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heterogeneous Catalysis with Metal-Containing Crystalline Porous Materials:Element-and Site-Specific Insights

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CCS Chemistry 2024年第5期6卷 1110-1129页

作者： Yan Li Andrew G.Walsh Peng Zhang Tianjun Zhang State Key Laboratory of New Pharmaceutical Preparations and Excipients College of Chemistry and Materials ScienceHebei UniversityBaoding 071002 Department of Chemistry Dalhousie UniversityHalifaxNova Scotia B3H 4R2

Metal-containing crystalline porous materials(CPMs)are gaining popularity in heterogeneous catalysis because of their highly crystalline and porous systems,and their excellent chemical *** of the metal species and framework structure permits them to have greater activity,selectivity,and stability over other *** in-depth understanding of the complex nature of metal active sites in CPMs is essential for revealing the structure-performance relationships and directing the rational design of such *** to conventional characterization techniques,the rapid development of X-ray absorption spectroscopy(XAS)has provided element-and site-specific deep insights into the electronic and structural information of metal species in *** such,this review begins by summarizing novel XAS techniques and analysis methods in accurately obtaining such ***,the combination of XAS with other high-level characterization methods into disclosing the configuration of active sites in metalcontaining CPMs is ***,the utilization of theory-assisted XAS data analysis in examining complex metal-containing CPM catalysts is ***,advanced in-situ/operando XAS studies into revealing the working sites in metal-containing CPMs under catalytic conditions are *** conclude by outlining the future challenges and prospects of XAS measurements,data analyses,and in-situ/operando setups in advancing the study of metal-in-CPM catalysts.

关键词： X-ray absorption spectroscopy in-situ metal species crystalline porous materials heterogeneous catalysis

blue economy:A new era of petroleum microbiology in a changing climate

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National Science Open 2024年第1期3卷 49-74页

作者： Yiqi Cao baiyu Zhang Guihua Dong bing Chen The Northern Region Persistent Organic Pollution Control(NRPOP)Laboratory Faculty of Engineering and Applied ScienceMemorial University of NewfoundlandSt.John’sN.L.A1B 3X5Canada

The productivity and health of our ocean hold some good solutions to the world’s challenges in ***,climate change and waste discharge are changing the marine capacity to buffer human impacts,further challenging the marine industry,primarily in offshore oil and gas,shipping,and fishery *** encourage the blue economy,a sustainable development approach to utilize marine *** microbiology dealing with microbes that can respond,degrade,and alter crude oils,offers an unprecedented opportunity to achieve the knowledge-and science-based blue ***,the new-era petroleum microbiology for supporting the blue economy has yet to be systematically *** review introduces the climate change impacts on key marine industrial sectors,highlights the critical role of advanced petroleum microbiology in supporting sustainable development,and offers insight into the challenges and future research opportunities in availing of petroleum microbiology for benefiting our marine environment and responsible economic growth.

关键词： blue economy sustainability climate change petroleum microbes bioproduction carbon neutrality

Enhancing Deep Learning Semantics:The Diffusion Sampling and Label-Driven Co-Attention Approach

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Computers, Materials & Continua 2024年第5期79卷 1939-1956页

作者： ChunhuaWang Wenqian Shang Tong Yi haibin Zhu State Key Laboratory of Media Convergence and Communication Communication University of ChinaBeijing100024China School of Computer and Cyber Sciences Communication University of ChinaBeijing100024China School of Computer Science and Engineering Guangxi Normal UniversityGuilin541004China Department of Computer Science Nipissing UniversityNorth BayON P1B 8L7Canada

The advent of self-attention mechanisms within Transformer models has significantly propelled the advancement of deep learning algorithms,yielding outstanding achievements across diverse ***,self-attention mechanisms falter when applied to datasets with intricate semantic content and extensive dependency *** response,this paper introduces a Diffusion Sampling and Label-Driven Co-attention Neural Network(DSLD),which adopts a diffusion sampling method to capture more comprehensive semantic information of the ***,themodel leverages the joint correlation information of labels and data to introduce the computation of text representation,correcting semantic representationbiases in thedata,andincreasing the accuracyof semantic ***,the model computes the corresponding classification results by synthesizing these rich data semantic *** on seven benchmark datasets show that our proposed model achieves competitive results compared to state-of-the-art methods.

关键词： Semantic representation sampling attention label-driven co-attention attention mechanisms

Starting materials, processes and characteristics of bio-based foams: A review

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Journal of bioresources and bioproducts 2024年第2期9卷 160-173页

作者： Xiaohan Wang Jinwon Jang Yanqun Su Jingang Liu hongjie Zhang Zhibin he Yonghao Ni National Engineering Laboratory for Pulp and Paper China National Pulp and Paper Research Institute Co.Ltd.Beijing 100102China Limerick Pulp and Paper Centre and Department of Chemical Engineering University of New BrunswickNew Brunswick E3B 5A3Canada

biofoam products have attracted considerable attention lately because there is a growing demand for green/sustainable *** this end,various biobased foams have either been developed or are currently in development,e.g.,bio-based polyurethanes(PUs),polylactic acid(PLA),starch,and polyhydroxyalkanotates(PhAs).Indeed,significant progress has been made;however,chal-lenges still persist,for example,biobased foam products have poor processability,inferior com-patibility,thermal and strength *** this review,we focus on five biofoam products:namely bio-based PUs,PLA,starch,PhAs,and cellulose biofoam products,along with their prop-erties and performance,as well as their manufacturing *** efforts are still needed to unlock the full potential of these bio-based products and meet the goal of complementing and gradually replacing some of their fossil-based ***,the challenges,as well as arising opportunities of future research directions are discussed.

关键词： biofoam bio-based polyurethanes Polylactic acid Polyhydroxyalkanotate Starch Cellulose Manufacturing process

Allergen degradation of bee pollen by lactic acid bacteria fermentation and its alleviatory effects on allergic reactions in bALb/c mice

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Food Science and human Wellness 2024年第1期13卷 349-359页

作者： Shuting Yin Qiangqiang Li Yuxiao Tao Enning Zhou Kun Wang Wanwen Chen Xiangxin Li Liming Wu Institute of Apicultural Research Chinese Academy of Agricultural SciencesBeijing 100093China Department of Animal Science McGill UniversityQuebec H9X 3V9Canada State Key Laboratory of Food Science and Technology School of Food Science and TechnologyJiangnan UniversityWuxi 214122China

Food allergy as a global health problem threatens food *** pollen(bP)is a typical food with allergenic potentials,although it performs various nutritional/pharmacological functions to *** this study,lactic acid bacteria(LAb)were used to ferment brassica napus bP for alleviating its *** novel allergens(glutaredoxin,oleosin-b2,catalase and lipase)were identified with significant decreases in LAb-fermented bP(FbP)than natural bP by ***,metabolomics analysis showed significant increases of 28 characteristic oligopeptides and amino acids in FbP versus bP,indicating the degradation of LAb on ***,FbP showed alleviatory effects in bALb/c mice,which relieved pathological symptoms and lowered production of allergic *** high-throughput sequencing analysis showed that FbP could regulate gut microbiota and metabolism to strengthen immunity,which were closely correlated with the alleviation of allergic *** findings could contribute to the development and utilization of hypoallergenic bP products.

关键词： Alleviatory effects Lactic acid bacteria fermentation bee pollen allergen Gut microbiota host metabolism

high-rate lithium-ion battery performance of a ternary sea urchin-shaped CoNiO_(2)@NiP_(6)Mo_(18)/CNTs composites

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Journal of Energy Chemistry 2024年第9期96卷 516-525页

作者： Li-ping Cui Shuang Sun Kai Yu Shu Zhang Mei-lin Wang Jia-jia Chen bai-bin Zhou Key Laboratory for Photonic1nd Electronic bandgap Materials Ministry of EducationSchool of Chemistry1nd Chemical EngineeringHarbin Normal UniversityHarbin 150025HeilongjiangChina State Key Laboratory of Physical Chemistry of Solid Surfaces Department of ChemistryCollege of Chemistry1nd Chemical EngineeringCollaborative Innovation Centre of Chemistry for Energy MaterialsXiamen UniversityXiamen 361005FujianChina

bimetallic oxides are attractive anode materials for lithium-ion batteries(LIbs)due to their large theoretical ***,the low conductivity,short cycle life,and poor rate capability are the bottlenecks for their further *** overcome above issues,the basket-like polymolybdate(NiP_(6)Mo_(18))and carbon nanotubes(CNTs)were uniformly embedded on the urchin-shaped CoNiO_(2)nanospheres to yield a ternary composites CoNiO_(2)@NiP_(6)Mo_(18)/CNTs via electrostatic *** multi-level morphology of urchin spinules accelerates the diffusion rate of Li^(+);CNT improves the conductivity and enhances cycle stability of the material;and heteropoly acid contributes more redox activity ***,CoNiO_(2)@NiP_(6)Mo_(18)/CNTs as an anode of LIbs exhibits a high initial capacity(1396.7 mA h g^(−1)at 0.1 A g^(−1)),long-term cycling stability(750.2 mA h g^(−1)after 300 cycles),and rate performance(450.3 mA h g^(−1)at 2 A g^(−1)),which are superior to reported metallic oxides anode of *** density functional theory(DFT)and kinetic mechanism suggest that CoNiO_(2)@NiP_(6)Mo_(18)/CNTs delivers an outstanding pseudocapacitance and rapid Li^(+)diffusion behaviors,which is due to the rich surface area of the urchin-like CoNiO_(2)with the uniform embeddedness of NiP_(6)Mo_(18)and *** study provides a new idea for optimizing the performance of bimetallic oxides and developing high-rate lithium-ion battery composites.

关键词： bi-metal oxides Transition metal oxides Polyoxometalates Nanocomposite LIbs

Preparation of maximally-entangled states with multiple cat-state qutrits in circuit QED

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Frontiers of physics 2024年第3期19卷 239-251页

作者： Chui-Ping Yang Jia-heng Ni Liang bin Yu Zhang Yang Yu Qi-Ping Su Department of Physics Hangzhou Normal UniversityHangzhou 311121China School of Physics Nanjing UniversityNanjing 210093China Institute for Quantum Science and Technology University of CalgaryAlberta T2N 1N4Canada

In recent years,cat-state encoding and high-dimensional entanglement have attracted much ***,previous works are limited to generation of entangled states of cat-state qubits(two-dimensional entanglement with cat-state encoding),while how to prepare entangled states of cat-state qutrits or qudits(high-dimensional entanglement with cat-state encoding)has not been *** here propose to generate a maximally-entangled state of multiple cat-state qutrits(three-dimensional entanglement by cat-state encoding)in circuit *** entangled state is prepared with multiple microwave cavities coupled to a superconducting flux ququart(a four-level quantum system).This proposal operates essentially by the cavity-qutrit dispersive *** circuit hardware resource is minimized because only a coupler ququart is *** higher intermediate level of the ququart is occupied only for a short time,thereby decoherence from this level is greatly suppressed during the state ***,the state preparation time does not depend on the number of the qutrits,thus it does not increase with the number of the *** an example,our numerical simulations demonstrate that,with the present circuit QED technology,the high-fidelity preparation is feasible for a maximally-entangled state of two cat-state ***,we numerically analyze the effect of the inter-cavity crosstalk on the scalability of this *** proposal is universal and can be extended to accomplish the same task with multiple microwave or optical cavities coupled to a natural or artificial four-level atom.

关键词： maximally-entangled states cat state qutrit circuit QED

Parallel Driving with big Models and Foundation Intelligence in Cyber-hysical-ocial Spaces

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Research 2024年第2期7卷 1-17页

作者： Xiao Wang Jun huang Yonglin Tian Chen Sun Lie Yang Shanhe Lou Chen Lv Changyin Sun Fei-Yue Wang School of Artificial Intelligence Anhui UniversityHefeiChina Macao University of Science and Technology MacaoChina State Key Laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijingChina MVSLab Department of Mechanical and Mechatronics EngineeringUniversity of Waterloo200 University Ave WestWaterlooON N2L3G1Canada School of Mechanical and Aerospace Engineering Nanyang Technological UniversitySingaporeSingapore

Recent years have witnessed numerous technical breakthroughs in connected and autonomous vehicles (CAVs). On the one hand, these breakthroughs have significantly advanced the development of intelligent transportation systems (ITSs);on the other hand, these new traffic participants introduce more complex and uncertain elements to ITSs from the social space. Digital twins (DTs) provide real-time, data-driven, precise modeling for constructing the digital mapping of physical-world ITSs. Meanwhile, the metaverse integrates emerging technologies such as virtual reality/mixed reality, artificial intelligence, and DTs to model and explore how to realize improved sustainability, increased efficiency, and enhanced safety. More recently, as a leading effort toward general artificial intelligence, the concept of foundation model was proposed and has achieved significant success, showing great potential to lay the cornerstone for diverse artificial intelligence applications across different domains. In this article, we explore the big models embodied foundation intelligence for parallel driving in cyber-physical-social spaces, which integrate metaverse and DTs to construct a parallel training space for CAVs, and present a comprehensive elucidation of the crucial characteristics and operational mechanisms. beyond providing the infrastructure and foundation intelligence of big models for parallel driving, this article also discusses future trends and potential research directions, and the ?S?goals of parallel driving.

关键词： breakthrough integrate corners

broad-spectrum ginsentides are principal bioactives in unraveling the cure-all effects of ginseng

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Acta Pharmaceutica Sinica b 2024年第2期14卷 653-666页

作者： Shining Loo Antony Kam bamaprasad Dutta Xiaohong Zhang Nan Feng Siu Kwan Sze Chuan-Fa Liu Xiaoliang Wang James P.Tam School of biological Sciences Nanyang Technological UniversitySingapore 637551Singapore Academy of Pharmacy Xi’an Jiaotong-Liverpool UniversitySuzhou 215123China Department of biological Sciences Xi’an Jiaotong-Liverpool UniversitySuzhou 215123China Institute of Materia Medica Chinese Academy of Medical SciencesBeijing 100050China Department of health Sciences Brock UniversityNiagara RegionON L2S 3A1Canada

Stress and illness connection is complex and involves multiple physiological *** ginsengs,reputed for their broad-spectrum“cure-all”effect,are widely prescribed to treat stress and related ***,the identity of ginseng’s“cure-all”medicinal compounds that relieve stress remains ***,we identify ginsentides as the principal bioactives that coordinate multiple systems to restore homeostasis in response to *** are disulfide-rich,cell-penetrating and proteolytic-stable *** affinity-enrichment mass spectrometry target identification together with in vitro,ex vivo and in vivo validations,we show that highly purified or synthetic ginsentides promote vasorelaxation by producing nitric oxide through endothelial cells via intracellular PI3K/Akt signaling pathway,alleviate a1-adrenergic receptor overactivity by reversing phenylephrine-induced constriction of aorta,decrease monocyte adhesion to endothelial cells via CD166/ESAM/CD40 and inhibit P2Y12 receptors to reduce platelet *** administered ginsentides were effective in animal models to reduce ADP-induced platelet aggregation,to prevent collagen and adrenalineinduced pulmonary thrombosis as well as anti-stress behavior of tail suspension and forced swimming tests in ***,these results strongly suggest that ginsentides are the principal panacea compounds of ginsengs because of their ability to target multiple extra-and intra-cellular proteins to reverse stress-induced damages.

关键词： Ginseng Cysteine-rich peptides Microproteins Cure-all Stress homeostasis