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Trace Element Mobility in Subducted Marble and Associated Eclogite:Constraints from UHP Rocks in the Shuanghe Area,Central-East China

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Journal of Earth Science 2024年第1期35卷 1-15页

作者： Xingao Hou Zhiqiang Yu Shefa Chen Lei Liu Yilin Xiao key laboratory of Metallogenic Prediction of Nonferrous Metals and Geological environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China key laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China cas key laboratory of Crust-Mantle Materials and environments School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

In order to decipher element mobility in UHP meta-sedimentary rocks in the continental subduction zone,major and trace element compositions are investigated for a continuous profile from a representative UHP region in the Dabie *** the lithologic contact zone,contents of K,Ca,LREE,and LILE exhibit varying degrees of downward trends in both marble and eclogite toward the contact zone,indicating that marble and their associated eclogite can release a large amount of K,Ca,and a small number of LILEs and *** is the main Ti phase in both marble and *** rims around rutile can occasionally be seen in *** of Ti and HFSE exhibit a well-coupled relation among marble and eclogite,indicating that substantial Ti and HFSEs were migrated from eclogite to marble,in accord with the capacity of a melt *** and titanites in marble exhibit a relatively limited variation in Nb/Ta ratios(12.9-16.2),similar to those of titanites in eclogite(14.2-16.7),which demonstrates that rutiles and titanites in marble were sourced from eclogite because of short-distance migrations of Ti and *** to the P-T path and the temperature and pressure conditions of the peak metamorphism reported by previous studies,the eclogite associated with marble may not form supercritical fluids in the subduction zone because of the addition of carbonate minerals.

关键词： UHP metamorphism eclogite marble element migration fluid actions geochemistry

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Influence of meteorological factors on open biomass burning at a background site in Northeast China

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Journal of environmental Sciences 2024年第4期138卷 1-9页

作者： Yulong Wang Linlin Liang Wanyun Xu Chang Liu Hongbing Cheng Yusi Liu Gen Zhang Xiaobin Xu Dajiang Yu Peng Wang Qingli Song Jiumeng Liu Yuan Cheng State key laboratory of Urban Water Resource and environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China State key laboratory of Severe Weather&key laboratory for Atmospheric Chemistry Chinese Academy of Meteorological SciencesBeijing 100081China Longfengshan Regional Background Station China Meteorological AdministrationHeilongjiang 150200China Heilongjiang Climate Center Heilongjiang 150030China

Biomass burning(BB)is a very important emission source that significantly adversely impacts regional air *** produces a large number of primary organic aerosol(POA)and black carbon(BC).Besides,BB also provides many precursors for secondary organic aerosol(SOA)*** this work,the ratio of levoglucosan(LG)to organic carbon(OC)and the fire hotspots map was used to identify the open biomass burning(OBB)events,which occurred in two representative episodes,October 13 to November 30,2020,and April1 to April 30,*** ratio of organic aerosol(OA)to reconstructed PM_(2.5)concentration(PM_(2.5)^(*))increased with the increase of LG/*** LG/OC ratio is higher than 0.03,the highest OA/PM_(2.5)^(*)ratio can reach 80%,which means the contribution of OBB to OA is *** to the ratio of LG to K^(+),LG to mannosan(MN)and the regional characteristics of Longfengshan,it can be determined that the crop residuals are the main *** occurrence of OBB coincides with farmers’preferred choices,i.e.,burning biomass in“bright weather”.The“bright weather”refers to the meteorological conditions with high temperature,low humidity,and without *** factors indirectly affect regional biomass combustion pollution by influencing farmers’active choices.

关键词： Air pollution Biomass burning Meteorological factors Organic trace Agricultural fires

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Role of methoxy and C_(α)-based substituents in electrochemical oxidation mechanisms and bond cleavage selectivity of β-O-4 lignin model compounds

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Green Energy & environment 2024年第1期9卷 114-125页

作者： Yang Zhou Qiang Zeng Hongyan He Kejia Wu Fuqiao Liu Xuehui Li School of Chemistry and Chemical Engineering The Guangdong Provincial Key Laboratory of Green Chemical Product TechnologyState Key Laboratory of Pulp and Paper EngineeringSouth China University of TechnologyGuangzhouGuangdong510640China cas key laboratory of Green Process and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing100190China

In order to better understand the specific substituent effects on the electrochemical oxidation process of β-O-4 bond, a series of methoxyphenyl type β-O-4 dimer model compounds with different localized methoxyl groups, including 2-(2-methoxyphenoxy)-1-phenylethanone, 2-(2-methoxyphenoxy)-1-phenylethanol, 2-(2-methoxyphenoxy)-1-(4-methoxyphenyl)ethanone, 2-(2-methoxyphenoxy)-1-(4-methoxyphenyl)ethanol, 2-(2,6-dimethoxyphenoxy)-1-(4-methoxyphenyl)ethanone, 2-(2,6-dimethoxyphenoxy)-1-(4-methoxyphenyl)ethanol have been selected and their electrochemical properties have been studied experimentally by cyclic voltammetry, and FT-IR spectroelectrochemistry. Combining with electrolysis products distribution analysis and density functional theory calculations, oxidation mechanisms of all six model dimers have been explored. In particular, a total effect from substituents of both para-methoxy(on the aryl ring closing to Cα) and Cα-OH on the oxidation mechanisms has been clearly observed, showing a significant selectivity on the Cα-Cβbond cleavage induced by electrochemical oxidations.

关键词： Lignin model compounds β-O-4 dimers Electrochemical oxidation Oxidation mechanisms Substituent effect

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Enhanced photoelectrochemical water splitting with a donor-acceptor polyimide

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Frontiers in Energy 2024年第4期18卷 463-473页

作者： Hongyu QU Xiaoyu XU Longfei HONG Xintie WANG Yifei ZAN Huiyan ZHANG Xiao ZHANG Sheng CHU key laboratory of Energy Thermal Conversion and Control of the Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China State key laboratory of Clean Energy Utilization Zhejiang UniversityHangzhou 310027China

Polyimide(PI)has emerged as a promising organic photocatalyst owing to its distinct advantages of high visible-light response,facile synthesis,molecularly tunable donor-acceptor structure,and excellent physicochemical ***,the synthesis of high-quality PI photoelectrode remains a challenge,and photoelectrochemical(PEC)water splitting for PI has been less ***,the synthesis of uniform PI photoelectrode films via a simple spin-coating method was reported,and their PEC properties were investigated using melamine as donor and various anhydrides as *** influence of the conjugate size of aromatic unit(phenyl,biphenyl,naphthalene,perylene)of electron acceptor on PEC performance were studied,where naphthalene-based PI photoelectrode exhibited the highest photocurrent *** is resulted from the unification of widerange light absorption,efficient charge separation and transport,and strong photooxidation *** paper expands the material library of polymer films for PEC applications and contributes to the rational design of efficient polymer photoelectrodes.

关键词： polyimide(PI)film photoelectrochemistry band structure engineering aromatic unit

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A systematic review of the inequality of health burdens related to climate change

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Frontiers of environmental Science & Engineering 2024年第5期18卷 137-153页

作者： Xinke Song Shihui Zhang Hai Huang Qun Ding Fang Guo Yaxin Zhang Jin Li Mingyu Li Wenjia Cai Can Wang State key Joint laboratory of environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Department of Earth System Science Tsinghua UniversityBeijing100084China

Climate change significantly impacts human health,exacerbating existing health inequalities and creating new *** study addresses the lack of systematic review in this area by analyzing 2440 publications,focusing on four key terms:health,disparities,environmental factors,and climate *** inclusion criteria limited the selection to English-language,peer-reviewed articles related to climate health hazards,ensuring the relevance and rigor of the synthesized *** process synthesized 65 relevant *** investigation revealed that recent research,predominantly from developed countries,has broadened its scope beyond temperature-related impacts to encompass diverse climate hazards,including droughts,extreme weather,floods,mental health issues,and the intersecting effects of Coronavirus Disease *** has highlighted exposure as the most studied element in the causal chain of climate change-related health inequalities,followed by adaptive capability and inherent *** most significant vulnerabilities were observed among populations with low socioeconomic status,ethnic minorities,and *** study further reveals research biases and methodological limitations,such as the paucity of attention to underdeveloped regions,a narrow focus on non-temperature-related hazards,challenges in attributing climate change effects,and a deficit of large-scale empirical *** findings call for more innovative research approaches and a holistic integration of physical,socio-political,and economic dimensions to enrich climate-health discourse and inform equitable policy-making.

关键词： Climate change Health impact Human well-being Inequality Vulnerability

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Molybdenum isotope composition of the upper mantle and its origin:insight from mid-ocean ridge basalt

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Journal of Oceanology and Limnology 2024年第3期42卷 705-708页

作者： Shuo CHEN key laboratory of Marine Geology and environment Institute of OceanologyChinese Academy of SciencesQingdao 266071China

The molybdenum(Mo)isotope system is pivotal in reconstructing marine redox changes throughout Earth’s history and has emerged as a promising tracer for igneous and metamorphic *** its composition and variation across major geochemical reservoirs is essential for its application in investigating high-temperature ***,there is debate regarding theδ^(98/95)Mo value of the Earth’s mantle,with estimates ranging from sub-chondritic to super-chondritic *** analyses of global mid-ocean ridge basalt(MORB)glasses revealed significantδ^(98/95)Mo variations attributed to mantle heterogeneity,proposing a two-component mixing model to explain the observed *** studies confirmed the sub-chondriticδ^(98/95)Mo of the depleted upper mantle,suggesting remixing of subduction-modified oceanic crust as a plausible *** findings underscore the role of Mo isotopes as effective tracers for understanding dynamic processes associated with mantle-crustal recycling.

关键词： molybdenum(Mo)isotope mantle crustal recycling mid-ocean ridge basalt(MORB)

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Passivation remediation of weakly alkaline Cd-contaminated soils using combined treatments of biochar and sepiolite

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Ecological Processes 2024年第1期13卷 40-52页

作者： Yuxin Zhang Shan Gao Hongtao Jia Tao Sun Shunan Zheng Shihang Wu Yuebing Sun key laboratory of Original Agroenvironmental Pollution Prevention and Control Ministry of Agriculture and Rural Affairs (MARA)/Tianjin Key Laboratory of Agro-Environment and Agro-Product Safety Agro–Environmental Protection InstituteMARA College of Resources and environment Sciences Xinjiang Agricultural University Rural Energy and environment Agency Ministry of Agriculture and Rural Affairs

Background Cadmium(Cd) pollution in agricultural soils has become a priority environmental concern globally. A reasonable application of passivators is critical to address the problem. In this study, we examined the remediation effects of rice husk biochar(r BC) and sepiolite(Sep) as single and combined(r BC + Sep) treatments on Cd pollution in a weakly alkaline soil using three maize cultivars(Liyu 16, Zhengdan 958, and Sanbei 218) as test crops. We also explained the mechanisms involved in the remediation *** The pseudo-second-order kinetic equation and Langmuir model could well describe the adsorption process of r BC + Sep for Cd2+. Compared with the control treatment(CK), soil available Cd concentration decreased by 29.51–36.34% under r BC + Sep treatment(p 0.05).Conclusions The application of 0.2% r BC + 0.5% Sep composite passivation material to weakly alkaline Cd-contaminated soil can effectively reduce the Cd concentration of soil and maize.

关键词： Cd Rice husk biochar Sepiolite Passivation restoration Weakly alkaline soil Maize

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Assessment of International GNSS Service Global Ionosphere Map products over China region based on measurements from the Crustal Movement Observation Network of China

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Earth and Planetary Physics 2024年第2期8卷 400-407页

作者： Jin Hu HaiBing Ruan FuQing Huang ShengYang Gu XianKang Dou Institute of Space Weather Nanjing University of Information Science and TechnologyNanjing 210044China State key laboratory of Space Weather Chinese Academy of Sciences(CAS)Beijing 100190China School of Electronic Information Wuhan UniversityWuhan 430072China Wuxi Research Institute Nanjing University of Information Science and TechnologyWuxi Jiangsu 214000China cas key laboratory of Geospace environment School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

The global ionosphere maps(GIM)provided by the International GNSS Service(IGS)are extensively utilized for ionospheric morphology monitoring,scientific research,and practical *** the credibility of GIM products in data-sparse regions is of paramount *** this study,measurements from the Crustal Movement Observation Network of China(CMONOC)are leveraged to evaluate the suitability of IGS-GIM products over China region in *** indices of mean error(ME),root mean square error(RMSE),and normalized RMSE(NRMSE)are then utilized to quantify the accuracy of IGS-GIM *** revealed distinct local time and latitudinal dependencies in IGS-GIM errors,with substantially high errors at nighttime(NRMSE:39%)and above 40°latitude(NRMSE:49%).Seasonal differences also emerged,with larger equinoctial deviations(NRMSE:33.5%)compared with summer(20%).A preliminary analysis implied that the irregular assimilation of sparse IGS observations,compounded by China’s distinct geomagnetic topology,may manifest as error *** results suggest that modeling based solely on IGS-GIM observations engenders inadequate representations across China and that a thorough examination would proffer the necessary foundation for advancing regional total electron content(TEC)constructions.

关键词： International GNSS Service(IGS)Global Ionosphere Maps(GIM) Crustal Movement Observation Network of China(CMONOC) total electron content(TEC) data assessment

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Effect of movability of water on the low-velocity pre-Darcy flow in clay soil

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3299-3310页

作者： Hui Cheng Fugang Wang Shengwei Li Xiaotong Guan Guohua Yang Zhongle Cheng Ceting Yu Yilong Yuan Guanhong Feng key laboratory of Groundwater Resources and environment Ministry of EducationJilin UniversityChangchun130012China Jilin Provincial key laboratory of Water Resources and Water environment Jilin UniversityChangchun130012China Chengdu Center China Geological SurveyChengdu610081China

Water seepage in soil is a fundamental problem involving various scientific and engineering *** to the literature,low-velocity water seepage in low-permeability porous media,such as clay,does not follow Darcy's law,also known as pre-Darcy *** formation of immovable water due to water adsorption on the pore wall is believed to be responsible for the formation of pre-Darcy ***,this view lacks direct solid *** investigate the pre-Darcy water flow in clay,head permeability experiments are conducted on six clay samples with different *** results indicate that water seepage in clay at low hydraulic gradients does not follow Darcy's law.A clear nonlinear relationship between flow velocity and hydraulic gradient is *** flow in clay can be divided into the pre-Darcy flow and Darcy flow regions by the critical hydraulic gradient,which is 10-12 for the Albic soil with dry density between 1.3 g/cm^(3)and 1.8 g/cm^(3).According to the disjoining pressure theory,immovable water due to water adsorption on the pore wall is the primary reason for water flow deviating from Darcy's law in *** results indicate that the percentage of movable water ranges from 39.7%to 59.3%for the six samples at a hydraulic gradient of *** the hydraulic gradient increases,the percentage of moveable water also ***,there is a strong correlation between the percentage of movable water and the variation in hydraulic conductivity with the hydraulic ***,a quantitative relationship between the percentage of movable water and the hydraulic conductivity has been *** results of this study suggest that water adsorption on the pore wall not only affects the water movability,but is also closely related to the pre-Darcy flow phenomenon in clay.

关键词： Pre-Darcy flow Clay Critical hydraulic gradient Water movability analysis

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Nitrite-driven anaerobic ethane oxidation

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environmental Science and Ecotechnology 2024年第5期21卷 361-368页

作者： Cheng-Cheng Dang Yin-Zhu Jin Xin Tan Wen-Bo Nie Yang Lu Bing-Feng Liu De-Feng Xing Nan-Qi Ren Guo-Jun Xie State key laboratory of Urban Water Resource and environment School of EnvironmentHarbin Institute of TechnologyHarbin150090China key laboratory of the Three Gorges Region's Eco-environment Ministry of EducationCollege of Environment and EcologyChongqing UniversityChongqing400044China Water Innovation and Smart environment laboratory School of Civil and Environmental EngineeringFaculty of EngineeringQueensland University of TechnologyBrisbaneQueensland4001Australia

Ethane,the second most abundant gaseous hydrocarbon in vast anoxic environments,is an overlooked greenhouse *** anaerobic oxidation of ethane can be driven by available electron acceptors such as sulfate and ***,despite nitrite being a more thermodynamically feasible electron acceptor than sulfate or nitrate,little is known about nitrite-driven anaerobic ethane *** this study,a microbial culture capable of nitrite-driven anaerobic ethane oxidation was enriched through the long-term operation of a nitrite-and-ethane-fed *** continuous operation,the nitrite removal rate and the theoretical ethane oxidation rate remained stable at approximately 25.0 mg NO_(2) eN L^(-1) d^(-1) and 11.48 mg C2H6 L^(-1) d^(-1),*** tests demonstrated that ethane is essential for nitrite removal in this microbial *** function analysis revealed that a species affiliated with a novel genus within the family Rhodocyclaceae,designated as'Candidatus Alkanivoras nitrosoreducens',may perform the nitrite-driven anaerobic ethane *** the proposed metabolic model,despite the absence of known genes for ethane conversion to ethyl-succinate and succinate-CoA ligase,'***'encodes a prospective fumarate addition pathway for anaerobic ethane oxidation and a complete denitrification pathway for nitrite reduction to *** findings advance our understanding of nitrite-driven anaerobic ethane oxidation,highlighting the previously overlooked impact of anaerobic ethane oxidation in natural ecosystems.

关键词： Anaerobic ethane oxidation Denitrification Microbial culture Fumarate addition pathway Greenhouse gas

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