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Development of a standardized in vitro approach to evaluate microphysical,chemical,and toxicological properties of combustion-derived fine and ultrafine particles

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Journal of Environmental Sciences 2022年第3期34卷 104-117页

作者： Ana Teresa Juarez-Facio Clement Castilla Cecile Corbiere Helene Lavanant Carlos Afonso Christophe Morin Nadine Merlet-Machour Laurence Chevalier Jean-Marie Vaugeois Jerome Yon Christelle Monteil Normandie Univ UNIROUENUNICAEN ABTE76000 RouenFrance Normandie Univ UNIROUENINSA RouenCNRSCOBRA76000 RouenFrance Normandie Univ UNIROUENINSA RouenCNRSGPM-UMR663476000 RouenFrance Normandie Univ UNIROUENINSA RouenCNRSCORIA76000 RouenFrance

Ultrafine particles represent a growing concern in the public health community but their precise role in many illnesses is still unknown. This lack of knowledge is related to the experimental difficulty in linking their biological effects to their multiple properties, which are important determinants of toxicity. Our aim is to propose an interdisciplinary approach to study fine(FP) and ultrafine(UFP) particles, generated in a controlled manner using a mini CAST(Combustion Aerosol Standard) soot generator used with two different operating conditions(CAST1 and CAST3). The chemical characterization was performed by an untargeted analysis using ultra-high resolution mass spectrometry. In conjunction with this approach, subsequent analysis by gas chromatography–mass spectrometry(GC–MS) was performed to identify polycyclic aromatic hydrocarbons(PAH). CAST1 enabled the generation of FP with a predominance of small PAH molecules, and CAST3 enabled the generation of UFP, which presented higher numbers of carbon atoms corresponding to larger PAH molecules. Healthy normal human bronchial epithelial(NHBE) cells differentiated at the air-liquid interface(ALI) were directly exposed to these freshly emitted FP and UFP. Expression of MUC5AC, FOXJ1, OCLN and ZOI as well as microscopic observation confirmed the ciliated pseudostratified epithelial phenotype. Study of the mass deposition efficiency revealed a difference between the two operating conditions, probably due to the morphological differences between the two categories of particles. We demonstrated that only NHBE cells exposed to CAST3 particles induced upregulation in the gene expression of IL-8 and NQO1. This approach offers new perspectives to study FP and UFP with stable and controlled properties.

关键词： In vitro Air-liquid interface MiniCAST Fine and ultrafine particles Organic compounds OC/TC

A 3D numerical simulation of laser-induced incandescence of soot particles in coal combustion products

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2009年第9期10卷 1320-1326页

作者： Ling-hong CHEN Ke-fa CEN Annie GARO Gerard GREHAN State Key Laboratory of Clean Energy Utilization Zhejiang University Hangzhou 310027 China LESP UMR 6614/CORIA CNRS/Universite et INSA de Rouen Saint Etienne du Rouvray 76800 France

Laser-induced incandescence (LII) has received increasing attention as a potentially powerful technique for in-situ measuring of the volume fraction and primary size of soot particles in combustion systems. In this study, a 3D Monte Carlo simulation combined with a Mie equation was developed to analyze the influence of spectral absorption and scattering on the measured LII flux emitted by soot particles. This paper represents a first attempt to analyze soot measurement using the LII technique in coal combustion products. The combustion products of gases (CO2, N2), soot, and fly-ash particles, present between the location of laser-excited soot and the LII flux receiver. The simulation results indicated that an almost Beer-Lambert exponential decrease in LII flux occurred with an increase in the volume fraction of soot particles, while a nearly linear decrease occurred with an increase in the volume fraction of fly-ash particles. The results also showed that scattering effects of both soot and fly-ash particles on the LII flux could be neglected. Compared with the absorption of gases, a decrease of 20% of LII flux was observed with soot particles, and a decrease of 10% with fly-ash particles.

关键词： Laser-induced incandescence (LII) Soot Fly-ash 3D Monte Carlo Scattering Absorption

Physical design and recent experimental results of the new ICRF antenna on EAST

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Plasma Science and Technology 2024年第6期26卷 169-176页

作者：杨桦张新军袁帅秦成明张伟 G.URBANCZYK 钱金平刘鲁南王高翔陈青青 Institute of Plasma Physics Chinese Academy of SciencesHefei 230031People’s Republic of China Institut Jean Lamour UMR 7198 cnrs-Universitéde Lorraine 2 allée André GuinierNancy 54011France University of Science and Technology of China Hefei 230026People’s Republic of China

Two new ICRF antennas operating in the ion cyclotron radio frequency(ICRF) range have been developed for EAST to overcome the low coupling problem of the original *** original ICRF antennas were limited in their power capacity due to insufficient *** new antenna design takes into account both wave coupling and absorption processes through comprehensive wave coupling and absorption codes,with the dominant parallel wave number k∥of 7.5 m-1at dipole *** the use of these new ICRF antennas,we are able to achieve 3.8 MW output power and 360 s operation,*** initial experimental results demonstrate the reliability of the antenna design method.

关键词： ICRF antenna coupling EAST

Exploring fs-laser irradiation damage subthreshold behavior of dielectric mirrors via electrical measurements

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High Power Laser Science and Engineering 2024年第2期12卷 24-32页

作者： Petrisor Gabriel Bleotu Radu Udrea Alice Dumitru Olivier Uteza Maria-Diana Mihai Dan Gh Matei Daniel Ursescu Stefan Irimiciuc Valentin Craciun Extreme Light Infrastructure-Nuclear Physics(ELI-NP) Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering(IFIN-HH)MagureleRomania Doctoral School of Physics University of BucharestMagureleRomania LULI-cnrs CEAUniversite SorbonneEcole PolytechniqueInstitut Polytechnique de ParisPalaiseau CEDEXFrance Apel Laser IlfovRomania Aix-Marseille University CNRSLP3 UMR 7341MarseilleFrance Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering(IFIN-HH) MagureleRomania University Politehnica of Bucharest BucharestRomania National Institute for Lasers Plasma and Radiation Physics MagureleRomania

With ultrafast laser systems reaching presently 10 PW peak power or operating at high repetition rates,research towards ensuring the long-term,trouble-free performance of all laser-exposed optical components is *** work is focused on providing insight into the optical material behavior at fluences below the standardized laser-induced damage threshold(LIDT)value by implementing a simultaneous dual analysis of surface emitted particles using a Langmuir probe(LP)and the target current(TC).HfO_(2) and ZrO_(2) thin films deposited on fused silica substrates by pulsed laser deposition at various O_(2) pressures for defect and stoichiometry control were irradiated by Gaussian,ultrashort laser pulses(800 nm,10 Hz,70 fs)in a wide range of *** TC and LP collected signals were in good agreement with the existing theoretical description of laser–matter interaction at an ultrashort time *** approach for an in situ LIDT monitoring system provides measurable signals for below-threshold irradiation conditions that indicate the endurance limit of the optical surfaces in the single-shot energy scanning *** LIDT value extracted from the LP-TC system is in line with the multipulse statistical analysis done with ISO 21254-2:2011(E).The implementation of the LP and TC as on-shot diagnostic tools for optical components will have a significant impact on the reliability of next-generation ultrafast and high-power laser systems.

关键词： HfO_(2) in situ detection Langmuir probe laser-induced damage threshold target current ZrO_(2)

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High-speed silicon photonic electro-optic Kerr modulation

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Photonics Research 2024年第1期12卷 51-60页

作者： JONATHAN PELTIER WEIWEI ZHANG LEOPOLD VIROT CHRISTIAN LAFFORGUE LUCAS DENIEL DELPHINE MARRIS-MORINI GUY AUBIN FARAH AMAR DENH TRAN XINGZHAO YAN CALLUM G.LITTLEJOHNS CARLOS ALONSO-RAMOS KE LI DAVID J.THOMSON GRAHAM REED LAURENT VIVIEN University Paris-Saclay CNRSCentre for Nanoscience and Nanotechnology(C2N)Palaiseau 91120France University Grenoble Alpes CEALETIGrenoble 38000France Optoelectronics Research Centre Zepler Institute for Photonics and NanoelectronicsFaculty of Engineering and Physical SciencesUniversity of SouthamptonSouthampton SO171BJUK

Silicon-based electro-optic modulators contribute to easing the integration of high-speed and low-power consumption circuits for classical optical communications and data *** the plasma dispersion modulation,an alternative solution in silicon is to exploit the DC Kerr effect,which generates an equivalent linear electro-optical effect enabled by applying a large DC electric *** some theoretical and experimental studies have shown its existence in silicon,limited contributions relative to plasma dispersion have been achieved in high-speed modulation so *** paper presents high-speed optical modulation based on the DC Kerr effect in silicon PIN *** contributions of both plasma dispersion and Kerr effects have been analyzed in different waveguide configurations,and we demonstrated that the Kerr induced modulation is dominant when a high external DC electric field is applied in PIN ***-speed optical modulation response is analyzed,and eye diagrams up to 80 Gbit/s in NRZ format are obtained under a *** of 30 *** work paves the way to exploit the Kerr effect to generate high-speed Pockels-like optical modulation.

关键词： waveguide dispersion effect

A phase field model for snow crystal growth in three dimensions

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npj Computational Materials 2017年第1期3卷 350-356页

作者： Gilles Demange Helena Zapolsky Renaud Patte Marc Brunel GPM UMR CNRS 6643University of RouenSaint Etienne du Rouvray 76575France coria UMR 6614 University of RouenSaintÉtienne du Rouvray 76575France

Snowflake growth provides a fascinating example of spontaneous pattern formation in *** to understand this phenomenon have led to important insights in non-equilibrium dynamics observed in various active scientific fields,ranging from pattern formation in physical and chemical systems,to self-assembly problems in ***,very few models currently succeed in reproducing the diversity of snowflake forms in three dimensions,and the link between model parameters and thermodynamic quantities is not ***,we report a modified phase field model that describes the subtlety of the ice vapour phase transition,through anisotropic water molecules attachment and condensation,surface diffusion,and strong anisotropic surface tension,that guarantee the anisotropy,faceting and dendritic growth of *** demonstrate that this model reproduces the growth dynamics of the most challenging morphologies of snowflakes from the Nakaya *** find that the growth dynamics of snow crystals matches the selection theory,consistently with previous experimental observations.

关键词： dimensions phase field

Large contributions of emission reductions and meteorological conditions to the abatement of PM_(2.5)in Beijing during the 24th Winter Olympic Games in 2022

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Journal of Environmental Sciences 2024年第2期136卷 172-188页

作者： Yaping Jiang Shaocai Yu Xue Chen Yibo Zhang Mengying Li Zhen Li Zhe Song Pengfei Li Xiaoye Zhang Eric Lichtfouse Daniel Rosenfeld Key Laboratory of Environmental Remediation and Ecological Health Ministry of EducationResearch Center for Air Pollution and HealthCollege of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China College of Science and Technology Hebei Agricultural UniversityBaoding 071000China Chinese Academy of Meteorological Sciences China Meteorological AdministrationBeijing 100081China Aix-Marseille Univ CNRSColl FranceCNRSIRDINRAEEuropole Mediterraneen de l’ArboisAvenue Louis Philibert13100 Aix en ProvenceFrance Xi’an Jiaotong University State Key Laboratory of Multiphase Flow in Power EngineeringXi’an 710049China Institute of Earth Sciences The Hebrew University of JerusalemJerusalemIsrael

To guarantee the blue skies for the 2022 Winter Olympics held in Beijing and Zhangjiakou from February 4 to 20,Beijing and its surrounding areas adopted a series of emission control *** provides an opportunity to determine the impacts of large-scale temporary control measures on the air quality in Beijing during this special ***,we applied the WRF-CMAQ model to quantify the contributions of emission reduction measures and meteorological *** show that meteorological conditions in 2022 decreased PM_(2.5)in Beijing by 6.9 and 11.8μg/m^(3)relative to 2021 under the scenarios with and without emission reductions,*** emission reduction measures implemented in Beijing and seven neighboring provinces resulted in an average decrease of 13.0μg/m^(3)(-41.2%)in PM_(2.5)in *** the entire period,local emission reductions contributed more to good air quality in Beijing than nonlocal emission *** the emission reduction scenario,local,controlled regions,other regions,and boundary conditions contributed 47.7%,42.0%,5.3%,and 5.0%to the PM_(2.5)concentrations in Beijing,*** results indicate that during the cleaning period with the air masses from the northwest,the abatements of PM_(2.5)were mainly caused by local emission ***,during the potential pollution period with the air masses from the east-northeast and west-southwest,the abatements of PM_(2.5)were caused by both local and nonlocal emission reductions almost *** implies that regional coordinated prevention and control strategies need to be arranged scientifically and rationally when heavy pollution events are forecasted.

关键词： PM_(2.5) WRF-CMAQ Meteorological conditions Emission reductions Winter Olympic games

Semi-analytical Monte Carlo simulation of laser-induced fluorescence propagation in an optically participating spray

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2007年第7期8卷 1170-1178页

作者： CHEN Ling-hong ROZE Claude GARO Annie GIRASOLE Thierry CEN Ke-fa GREHAN Gérard State Key Laboratory of Clean Energy Utilization Zhejiang University Hangzhou 310027 China Laboratoire d＇Electromagnétisme et Systémes Particulaires Universite ＆ INSA Rouen CORIA/CNRS UMR 6614 France

A semi-analytical Monte Carlo (SMC) simulation was developed to simulate the propagation of laser-induced fluo- rescence (LIF) in an optically participating spray, which simultaneously exhibits spectrally dependent emission, anisotropic scattering, absorption, and re-emission. The SMC simulation is described and then applied to an experimental configuration of a cloud of polydisperse droplets composed of water and sulforhodamine B dye. In the SMC simulation, the collected LIF flux on the remote receptor element is calculated as the global contribution from the emissive source, single, twice, … and nth collision events in any sequence. The effects on the fluorescence photons propagation of spray parameters like the dye concentration, droplets concentration, and droplets size are examined. Three spectral bands representing different optical properties are chosen to analyze the interference of absorption, scattering and re-emission on the detected LIF flux. The obtained spectral LIF flux distribution on the receptor demonstrates a “red shift” phenomenon.

关键词： Laser-induced fluorescence (LIF) Semi-analytical Monte Carlo (SMC) simulation Absorption Anisotropic scattering Re-emission Spray

How Marie Sklodowska-Curie Doctoral Networks Can Support European Refractory Ecosystem in Context of The European Green Deal

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China's Refractories 2024年第2期33卷 1-9页

作者： Marc HUGER Glyn DERRICK Mossaab MOUIYA Andrea SALERNO Kwasi Addo BOATENG Hrikeshava RANGANATHAN Amit Kumar GOPE Institute of Research for Ceramics(IRCER-UMR cnrs 7315) University of LimogesLimoges 87000France

The movement of the Iron&Steelmaking(I&S)industry towards Net-Zero emissions and digitalized processes through disruptive,breakthrough technologies will be achieved through the use of *** biggest challenge for the refractory industry is to continue to meet the performance expectations while,at the same time,moving to a more sustainable production *** complexity and urgency of these technological changes,highlighted by the European Green Deal,requires ambitious,international,interdisciplinary and intersectoral projects,bringing together institutes from across the global value chain,to carry out cutting edge *** European Union,through its flagship doctoral training program,MSCA,has,and continues to support research and development as well as the promotion of the refractory industry in *** introduction to two MSCA projects and some of the results achieved are highlighted within this article.

关键词： FIRE network Horizon 2020 Horizon Europe Marie Sklodowska-Curie Actions Doctoral networks European Green Deal