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Development of a model to simulate soil heavy metals lateral migration quantity based on SWAT in Huanjiang watershed,China

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Journal of Environmental Sciences 2019年第3期31卷 115-129页

作者： Pengwei Qiao Mei Lei Sucai Yang Jun Yang Xiaoyong Zhou Nan Dong Guanghui Guo Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences beijing key laboratory of remediation of industrial pollution sites Environmental Protection Research Institute of Light Industry Comprehensive Institute of Geotechnical Investigation and Surveying Ltd.

Lateral transportation of soil heavy metals in rainfall events could significantly increase the scope of pollution. Therefore, it is necessary to develop a model with high accuracy to simulate the migration quantity of heavy metals. A model for heavy metal migration simulation was developed based on the SWAT(Soil and Water Assessment Tool) model. This model took into consideration the influence of soil p H value, soil particle size, runoff volume, sediment amount,concentration of water-soluble heavy metals dissolved in runoff and insoluble absorbed to the soil particles. This model was reasonable in Huanjiang watershed, Guangxi Zhuang Autonomous Region, south China, covering an area of 273 km^2. The optimal drainage area threshold was determined by analyzing the effects of watershed subdivision on the simulation results to ensure the simulation accuracy. The main conclusions of this paper were:(1) watershed subdivision could affect simulation migration quantity of heavy metals;(2) the quantity of heavy metals transported by sediment accounted for 97%–99% of the total migration quantity in the study watershed. Therefore, sediment played the most important role in heavy metal migration;(3) the optimal drainage area threshold percentage to ensure high simulation accuracy was determined to be 2.01% of the total watershed;(4) with the optimal threshold percentage, this model could simulate the migration quantity of As, Pb and Cd accurately at the total watershed and subwatershed level. The results of this paper were useful for identifying the key regions with heavy metal migration.

关键词： Soil heavy metal migration Simulation model Watershed subdivision Optimal drainage area threshold percentage Simulation accuracy

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Identifying factors that influence soil heavy metals by using categorical regression analysis:A case study in beijing,China

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Frontiers of Environmental Science & Engineering 2020年第3期14卷 1-14页

作者： Jun Yang Jingyun Wang Pengwei Qiao Yuanming Zheng Junxing Yang Tongbin Chen Mei Lei Xiaoming Wan Xiaoyong Zhou Center for Environmental remediation Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China beijing key laboratory of remediation of industrial pollution sites Environmental Protection Research Institute of Light IndustryBeijing 100048China

Identifying the factors that influence the heavy metal contents of soil could reveal the sources of soil heavy metal *** this study,a categorical regression was used to identify the factors that influence soil heavy ***,environmental factors were associated with soil heavy metal data,and then,the degree of influence of different factors on the soil heavy metal contents in beijing was analyzed using a categorical *** results showed that the soil parent material,soil type,land use type,and industrial activity were the main influencing factors,which suggested that these four factors were important sources of soil heavy metals in *** addition,population density had a certain influence on the soil Pb and Zn *** distribution of soil As,Cd,Pb,and Zn was markedly influenced by interactions,such as traffic activity and land use type,industrial activity and population *** spatial distribution of soil heavy metal hotspots corresponded well with the influencing factors,such as industrial activity,population density,and soil parent *** this study,the main factors affecting soil heavy metals were identified,and the degree of their influence was ranked.A categorical regression represents a suitable method for identifying the factors that influence soil heavy metal contents and could be used to study the genetic process of regional soil heavy metal pollution.

关键词： Soil Heavy metal Influencing factor Categorical regression Identification method

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Colloid-facilitated release of polybrominated diphenyl ethers at an e-waste recycling site: evidence from undisturbed soil core leaching experiments

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Frontiers of Environmental Science & Engineering 2024年第2期18卷 91-101页

作者： Zebin Huo Mengjun Xi Lianrui Xu Chuanjia Jiang Wei Chen College of Environmental Science and Engineering Ministry of Education Key Laboratory of Pollution Processes and Environmental CriteriaTianjin Key Laboratory of Environmental Remediation and Pollution ControlNankai UniversityTianjin 300350China

Polybrominated diphenyl ethers (PBDEs), a class of persistent organic pollutants, have been frequently detected in soil at e-waste recycling sites. However, the key factors controlling the transport of PBDEs from surface soil to the vadose zone and groundwater are unclear. Here, colloid-enhanced leaching of PBDEs from undisturbed soil cores collected at an e-waste recycling site in Tianjin, China, is reported. Spatially heterogeneous release of colloids and PBDEs was observed in all the tested soil cores under chemical and hydrodynamic perturbations, indicating the presence of preferential flow paths. Colloid concentration in the effluent significantly increased as ionic strength decreased (from 10 to 0.01 mmol/L), probably due to the stronger electrostatic repulsion between colloidal particles and the soil matrix at lower ionic strength. In contrast, colloid mobilization was not significantly affected by the changes in pH of the influent (from 4.0 to 10.0) and flow rate (from a Darcy velocity of 1.5 to 6.0 cm/h). The concentrations of 2,2′,3,3′,4,4′,5,5′,6,6′-decabromodiphenyl ether (BDE-209), the predominant PBDE congener at the site, detected in the leachate (ranging from 1.09 to 3.43 ng/L) were much lower than previously reported results from packed column leaching tests, and were positively correlated with colloid concentrations. This indicates that remobilization of colloids at e-waste recycling sites can promote the leaching and downward migration of PBDEs from surface soil. The findings highlight the potential risk of surface soil PBDE contamination to groundwater quality and call for further understanding of colloid-facilitated transport for predicting the fate of PBDEs at e-waste recycling sites.

关键词： Polybrominated diphenyl ether Colloid-facilitated transport E-waste recycling site Undisturbed soil core Groundwater quality

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Evolution of soil DOM during thermal remediation below 100℃:concentration,spectral characteristics and complexation ability

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 31-41页

作者： Wan Huang Ziren Wan Di Zheng Lifeng Cao Guanghe Li Fang Zhang State key Joint laboratory of Environment Simulation and pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China National Engineering laboratory for Site remediation Technologies Beijing 100015China

The impact of thermal remediation on soil function has drawn increasing *** far,as the most active fraction of soil organic matter,the evolution of dissolved organic matter(DOM)during the thermal remediation lacks in-depth investigation,especially for the temperatures value below 100℃.In this study,a series of soil thermal treatment experiments was conducted at 30,60,and 90℃ during a 90-d period,where soil DOM concentration increased with heating temperature and *** molecular weight,functional groups content and aromaticity of DOM all decreased during the thermal *** excitation-emission matrices(EEM)results suggested that humic acid-like substances transformed into fulvic acid-like substances(FIII/FV increased from 0.27 to 0.44)during the heating process,and five DOM components were further identified by *** change of DOM structures and components indicated the decline of DOM stability and hydrophilicity,and can potentially change the bioavailability and *** temperature also resulted in the decline of DOM complexation ability,which may be caused by the loss of binding sites due to the decrease of polar function groups,aromatic structures and hydrophilic *** study provides valuable information about the evolution of DOM during thermal remediation,which would potentially change the fate of metal ions and the effectiveness of the post-treatment technologies in the treated region.

关键词： Thermal remediation below 100℃ Heating temperature Soil DOM concentration DOM spectral characteristics Excitation-emission matrices(EEM) Complexation ability

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Toxicity of the xenoestrogen nonylphenol and its biodegradation by the alga Cyclotella caspia

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Journal of Environmental Sciences 2013年第8期25卷 1662-1671页

作者： Yu Liu Xiaokang Dai Jie Wei School of Environmental Science and Engineering Sun Yat-Sen University Guangdong Provincial key laboratory of Environmental pollution Control and remediation Technology

Alkylphenols （APs）, the breakdown products of alkylphenol polyethoxylates that are widely used as surfactants, have been proven to exert estrogenic effects. With industrial development, higher concentrations of APs are discharged into aquatic environments. Nonylphenol （NP）, the most noxious AP, is included in the blacklist of several countries. The toxicity of NP to the alga Cyclotella caspia and the biodegradation of NP by C. caspia were studied in the laboratory. The median effective concentration at 96 hr （96 hr EC50 ） of NP for C. caspia was found to be 0.18 mg/L. Five toxicity and three degradation indices were selected for toxicity and biodegradation experiments, respectively, in five or three concentrations of NP set by the 96 hr EC50 of NP. The algal growth rate and chlorophyll a contents decreased as NP concentration increased. The main manifestations of morphological deformity of the cells included volume expansion and the presence of cytoplasmic inclusions （lipid droplets）. The abnormality rate of the cells increased with NP concentration and time, and was 100% at 0.22 and 0.26 mg/L of NP after 192 hr of culture. Superoxide dismutase activity initially increased and then declined at a higher NP toxicity of greater than 0.18 mg/L. After 192 hr of culture, the biodegradation rates of NP by C. caspia with initial concentrations of 0.14, 0.18, and 0.22 mg/L were 37.7%, 31.7%, and 6.5%, respectively. The kinetic equation of C. caspia biodegradation on NP was correlated with algal growth rate and initial NP concentration.

关键词： alkylphenol nonylphenol Cyclotella caspia toxicity biodegradation

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remediation of soil heavily polluted with polychlorinated biphenyls using a low-temperature plasma technique

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Frontiers of Environmental Science & Engineering 2014年第2期8卷 277-283页

作者： Xiuhua LI Haibo ZHANG Yongming LUO Ying TENG key laboratory of Soil Environment and pollution remediation Institute of Soil Science Chinese Academy of Sciences Nanjing 210008 China

Polychlorinated biphenyls （PCBs） were removed by low-temperature plasma technique （dielectric barrier discharge） from heavily polluted soil and their intermediate products were analyzed. The removal rate ranged from 40.1 to 84.6% by different treatments, and they were also influenced significantly （P 〈 0.01） by soil particle-size, electric power, gas flow rate and reaction time. The optimal reaction conditions of PCB removal from the soil were obtained experimentally when soil particle-size, electrical power, flow rate and reaction time were 5-10mm, 21w, 120mL. rain and 90rain, respectively. However, decreasing electrical power, flow rate and reaction time to 18 w, 60 mL. min- and 60 min respectively were also acceptable in view of the cost of remediation. This technique was characterized by the additional advantage of thorough oxidation of PCBs in the soil, with no formation of intermediate products after reaction. The technique therefore shows some promise for application in the remediation of soils contaminated with persistent organic pollutants in brown field sites in urban areas.

关键词： polychlorinated biphenyls low-temperature plasma soil contamination intermediate products

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Advances and challenges of sulfur-driven autotrophic denitrification(SDAD)for nitrogen removal

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Chinese Chemical Letters 2020年第10期31卷 2567-2574页

作者： Jiao-Jiao Wang Bao-Cheng Huang Jun Li Ren-Cun Jin key laboratory of Microbial Technology for industrial pollution Control of Zhejiang Province College of EnvironmentZhejiang University of TechnologyHangzhou 310014China laboratory of Water pollution remediation School of Life and Environmental SciencesHangzhou Normal UniversityHangzhou 311121China

Sulfur-driven autotrophic denitrification(SDAD),a process suited for the treatment of nitrogen and sulfur-polluted wastewater without extra supplement of organic carbon,is a promising biological nitrogen removal ***,the SDAD process was affected by many factors such as various electron donors,organic carbon and exogenous substances(e.g.,antibiotics and heavy metal),which prevent further ***,we conducted a detailed review of previous studies on such influence factors and its current ***,a comparative analysis was adopted to recognize the current challenges and future needs for feasible application,so as to ultimately perfect the SDAD process and extend its application scope.

关键词： Biological nitrogen removal Microbial fuel cell Mixotrophic denitrification Sulfur-oxidizing bacteria(SOB) Sulfur-driven autotrophic denitrification Anammox

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In-situ construction of abundant active centers on hierarchically porous carbon electrode toward high-performance phosphate electrosorption: Synergistic effect of electric field and capture sites

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Green Energy & Environment 2024年第1期9卷 126-137页

作者： Peng Zhang Fukuan Li Mingming He Silu Huo Xueli Zhang Benqiang Cen Dezhi Fang Kexun Li Hao Wang College of Environmental Science and Engineering Nankai UniversityTianjin300350China MOE key laboratory of pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution ControlTianjin Key Laboratory of Environmental Technology for Complex Trans-Media PollutionNankai UniversityTianjin300350China State key laboratory of Simulation and Regulation of Water Cycles in River Basins China Institute of Water Resources and Hydropower ResearchBeijing100038China

Phosphate removal is crucial for eutrophication control and water quality ***-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater ***,there are few works focused on phosphate electro-sorption,and reported electrodes cannot attach satisfactory removal capacities and ***,electro-assisted adsorption of phosphate via in-situ construction of La active centers on hierarchically porous carbon(LaPC)has been originally *** resulted LaPC composite not only possessed a hierarchically porous structure with uniformly dispersed La active sites,but also provided good conductivity for interfacial electron *** LaPC electrode achieved an ultrahigh phosphate electrosorption capability of 462.01 mg g^(-1) at 1 V,outperforming most existing *** superior phosphate removal performance originates from abundant active centers formed by the coupling of electricﬁeld and capture ***,the stability and selectivity toward phosphate capture were maintained well even under comprehensive ***,a series of kinetics and isotherms models were employed to validate the electrosorption *** work demonstrates a deep understanding and promotes a new level of phosphate electrosorption.

关键词： Electro-assisted adsorption Electrosorption Phosphate removal Active centers MOF-derived carbon

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Engineering practice of mechanical soil aeration for the remediation of volatile organic compound-contaminated sites in China： Advantages and challenges

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Frontiers of Environmental Science & Engineering 2016年第6期10卷 17-27页

作者： Yan Ma Xiaoming Du Yi Shi Deyi Hou Binbin Dong Zhu Xu Huiying Li Yunfeng Xie Jidun Fang Zheng Li Yunzhe Cao Qingbao Gu Fasheng Li School of Chemical and Environmental Engineering China University of Mining & Technology Beijing 100083 China Department of Soil pollution Control State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental Sciences Beijing 100012 China School of Environment Tsinghua University Beijing 100084 China beijing key laboratory for Risk Modeling and remediation of Contaminated sites Beijing Municipal Research Institute of Environmental Protection Beijing 100037 China Shandong key laboratory of Eco-Environmental Science for Yellow River Delta Binzhou University Binzhou 256600 China

In recent years, many industrial enterprises located in the urban centers of China have been relocated owing to the rapid increase in urban development. At the sites abandoned by these enterprises, volatile organic compounds have frequently been detected, sometimes at high concentrations, particularly at sites abandoned by chemical manufacturing enterprises. With the redevelopment of sites and changes in land-use tvpe associated with these sites, substantial amounts of contaminated soils now require remediation. ＂Since China is a developing country, soil remediation warrants the usage of techniques that are suitable for addressing the unique challenges faced in this country. Land shortage is a common problem in China; the large numbers of contaminated sites, tight development schedules, and limited financial resources necessitate the development of .cost-effective methods for land *** soil aeration is a simple, effective, and low-cost soil remediation tectm^que mat is particularly suitable for the remediation of large volatile organic compound-contaminated sites. Its effectiveness has been confirmed by conducting laboratory studies, pilot tests, and full-scale *** study reviews current engineei-ing practice and developmental trends of mechanical soil aeration and analyzes the advantages and disadvantages of this technology for application in China as an emerging soil remediation market. The findings of this study might aid technology development in China, as well as assist other developing countries in the assessment and implementation of costeffective hazardous waste site soil remediation programs.

关键词： Soil contamination Volatile organic compound Mechanical soil aeration Engineering practice China

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Effect of Land Use Conversion from Rice Paddies to Vegetable Fields on Soil Phosphorus Fractions

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Pedosphere 2010年第2期20卷 137-145页

作者： J. L. DARILEK HUANG Biao LI De-Cheng WANG Zhi-Gang ZHAO Yong-Cun SUN Wei-Xia SHI Xue-Zheng key laboratory of Soil Environment and pollution remediation Institute of Soil Science Chinese Academy of SciencesNanjing 210008 (China) Graduate University of the Chinese Academy of Sciences Beijing 100039 (China)

Excess phosphorus （P） from agricultural soils contributes to eutrophication in water bodies. Samples （n = 60） were taken from sites where rice paddies have been converted to vegetable fields for 0, 〈 10, 10-20, and 〉 20 years and analyzed for five inorganic P （Pi） fractions, three organic P （Po） fractions, and several soil parameters to investigate how land use conversion affects Pi and Po fractions in a peri-urban area of China with soils characteristic of many agricultural areas of Asia. Significant increases of 33, 281, 293, and 438 mg kg-i were found for soluble and loosely bound Pi （SL-Pi）, aluminum-bound Pi （Al-Pi）, calcium-bound Pi （Ca-Pi）, and iron-bound Pi （Fe-Pi）, respectively, after conversion from rice paddies to vegetable fields. Most of the increase in Pi was in the form of Fe-Pi, which increased from 8% of total P （TP） on paddy soil to 31% on the soil with 〉 20-year vegetable cultivation, followed by Al-Pi, which increased from 2% to 19% of TP. For Po fractions, there was no significant change in P concentrations. The conversion of land use from paddy fields to high intensity vegetable fields was causing significant changes in soil P fractious. Management practices were causing a buildup of soil P, primarily in the Fe-Pi fraction, followed by Ca-Pi and Al-Pi fractions. If current trends continue, a 30%-70% increase in TP could be expected in the next 20 years. Farmers in the area should reduce P application and use to maximize P uptake.

关键词： inorganic phosphorus organic phosphorus peri-urban agriculture phosphorus accumulation soil fertility

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