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Enhanced conductivity and weakened magnetism in Pb-doped Sr_(2)IrO_(4)

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Chinese Physics B 2024年第1期33卷 680-685页

作者：岳智来甄伟立牛瑞焦珂珂朱文卡皮雳张昌锦 High Magnetic field Laboratory Hefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

Group IV element Pb has been selected as the dopant to dope at the Sr site of Sr_(2)IrO_(4). It is exciting to find that the single-phase crystal structure could be maintained with a high Pb doping level of up to x=0.3 in Sr_(2-x)Pb_(x)IrO_(4). The mapping data obtained from energy-dispersive x-ray spectroscopy analyses give solid evidence that the Pb ions are uniformly distributed in the Sr_(2)IrO_(4) matrix. The incorporation of Pb leads to a moderate depression of the canted antiferromagnetic ordering state. The electrical conductivity could be greatly enhanced when the Pb doping content is higher than x=*** present results give a fresh material base to explore new physics in doped Sr_(2)IrO_(4) systems.

关键词： iridates doping conductivity magnetism

Textured Asymmetric Membrane Electrode Assemblies of Piezoelectric Phosphorene and Ti_(3)C_(2)T_(x)MXene Heterostructures for Enhanced Electrochemical Stability and Kinetics in LIBs

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Nano-Micro Letters 2024年第4期16卷 394-414页

作者： Yihui Li Juan Xie Ruofei Wang Shugang Min Zewen Xu Yangjian Ding Pengcheng Su Xingmin Zhang Liyu Wei Jing‑Feng Li Zhaoqiang Chu Jingyu Sun Cheng Huang Volta and DiPole Materials Labs College of EnergySoochow Institute for Energy and Materials InnovationS(SIEMIS)Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceKey Laboratory of Core Technology of High Specific Energy Battery and Key Materials for Petroleum and Chemical IndustrySoochow UniversitySuzhou 215006People’s Republic of China School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013People’s Republic of China College of Underwater Acoustic Engineering Harbin Engineering UniversityHarbin 150001People’s Republic of China Shanghai Synchrotron Radiation facility Shanghai Advanced Research InstituteShanghai Institute of Applied PhysicsChinese Academy of SciencesShanghai 201204People’s Republic of China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084People’s Republic of China High Density Materials Technology Center for Flexible Hybrid Electronics Suzhou Institute of Electronic Functional Materials TechnologySuzhou Industrial Technology Research InstituteSuzhou 215151People’s Republic of China Institute of Advanced Materials and Institute of Membrane Science and Technology Jiangsu National Synergistic Innovation Center for Advanced MaterialsSuzhou Laboratory and Nanjing Tech UniversityNanjing 211816People’s Republic of China

Black phosphorus with a superior theoretical capacity(2596 mAh g^(-1))and high conductivity is regarded as one of the powerful candidates for lithium-ion battery(LIB)anode materials,whereas the severe volume expansion and sluggish kinetics still impede its applications in *** contrast,the exfoliated two-dimensional phosphorene owns negligible volume variation,and its intrinsic piezoelectricity is considered to be beneficial to the Li-ion transfer kinetics,while its positive influence has not been discussed ***,a phosphorene/MXene heterostructure-textured nanopiezocomposite is proposed with even phosphorene distribution and enhanced piezo-electrochemical coupling as an applicable free-standing asymmetric membrane electrode beyond the skin effect for enhanced Li-ion *** experimental and simulation analysis reveals that the embedded phosphorene nanosheets not only provide abundant active sites for Li-ions,but also endow the nanocomposite with favorable piezoelectricity,thus promoting the Li-ion transfer kinetics by generating the piezoelectric field serving as an extra *** waltzing with the MXene framework,the optimized electrode exhibits enhanced kinetics and stability,achieving stable cycling performances for 1,000 cycles at 2 A g^(-1),and delivering a high reversible capacity of 524 m Ah g^(-1)at-20℃,indicating the positive influence of the structural merits of self-assembled nanopiezocomposites on promoting stability and kinetics.

关键词： Phosphorene Nanopiezocomposite Piezo-electrochemical coupling Membrane electrode assembly Lithium-ion storage

Optimizing laser coupling,matter heating,and particle acceleration from solids using multiplexed ultraintense lasers

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Matter and Radiation at Extremes 2024年第4期9卷 16-28页

作者： Weipeng Yao Motoaki Nakatsutsumi Sébastien Buffechoux Patrizio Antici Marco Borghesi Andrea Ciardi Sophia N.Chen Emmanuel d’Humières Laurent Gremillet Robert Heathcote Vojtech Horny Paul McKenna Mark N.Quinn Lorenzo Romagnani Ryan Royle Gianluca Sarri Yasuhiko Sentoku Hans-Peter Schlenvoigt Toma Toncian Olivier Tresca Laura Vassura Oswald Willi Julien Fuchs LULI-CNRS CEASorbonne UniversitéEcole PolytechniqueInstitut Polytechnique de ParisF-91128 Palaiseau CedexFrance Sorbonne Université Observatoire de ParisUniversité PSLCNRSLERMAF-75005 ParisFrance INRS-EMT 1650 BoulLionel-BouletVarennesQuebec J3X 1S2Canada Center for Plasma Physics School of Mathematics and PhysicsQueen’s University BelfastBelfast BT71NNUnited Kingdom “Horia Hulubei”National Institute for Physics and Nuclear Engineering 30 Reactorului StreetRO-077125 Bucharest-MagureleRomania University of Bordeaux Centre Lasers Intenses et ApplicationsCNRSCEAUMR 5107F-33405 TalenceFrance CEA DAMDIFF-91297 ArpajonFrance Université Paris-Saclay CEALMCE91680 Bruyères-le-ChatelFrance Central Laser facility STFC Rutherford Appleton LaboratoryDidcotUnited Kingdom SUPA Department of PhysicsUniversity of StrathclydeGlasgow G40NGUnited Kingdom Department of Physics University of NevadaRenoNevada 89557USA Institute of Laser Engineering Osaka University2-6 YamadaokaSuitaOsaka 565-0871Japan Institut fur Laser und Plasmaphysik Heinrich Heine Universitat DusseldorfDusseldorfGermany

Realizing the full potential of ultrahigh-intensity lasers for particle and radiation generation will require multi-beam arrangements due to technology ***,we investigate how to optimize their coupling with solid ***,we show that overlapping two intense lasers in a mirror-like configuration onto a solid with a large preplasma can greatly improve the generation of hot electrons at the target front and ion acceleration at the target *** underlying mechanisms are analyzed through multidimensional particle-in-cell simulations,revealing that the self-induced magnetic fields driven by the two laser beams at the target front are susceptible to reconnection,which is one possible mechanism to boost electron *** addition,the resistive magnetic field generated during the transport of the hot electrons in the target bulk tends to improve their *** simulations also indicate that such effects can be further enhanced by overlapping more than two laser beams.

关键词： laser acceleration particle

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基于格点有效场论的原子核电荷半径微扰计算

原子核物理评论 2024年第1期41卷 172-177页

作者：马远卓吕炳楠李宁王倩华南师范大学量子物质研究院原子亚原子结构与量子调控教育部重点实验室广州510006 facility for Rare Isotope Beams Michigan State UniversityMI 48824USA 中国工程物理研究院研究生院北京100193 中山大学物理学院广州510275

原子核格点有效场论(Nuclear Lattice Effective field Theory)是近些年发展起来的一种高精度原子核第一性原理计算方法。它将手征有效场论与格点量子蒙特卡罗方法有机结合起来,能够在统一的理论框架下构建核力与求解量子多体问题。近... 详细信息

原子核格点有效场论(Nuclear Lattice Effective field Theory)是近些年发展起来的一种高精度原子核第一性原理计算方法。它将手征有效场论与格点量子蒙特卡罗方法有机结合起来,能够在统一的理论框架下构建核力与求解量子多体问题。近年来新发展出来的波函数匹配(wave function matching)方法与微扰量子蒙特卡罗方法(perturbative quantum Monte Carlo method)为解决著名的“符号问题”开辟了全新的路径。本工作在这些方法的基础上,通过计算两点关联函数发展出格点上电荷半径的微扰计算方法,验证计算表明了本工作的可靠性。使用手征N^(3)LO核力的计算能够很好地复现^(4)He、^(12)C与^(16)O的实验测量结果。

关键词：原子核电荷半径手征有效场论格点微扰计算

Plasma optics:A perspective for high-power coherent light generation and manipulation

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Matter and Radiation at Extremes 2023年第2期8卷 1-5页

作者： C.Riconda S.Weber LULI Sorbonne UniversitéCNRSÉcole PolytechniqueCEA75252 ParisFrance Extreme Light Infrastructure ERIC ELI Beamlines Facility25241 Dolni BrezanyCzech Republic

Over the last two decades,the importance of fully ionized plasmas for the controlled manipulation of high-power coherent light has increased *** ideas have been put forward on how to control or change the properties of laser pulses such as their frequency,spectrum,intensity,and *** corresponding interaction with a plasma can take place either in a self-organizing way or by prior *** work has been done in theoretical studies and in simulations,but at present there is a backlog of demand for experimental veri-ﬁcation and the associated detailed characterization of plasma-optical *** proof-of-principle experiments need to be pushed to higher power *** is little doubt that plasmas have huge potential for future use in high-power *** introduction to the special issue of Matter and Radiation at Extremes devoted to plasma optics sets the framework,gives a short historical overview,and brieﬂy describes the various articles in this collection.

关键词： power optics coherent

The new X-ray imaging and biomedical application beamline BL13HB at SSRF

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Nuclear Science and Techniques 2023年第12期34卷 190-205页

作者： Jian‑Feng Ji Han Guo Yan‑Ling Xue Rong‑Chang Chen Ya‑Nan Fu Guo‑Hao Du Biao Deng Hong‑Lan Xie Ti‑Qiao Xiao Shanghai Synchrotron Radiation facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China Shanghai Institute of Applied Physics China Academy of ScienceShanghai 201800China

A new X-ray imaging and biomedical application beamline(BL13HB)has been implemented at the Shanghai Radiation Synchrotron facility(SSRF)as an upgrade to the old X-ray imaging and biomedical application beamline(BL13W1).This is part of the Phase II construction project of the *** BL13HB is dedicated to 2D and 3D static and dynamic X-ray imaging,with a field of view of up to 48.5 mm×5.2 mm and spatial resolution as high as 0.8μm.A super-bending magnet is used as the X-ray source in BL13HB,which has a maximum magnetic field of 2.293 *** energy range of monochromatic X-ray photons from a double-multiplayer monochromator was 8–40 keV,and the white beam mode was provided on the beamline for dynamic X-ray imaging and dynamic X-ray *** maintaining the previous experimental setup of BL13W1,new equipment was added to the beamline experimental *** beamline is equipped with different sets of X-ray imaging detectors for several experimental methods such as micro-CT,dynamic micro-CT,and pair distribution *** experimental station of BL13HB is designed specifically for various in situ dynamic experiments,and BL13HB has been open to users since June 2021.

关键词： X-ray imaging Dynamic micro-CT Shanghai Synchrotron Radiation facility

Activating coordinative conjugated polymer via interfacial electron transfer for efficient CO_(2) electroreduction

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能源化学:英文版 2023年第8期83卷 313-323,I0009页

作者： Jing Zhang Jia-Jun Dai De-Quan Cao Heng Xu Xing-Yu Ding Chun-Hua Zhen Beate Paulus Jin-Yu Ye Qian Liang Jun-Ke Liu Shi-Jun Xie Sai-Sai Deng Zhen Wang Jun-Tao Li Yao Zhou Shi-Gang Sun College of Energy XiamenUniversityXiamen 361005FujianChina College of Chemistry and Chemical Engineering Xiamen UniversityXiamen 361005FujianChina Institute of Chemistry and Biochemistry Freie Universitat BerlinArnimallee 2214195 BerlinGermany

With tunable local electronic environment,high mass density of MN4sites,and ease of preparation,metal-organic conjugated coordinative polymer(CCP) with inherent electronic conductivity provides a promising alternative to the well-known M-N-C ***,the coordination reaction between Cu^(2+)and 1,2,4,5-tetraaminobenzene(TAB) was conducted on the surface of metallic Cu nanowires,forming a thin layer of CuN4-based CCP(Cu-TAB) on the Cu *** importantly,interfacial transfer of electrons from Cu core to the CuN4-based CCP nanoshell was observed within the resulting CuTAB@Cu,which was found to enrich the local electronic density of the *** such,the CuTAB@Cu demonstrates much improved affinity to the*COOH intermediate formed from the rate determining step;the energy barrier for C-C coupling,which is critical to convert CO_(2)into C2products,is also ***,it delivers a current density of-9.1 mA cm^(-2)at a potential as high as 0.558 V(***) in H-type cell and a Faraday efficiency of 46.4% for *** work emphasizes the profound role of interfacial interaction in tuning the local electronic structure and activating the CuN4-based CCPs for efficient electroreduction of CO_(2).

关键词： Metal-organic solid compounds Conjugated coordinative polymer Solid-solid interfacial electron transfer MN_(4)sites Electrocatalysis

Automatic identification of crystal structures and interfaces via artificial-intelligence-based electron microscopy

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npj Computational Materials 2023年第1期9卷 489-499页

作者： Andreas Leitherer Byung Chul Yeo Christian H.Liebscher Luca M.Ghiringhelli The NOMAD Laboratory at the Fritz-Haber-Institut of the Max-Planck-Gesellschaft and IRIS-Adlershof of the Humboldt-Universität zu berlin BerlinGermany Department of Energy Resources Engineering Pukyong National UniversityBusan 48513Republic of Korea Max-Planck-Institut für Eisenforschung 40237 DüsseldorfGermany Physics Department and IRIS Adlershof Humboldt-Universität zu BerlinBerlinGermany Present address:Department of Materials Science and Engineering Friedrich-Alexander Universität Erlangen-NürnbergErlangenGermany

Characterizing crystal structures and interfaces down to the atomic level is an important step for designing advanced *** electron microscopy routinely achieves atomic resolution and is capable to resolve complex arrangements of atoms with picometer ***,we present AI-STEM,an automatic,artificial-intelligence based method,for accurately identifying key characteristics from atomic-resolution scanning transmission electron microscopy(STEM)images of polycrystalline *** method is based on a Bayesian convolutional neural network(BNN)that is trained only on simulated ***-STEM automatically and accurately identifies crystal structure,lattice orientation,and location of interface regions in synthetic and experimental *** model is trained on cubic and hexagonal crystal structures,yielding classifications and uncertainty estimates,while no explicit information on structural patterns at the interfaces is included during *** work combines principles from probabilistic modeling,deep learning,and information theory,enabling automatic analysis of experimental,atomic-resolution images.

关键词： materials crystal estimates

Eddy current septum magnets for injection and extraction at SSRF

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Chinese Physics C 2010年第3期34卷 389-393页

作者：欧阳联华谷鸣刘波陈嵘 Shanghai Synchrotron Radiction facility

There are 6 in-vacuum eddy current septum magnets used for booster injection, extraction, and storage ring injection in SSRF. Special attention was paid to coils and their support designs because of the shock force they bear in the magnetic fields and the high heat which is hard to be dissipated in vacuum environment. For the storage ring magnets, good transverse homogeneity in the gap was achieved by careful design, precise machining and accurate assembly; and an extremely low leakage field on the stored beam is another key feature thanks to the high permeability Mu metal. Magnetic field measurement was conducted with both a point coil and a long integral coil, and the results agree well with the OPERA-2d/3d simulations. An inner tube is added to keep the continuity of impedance for the circulating beam with two RF finger flanges at each end. There is no vacuum separation between the inner tube and the magnet chamber. Sputter ion pumps integrated with NEG are used to acquire the UHV for the chamber.

关键词： injection and extraction eddy current septum magnets leakage field