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A novel strategy of tannery sludge disposal–converting into biochar and reusing for Cr(Ⅵ)removal from tannery wastewater

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Journal of environmental Sciences 2024年第4期138卷 637-649页

作者： Zhiwei Li Di Yu Xingdong Wang Xuejiao Liu Zhen Xu Yin Wang cas key laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China Zhejiang key laboratory of Urban environmental Processes and Pollution Control CAS Haixi Industrial Technology Innovation Center in BeilunNingbo 315830China key laboratory of Urban environment and Health Ningbo Observatio

Tannery sludge with high chromium content has been identified as hazardous solid waste due to its potential toxic *** safety disposal and valorization of the tannery sludge remains a *** this study,the chromium stabilization mechanism was systematically investigated during chromium-rich tannery sludge was converted to biochar and the removal performance of the sludge biochar(SBC)for Cr(Ⅵ)from tannery wastewater was also *** results showed that increase in pyrolysis temperature was conductive to the stabilization of Cr and significant reduction of the proportion of Cr(Ⅵ)in *** was confirmed that the stabilization of chromium mainly was attributed to the embedding of chromium in the C matrix and the transformation of the chromium-containing substances from the amorphous Cr(OH)_(3)to the crystalline state,such as(FeMg)Cr_(2)O_(5).The biochar presented high adsorption capacity of Cr(Ⅵ)at low pH and the maximal theoretical adsorption capacity of SBC produced at 800°C can reach 352 mg Cr(Ⅵ)/g,the process of which can be well expressed by Langmuir adsorption isotherm and pseudo second order *** electrostatic effect and reduction reaction were dominantly responsible for the Cr(Ⅵ)adsorption by ***,this study provided a novel strategy for the harmless disposal and resource utilization for the solid waste containing chromium in leather industry.

关键词： Chromium-rich tannery sludge Pyrolysis Biochar Stabilizationmechanisms Cr(Ⅵ)adsorption

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The interannual periodicity of precipitation and its links to the large-scale circulations over the Third Pole

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Journal of Geographical Sciences 2024年第8期34卷 1457-1471页

作者： LIANG Liqiao LIU Qiang LI Jiuyi State key laboratory of Tibetan Plateau Earth System Environment and Resources(TPESER)Institute of Tibetan Plateau ResearchCASBeijing 100101China State key laboratory of Water environment Simulation School of EnvironmentBeijing Normal UniversityBeijing 100875China key laboratory for Water and Sediment Sciences Ministry of EducationSchool of EnvironmentBeijing Normal UniversityBeijing 100875China key laboratory of Water Cycle and Related Land Surface Processes Institute of Geographic Sciences and Natural Resources ResearchCASBeijing 100101China

To understand the spatio-temporal variability of precipitation(P)in the Third Pole region(centered on the Tibetan Plateau-TP),it is necessary to quantify the interannual periodicity of P and its relationship with large-scale *** this study,Morlet wavelet transform was used to detect significant(p<0.05)periodic characteristics in P data from meteorological stations in four climate domains in the Third Pole,and to reveal the major large-scale circulations that triggered the variability of periodic P,in addition to bringing large amounts of water *** wavelet transform results were as follows.(1)Significant quasiperiodicity varied from 2 to 11 *** high-frequency variability mode(2 to 6 years quasi-periods)was universal,and the low-frequency variability mode(7 to 11 years quasi-periods)was rare,occurring mainly in the westerlies and Indian monsoon domains.(2)The majority of periods were base periods(53%),followed by two-base *** all stations in the Third Pole(95%)showed one or two periods.(3)Periodicity was widely detected in the majority of years(84%).(4)The power spectra of P in the four domains were dominated by statistically significant high-frequency oscillations(ie.,with short periodicity).(5)Large-scale circulations directly and indirectly influenced the periodic P variability in the different *** mode of P variability in the different domains was influenced by interactions between large-scale circulation features and not only by the dominant circulation and its control of water vapour *** results of this study will contribute to better understanding of the causal mechanisms associated with P variability,which is important for hydrological science and waterresourcemanagement.

关键词： precipitation interannual periodicity Morlet wavelet large-scale circulations Third Pole

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The risk factors and threshold level of subchronic inhalation exposure of reclaimed water

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Journal of environmental Sciences 2024年第3期137卷 639-650页

作者： Jiayang Kong Yun Lu Yunru Ren Menghao Chen Gang Liu Liangliang Shi State key Joint laboratory of environment Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Inhalation of reclaimed water is known to cause lung infammation,and free endotoxins have been shown to be a major risk factor for acute *** exposure has also been shown to induce infammatory responses with visible tissue ***,subchronic risk factors have yet to be identified,and a threshold for the protection of occupational populations during urban reuse is *** this study,potential risk factors in reclaimed water were examined by subchronic exposure with fractionated reclaimed water,and the health risk threshold was tested with a series of diluted reclaimed ***,following a 12-week exposure,macromolecules and microorganisms were found to be two major risk factors in reclaimed water that could cause pulmonary infammation,including increased proportion of polymorphonuclear leukocytes in bronchoalveolar fuid,formation of inducible bronchus-associated lymphoid tissue,and elevation of Immunoglobulin A ***,infammation persisted after a 4-week recovery *** calculated threshold of reclaimed water exposure for mice was 31.8 Endotoxin Unit(EU)/(kg·day)under when exposed to 50%additional relative humidity from reclaimed water at 25℃ for 2 hr/***,the subchronic threshold estimate for humans under the same exposure conditions was found to be 12.2 EU/(kg·day),corresponding to endotoxin levels of 61.7 EU/mL in reclaimed *** threshold level of endotoxin was lower than that in most non-potable reclaimed *** findings of this study suggest that occupational exposure of reclaimed water can serve as a potential risk to workers.

关键词： Reclaimed water Inhalation exposure Risk factor Threshold Infammation Endotoxin

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Selective adsorption of tetracycline by β-CD-immobilized sodium alginate aerogel coupled with ultrafiltration for reclaimed water

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Chinese Journal of Chemical Engineering 2024年第4期68卷 27-34页

作者： Xi Quan Jun Zhang Linlin Yin Wei Zuo Yu Tian State key laboratory of Urban Water Resource and environment(SKLUWRE) School of EnvironmentHarbin Institute of TechnologyHarbin 150090China

In this work,a novel composite material based on β-cyclodextrin-immobilized sodium alginate aerogel(β-CD/NaAlg) was developed utilizing cross-linker of epichlorohydrin and applied as an adsorbent to remove tetracycline antibiotics from reclaimed wastewater.A series of characterizations were utilized to confirm the successful synthesis of the adsorbent and this β-CD/NaAlg presented a three-dimensional network at the nanoscale or *** optimal conditions(pH=4,t=8 h,β-CD:NaAlg=9,adsorbent dosage = 1.5 g·L-1),the maximum removal rate of β-CD/NaAlg to tetracycline was 70%.The adsorption behavior of tetracycline on β-CD/NaAlg conformed to the Freundlich isotherm model(R2=0.9977) and the pseudo-second-order kinetic model(R^(2)=0.9993).Moreover,the adsorbent still removed 55.3% of tetracycline after five ***,the adsorbent was integrated with ultrafiltration to adsorb tetracycline antibiotics from simulated reclaimed wastewater,and the removal rate of tetracycline reached 78.9% within 2 *** existence of Cr(Ⅵ) had a negligible impact on tetracycline removal,while the presence of humic acid exhibited a promoting *** possible adsorption mechanisms were also elucidated through X-ray photoelectron spectroscopy and density functional theory *** summary,β-CD/NaAlg represents an environmentally friendly,efficient,and sustainable adsorbent for removing tetracycline antibiotics from reclaimed water.

关键词： b-CD/NaAlg aerogel Covalent grafting Tetracycline antibiotics Ultrafiltration Selective adsorption Reclaimed water

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How the enhanced East Asian summer monsoon regulates total gross primary production in eastern China

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Advances in Climate Change Research 2024年第2期15卷 244-252页

作者： Ming-Yu HAN Yong ZHANG Jing PENG China State key laboratory of Severe Weather Chinese Academy of Meteorological SciencesBeijing 100081China China Meteorological Administration Institute for Development and Programme Design Beijing 100081China cas key laboratory of Regional Climate-environment for Temperate East Asia Institute of Atmospheric PhysicsChinese Academy of Sciences(CAS)Beijing 100029China

Recognizing the relationship between gross primary production(GPP)and precipitation in eastern China,the East Asian Summer Monsoon(EASM)plays a crucial role in shaping *** confirmation of the strong link between EASM and GPP,there remains a notable research gap in understanding the specific impact of the EASM on GPP in different regions of eastern *** we used simulations from Trends in Net Land-Atmosphere Carbon Exchanges(TRENDY)models from 1951 to 2010 and divided eastern China into five subregions for the *** also used the New East Asian Summer Monsoon Index(NEWI)as a quantitative metric to distinguish between periods of strong and weak *** on this,this study aims to investigate the response of GPP in different subregions of eastern ***,under strengthened EASM years(1954,1957,1965,1969,1977,1980,1983,1987,1993 and 1998),East China experienced the most pronounced increase in GPP at 12±21(mean±1 sigma)gC m^(-2) mon^(-1) compared to the weak EASM years(1958,1961,1972,1973,1978,1981,1985,1994,1997 and 2004).In contrast,Southwest China showed a decline in GPP at-4±10 gC m^(-2) mon^(-1).Moreover,GPP also increased in Northeast and North China when EASM strengthened,while South China showed a decline in *** indicated that GPP changed with monsoon *** to the mechanism analysis,during strong EASM,there was intense moisture convergence through alterations in the atmospheric circulation field over East China and abundant precipitation,which further contributed to the increase in *** solar radiation in Southwest China decreased with EASM enhancement,which suppressed GPP and hindered vegetation ***,the results highlight the importance of accurately predicting the impact of different EASM intensities of regional carbon fluxes.

关键词： Gross primary production Surface air temperature Precipitation Solar radiation Eastern China Carbon cycle

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Disastrous effects of climate change on High Mountain Asia

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Advances in Climate Change Research 2024年第3期15卷 365-366页

作者： Peng CUI Yao-Ming MA Yan WANG Bin-BinWANG Institute of Geographic Sciences and Natural Resources Research The Chinese Academy of Sciences(CAS)Beijing 100101China Institute of Mountain Hazards and environment CASChengdu 610041China China-Pakistan Joint Research Center on Earth Sciences CAS-HECIslamabad 45320Pakistan State key laboratory of Tibetan Plateau Earth System Environment and Resources(TPESER)Institute of Tibetan Plateau ResearchCASBeijing 100101China

High Mountain Asia(HMA),encompassing the Tibetan Plateau and the surrounding high mountain ranges of the Hindu Kush and Tianshan,is a region characterised by large terrain,complex topography and the interplay of vario... 详细信息

关键词： terrain Tianshan Tibetan

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Sustainable, thermoplastic and hydrophobic coating from natural cellulose and cinnamon to fabricate eco-friendly catering packaging

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Green Energy & environment 2024年第5期9卷 927-936页

作者： Rumeng Xu Chunchun Yin Jingxuan You Jinming Zhang Qinyong Mi Jin Wu Jun Zhang cas key laboratory of Engineering Plastics Institute of ChemistryChinese Academy of Sciences(CAS)Beijing100190China University of Chinese Academy of Sciences Beijing100049China

Non-degradable polymers cause serious environmental pollution problem,such as the widely-used while unrecyclable coatings which signiﬁcantly affect the overall degradation performance of *** is imperative and attractive to develop biodegradable functional ***,we proposed a novel strategy to successfully prepare biodegradable,thermoplastic and hydrophobic coatings with high transparence and biosafety by weakening the interchain interactions between cellulose *** natural cellulose and cinnamic acid were as raw *** reducing the degree of polymerization(DP)of cellulose and regulating the degree of substitution(DS)of cinnamate moiety,the obtained cellulose cinnamate(CC)exhibited not only the thermalﬂow behavior but also good biodegradability,which solves the conﬂict between the thermoplasticity and biodegradability in cellulose-based *** glass transition temperature(T_(g))and thermalﬂow temperature(T_(f))of the CC could be adjusted in a range of 150–200℃ and 180–210℃,*** CC with DS<1.2 and DP≤100 degraded more than 60%after an enzyme treatment for 7 days,and degraded more than 80%after a composting treatment for 42 ***,CC had no toxicity to human epidermal cells even at a high concentration(0.5 mg mL^(-1)).In addition,CC could be easily fabricated into multifunctional coating with high hydrophobicity,thermal adhesion and high ***,after combining with cellophane and paperboard,CC coating with low DP and DS could be used to prepare fully-biodegradable heat-sealing packaging,art paper,paper cups,paper straws and food packaging boxes.

关键词： Thermoplastic coating Bio-degradable adhesive Natural products Cellulose Eco-friendly packaging

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Masculinizer gene controls sexual differentiation in Hyphantria cunea

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Insect Science 2024年第2期31卷 405-416页

作者： Xiaowei Li Huihui Liu Honglun Bi Yaohui Wang Jun Xu Sufang Zhang Zhen Zhang Ze Zhang Yongping Huang laboratory of Evolutionary and Functional Genomics School of Life SciencesChongqing UniversityChongqingChina cas key laboratory of Insect Developmental and Evolutionary Biology CAS Centerfor Excellence in Molecular Plant SciencesInstitute of Plant Physiology and EcologyShanghaiChina key laboratory of Forest Protection Research Institute of Forest EcologyEnvironment and ProtectionChinese Academy of ForestryState Forestry AdministrationBeijingChina

The Masculinizer gene,Masc,encodes a lepidopteran-specific novel CCCHtype zinc finger protein,which controls sex determination and dosage compensation in Bombyx *** the potential application of it in pest control,it is necessary to investigate the function of Masc gene in Hyphantria cunea,a globally invasive forest *** the present study,we identified and functionally characterized the Masc gene,HcMasc,in *** analysis revealed that HcMASC contained the conserved CCCH-type zinc finger domain,nuclear localization signal,and male determining domain,in which the last was confirmed to be required for its masculinization in BmN cell ***,expression data showed that unlike male-biased expression in ***,Hc-Masc gene expresses in main all developmental stages or tissues in both *** regularly interspaced palindromic repeats(CRISPR)/CRISPR-associated protein 9-based disruption of the common exons 1 and 3 of the HcMasc gene resulted in imbalanced sex ratio and abnormal external genitalia of both *** results suggest that the HcMasc gene is required for both male and female sexual differentiation and dosage compensation in *** and provide a foundation for developing better strategies to control this pest.

关键词： CRISPR/cas9 dosage compensation Hyphantria cunea Masc sexual differentiation

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Evolution of soil DOM during thermal remediation below 100℃:concentration,spectral characteristics and complexation ability

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Frontiers of environmental Science & Engineering 2024年第8期18卷 31-41页

作者： Wan Huang Ziren Wan Di Zheng Lifeng Cao Guanghe Li Fang Zhang State key Joint laboratory of environment Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China National Engineering laboratory for Site Remediation Technologies Beijing 100015China

The impact of thermal remediation on soil function has drawn increasing *** far,as the most active fraction of soil organic matter,the evolution of dissolved organic matter(DOM)during the thermal remediation lacks in-depth investigation,especially for the temperatures value below 100℃.In this study,a series of soil thermal treatment experiments was conducted at 30,60,and 90℃ during a 90-d period,where soil DOM concentration increased with heating temperature and *** molecular weight,functional groups content and aromaticity of DOM all decreased during the thermal *** excitation-emission matrices(EEM)results suggested that humic acid-like substances transformed into fulvic acid-like substances(FIII/FV increased from 0.27 to 0.44)during the heating process,and five DOM components were further identified by *** change of DOM structures and components indicated the decline of DOM stability and hydrophilicity,and can potentially change the bioavailability and *** temperature also resulted in the decline of DOM complexation ability,which may be caused by the loss of binding sites due to the decrease of polar function groups,aromatic structures and hydrophilic *** study provides valuable information about the evolution of DOM during thermal remediation,which would potentially change the fate of metal ions and the effectiveness of the post-treatment technologies in the treated region.

关键词： Thermal remediation below 100℃ Heating temperature Soil DOM concentration DOM spectral characteristics Excitation-emission matrices(EEM) Complexation ability

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Optimization of Gas Production from Hydrate-Bearing Sediments with Fluctuation Characteristics

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Journal of Ocean University of China 2024年第3期23卷 618-632页

作者： LI Yaobin XU Tianfu XIN Xin YU Han YUAN Yilong ZHU Huixing key laboratory of Groundwater Resources and environment Ministry of EducationJilin UniversityChangchun 130021China Jilin Provincial key laboratory of Water Resources and environment Jilin UniversityChangchun 130021China

As an important source of low-carbon,clean fossil energy,natural gas hydrate plays an important role in improving the global energy consumption *** the hydrate industry in the South China Sea is important to achieving‘carbon peak and carbon neutrality’goals as soon as ***-water areas subjected to the action of long-term stress and tectonic movement have developed complex and volatile terrains,and as such,the morphologies of hydrate-bearing sediments(HBSs)fluctuate *** key to numerically simulating HBS morphologies is the establishment of the conceptual model,which represents the objective and real description of the actual geological ***,current numerical simulation models have characterized HBSs into horizontal strata without considering the fluctuation *** representing the HBS as a horizontal element reduces simulation ***,the commonly used horizontal HBS model and a model considering the HBS’s fluctuation characteristics with the data of the SH2 site in the Shenhu Sea area were first constructed in this ***,their production behaviors were compared,and the huge impact of the fluctuation characteristics on HBS production was *** this basis,the key parameters affecting the depressurization production of the fluctuating HBSs were studied and *** research results show that the fluctuation characteristics have an obvious influence on the hydrate production of HBSs by affecting their temperatures and pressure distributions,as well as the transmission of the pressure drop and methane gas ***,the results show that the gas productivity of fluctuating HBSs was about 5%less than that of horizontal *** optimizing the depressurization amplitude,well length,and layout location of vertical wells,the productivity of fluctuating HBSs increased by about 56.6%.

关键词： natural gas hydrate numerical simulation fluctuation characteristics depressurization production production well optimization

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