang UniversityHangzhou310027China Key Laboratory of Clean energy and Carbon Neutrality of Zhejiang Province Jiaxing Research InstituteZhejiang UniversityJiaxing314031China

The atomization characteristics play a key role in the highly efficient combustion of pyrolysis oil derived from waste *** this study,the fuel properties of tire pyrolysis oil(TPO)were initially studied,and then a high-speed camera and a phase Doppler particle analyzer were employed to characterize the atomization feature of *** influence of pressure and nozzle orifice diameter on atomization characteristics such as spray angle,droplet velocity,and droplet size distribution was *** results showed that TPO had a high calorific value of about 43.6 MJ/kg and a low viscosity of 3.84×10^(–6)m^(2)/s at 40℃,which made it have the potential to be used as an alternative *** pressure expanded the spray angle and extended the spray in both the axial and radial *** increasing pressure,spray angle and droplet velocity raised,and the increase in crushing effect of air reduced the Sauter mean diameter(SMD)of the *** obtain proper atomization quality for combustion,the pressure is expected to be higher than 1.25 *** increasing nozzle orifice diameter,droplet velocity increased,and the SMD of the droplets increased as well due to weakened crushing effect of the ***,the pressure must be increased to maintain the atomization quality when using a nozzle with a larger *** to the lower viscosity,the velocity and particle size distribution of TPO droplets after atomization were smaller than those of diesel *** extremely small carbon black contained in TPO also contributed to the breaking of droplets and played a certain role in the size reduction of the oil droplets,but it may cause the risk of nozzle *** summary,TPO showed great atomization characteristics for alternative fuel applications.

关键词： Pyrolysis oil Atomization characteristics Spray angle Droplet velocity Droplet size distribution

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Facile low-temperature supercritical carbonization method to prepare high-loading nickel single atom catalysts for efficient photodegradation of tetracycline

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Journal of environmental Sciences 2024年第4期138卷 373-384页

作者： Han Qiao Lirong Zheng Shiwen Hu Gang Tang Hongri Suo Chongxuan Liu School of Environment Harbin Institute of TechnologyHarbin 150090China State environmental protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China Beijing Synchrotron Radiation Facility(BSRF) Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China

environmental photocatalysis is a promising technology for treating antibiotics in *** this study,a supercritical carbonization method was developed to synthesize a single-atom photocatalyst with a high loading of Ni(above 5 wt.%)anchored on a carbonnitrogen-silicate substrate for the efficient photodegradation of a ubiquitous environmental contaminant of tetracycline(TC).The photocatalyst was prepared from an easily obtained metal-biopolymer-inorganic supramolecular hydrogel,followed by supercritical drying and carbonization *** low-temperature(300℃)supercritical ethanol treatment prevents the excessive structural degradation of hydrogel and greatly reduces the metal clustering and aggregation,which contributed to the high Ni *** characterizations confirmed that Ni was present at isolated sites and stabilized by Ni-N and Ni-O bonds in a Ni-(N/O)_(6)-C/SiC configuration.A 5%Ni-C-Si catalyst,which performed the best among the studied catalysts,exhibited a wide visible light response with a narrow bandgap of 1.45 eV that could efficiently and repeatedly catalyze the oxidation of TC with a conversion rate of almost 100% within 40 *** reactive species trapping experiments and electron spin resonance(ESR)tests demonstrated that the h+,and·O_(2)-were mainly responsible for TC *** TC degradation mechanism and possible reaction pathways were provided ***,this study proposed a novel strategy to synthesize a high metal loading singleatom photocatalyst that can efficiently remove TC with high concentrations,and this strategy might be extended for synthesis of other carbon-based single-atom catalysts with valuable properties.

关键词： Carbon-based single-atom catalyst Nickel Photocatalytic degradation Tetracycline Visible light

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Feasibility of low-intensity ultrasound treatment with hydroxylamine to accelerate the initiation of partial nitrification and allow operation under intermittent aeration

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Journal of environmental Sciences 2024年第5期139卷 446-459页

作者： Jianxiong Jian Xiaojian Liao Zhihua Mo Shoupeng Li Lei Li Shaojin Chen Zhenhua Huang Junhao Chen Wencan Dai Shuiyu Sun Guangzhou Key Laboratory environmental Catalysis and Pollution Control Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlSchool of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangdong Province Solid Waste Recycling and Heavy Metal Pollution Control Engineering Technology Research center Guangdong Polytechnic of Environmental Protection EngineeringFoshan 528216China Analysis and Test center Guangdong University of TechnologyGuangzhou 510006China

Partial nitrification is a key aspect of efficient nitrogen removal,although practically it suf-fers from long start-up cycles and unstable long-term operational *** address these drawbacks,this study investigated the effect of low intensity ultrasound treatment combined with hydroxylamine(NH2OH)on the performance of partial *** showthat compared with the control group,low-intensity ultrasound treatment(0.10W/mL,15 min)combined with NH2OH(5 mg/L)reduced the time required for partial nitrification initiation by 6 days,increasing the nitrite accumulation rate(NAR)and ammonia nitro-gen removal rate(NRR)by 20.4% and 6.7%,respectively,achieving 96.48% ***-tic analysis showed that NH2OH enhanced ammonia oxidation,inhibited nitrite-oxidizing bacteria(NOB)activity and shortened the time required for partial nitrification ***,ultrasonication combined with NH2OH dosing stimulated EPS(extracellular polymeric substances)secretion,increased carbonyl,hydroxyl and amine functional group abundances and enhanced mass *** addition,16S rRNA gene sequencing results showed that ultrasonication-sensitive Nitrospira disappeared from the ultrasound+NH_(2)OH system,while Nitrosomonas gradually became the dominant ***,the results of this study provide valuable insight into the enhancement of partial nitrification start-up during the process of wastewater nitrogen removal.

关键词： Partial nitrification Low-intensity ultrasound Hydroxylamine Ammonia oxidizing bacteria Nitrite oxidizing bacteria

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Lithium Salt Combining Fluoroethylene Carbonate Initiates Methyl Methacrylate Polymerization Enabling Dendrite-Free Solid-State Lithium Metal Battery

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energy & environmental Materials 2024年第6期7卷 50-59页

作者： Xue Ye Jianneng Liang Baorong Du Yongliang Li Xiangzhong Ren Dazhuan Wu Xiaoping Ouyang Qianling Zhang Jianhong Liu institute of Process Equipment College of Energy EngineeringZhejiang UniversityHangzhou310000 China Graphene Composite Research center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen518061 China

This work demonstrates a novel polymerization-derived polymer electrolyte consisting of methyl methacrylate,lithium bis(trifluoromethanesulfonyl)imide and fluoroethylene *** polymerization of MMA was initiated by the amino compounds following an anionic catalytic *** plays both roles including the initiator and Li ion source in the polymer ***,lithium bis(trifluoromethanesulfonyl)imide has difficulty in initiating the polymerization reaction of methyl methacrylate monomer,a very high concentration of lithium bis(trifluoromethanesulfonyl)imide is needed for initiating the ***,the fluoroethylene carbonate additive can work as a supporter to facilitate the degree of dissociation of lithium bis(trifluoromethanesulfonyl)imide and increase its initiator capacity due to the high dielectric *** as-prepared poly-methyl methacrylate-based polymer electrolyte has a high ionic conductivity(1.19×10^(−3)S cm^(−1)),a wide electrochemical stability window(5 V vs Li^(+)/Li),and a high Li ion transference number(t_(Li^(+)))of 0.74 at room temperature(RT).Moreover,this polymerization-derived polymer electrolyte can effectively work as an artificial protective layer on Li metal anode,which enabled the Li symmetric cell to achieve a long-term cycling performance at 0.2 mAh cm^(−2)for 2800 *** LiFePO_(4)battery with polymerization-derived polymer electrolyte-modified Li metal anode shows a capacity retention of 91.17%after 800 cycles at 0.5 *** work provides a facile and accessible approach to manufacturing poly-methyl methacrylate-based polymerization-derived polymer electrolyte and shows great potential as an interphase in Li metal batteries.

关键词： in situ polymerization lithium anode polymer electrolyte solid-state lithium batteries

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Quantifying China's iron and steel industry's CO2 emissions and environmental health burdens:A pathway to sustainable transformation

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environmental Science and Ecotechnology 2024年第4期20卷 189-197页

作者： Weiling Wu Qian Tang Wenbo Xue Xurong Shi Dadi Zhao Zeyuan Liu Xin Liu Chunlai Jiang Gang Yan Jinnan Wang State environmental protection Key Laboratory of environmental Pollution and Greenhouse Gases Co-control Chinese Academy of Environmental PlanningBeijing100041China center of Air Quality Simulation and System Analysis Chinese Academy of Environmental PlanningBeijing100041China State environmental protection Key Laboratory of environmental Planning and Policy Simulation Chinese Academy of Environmental PlanningBeijing100041China College of environmental&Resource Sciences Zhejiang UniversityHangzhou310058China

Assessing the iron and steel industry's(ISI)impact on climate change and environmental health is vital,particularly in China,where this sector significantly influences air quality and CO_(2)*** is a lack of comprehensive analyses that consider the environmental and health burdens of manufacturing processes for ISI ***,we present an integrated emission inventory that encompasses air pollutants and CO_(2)emissions from 811 ISI enterprises and five key manufacturing processes in *** analysis shows that sintering is the primary source of air pollution in the *** contributes 71%of SO_(2),73%of NO_(x),and 54%of PM_(2.5)*** the other hand,81%of total CO_(2)emissions come from blast ***,the contributions of ISI have resulted in an increase of 3.6 mg m^(-3)in national population-weighted PM_(2.5)concentration,causing approximately 59,035 premature deaths in *** from Hebei,Jiangsu,Shandong,Shanxi,and Inner Mongolia provinces contributed to 48%of PM_(2.5)-related deaths in ***,the transportation of air pollutants across provincial borders highlights a concerning trend of environmental health *** on the research findings,it is crucial for ISI manufacturers to prioritize the removal of outdated production capacities and adopt energy-efficient and advanced techniques,along with ultra-low emission *** is particularly important for those manufacturers with substantial environmental *** transformative actions are essential in mitigating the environmental and health impacts in the affected regions.

关键词： Iron and steel industry CO_(2)emissions Air pollutants emissions environmental health

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A passive sampler for synchronously measuring inorganic and organic pollutants in sediment porewater:Configuration and field application

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Journal of environmental Sciences 2024年第2期136卷 201-212页

作者： Pei Lei Mingying Chen Nan Rong Wenzhong Tang Hong Zhang School of Environment Nanjing Normal UniversityNanjing 210023China State Key Laboratory of environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China South China institute of environmental Sciences Ministry of Ecology and EnvironmentGuangzhou 510530China State environmental protection Key Laboratory of Water environmental Simulation and Pollution Control Guangzhou 510530China University of Chinese Academy of Sciences Beijing 100049China

In situ measurement of multiple pollutants coexisting in sediment porewater is an essential step in comprehensively assessing the bioavailability and risk of pollutants,but to date,this needs to be better *** this study,a passive sampler,consisting of an“I-shaped”supporting frame and inorganic/organic sampling units,incorporating equilibrium dialysis theory and kinetic/equilibrium sorption principle,was developed for the synchronous measurement of inorganic(e.g.,phosphorus and metal(loid)s)and organic pollutants(e.g.,parent and substituted PAHs).The equilibrium time and sampling rates were explored in laboratory tests to support in situ *** of pollutants in porewater within a vertical resolution of centimeters,i.e.,1 cm and 2 cm for inorganic and organic pollutants,respectively,were obtained by field deployment of the sampler for further estimation of diffusive fluxes across the sediment-water *** results suggested that the role of sediments for a specific pollutant may change(e.g.,from“sink”to“source”)during the sampling *** study demonstrated the feasibility of synchronous measurement of inorganic and organic pollutants in sediment porewater by the passive *** addition,it provided new insight for further investigation into the combined pollution effects of various pollutants in sediments.

关键词： Passive sampling Bioavailability Polycyclic aromatic hydrocarbons Combined pollution Diffusive flux

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Novel process for facile preparation of mesoporous silica-based materials with controllable pore structure from coal fly ash Author links open overlay panel

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Particuology 2024年第8期91卷 128-137页

作者： Jian-ming Gao Zhen Li Shujia Ma Yuanyuan Zhang Fangqin Cheng institute of Resources and Environment Engineering State Environmental Protection Key Laboratory of Efficient Utilization Technology of Coal Waste ResourcesShanxi Collaborative Innovation Center of High Value-added Utilization of Coal-related WastesShanxi UniversityTaiyuan 030006China

Extraction of silica from fly ash to produce mesoporous silica materials is one of the most important utilization *** silica could not be synthesized on a large-scale by conventional sol-gel *** this paper,facile preparation of mesoporous silica with controllable pore structure from fly ash by the template-free process via two steps of mineral phase transformation and selective acid etching was *** influence of crystalline structure and acid etching degree on structure of as-synthesized mesoporous silica materials was revealed,as well as mechanism of crystalline structure transformation and pore structure *** results show that mullite and quartz could be transformed into acid-soluble kaliophilite when fly ash reacted with K_(2)CO_(3)at temperature of 800-1100℃.The hexagonal kaliophilite would be transformed into orthorhombic KAlSiO_(4)-O1 phase when the temperature is controlled at 1100℃.Mesoporous silica with specific surface area of 475.93 m^(2)/g and 642.57 m^(2)/g could be synthesized from activated fly ash with kaliophilite and KAlSiO_(4)-O1 phase crystalline *** controlling the degree of acid etching,mesoporous silica materials with different pore structures can be *** paper provides a cost-effective and large-scale process for the preparation of mesoporous silica materials with controllable pore structure from solid waste fly ash.

关键词： Fly ash Mesoporous silica Crystal transformation Acid etching Controllable pore structure

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Spatiotemporal drivers of urban water pollution:Assessment of 102 cities across the Yangtze River Basin

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environmental Science and Ecotechnology 2024年第4期20卷 300-314页

作者： Yi-Lin Zhao Han-Jun Sun Xiao-DanWang Jie Ding Mei-Yun Lu Ji-Wei Pang Da-Peng Zhou Ming Liang Nan-Qi Ren Shan-Shan Yang State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China China energy Conservation and environmental protection Group Beijing 100082China China energy Conservation and environmental protection Group CECEP Digital Technology Co.Ltd.Beijing 100089China China Railway Engineering Design and Consulting Group Co. Ltd.Beijing 100055China

Effective management of large basins necessitates pinpointing the spatial and temporal drivers of primary index exceedances and urban risk factors,offering crucial insights for basin ***,comprehensive examinations of multiple pollutants within the Yangtze River Basin remain *** we introduce a pollution inventory for urban clusters surrounding the Yangtze River Basin,analyzing water quality data from 102 cities during *** assessed the exceedance rates for six pivotal indicators:dissolved oxygen(DO),ammonia nitrogen(NH_(3)-N),chemical oxygen demand(COD),biochemical oxygen demand(BOD),total phosphorus(TP),and the permanganate index(COD_(Mn))for each *** random forest regression and SHapley Additive exPlanations(SHAP)analyses,we identified the spatiotemporal factors influencing these key *** results highlight agricultural activities as the primary contributors to the exceedance of all six indicators,thus pinpointing them as the leading pollution source in the ***,forest coverage,livestock farming,chemical and pharmaceutical sectors,along with meteorological elements like precipitation and temperature,significantly impacted various indicators'***,we delineate five core urban risk components through principal component analysis,which are(1)anthropogenic and industrial activities,(2)agricultural practices and forest extent,(3)climatic variables,(4)livestock rearing,and(5)principal polluting *** cities were subsequently evaluated and categorized based on these risk components,incorporating policy interventions and administrative performance within each *** comprehensive analysis advocates for a customized strategy in addressing the discerned risk factors,especially for cities presenting elevated risk levels.

关键词： Basin management Primary indices Urban risk factors Yangtze river basin Local conditions

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New Insights into Microplastic Contamination in Different Types of Leachates: Abundances, Characteristics, and Potential Sources

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Engineering 2024年第6期37卷 62-68页

作者： Lei Zhang Wentao Zhao Liang Zhang Zhenxiao Cai Ruiqi Yan Xia Yu Damià Barceló Qian Sui State environmental protection Key Laboratory of environmental Risk Assessment and Control on Chemical Process School of Resources and Environmental EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai institute of Pollution Control and Ecological Security Shanghai 200092China PerkinElmer Inc.Shanghai 201203China Maihai environmental protection Technology Co. Ltd.SuzhouJiangsu 215000China Department of environmental Chemistry Institute of Environmental Assessment and Water ResearchSpanish Council for Scientific Research(IDAEA-CSIC)Barcelona 08034Spain

Municipal solid waste(MSW)is an important destination for abandoned *** the waste disposal process,large plastic debris is broken down into microplastics(MPs)and released into the ***,current research only focuses on landfill leachates,and the occurrence of MPs in other leachates has not been ***,herein,the abundance and characteristics of MPs in three types of leachates,namely,landfill leachate,residual waste leachate,and household food waste leachate,were studied,all leachates were collected from the largest waste disposal center in *** results showed that the average MP abundances in the different types of leachates ranged from(129±54)to(1288±184)MP particles per liter(particlesL1)and the household food waste leachate exhibited the highest MP abundance(p80%)of small MPs(20–100 lm)in landfill leachates compared to other *** the best of our knowledge,this is the first study discussing the sources of MPs in different leachates,which is important for MP pollution control during MSW disposal.

关键词： Microplastics Landfill leachate Residual waste leachate Household food waste leachate Source

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Risk assessment of oil and gas investment environment in countries along the Belt and Road Initiative

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Petroleum Science 2024年第2期21卷 1429-1443页

作者： Bao-Jun Tang Chang-Jing Ji Yu-Xian Zheng Kang-Ning Liu Yi-Fei Ma Jun-Yu Chen center for energy and environmental Policy Research Beijing Institute of TechnologyBeijing100081China School of Management and Economics Beijing Institute of TechnologyBeijing100081China Collaborative Innovation center of Electric Vehicles in Beijing BeijingChina Sustainable Development Research institute for Economy and Society of Beijing BeijingChina institute of Carbon Neutrality ShanghaiTech UniversityShanghai201210China

With the implementation of the Belt and Road Initiative, China is deepening its cooperation in oil and gas resources with countries along the Initiative. In order to better mitigate risks and enhance the safety of investments, it is of significant importance to research the oil and gas investment environment in these countries for China's overseas investment macro-layout. This paper proposes an indicator system including 27 indicators from 6 dimensions. On this basis, game theory models combined with global entropy method and analytic hierarchy process are applied to determine the combined weights, and the TOPSIS-GRA model is utilized to assess the risks of oil and gas investment in 76 countries along the Initiative from 2014 to 2021. Finally, the GM(1,1) model is employed to predict risk values for 2022-2025. In conclusion, oil and gas resources and political factors have the greatest impact on investment environment risk, and 12 countries with greater investment potential are selected through cluster analysis in conjunction with the predicted results. The research findings may provide scientific decisionmaking recommendations for the Chinese government and oil enterprises to strengthen oil and gas investment cooperation with countries along the Belt and Road Initiative.

关键词： Belt and Road Initiative Oil and Gas Investment Risk assessment

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