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An investigation of the effects of hydrochar application rate on soil amelioration and plant growth in three diverse soils

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Biochar 2021年第3期3卷 349-365页

作者： Megan de Jager Luise Giani carl von ossietzky Universität Institut Für Biologie Und UmweltwissenschaftenOldenburgGermany

The hydrothermal carbonization(HTC)of biogas digestate alters the raw materials inherent characteristics to produce a carbon(C)-rich hydrochar(HC),with an improved suitability for soil *** studies report conflicting impacts of various HC application rates on soil properties and plant *** this study,the influence of HC application rate on soil improvement and plant growth aspects was investigated in three diverse soils(Chernozem,Podzol,and Gleysol).Pot trials were conducted in which all soils were amended with 5,10,20 and 30%(w/w)HC in quintuplicate,with two controls of pure soil(with and without plants,respectively)also *** to potting,soil samples were collected from all HC-amended soils and controls and analyzed for soil pH,plant available nutrients(PO4-P and K),and microbial activity using standard laboratory and statistical *** after potting,a 6-week seed germination experiment using Chinese cabbage was conducted to determine germination success,followed by a plant growth experiment of equal duration and plant species to determine biomass *** the end of the study(after a total plant growth period of 12 weeks),each pot was sampled and comparatively analyzed for the same soil properties as at the beginning of the *** pH shifted toward the pH of the HC(6.6)in all soils over the course of the study,but was most expressed in the 20%and 30%application rates,confirming the well-documented liming effect of *** addition of HC increased the PO4-P and K contents,particularly with 20%and 30%HC *** results are proposedly due to the large labile C fraction of the HC,which is easily degradable by *** rapid decomposition of this C fraction prompted the quick release of the HCs inherently high PO4-P and K content into the soil,and in turn,further stimulated microbial activity,until this fraction was essentially *** addition did not inhibit seed germination at any rate,presumabl

关键词： Biogas digestate Hydrochar application rate Soil improvement Nutrient availability Microbial activity

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On Unsupervised Training of Multi-Class Regularized Least-Squares Classifiers

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Journal of Computer Science & Technology 2014年第1期29卷 90-104页

作者： Tapio Pahikkala Antti Airola Fabian Gieseke Oliver Kramer ACM IEEE Department of Information Technology University of Turku Department of Computer Science University of Copenhagen Computer Science Department Carl von Ossietzky University of Oldenburg

In this work we present the first efficient algorithm for unsupervised training of multi-class regularized least- squares classifiers. The approach is closely related to the unsupervised extension of the support vector machine classifier known as maximum margin clustering, which recently has received considerable attention, though mostly considering the binary classification case. We present a combinatorial search scheme that combines steepest descent strategies with powerful meta-heuristics for avoiding bad local optima. The regularized least-squares based formulation of the problem allows us to use matrix algebraic optimization enabling constant time checks for the intermediate candidate solutions during the search. Our experimental evaluation indicates the potential of the novel method and demonstrates its superior clustering performance over a variety of competing methods on real world datasets. Both time complexity analysis and experimental comparisons show that the method can scale well to practical sized problems.

关键词： unsupervised learning multi-class regularized least-squares classification maximum margin clustering combinatorial optimization

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Chapter model systems in heterogeneous catalysis at the atomic level: a personal view

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Science China Chemistry 2020年第4期63卷 426-447页

作者： Hans-Joachim Freund Markus Heyde Helmut Kuhlenbeck Niklas Nilius Thomas Risse Thomas Schmidt Shamil Shaikhutdinov Martin Sterrer Fritz Haber Institute of the Max Planck Society Faradayweg 4-6Berlin D-14195Germany Fakultat V-Mathematik und Naturwissenschaften Carl von Ossietzky Universitat OldenburgGermany Institut fur Chemie und Biochemie Freie UniversitatBerlinGermany Institute of Physics University of GrazGrazAustria

The review presents an overview of studies in the surface science of oxide and related surfaces with an emphasis of the studies performed in the authors’ group. Novel instruments and technique developments, as well as their applications are reported, in an attempt to cover studies on model systems of increasing complexity, including some of the key ingredients of an industrially applied heterogeneous catalyst and its fabrication. The review is intended to demonstrate the power of model studies in understanding heterogeneous catalysis at the atomic level. The studies include those on supported nano-particles, both, prepared in vacuum and from solution, interaction of surfaces and the underlying bulk with molecules from the gas phase, strong metal support interaction, as well as the first attempt to include studies on reactions in confined spaces.

关键词： model catalysts oxide surfaces structure and spectroscopy supported nanoparticles reactions in the confined space

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Catalyst-Free Synthesis and Shape Control of CdTe Nanowires

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Nano Research 2011年第9期4卷 824-835页

作者： Xiaoping Jin Marta Kruszynska Jurgen Parisi Joanna Kolny-Olesiak University of Oldenburg Department of Physics Energy and Semiconductor Research Laboratory Carl-von-Ossietzky-Str. 9-11 26129Oldenburg Germany

The procedure reported here allows for the size and shape control of CdTe nanowires by means of colloidal chemistry. Thus, ultrathin, straight, saw-tooth-like and one-sided branched nanowires with zinc blende structures could be synthesized. Their formation does not require any catalyst and is most likely due to the oriented attachment of nanoparticles formed in the beginning of the reaction. The use of oleylamine as a solvent turned out to be crucial in order to achieve CdTe nanowires. The reaction between oleic acid and oleylamine in the presence of CdO proved to be essential, not only to activate the Cd precursor but also to provide reaction conditions facilitating nanowire formation by oriented attachment.

关键词： Nanowires CdTe amine activation oriented attachment shape control

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Model evaluation for the prediction of solubility of active pharmaceutical ingredients(APIs) to guide solid–liquid separator design

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Asian Journal of Pharmaceutical Sciences 2018年第3期13卷 265-278页

作者： Kuveneshan Moodley Jürgen Rarey Deresh Ramjugernath Thermodynamics Research Unit School of Engineering University of KwaZulu-Natal Howard College Campus Industrial Chemistry Carl von Ossietzky University Oldenburg

The assumptions and models for solubility modelling or prediction in systems using nonpolar solvents, or water and complex triterpene and other active pharmaceutical ingredients as solutes aren't well studied. Furthermore, the assumptions concerning heat capacity effects(negligibility, experimental values or approximations) are explored, using non-polar solvents(benzene), or water as reference solvents, for systems with solute melting points in the range of 306–528 K and molecular weights in the range of 90–442 g/mol. New empirical estimation methods for the Δ_(fus)C_(pi) of APIs are presented which correlate the solute molecular masses and van der Waals surface areas with Δ_(fus)C_(pi). Separate empirical parameters were required for oxygenated and non-oxygenated solutes. Subsequently, the predictive capabilities of the various approaches to solubility modelling for complex pharmaceuticals,for which data is limited, are analysed. The solute selection is based on a principal component analysis, considering molecular weights, fusion temperatures, and solubilities in a non-polar solvent, alcohol, and water, where data was available. New NRTL-SAC parameters were determined for selected steroids, by regression. The original UNIFAC, modified UNIFAC(Dortmund), COSMO-RS(OL), and COSMO-SAC activity coefficient predictions are then conducted, based on the availability of group constants and sigma profiles. These are undertaken to assess the predictive capabilities of these models when each assumption concerning heat capacity is employed. The predictive qualities of the models are assessed, based on the mean square deviation and provide guidelines for model selection, and assumptions concerning phase equilibrium, when designing solid–liquid separators for the pharmaceutical industry on process simulation software. The most suitable assumption regarding Δ_(fus)C_(pi) was found to be system specific, with modified UNIFAC(Dortmund) performing well in benzene as a solvent system,

关键词： Solubility Solid–Liquid Equilibrium Model prediction Active pharmaceutical ingredients

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Competitive effect, but not competitive response, varies along a climatic gradient depending on tree species identity

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Forest Ecosystems 2024年第2期11卷 142-151页

作者： Teresa Valor Lluís Coll David I.Forrester Hans Pretzsch Miren del Río Kamil Bielak Bogdan Brzeziecki Franz Binder Torben Hilmers Zuzana Sitková Roberto Tognetti Aitor Ameztegui Department of Agricultural and Forest Sciences and Engineering(DCEFA) University of LleidaAv.Alcalde Rovira Roure 191E25198 LleidaSpain Joint Research Unit CTFC-AGROTECNIO-CERCA Ctra.Sant LlorençKm.225280SolsonaSpain Swiss Federal Institute of Forest Snow and Landscape Research WSLZürcherstrasse 1118903BirmensdorfSwitzerland CSIRO Land and Water GPO Box 1700CanberraACT2601Australia Chair of Forest Growth and Yield Science School of Life Sciences WeihenstephanTechnical University of MunichHans-Carl-Von-Carlowitz-Platz 285354FreisingGermany Forest Research Center INIA-CSICCtra.A Coruña Km 7.528040MadridSpain IuFOR Sustainable Forest Management Research InstituteUniversity of Valladolid&INIASpain Department of Silviculture Institute of Forest SciencesWarsaw University of Life SciencesNowoursynowska 159/3402776WarsawPoland Bavarian State Institute of Forestry(LWF) Hans-Carl-von-Carlowitz-Platz 1D-85354FreisingGermany National Forest Centre Forest Research InstituteT.G.Masaryka 2296001ZvolenSlovakia Faculty of Agricultural Environmental and Food SciencesFree University of Bozen-Bolzano Piazza Università1 I-39100Bolzano

Background: Understanding the role of species identity in interactions among individuals is crucial for assessing the productivity and stability of mixed forests over time. However, there is limited knowledge concerning the variation in competitive effect and response of different species along climatic gradients. In this study, we investigated the importance of climate, tree size, and competition on the growth of three tree species: spruce(Picea abies), fir(Abies alba), and beech(Fagus sylvatica), and examined their competitive response and effect along a climatic ***: We selected 39 plots distributed across the European mountains with records of the position and growth of 5,759 individuals. For each target species, models relating tree growth to tree size, climate and competition were proposed. Competition was modelled using a neighbourhood competition index that considered the effects of inter-and intraspecific competition on target trees. Competitive responses and effects were related to *** methods and information theory were used to select the best ***: Our findings revealed that competition had a greater impact on target species growth than tree size or climate. Climate did influence the competitive effects of neighbouring species, but it did not affect the target species? response to competition. The strength of competitive effects varied along the gradient, contingent on the identity of the interacting species. When the target species exhibited an intermediate competitive effect relative to neighbouring species, both higher inter-than intraspecific competitive effects and competition reduction occurred along the gradient. Notably, species competitive effects were most pronounced when the target species' growth was at its peak and weakest when growing conditions were far from their ***: Climate modulates the effects of competition from neighbouring trees on the target tree and not the susceptibility of th

关键词： Competition coefficient Competition reduction Interspecific competition Intraspecific competition Mixing effects Mixed species forest Neighbourhood models Plant-plant interactions

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Disentangling the effects of management and climate change on habitat suitability for saproxylic species in boreal forests

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Journal of Forestry Research 2024年第2期35卷 121-133页

作者： Ellinoora Ekman María Triviño Clemens Blattert Adriano Mazziotta Maria Potterf Kyle Eyvindson Department of Biological and Environmental Science University of JyvaskylaP.O.Box 3540014 JyvaskylaFinland Institute for Atmospheric and Earth System Research(INAR)/Physics Faculty of ScienceUniversity of HelsinkiP.O.Box 6800014 HelsinkiFinland School of Resource Wisdom University of JyvaskylaP.O.Box 3540014 JyvaskylaFinland Natural Resources Institute Finland(LUKE) Latokartanonkaari 900790 HelsinkiFinland Ecosystem Dynamics and Forest Management Group Technical University of MunichHans‑Carl‑Von‑Carlowitz‑Platz 285354 FreisingGermany Faculty of Environmental Sciences and Natural Resource Management Norwegian University of Life SciencesP.O.Box 50031433ÅsNorway

Forest degradation induced by intensive forest management and temperature increase by climate change are resulting in biodiversity decline in boreal *** forest management and high-end climate emission scenarios can further reduce the amount and diversity of deadwood,the limiting factor for habitats for saproxylic species in European boreal *** magnitude of their combined effects and how changes in forest management can affect deadwood diversity under a range of climate change scenarios are poorly *** used forest growth simulations to evaluate how forest management and climate change will individually and jointly affect habitats of red-listed saproxylic species in *** simulated seven forest management regimes and three climate scenarios(reference,RCP4.5 and RCP8.5)over 100 *** regimes included set aside,continuous cover forestry,business-as-usual(BAU)and four modifications of *** suitability was assessed using a speciesspecific habitat suitability index,including 21 fungal and invertebrate species groups.“Winner”and“loser”species were identified based on the modelled impacts of forest management and climate change on their habitat *** found that forest management had a major impact on habitat suitability of saproxylic species compared to climate *** suitability index varied by over 250%among management regimes,while overall change in habitat suitability index caused by climate change was on average only 2%.More species groups were identified as winners than losers from impacts of climate change(52%–95%were winners,depending on the climate change scenario and management regime).The largest increase in habitat suitability index was achieved under set aside(254%)and the climate scenario RCP8.5(>2%),while continuous cover forestry was the most suitable regime to increase habitat suitability of saproxylic species(up to+11%)across all climate change *** results show that close-to-na

关键词： Biodiversity Simulations Finland Forest planning Habitat suitability Deadwood

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Comparison of Nitric Oxide Concentrations in μs-and ns-Atmospheric Pressure Plasmas by UV Absorption Spectroscopy

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Plasma Science and Technology 2016年第4期18卷 406-411页

作者： F.PETERS J.HIRSCHBERG N.MERTENS S.WIENEKE W.VIOL HAWK University of Applied Sciences and Arts Von-Ossietzky-Straβe 9937085 Gottingen Germany Fraunhofer Application Center for Plasma and Photonics Fraunhofer Institute for Surface Engineering and Thin Films IST Von-Ossietzky-Stratte 100 37085 Gottingen Germany

In this paper,an absorption spectroscopy measurement method was applied on two atmospheric pressure plasma sources to determine their production of nitric *** concentrations are essential for evaluating the plasma sources based on the principle of the Dielectric Barrier Discharge（DBD）for applications in plasma *** described method is based on a setup with an electrodeless discharge lamp filled with a mixture of oxygen and *** of the emitted wavelengths is an important resonance wavelength of nitric oxide（λ = 226.2 nm）.By comparing the absorption behaviour at the minimum and maximum of the spectral absorption cross section of nitric oxide around that wavelength,and measuring the change in intensity by the absorbing plasma,the concentration of nitric oxide inside the plasma can be *** produced nitric oxide concentrations depend on the pulse duration and are in the range of 180 ppm to 1400 ppm,so that a distance of about 10 cm to the respiratory tract is enough to conform to the VDI Guideline 2310.

关键词： nitric oxide(NO)concentration dielectric barrier discharge(DBD) ultraviolet(UV)absorption spectroscopy plasma medicine pulse duration ns-source μs-source

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Assessing the sensitivity of Melanoplus frigidus （Orthoptera： Acrididae） to different weather conditions＂ A modeling approach focussing on development times

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Insect Science 2008年第2期15卷 167-178页

作者： Oliver-D. Finch Jorg Loffler Roland Pape carl-von-ossietzky University of Oldenburg Fk V Institute of Biology and Environmental-Sciences Terrestrial Ecology D-26111 Oldenburg University of Bonn Department of Geography Meckenheimer AIlee 166 D-53115 Bonn Germany

The temperature and soil moisture conditions as well as vegetation patterns were studied to describe the habitat and to model the life cycle of Melanoplusfrigidus, a true alpine grasshopper of the Scandes. In the low alpine belt of the Norwegian Scandes the species colonizes only the warmest microhabitats with maximum soil surface temperatures of 31℃. Vegetation of these habitats consists of shrub-rich heath dominated by Vaccinium myrtillus and Calluna vulgaris. Using continuously measured temperature data, the development times for four different seasons were modeled and related to field observations. The maximum delay of adult molt was estimated to amount to 3 weeks, the delay being determined by the variation in spring temperature conditions between different years. The possibilities of using M. frigidus as an indicator organism of climate change effects on alpine zoo-coenoses of the Scandes are discussed.

关键词： alpine insects climate change indicator life history thermal effective environment

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Surface Activation of Plane and Curved Automotive Polymer Surfaces by Using a Fittable Multi-Pin DBD Plasma Source

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Plasma Science and Technology 2014年第6期16卷 593-597页

作者： Jrn HEINE Roland DAMM Christoph GERHARD Stephan WIENEKE Wolfgang VIL University of Applied Sciences and Arts Laboratory of Laser and Plasma TechnologyVon-Ossietzky-Stra?e 99 37085 Gttingen Germany Fraunhofer Institute for Surface Engineering and Thin Films Application Center for Plasma and Photonic Von-Ossietzky-Stra?e 99 37085 Gttingen Germany

In this work, surface activation of automotive polymers using atmospheric pressure plasmas was investigated. The aim was to increase the polar fraction of the surface energy of both plane and convex polymer devices with a radius in the range of 30 mm. For this purpose, a fittable low temperature atmospheric pressure plasma source based on capacitively coupled multi-pin electrodes was set up and applied. Each single electrode generates a treatment spot of approximately 2 cm2 with a tunable power density of up to 1.4 W/cm2. The surface energy was evaluated by contact angle measurements. After treatment at a low energy density of 1.01 J/cm2, the polar fraction of the surface energy of the investigated polymers was increased by a factor of 3.3 to 132, depending on the polymer materials. It was shown that by applying the presented fittable plasma source, this effect is independent of the surface radius of the polymer sample.

关键词： surface activation atmospheric pressure plasma adhesion lacquering surfaceenergy

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