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A double-layer radiative cooling coating that utilizes the refractive index difference between layers to achieve extremely high solar reflectivity

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Science China Technological Sciences 2024年第10期67卷 3182-3189页

作者： WANG FuQiang LI ChunZhe YANG ZhenNing XIE WeiXin LI Xiang XU ZengHui YAN YuYing CHENG ZiMing School of energy Science and Engineering Harbin Institute of Technology School of New energy Harbin Institute of Technology at Weihai China Construction Eco-environmental protection Technology Co. Ltd. Faculty of Engineering University of Nottingham

Passive daytime radiative cooling（PDRC） technology has great potential in reducing cooling energy consumption. In order to further improve the spectral performance of PDRC coatings, current researchers mostly focus on the selection and size design of functional particles, while ignoring the optical properties enhancement effect caused by the interlayer binder. In this study, based on the principle that the refractive index difference between layers enhanced the backscattering performance of the solar spectrum, we proposed and manufactured a double-layer PDRC coating with polyvinylidene difluoride（PVDF） as the filmforming material in the upper layer and polydimethylsiloxane（PDMS） as the film-forming material in the lower layer, both filled with Al2O3and SiO2particles. The double-layer PDRC coating exhibited excellent spectral performance that a high solar reflectivity of 98% and an emissivity of 0.95 at the “atmospheric window” band. In comparison, the solar spectrum reflectivity of the single-layer PDRC coatings based on PVDF and PDMS of the same thickness was 95% and 94.7%, respectively. Outdoor tests showed that the PDRC coating achieved a temperature decrease of up to 7.1℃ under direct sunlight at noon time. In addition, the PDRC coating had excellent weather resistance, water resistance, and other basic properties. This article opens up a new idea and provides methodological guidance for the design of double-layer PDRC coatings.

关键词： double-layer radiative cooling coating spectral modulation interlayer refractive index solar energy radiative transfer

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Three-dimensionally ordered macroporous(3DOM) structure promoted the activity and H_(2)O poisoning resistance of Ce Mn/3DOM-TiO_(2) catalyst in NH_(3)-SCR

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Journal of Rare Earths 2024年第3期42卷 523-533,I0004页

作者： Yaqin Hu Shipeng Ding Chenchen Tan Peng Wu Guobo Li Sheng Wang Hongqiang Yang Yaping Zhang Key Laboratory of energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing210096China State Power environmental protection Research institute Nanjing210031China

NH_(3)-SCR is an effective mean of NOxremoval in the non-electric industry, however, the high activation temperature and poor H_(2)O resistance of SCR catalysts posed a barrier to its application. In this work, a series of three-dimensionally ordered macroporous(3DOM) catalysts were synthesized via a colloidal crystal template(CCT) method, and various characterizations were carried out to explore the physicochemical property of catalysts. The experiment results reveal that Ce_(0.2)Mn_(0.2)/3DOM-TiO_(2) catalyst presents the excellent low-temperature catalytic activity of nearly 100% at 100℃. Furthermore, the enhanced H_(2)O resistance is achieved, certified by the unaffected NO remove at 150℃ in the participation of 15 vol% H_(2)O. The characterizations results exhibit that the improved dispersion of the active component and enhanced redox ability are conducive to the low-temperature catalytic activity. N_(2) adsorption and desorption experiments indicate that catalyst with 3DOM support possesses a larger pore diameter and specific surface area, which may weaken the condensation of H_(2)O in the microporosity of catalysts and improved the H_(2)O resistance of the catalyst. In situ DRIFTS results manifest that Ce_(0.2)Mn_(0.2)/3DOM-TiO_(2) catalyst could not only absorb more NH_(3) and generate more surface-active sites, but inhibit the competitive adsorption between H_(2)O and SCR reactants.

关键词： 3DOM material NH_(3)-SCR H_(2)O resistance Low-temperature Cerium Rare earths

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Cloud-Model-Based Feature Engineering to Analyze the energy-Water Nexus of a Full-Scale Wastewater Treatment Plant

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Engineering 2024年第5期36卷 63-75页

作者： Shan-Shan Yang Xin-Lei Yu Chen-Hao Cui Jie Ding Lei He Wei Dai Han-Jun Sun Shun-Wen Bai Yu Tao Ji-Wei Pang Nan-Qi Ren State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150000China Key Laboratory of environmental Biotechnology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China School of Civil and environmental Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China China energy Conservation and environmental protection Group Beijing 100089China

Wastewater treatment plants(WWTPs)are important and energy-intensive municipal *** energy consumption and relatively low operating performance are major challenges from the perspective of carbon ***,water-energy nexus analysis and models for WWTPs have rarely been reported to *** this study,a cloud-model-based energy consumption analysis(CMECA)of a WWTP was conducted to explore the relationship between influent and energy consumption by clustering its influent’s *** principal component analysis(PCA)and K-means clustering were applied to classify the influent condition using water quality and volume *** energy consumption of the WWTP is divided into five standard evaluation levels,and its cloud digital characteristics(CDCs)were extracted according to bilateral constraints and golden ratio *** results showed that the energy consumption distribution gradually dispersed and deviated from the Gaussian distribution with decreased water concentration and *** days with high energy efficiency were extracted via the clustering method from the influent category of excessive energy consumption,represented by a compact-type energy consumption distribution curve to identify the influent conditions that affect the steady distribution of energy *** local WWTP has high energy consumption with 0.3613 kW·h·m^(-3)despite low influent concentration and volumes,across four consumption levels from low(I)to relatively high(IV),showing an unsatisfactory operation and management *** average oxygenation capacity,internal reflux ratio,and external reflux ratio during high energy efficiency days recognized by further clustering were obtained(0.2924-0.3703 kg O_(2)·m^(-3),1.9576-2.4787,and 0.6603-0.8361,respectively),which could be used as a guide for the days with low energy ***,this study offers a water-energy nexus analysis method to identify influent conditions with operational manageme

关键词： Wastewater treatment plants Cloud-model theory Data mining Principal component analysis K-means clustering Cloud-model-based energy consumption analysis

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Electrostatic removal of ultrafine carbon black with square-grooved collecting plates:Insights for capturing black carbon emitted from ships

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Journal of environmental Sciences 2024年第2期136卷 559-569页

作者： Zhicheng Wu YifanWang Lingyu Shao Hao Zhang Haobo Dai Haidong Fan Chenghang Zheng Xiang Gao State Key Lab of Clean energy Utilization State Environmental Protection Engineering Center for Coal-Fired Air Pollution ControlZhejiang UniversityHangzhou 310027China Department of Earth and environmental Sciences University of ManchesterOxford RoadUnited Kingdom Zhejiang Tiandi environmental protection Engineering Co. Ltd.Hangzhou 310012China Baima Lake Laboratory(Zhejiang Provincial Laboratory of energy and Carbon Neutrality) Hangzhou 310000China

Ships and other mobile pollution sources emitted massive ultrafine and low-resistivity particles containing black carbon(BC),which were harmful to human health and were difficult to capture by conventional electrostatic precipitators(ESPs).In this study,nanoscale carbon black was adopted as simulated particles(SP)with similar physicochemical properties for black carbon emitted from ships(SP-BC)to investigate the feasibility of using an ESP with square-grooved collecting plates for the removal of SP-BC at low *** increased applied voltage significantly improved the total collection of SP-BC whereas may also promote the conversion of relatively larger particle size SP-BC into nano-size below *** outlet number concentration of SP-BC under 27 kV at 130℃was three times that of the *** the reduction of the flow rate could strengthen the capture of SP-BC below20 nm,and under the combined action of low flow rate and maximum applied voltage,the collection efficiency of 20-100 nm SP-BC could exceed 90%.In addition,the escape and capture characteristics of SP-BC under long-term rapping were *** square-grooved collecting plate could effectively restrain the re-entrainment of collected SP-BC generated by rapping,and the nanoscale SP-BC was trapped in the grooves after *** results could provide insights into the profound removal of massive nanoscale black carbon emissions from mobile sources.

关键词： Simulated ship black carbon Electrostatic removal Square-grooved collecting plate Long-term rapping

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The underappreciated role of fugitive VOCs in ozone formation and health risk assessment emitted from seven typical industries in China

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Journal of environmental Sciences 2024年第2期136卷 647-657页

作者： Zhiling Liang Yunjiang Yu Bingbing Sun Qian Yao Xihua Lin Yongsheng Wang Jianping Zhang Yingzi Li Xuefeng Wang Zhengzheng Tang Shexia Ma College of environmental and Chemical Engineering Shanghai University of Electric PowerShanghai 200090China State environmental protection Key Laboratory of environmental protection Health Risk Assessment South China Institute of Environmental SciencesMinistry of Ecology and EnvironmentGuangzhou 510535China Henan Jiyuan Ecological Environment Testing center Jiyuan 454650China Ecological Environment Bureau of Jiyuan Production City Integration Demonstration Zone Jiyuan 454650China

Fugitive emission from industrial sources may result in ozone formation and health risk,while the exact contribution of this source remains incompletely *** this study,emission characteristics,ozone formation potential(OFP)and health risk of fugitive VOCs in7 representative industries were *** material industry was the dominant contributor to VOCs of fugitive emission in comparison with other *** OFP of VOCs from fugitive emission was in the range of 1.45×10^(3)-3.98×10^(5)μg/m^(3),with a higher value than that of organized emission in seven industries except for the coking industry and the chemical material industry,suggesting that fugitive VOCs should be taken into account while developing control ***,m,p-xylene,n-nonane,ethylene,vinyl chloridethe and other high OFP-contributing species were the major reactive species that should be *** risk assessment investigated non-cancer and cancer risks of fugitive VOCs in 7 industries were all above safe level(HR>1 and LCR>1×10^(-4)),posing remarkable health threats to human *** were the main contributor to non-cancer risk,while halohydrocarbons and aromatics contributed most to cancer risks,posing remarkable health threat on human *** findings highlighted the contribution of fugitive VOCs on ozone formation and health risk was underestimated,indicating which should be considered in emission control strategies of industrial sources.

关键词： Industrial sources Volatile organic compounds Fugitive emission Ozone formation potential Health risk assessment

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Anion exchange membranes with a semi-interpenetrating polymer network using 1,6-dibromohexane as bifunctional crosslinker

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Chinese Journal of Chemical Engineering 2024年第8期72卷 199-208页

作者： Aijie Li Zhanliang Wang Zhihao Si Lu Lu Peipei Huang Jinhong Liu Songyuan Yao Peiyong Qin Xinmiao Zhang National energy R&D center for Biorefinery College of Life Science and TechnologyBeijing University of Chemical TechnologyBeijing 100029China Paris Curie Engineer School Beijing University of Chemical TechnologyBeijing 100029China environmental protection Research institute Beijing Research Institute of Chemical IndustryBeijing 100000China

An anion exchange membrane(AEM)is generally expected to possess high ion exchange capacity(IEC),low water uptake(WU),and high mechanical strength when applied to electrodialysis *** different types of AEMs,semi-interpenetrating polymer networks(SIPNs)have been suggested for their structural superiorities,i.e.,the tunable local density of ion exchange groups for IEC and the restrained leaching of hygroscopic groups by insolubility for ***,the conventional SIPN AEMs still struggle to balances IEC,WU,and mechanical strength simultaneously,due to the lack of the compact crosslinking *** this work,we proposed a novel SIPN structure of polyvinylidene difluoride/polyvinylimidazole/1,6-dibromohexane(PVDF/PVIm/DBH).On the one hand,DBH with two cationic groups of imidazole groups are introduced to enhance the ion conductivity,which is different from the conventional monofunctional modifier with only one cationic *** the other hand,DBH has the ability to bridge with PVIm,where the mechanical strength of the resulting AEM is increased by the increase of crosslinking *** show that a low WU of 38.1%to 62.6%,high IEC of 2.12—2.22 mmol·g^(-1),and excellent tensile strength of 3.54—12.35 MPa for PVDF/PVIm/DBH membrane are *** work opens a new avenue for achieving the high-quality AEMs.

关键词： Anion exchange membrane Polyvinylidene difluoride Electrodialysis Semi-interpenetrating polymer networks

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Dynamic emission characteristics and control strategies of air pollutants from motor vehicles in downtown Beijing,China

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Journal of environmental Sciences 2024年第2期136卷 637-646页

作者： Yan Shen Tongran Wu Aiping Lian Jie Gao Fei Peng Guohua Song Xuefang Wu Yangyang Cui Xinyu Liu Yunfei Wan Jing Yan Yifeng Xue National Engineering Research center of Urban environmental Pollution Control Beijing Municipal Research Institute of Eco-Environmental ProtectionBeijing 100037China Beijing Municipal Ecology and Environment Bureau Beijing 100048China Beijing Jiaotong University Beijing 100091China

This study combined the real-time monitoring and investigation of traffic flows to comprehensively analyze the road traffic flow and vehicle structure in downtown Beijing.A dynamic emission inventory of motor vehicle air pollutants in downtown Beijing in 2021 was established,and the impact of these emissions on air quality was simulated and quantified,and different emission reduction control scenarios were proposed to evaluate their environmental improvement effects and explore measures to mitigate the impact of pollution *** results show that the high traffic flow and the structure of the motor vehicle emissions in downtown Beijing are the main causes of severe motor vehicle *** data shows that traffic flow in central Beijing is dominated by small passenger vehicles,while the vehicle mix is better than in other regions,with 72.0%of vehicles meeting"National V"or higher emission ***,to achieve higher air quality goals,further reducing vehicle emissions is *** on dynamic traffic flow,the average daily emissions of nitrogen oxides(NOX),particulate matters(PM_(2.5))and volatile organic compounds(VOC)from motor vehicles in central Beijing are 17.7 tons,0.6 tons and 14.0 tons,respectively,accounting for 23.0%of the city’s average daily motor vehicle *** a zero-emission zone for motor vehicles were implemented in central Beijing,the annual average emission level of pollutants will be reduced by 10.4%to 21.0%.The designation of ultra-low emission zones for motor vehicles could be effective in improving the air quality in the center of Beijing.

关键词： Motor vehicle Air pollutant Emission characteristics Control strategy Beijing

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Nutrient transport following water transfer through the world's largest water diversion channel

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Journal of environmental Sciences 2024年第1期135卷 703-714页

作者： Yuanhui Cheng Hong Zhang Wei Yin State Key Laboratory of environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085 China Changjiang Water Resources protection institute Wuhan 430051China University of Chinese Academy of Sciences Beijing 100049China

Nutrient levels in the artificial channel constructed for the Middle Route Project are significant indicators of water quality safety and aquatic ecological integrity for this large,interbasin ***,the distribution and transport of nutrients along the channel were poorly *** on a time-series dataset as well as mass balance and material flow analysis methods,the water and nutrient transport fluxes in the Middle Route of the South-to-North Water Diversion Project were identified in this *** results indicate that the nutrient concentrations varied considerably with time,but there was no significant difference among the 30 stations of the main *** temperature difference was the major factor in the large fluctuations of water quality indicators over *** nutrient loadings varied with the water volume outputs from the main channel to the waterreceiving *** deposition was an important source of nutrients in the main channel,accounting for 9.13%,20.6%,and 0.635%of the nitrogen,phosphorus,and sulfur input from the Danjiangkou Reservoir,*** 2021,a net accumulation of 988 tons of N,29 tons of P,and 2,540 tons of S,respectively,were present in the main *** increase of these external and internal nutrient loadings would cause water quality fluctuation and deterioration in some local sections of the main *** study quantified the spatial and temporal patterns of nutrient transport in the Middle Route and revealed the ecological effects on the aquatic environment,assisting authorities on the project to develop effective water conservation strategies.

关键词： Nutrient transport Spatiotemporal patterns The Middle Route The South-to-North Diversion Project Hydro-ecological effects Water-receiving cities

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Effects of Diesel Concentration on the Thermal Conductivity,Specific Heat Capacity and Thermal Diffusivity of Diesel-Contaminated Soil

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Journal of Thermal Science 2024年第2期33卷 696-709页

作者： WU Yuhao WU Yuefei LUO Gubai ZHANG Teng WANG Qing FAN Liwu SONG Xin YU Zitao Key Laboratory of Clean energy and Carbon Neutrality of Zhejiang Province Zhejiang UniversityHangzhou310027China State Key Laboratory of Clean energy Utilization Zhejiang UniversityHangzhou310027China institute of Thermal Science and Power Systems School of Energy EngineeringZhejiang UniversityHangzhou310027China center environmental protection Technology Company Limited Beijing100176China institute of Soil Science Chinese Academy of SciencesNanjing210008China

High energy consumption is a serious issue associated with in situ thermal desorption(TD)remediation of sites contaminated by petroleum hydrocarbons(PHs).The knowledge on the thermophysical properties of contaminated soil can help predict accurately the transient temperature distribution in a remediation site,for the purpose of energy ***,such data are rarely reported for PH-contaminated *** this study,by taking diesel as a representative example for PHs,soil samples with constant dry bulk density but different diesel mass concentrations ranging from 0% to 20% were prepared,and the variations of their thermal conductivity,specific heat capacity and thermal diffusivity were measured and analyzed over a wide temperature range between 0℃ and 120℃.It was found that the effect of diesel concentration on the thermal conductivity of soil is negligible when it is below 1%.When diesel concentration is below 10%,the thermal conductivity of soil increases with raising the ***,when diesel concentration becomes above 10%,the change of the thermal conductivity of soil with temperature exhibits the opposite *** is mainly due to the competition between soil minerals and diesel,because the thermal conductivity of minerals increases with temperature,whereas the thermal conductivity of diesel decreases with *** analysis results showed that,compared with temperature,the diesel concentration has more significant effects on soil thermal *** of the diesel concentration,with the increase of temperature,the specific heat capacity of soil increases,while the thermal diffusivity of soil *** addition,the results of a control experiment exhibited that the relative differences of the thermal conductivity of the soil samples containing the same concentration of both diesel and a pure alkane are all below 10%,indicating that the results obtained with diesel in this study can be extended to the family of PHs.A theo

关键词： contaminated soil diesel concentration thermal conductivity specific heat capacity thermal diffusivity thermal desorption fractal model

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A global perspective on microbial risk factors in effluents of wastewater treatment plants

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Journal of environmental Sciences 2024年第4期138卷 227-235页

作者： Kejing Chen Jinsong Liang Yuhan Wang Yechen Tao Yun Lu Aijie Wang School of Civil and environmental Engineering Harbin Institute of TechnologyShenzhen 518055China Shenzhen Guohuan environmental protection Technology Development Co. LTD.Shenzhen 518055China State Key Joint Laboratory of environmental Simulation and Pollution Control State Environmental Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Effective monitoring and management of microbial risk factors in wastewater treatment plants(WWTPs)effluents require a comprehensive investigation of these risks.A global survey on microbial risk factors in WWTP effluents could reveal important insights into their risk *** study aims to explore the abundance and types of antibiotic resistance genes(ARGs),virulence factor genes(VFGs),the vector of ARG/VFG,and dominant pathogens in global WWTP *** collected 113 metagenomes of WWTP effluents from the Sequence Read Archive of the National center for Biotechnology Information and characterized the microbial risk *** results showed that multidrug resistance was the dominant ARG type,while offensive virulence factors were the most abundant type of *** most dominant types of ARGs in the vector of plasmid and phage were both aminoglycoside resistance,which is concerning as aminoglycosides are often a last resort for treating multi-resistant *** baumannii was the most dominant pathogen,rather than Escherichia coli,and a weak negative correlation between Escherichia coli and two other dominant pathogens(Acinetobacter baumannii and Bacteroides uniformis)suggests that using Escherichia coli as a biological indicator for all pathogens in WWTP effluents may not be *** Getah virus was the most dominant virus found in global WWTP *** study presents a comprehensive global-scale investigation of microbial risk factors in WWTP effluents,providing valuable insights into the potential risks associated with WWTP effluents and contributing to the monitoring and control of these risks.

关键词： Wastewater treatment plant Microbial risk factor Effluent Pathogen Antibiotic resistance gene Virulence factor gene

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