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Tuning microstructures of TC4 ELI to improve explosion resistance

Defence technology（防务技术） 2024年第3期33卷 78-99页

作者： Changle Zhang Yangwei Wang Lin Wang Zixuan Ning Guoju Li Dongping Chen Zhi-Wei Yan Yuchen Song Xucai Wang School of Materials science and Engineering Beijing Institute of TechnologyBeijing 100081China National Key Laboratory of science and technology on Materials under Shock and Impact Beijing 100081China State Key Laboratory of Explosive science and technology Beijing Institute of TechnologyBeijing 100081China Aerospace Information research institute Chinese Academy of SciencesBeijing 100094China School of aeronautical Engineering Zhengzhou University of AeronauticsHenan ProvinceZhengzhou 450046China Shanxi Jiangyang Chemical Co. Ltd.Shanxi ProvinceTaiyuan 030041China Shandong institute of Non-metallic Materials Shandong ProvinceJinan 250031China

A reasonable heat treatment process for TC4 ELI titanium alloy is crucial to tune microstructures to improve its explosion ***,there is limited investigation on tuning microstructures of TC4 ELI to improve explosion ***,the current challenge is quantifying microstructural changes'effects on explosion resistance and incorporating microstructural changes into finite element *** work aims to tune microstructures to improve explosion resistance and elucidate their anti-explosion mechanism,and find a suitable method to incorporate microstructural changes into finite element *** this work,we systematically study the deformation and failure characteristics of TC4 ELI plates with varying microstructures using an air explosion test and LS-DYNA finite element *** Johnson-Cook(JC)constitutive parameters are used to quantify the effects of microstructural changes on explosion resistance and incorporate microstructural changes into finite element *** of the heat treatment,one plate has equiaxed microstructure and the other has bimodal *** convex of the plate after the explosion has a quadratic relationship with the charge mass,and the simulation results demonstrate high reliability,with the error less than 17.5%.Therefore,it is feasible to obtain corresponding JC constitutive parameters based on the differences in microstructures and mechanical properties and characterize the effects of microstructural changes on explosion *** bimodal target exhibits excellent deformation *** response of bimodal microstructure to the shock wave may be more intense under explosive *** well-coordinated structure of the bimodal target enhances its resistance to deformation.

关键词： Microstructure Finite element modelling Parameter optimization Failure characteristics Explosion resistance

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Ultra reliability and massive connectivity provision in integrated internet of military things(IoMT)based on tactical datalink

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Defence technology（防务技术） 2024年第3期33卷 386-398页

作者： Li Bing Yating Gu Lanke Hu Li Bowen Yang Lihua Jue Wang Yue Yin Northwestern Polytechnical University Xi'an 710072China china Academy of Information and Communications technology Beijing 100191China china Intelligent and Connected Vehicles(beijing)research institute Co. LtdBeijing 100176China The 20th research institute of china Electronic technology Group Corporation Xi’an 710068China Xidian University Xi'an 710071China

One of the major challenges arising in internet of military things(IoMT)is accommodating massive connectivity while providing guaranteed quality of service(QoS)in terms of ultra-high *** this regard,this paper presents a class of code-domain nonorthogonal multiple accesses(NOMAs)for uplink ultra reliable networking of massive IoMT based on tactical datalink such as Link-16 and joint tactical information distribution system(JTIDS).In the considered scenario,a satellite equipped with Nr antennas servers K devices including vehicles,drones,ships,sensors,handset radios,*** coded modulation,a special form of multiple input multiple output(MIMO)-NOMA is *** discussion starts with evaluating the output signal to interference-plus-noise(SINR)of receiver filter,leading to the unveiling of a closed-form expression for overloading systems as the number of users is significantly larger than the number of devices admitted such that massive connectivity is *** expression allows for the development of simple yet successful interference suppression based on power allocation and phase shaping techniques that maximizes the sum rate since it is equivalent to fixed-point programming as can be *** proposed design is exemplified by nonlinear modulation schemes such as minimum shift keying(MSK)and Gaussian MSK(GMSK),two pivotal modulation formats in IoMT standards such as Link-16 and *** results show that near capacity performance is ***,the performance is obtained using simple forward error corrections(FECs)of higher coding rate than existing schemes do,while the transmit power is reduced by 6 *** proposed design finds wide applications not only in IoMT but also in deep space communications,where ultra reliability and massive connectivity is a keen concern.

关键词： Satellite network Deep space communications Internet of military things Non-orthogonal multiple access MIMO Link-16 JITDS

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Highly sensitive nanozyme strip:An effective tool for forensic material evidence identification

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Nano research 2024年第3期17卷 1785-1791页

作者： Juanji Hong Zhanjun Guo Dihan Duan Yi Zhang Xin Chen Yongjiu Li Zheng Tu Lei Feng Lei Chen Xiyun Yan Lizeng Gao Minmin Liang Demin Duan Experimental Center of Advanced Materials School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing 100081China College of Bioscience and Biotechnology Shenyang Agricultural UniversityShenyang 110866China Chongqing kangjuquanhong biology science and technology Co. ltdChongqing 400026China Key Laboratory of Forensic Genetics Institute of Forensic ScienceMinistry of Public SecurityBeijing 100038China CAS Engineering Laboratory for Nanozyme Key Laboratory of BiomacromoleculesInstitute of BiophysicsChinese Academic of ScienceBeijing 100101China

During criminal case investigations,blood evidence tracing is critical for criminal ***,the blood stains are often cleaned or covered up after the crime,resulting in trace residue and difficult ***,a highly sensitive and specific method for the rapid detection of human blood stains remains *** solve this problem,we established a nanozyme-based strip for rapid detection of blood evidence with high sensitivity and *** construct reliable nanozyme strips,we synthesized CoFe_(2)O_(4) nanozymes with high peroxidase-like activity by scaling up to gram level,which can be supplied for six million tests,and conjugated antibody as a detection probe in nanozyme *** developed CoFe_(2)O_(4) nanozyme strip can detect human hemoglobin(HGB)at a concentration as low as 1 ng/mL,which is 100 times lower than the commercially available colloidal gold strips(100 ng/mL).Moreover,this CoFe_(2)O_(4) nanozyme strip showed high generality on 12 substrates and high specificity to human HGB among 13 animal blood ***,we applied the developed CoFe_(2)O_(4) nanozyme strip to successfully detect blood stains in three real cases,where the current commercial colloidal gold strip failed to *** results suggest that the CoFe_(2)O_(4) nanozyme strip can be used as an effective on-scene detection method for human blood stains,and can further be used as a long-term preserved material evidence for traceability inquiry.

关键词： CoFe_(2)O_(4)nanozyme nanozyme strip peroxidase-like activity human hemoglobin blood evidence

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Atomistic mechanism of high ionic conductivity in lithium ytterbium-based halide solid electrolytes:A first-principles study

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Journal of Rare Earths 2024年第1期42卷 155-162,I0006页

作者： Limin Wang Wei Xiao Lu Sun Rong Yang Jinqiu Yu Ligen Wang State Key Laboratory of Nonferrous Metals and Processes China GRINM Group Co.Ltd.Beijing100088China GRIMAT Engineering institute Co. Ltd.Beijing101407China General research institute for Nonferrous Metals Beijing100088China china Automotive Battery research institute Co. Ltd.Beijing101407China Rare Earth Functional Materials(Xiong'an)Innovation Center Co. Ltd.Xiong'an071700China

As the next generation of commercial automotive power batteries begins replacing liquid lithium batteries,many look towards all-solid-state batteries to pioneer the ***-so lid-state batteries have attracted the attention of countless researchers around the world because of their high safety and high energy *** recent times,halide solid-state electrolytes have become a research hotspot within solid-state electrolytes because of their potentially superior *** this paper,in the framework of DFT,we investigated the atomic mechanisms of improving the ionic conductivity and stability of Li_(3)YbCl_(6).Our calculations show that both trigonal and orthorhombic Li_(3)YbCl_(6) exhibit wide electrochemical windows and metastable properties(100 meV/atom>Ehull>0 meV/atom).However,the orthorhombic Li_(3)YbCl_(6) can be stabilized at high temperatures by taking the vibrational entropy into account,which is supported by the experimental ***,it is expected that because of the Yb/Li synergistic interactions that,due to their strong mutual coulomb repulsion,influence the Li^(+)transport behavior,the orthorhombic Li_(3)YbCl_(6) might have superior ionic conductivities with appropriate Li+migration paths determined by the Yb^(3+) ***,higher ionic conductivities can be obtained by regulating the random distribution of Li^(+) *** Li^(+)-deficiency can also largely increase the ionic conductivity by invoking *** study helps gain a deeper understanding of the laws that govern ionic conductivities and stabilities and provides a certain theoretical reference for the experimental development and design of halide solid-state electrolytes.

关键词： Halide solid-state electrolytes Phase stability Ionic conductivity First-principles calculations Rare earths

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Exciton-harvesting enabled efficient charged particle detection in zero-dimensional halides

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Light(science & Applications) 2024年第9期13卷 1944-1955页

作者： Qian Wang Chenger Wang Hongliang Shi Jie Chen Junye Yang Alena Beitlerova Romana Kucerkova Zhengyang Zhou Yunyun Li Martin Nikl Xilei Sun Xiaoping OuYang Yuntao Wu Shanghai institute of Ceramics Chinese Academy of SciencesShanghai 201899China institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China National Engineering research Center for Rare Earth Grirem Advanced Materials Co.Ltd.and General Research Institute for Nonferrous MetalsBeijing 100088China Department of Physics Beihang UniversityBeijing 100191China Spallation Neutron Source science Center Dongguan 523803China Department of Optical Materials Institute of Physics of the Czech Academy of SciencesPrague 16200Czech Republic Northwest institute of Nuclear technology Xi’an 710024China

Materials for radiation detection are critically important and urgently demanded in diverse fields,starting from fundamental scientific research to medical diagnostics,homeland security,and environmental *** halides(LDHs)exhibiting efficient self-trapped exciton(STE)emission with high photoluminescence quantum yield(PLQY)have recently shown a great potential as ***,an overlooked issue of excitonexciton interaction in LDHs under ionizing radiation hinders the broadening of its radiation detection ***,we demonstrate an exceptional enhancement of exciton-harvesting efficiency in zero-dimensional(0D)Cs3Cu2I5:Tl halide single crystals by forming strongly localized Tl-bound *** of the suppression of nonradiative exciton-exciton interaction,an excellentα/βpulse-shape-discrimination(PSD)figure-of-merit(FoM)factor of 2.64,a superior rejection ratio of 10−9,and a high scintillation yield of 26000 photons MeV−1 under 5.49 MeVα-ray are achieved in Cs3Cu2I5:Tl single crystals,outperforming the commercial ZnS:Ag/PVT composites for charged particle detection ***,a radiation detector prototype based on Cs3Cu2I5:Tl single crystal demonstrates the capability of identifying radioactive 220Rn gas for environmental radiation monitoring *** believe that the exciton-harvesting strategy proposed here can greatly boost the applications of LDHs materials.

关键词： composites particle dimensional

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Unveiling the surface-interface properties of perovskite crystals and pivotal regulation strategies

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Nano research 2024年第5期17卷 3950-3981页

作者： Qin Li Ziyu Wang Junjie Ma Mengqi Han Peng Gao Meng Cai Yiqiang Zhang Yanlin Song Shou Peng Henan institute of Advanced technology College of ChemistryZhengzhou UniversityZhengzhou 450001China Key Laboratory of Green Printing Institute of ChemistryChinese Academy of Sciences(ICCAS)Beijing 100190China china National Building Material Group Co. Ltd.Beijing 100036China State Key Laboratory of Advanced technology for Float Glass Beijing 100036China

Metal-halide perovskite solar cells have garnered significant research attention in the last decade due to their exceptional photovoltaic performance and potential for *** achieving remarkable power conversion efficiency of up to 26.1%,a substantial discrepancy persists when compared to the theoretical Shockley-Queisser(SQ)*** of the most serious challenges facing perovskite solar cells is the energy loss incurred during photovoltaic conversion,which affects the SQ limits and stability of the *** significant than the energy loss occurring in the bulk phase of the perovskite is the energy loss occurring at the ***,we provide a systematic overview of the physical and chemical properties of the ***,we delve into the underlying mechanism causing the energy deficit and structural degradation at the surface-interface,aiming to enhance the understanding of carrier transport processes and structural chemical ***,we systematically summarized the primary modulating pathways,including surface reconstruction,dimensional construction,and electric-field ***,we propose directions for future research to advance the efficiency of perovskite solar cells towards the radiative limit and their widespread commercial application.

关键词： perovskite solar cells surface-interface treatment defect modification dimensional design energy regulation heterojunction and homojunction

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Tuning electronic properties of cobalt phthalocyanines for oxygen reduction and evolution reactions

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science china Chemistry 2024年第1期67卷 398-407页

作者： Jianlin Jiang Zhen Liu Shuaijun Pan Xinnian Xia Bing Qin Yang Hu Xuxu Wang Jiamin Lan Yu Gu Encai Ou Weijian Xu Joseph J.Richardson Rui Guo SINOPEC research institute of Petroleum Processing Co. Ltd.Beijing 100083China College of Chemistry and Chemical Engineering Hunan UniversityChangsha 410082China College of Chemistry and Materials science Hunan Agricultural UniversityChangsha 410128China Department of Chemical Engineering The University of MelbourneParkville 3010Australia College of Environmental science and Engineering Hunan UniversityChangsha 410082China School of Engineering RMIT UniversityMelbourneVictoria 3001Australia

Metal–phthalocyanines are a class of catalytically active materials promising in energy conversion and storage fields(e.g.,electrocatalysis).However,understanding and controlling the electrochemical properties in metal-phthalocyanine systems is ***,we elucidate the electrocatalytic origins of a series of cobalt-phthalocyanine molecular catalysts and finetune their electronic properties at the atomic level,both experimentally and *** interactions between the cobalt center and the local coordination environment are regulated by introducing either electron-donating or electron-withdrawing groups on the phthalocyanine ligand,and the spin-orbit splitting of cobalt is increased by~0.15 eV compared with the nonsubstituted ***,the aminated cobalt phthalocyanine-based electrocatalysts exhibit low free energies in the ratedetermining steps of the oxygen reduction(-1.68 eV)and oxygen evolution reactions(0.37 eV).This contributes to the high electrocatalytic activity(e.g.,a halfwave potential of 0.84 V and an overpotential of 0.30 V at 10 mAcm^(-2)),featuring a high selectivity of a four-electron pathway(i.e.,a negligible by-product of hydrogen peroxide).These catalysts also exhibit exceptional kinetic current density(Tafel slope of 100 mV dec^(-1))in oxygen reduction reactions,in addition to a superior power density(158 mWcm^(-2))and a high cycling stability(>1,300 cycles)in Zn-air batteries,outperforming the commercial Pt/C and/or RuO2counterparts.

关键词： interfacial wettability molecular catalysts carbon nanotubes density functional theory electrochemistry

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A model-scale test on noise from single-stream nozzle exhaust geometries in static conditions

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Chinese Journal of Aeronautics 2018年第12期31卷 2206-2220页

作者： Incheol LEE Yingzhe ZHANG Dakai LIN beijing aeronautical science and technology research institute of commercial aircraft Corporation of china Ltd. Beijing Key Laboratory of Simulation Technology for Civil Aircraft Design

A model-scale test with single-stream nozzle exhaust geometries was carried out at the anechoic chamber of Beihang University in beijing, china. The spectral characteristics are investigated, and the effects of the following parametric variations are reported in this paper: impact of nozzle operating conditions on spectra; impact of the presence of a plug; and effectiveness of chevron configurations for noise mitigation. The measurement shows that the change of pressure values has more impact on spectra than the change of temperature values. The spectral change due to pressure is shown at all band numbers for unheated conditions whereas it is more pronounced at highfrequency ranges for heated conditions. An impact of the presence of a plug is also clearly *** reduction of noise is moderate up to band number of 35, and becomes more significant at higher band numbers. It is observed that chevron nozzles are more efficient at high pressure and temperature values. It is expected that the quantified analysis will be used to develop an empirical model of single jet noise, which will be the baseline for the development of prediction of noise from turbofan engines of high bypass ratios.

关键词： Chevron Engine noise Engine plug Jet noise Single-stream jet

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New actuator disk model for propeller-aircraft computation

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science china(Technological sciences) 2016年第8期59卷 1201-1207页

作者： JIANG Zhe CHEN YaoSong AN YiRan WANG QiFeng Department of Mechanics and Engineering science College of Engineering Peking University Beijing 100871 China beijing aeronautical science & technology research institute of commercial aircraft of china ltd Beijing 102211 China

There is a growing interest in propellers for transport aircraft as well as regional airliners from the viewpoint of energy saving. An important consideration for utilizing a propeller propulsion system on aircraft is the aerodynamic interaction between the propeller slipstream and other aerodynamic surfaces. It is therefore necessary to use a simplified but relatively accurate tool for propeller modeling, with the widely used actuator disk model. The advantage of this model is that it is easy to use and inex- pensive in terms of computation time required. In addition, it also produces acceptable results. In this study, a new regionalized actuator disk model was utilized in the analysis of propeller slipstream interference effects on a real four-propeller aircraft. The results are compared with the cases of inactive actuator disks, which shows that the propeller slipstream causes an increase in the lift and drag coefficients. An evident yawing effect caused by the rotating slipstream was noticed, which should be taken into account in the design phase. The regionalized actuator disk model is evaluated as a fast and relatively accurate model for propeller preliminary design.

关键词： four-propeller aircraft propeller slipstream regionalized actuator disk model

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Discrimination of polysorbate 20 by high-performance liquid chromatography-charged aerosol detection and characterization for components by expanding compound database and library

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Journal of Pharmaceutical Analysis 2024年第5期14卷 722-732页

作者： Shi-Qi Wang Xun Zhao Li-Jun Zhang Yue-Mei Zhao Lei Chen Jin-Lin Zhang Bao-Cheng Wang Sheng Tang Tom Yuan Yaozuo Yuan Mei Zhang Hian Kee Lee Hai-Wei Shi Jiangsu institute for Food and Drug Control Nanjing210019China School of Pharmacy China Pharmaceutical UniversityNanjing211112China School of Pharmacy Nanjing University of Chinese MedicineNanjing210046China Chinese Pharmacopoeia Commission Beijing100061China Nanjing Well Pharmaceutical Group Co. Ltd.Nanjing210018China School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiangJiangsu212003China University of Massachusetts Amherst Amherst01003USA Department of Chemistry National University of SingaporeSingapore117543Singapore

Analyzing polysorbate 20(PS20)composition and the impact of each component on stability and safety is crucial due to formulation variations and individual *** similar structures and polarities of PS20 components make accurate separation,identification,and quantification *** this work,a high-resolution quantitative method was developed using single-dimensional high-performance liquid chromatography(HPLC)with charged aerosol detection(CAD)to separate 18 key components with multiple *** separated components were characterized by ultra-high-performance liquid chromatography-quadrupole time-of-flight mass spectrometry(UHPLC-Q-TOF-MS)with an identical gradient as the HPLC-CAD *** polysorbate compound database and library were expanded over 7-time compared to the commercial *** method investigated differences in PS20 samples from various origins and grades for different dosage forms to evaluate the composition-process ***-Q-TOF-MS identified 1329 to 1511 compounds in 4 batches of PS20 from different *** method observed the impact of 4 degradation conditions on peak components,identifying stable components and their tendencies to ***-CAD and UHPLC-Q-TOF-MS results provided insights into fingerprint differences,distinguishing quasi products.

关键词： Polysorbate 20 Component Database Discrimination Degradation

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