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MOF-derived Se doped MnS/Ti_(3)C_(2)T_(x) as cathode and Zn-Ti_(3)C_(2)T_(x) membrane as anode for rocking-chair zinc-ion battery

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Nano Research 2024年第4期17卷 2781-2789页

作者： Kaisheng Sun Zemao Xiao Yunfei Shen Heng Lv Jianpeng Zhu Jianxiang Pang Yang Zheng Wenwen Kong Long Chen School of chemistry and Chemical Engineering/State key laboratory Incubation Base for Green Processing of Chemical Engineering Shihezi UniversityShihezi 832003China cas key laboratory of functional materials and devices for special environments Xinjiang Key Laboratory of Electronic Information Materials and DevicesCenter of Materials Science and Optoelectronics EngineeringXinjiang Technical Institute of Physics and Chemistry of CASUrumqi 830011China

Mn-based zinc ion battery has the advantages of low cost and high performance,which makes it the promising energy storage ***,the poor conductivity and the agglomeration in the synthesis process of manganese-based materials restrict the performance of ***,the Se-doped MnS/Ti_(3)C_(2)T_(x)(Se-MnS/Ti_(3)C_(2)T_(x))composite material derived from Mn-based metal-organic framework is *** tests show that Se-doped could generate S defects and enhance the electrochemical activity of *** the same time,the introduction of Ti_(3)C_(2)T_(x) substrate is conducive to exposing more sulfur defects and improving the utilization rate of *** the mechanism study,it is found that Se-MnS/Ti_(3)C_(2)T_(x) is transformed into S/Se co-doped Mn3O_(4) at the first charge,which innovatively elucidated the behavior of S/Se during *** the electrochemical performance test,the specific capacity can reach 74.7 mAh·g^(-1) at 5.0 A·g^(-1).In addition,the Zn-Ti_(3)C_(2)T_(x) membrane electrode is prepared by vacuum filtration as the zinc-poor anode,which is assembled into the rocking chair full battery to avoid dendrite growth and exhibit excellent rate *** addition of Zn2+weakens the electrostatic repulsion between the interlayers of MXene,and the formation of the folded morphology aids the penetration of the *** 1.0 A·g^(-1),the capacity can reach 50.6 mAh·g^(-1).This work is helpful to promote the research and development of the reaction mechanism of manganese based rocking chair batteries.

关键词： rocking-chair zinc-ion battery MnS Zn-Ti_(3)C_(2)T_(x) membrane Se doped Ti_(3)C_(2)T_(x) composite

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Review on birefringence in borates based on birefringence-active functional groups and arrangements

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Science China chemistry 2024年第7期67卷 2155-2170页

作者： Qianzhen Zhang Ran An Zhihua Yang Xifa Long Shilie Pan Yun Yang Research Center for Crystal materials State Key Laboratory of Functional Materials and Devices for Special Environmental ConditionsXinjiang Key Laboratory of Functional Crystal MaterialsThe Xinjiang Technical Institute of Physics&ChemistryChinese Academy of SciencesUrumqi 830011China Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

As a fundamental parameter of the optical crystals,birefringence plays a vital role in many optical applications,such as phase modulation,light splitting,and polarization,especially the phase matching process of the nonlinear optical *** big birefringence not only benefits to the miniaturization of related devices,but also broadens the phase-matching wavelength range of nonlinear optical *** design and synthesis of crystals with large birefringence becomes a hot research topic due to its more and more important applications in the optical modulation and laser technology ***,crystals with birefringence greater than 0.05 in the borate system are reviewed and classified according to different birefringent active groups,and the relationship between structure and properties is thoroughly *** is hoped that this review will provide a clear understanding of what kinds of building units and arrangements would have more opportunity to get adequate birefringence in borate systems and provide the statistical references to encourage the emergence of better crystal materials with large birefringence.

关键词： birefringence borate optical functional crystal structural anisotropy arrangement of functional units

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Zincophilic Ti_(3)C_(2)Cl_(2)MXene and anti-corrosive Cu NPs for synergistically regulated deposition of dendrite-free Zn metal anode

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Journal of materials Science & Technology 2024年第2期169卷 137-147页

作者： Yunfei Shen Yi Liu Kaisheng Sun Tiantian Gu Gang Wang Yue Yang Jianxiang Pang Yang Zheng Xiaodong Yang Long Chen key laboratory for Green Process of Chemical Engineering of xinjiang Bingtuan School of Chemistry and Chemical EngineeringShihezi UniversityShihezi 832003China institute for chemistry Chemnitz University of TechnologyChemnitz 09107Germany cas key laboratory of functional materials and devices for special environments Xinjiang Key Laboratory of Electronic Information Materials and DevicesCenter of Materials Science and Optoelectronics EngineeringXinjiang Technical Institute of Physics and Chemistry of CASUrumqi 830011China key laboratory of Ecophysics and Department of physics College of ScienceShihezi UniversityShihezi 832003China

Dendrites growth,chemical corrosion,and hydrogen evolution reaction(HER)on zinc anodes are the main barriers for the development of aqueous zinc-ion batteries(AZIBs).Constructing interfacial protec-tive layer is an effective way to alleviate the side reactions on the ***,Cu/Ti_(3)C_(2)Cl_(2)MXene(CMX)with high zincophilic and hydrophobic property is prepared by the lewis molten salts etching method,and the CMX interface protection layer is constructed by a simple spin *** CMX coat-ing layer can provide abundant nucleation sites and uniformize the charge distribution through the zin-cophilic Ti_(3)C_(2)Cl_(2)MXene matrix,leading to homogenous Zn *** addition,the hydrophobic coat-ing contained anti-corrosive Cu nanoparticles can prevent the Zn anode from the electrolyte,beneficial for suppressing the chemical corrosion and ***,the stable and reversible Zn plating/stripping is achieved for the Zn anode coated by the CMX,which exhibits the lifespan of over 1400 h at 0.5 mA cm^(−2),and even can steadily run for 700 h with 65 mV at 10 mA cm^(−2).Furthermore,CMX@Zn shows a high coulombic efficiency of over 100%for 3800 cycles,which indicates that the CMX@Zn electrode has excellent stability and reversibility of Zn stripping/*** full batteries assembled with ZnCoMnO/C(ZCM)cathodes also exhibits higher capacity(450.6 mAh g^(−1)at 0.1 A g^(−1))and cycle stability(capacity retention of 70%after 1500 cycles).This work enhanced the lifespan of AZIBs and broaden the research of multifunctional coating layer to other secondary batteries based on metal anodes.

关键词： Zinc anode Spin coating Zincophilic MXene Anti-corrosive Cu NPs Multifunctional coating

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Iron-based layered double hydroxide packed with metal-organic frameworks for enhanced overall water-splitting electrocatalysis

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Tungsten 2024年第4期6卷 859-868页

作者： Long Chen Yun Luo Zhi-Peng Yu Yi-Kun Cheng Yang Zheng Li He Jia-Hao Xiong Wen-Wen Kong key laboratory for Green Process of Chemical Engineering of xinjiang Bingtuan School of Chemistry and Chemical Engineering Shihezi University institute of Scientific Research Luzhou North Chemistry Industry Co.Ltd International Iberian Nanotechnology laboratory (INL) cas key laboratory of functional materials and devices for special environments Xinjiang Key Laboratory of Electronic Information Materials and Devices Center of Materials Science and Optoelectronics Engineering Xinjiang Technical Institute of Physics and Chemistry of CAS

Designing hybrid materials with numerous catalytic active sites,high specific surface area,and interfacial interactions is an effective strategy to improve electrocatalytic *** this work,iron-based metal organic frameworks（Fe-MOFs）@（Co,Ni）Fe-layered double hydroxide（LDH） is successfully constructed using the similar "MOF growing on LDH" strategy for oxygen evolution reaction and hydrogen evolution reaction in the alkaline *** synthesized hybrid materials in this particular way show excellent electrochemical overall water-splitting performance with the cell voltage of 1.62 V at10 mA·cm-2in the alkaline environment due to the optimized adsorption/desorption properties of metal ions on oxygencontaining species and interfacial effects of hybrid ***-MOFs@（Co,Ni）Fe-LDH also exhibits excellent hydrogen and oxygen production efficiency of 370 and 175 μL·min-1,*** work draws on an effective approach to the fabrication of MOF@LDH structures and provides new insights into overall water-splitting in alkaline conditions.

关键词： Electrocatalysis Interfacial interactions Layered double hydroxide Metal–organic frameworks (MOFs) Water splitting

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Realization of flexible in-memory computing in a van der Waals ferroelectric heterostructure tri-gate transistor

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Nano Research 2024年第3期17卷 1886-1892页

作者： Xinzhu Gao Quan Chen Qinggang Qin Liang Li Meizhuang Liu Derek Hao Junjie Li Jingbo Li Zhongchang Wang Zuxin Chen School of Semiconductor Science and Technology South China Normal UniversityFoshan 528225China Guangdong Provincial key laboratory of Chip and Integration Technology Guangzhou 510631China institute of Solid State physics Hefei institutes of Physical Science Chinese Academy of SciencesHefei 230601China School of Science STEM CollegeRMIT UniversityMelbourne 3000Australia cas key laboratory of functional materials and devices for special environments Xinjiang Technical Institute of Physics&ChemistryChinese Academy of SciencesUrumqi 830011China Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China College of Optical Science and Engineering Zhejiang UniversityHangzhou 310027China International Iberian Nanotechnology laboratory(INL) Av.Mestre Jose Veiga s/nBraga 4715-330Portugal

Combining logical function and memory characteristics of transistors is an ideal strategy for enhancing computational efficiency of transistor ***,we rationally design a tri-gate two-dimensional(2D)ferroelectric van der Waals heterostructures device based on copper indium thiophosphate(CuInP_(2)S_(6))and few layers tungsten disulfide(WS_(2)),and demonstrate its multi-functional applications in multi-valued state of data,non-volatile storage,and logic *** co-regulating the input signals across the tri-gate,we show that the device can switch functions flexibly at a low supply voltage of 6 V,giving rise to an ultra-high current switching ratio of 107 and a low subthreshold swing of 53.9 mV/*** findings offer perspectives in designing smart 2D devices with excellent functions based on ferroelectric van der Waals heterostructures.

关键词： two-dimensional(2D)ferroelectric heterostructure tri-gate polymorphic regulation in-memory computing

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以LiB_(3)O_(5)为模板设计深紫外零级波片材料

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Science China materials 2024年第3期67卷 914-920页

作者：张志远徐蝶 Abudukadi Tudi 杨志华韩树娟潘世烈 Research Center for Crystal materials State Key Laboratory of Functional Materials and Devices for Special Environmental ConditionsXinjiang Key Laboratory of Functional Crystal MaterialsXinjiang Technical Institute of Physics and ChemistryChinese Academy of SciencesUrumqi 830011China Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

以著名的LiB_(3)O_(5)为模板,通过增强其结构中B_(2)O_(5)的夹角使双折射更小,在封闭体系中通过高温溶液法获得了两种新的用于制造零级波片的双折射晶体Li_(2)MLaB_(18)O_(30)(M=Rb,Cs).有趣的是,相邻的B_(2)O_(5)接近垂直排列,使得它... 详细信息

以著名的LiB_(3)O_(5)为模板,通过增强其结构中B_(2)O_(5)的夹角使双折射更小,在封闭体系中通过高温溶液法获得了两种新的用于制造零级波片的双折射晶体Li_(2)MLaB_(18)O_(30)(M=Rb,Cs).有趣的是,相邻的B_(2)O_(5)接近垂直排列,使得它们表现出比商用石英晶体(Δn~0.0092在可见光区域)小得多的双折射率(分别为0.0032@532 nm和0.0027@532 nm).此外,Li_(2)MLaB_(18)O_(30)(M=Rb,Cs)晶体的紫外截止边均低于200 nm,表明它们可用作深紫外区域的零级波片材料.

关键词： tiny birefringence zero-order waveplate deep-ultraviolet region angle of B_(2)O_(5)

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共价键合氟优化氟化硼酸盐的深紫外非线性光学性能

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Science Bulletin 2024年第9期69卷 1192-1196页

作者：李富明靳文琪安然米日丁·穆太力普潘世烈杨志华 Research Center for Crystal materials State Key Laboratory of Functional Materials and Devices for Special Environmental ConditionsXinjiang Key Laboratory of Functional Crystal MaterialsXinjiang Technical Institute of Physics and ChemistryChinese Academy of SciencesUrumqi 830011China Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

Nonlinear optical (NLO) crystals are pivotal in laser application technology, which can convert the laser frequency to generate coherent light in the deep-ultraviolet (deep-UV, wavelengthλ≤200 nm) to far-infrared spectral range, and widely used in solid-state system detection, tissue imaging, quantum information,and more [1]. To expand the diversity of optical functional units and then discover novel NLO materials.

关键词：非线性光学性能共价键合硼酸盐深紫外

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图神经网络指导新型深紫外大双折射晶体材料的设计（英文）

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Science China materials 2024年

作者：克鲁格洛夫伊万柳德米拉别列兹尼科娃谢聪伟储冬冬李珂吉洪诺夫叶夫格尼阿布都卡地吐地阿尔斯兰马齐托夫张敏潘世烈杨志华 Research Center for Crystal materials State Key Laboratory of Functional Materials and Devices for Special Environmental Conditions Xinjiang Key Laboratory of Functional Crystal Materials Xinjiang Technical Institute of Physics and Chemistry Chinese Academy of Sciences Moscow institute of physics and Technology 9 Institutsky Lane Emerging Technologies Research Center XPANCEO Internet CityEmmay Tower

寻找具有大双折射率（Δn）的晶体材料,尤其是深紫外大双折射晶体材料,对于制备光纤传感器等偏振器件非常重要.具有大双折射率的晶体材料通常需借助实验技术发现.然而,大量耗时的实验并不利于高效寻找具有大双折射率的晶体材料.在本文中...

寻找具有大双折射率（Δn）的晶体材料,尤其是深紫外大双折射晶体材料,对于制备光纤传感器等偏振器件非常重要.具有大双折射率的晶体材料通常需借助实验技术发现.然而,大量耗时的实验并不利于高效寻找具有大双折射率的晶体材料.在本文中,我们收集了一个包含数千晶体结构及其光学性质的数据集,并采用原子线图神经网络（ALIGNN）训练了可用于快速预测晶体材料双折射率的机器学习模型.我们采用D-optimality准则评估所构建机器学习模型的预测可信度.基于该双折射率机器学习模型,我们从materials Project数据库中搜索了具有大双折射率的晶体材料,发现了两种新型深紫外大双折射候选材料NaYCO3F2和SClO2F,它们的双折射率分别为0.202和0.101@1064 nm.进一步分析表明,具有强各向异性的多阴离子基团和π共轭平面基团有利于产生大的双折射率.

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Low-Dose 1 MeV Electron Irradiation-Induced Enhancement in the Photoluminescence Emission of Ga-Rich InGaN Multiple Quantum Wells

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Chinese physics Letters 2013年第7期30卷 135-137页

作者： ZHANG Xiao-Fu LI Yu-Dong GUO Qi LU Wu key laboratory of functional materials and devices for special environments Xinjiang Technical Institute of Physics&ChemistryChinese Academy of SciencesUrumqi 830011

We investigate the photoluminescence(PL)emission from InGaN/GaN multiple quantum-well structures before and after 1 MeV electron *** PL peak intensity exhibits a slight enhancement after low-dose electron irradiation(2×10^(13) e/cm^(2)),and then decreases with the cumulative electron ***,the full width at half maximum of the PL spectrum narrows after low-dose electron irradiation and widens when the irradiation dose is relatively *** respect to the yellow photoluminescence,there is no significant change until the electron fluence has accumulated up to 10^(14) e/cm^(2).

关键词： InGaN/GaN Electron Quantum

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Growth Mechanism,Modified Morphology and Optical Properties of Coral-like BaTiO_3 Architecture through CTAB Assisted Synthesis

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Journal of materials Science & Technology 2015年第2期31卷 223-228页

作者： Pengjun Zhao Lei Wang Liang Bian Jinbao Xu Aimin Chang Xinqian Xiong Fanglong Xu Jiaqi Zhang key laboratory of functional materials and devices for special environments of cas Xinjiang Key Laboratory of Electronic Information Materials and DevicesXinjiang Technical Institute of Physics & Chemistry of CAS University of Chinese Academy of Sciences

Three-dimensional hierarchical structure coral-like BaTiO3 nanoparticles have been self-assembled by a facile one step hydrothermal method. Cetyltrimethyl ammonium bromide(CTAB),Ba(OH)2·8H2O and tetrabutyl titanate have been used as precursors. The prepared Ba TiO3 exhibits cubic perovskite phase at room temperature,and the coral-like architecture is a micro-nano hiberarchy consisted of dendrimer-like structure and trunk-like structure. By adjusting the hydrothermal duration and the precursor substances,a surfactant induced mechanism is proposed to understand the self-assembly process. UV-vis measurement demonstrates that the as-prepared Ba TiO3 nanoparticles exhibit dozens of times overwhelming absorptive character compared to the ordinary nanospheres at ultraviolet band,which is benefited from the coral-like porous framework. Moreover,halogen anions( F,Cl,Br,and I) have been chosen to adjust the coral-like Ba TiO3 physical properties. Results show the halogen doping produces distinct modulation effect on the grain size,UV-vis absorbance and photoluminescence properties of the materials. The coral-like BaTiO3 nanoparticle and its halogen modified ramifications offer significant opportunities to develop nano-laser devices,photon detectors,photocatalyst based on BaTiO3 perovskite materials.

关键词： BaTiO3 Halogen doping Hydrothermal synthesis Coral

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