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Synergistic effect of adsorption and photocatalytic degradation of oilfield-produced water by electrospun photocatalytic fibers of Polystyrene/Nanorod-Graphitic carbon nitride

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Journal of Environmental Sciences 2024年第7期141卷 287-303页

作者： Parisa Azmoon Mehrdad Farhadian Alireza Pendashteh Amir H.Navarchian Department of Chemical Engineering Faculty of EngineeringUniversity of IsfahanIsfahanIran Department of Chemical Engineering Faculty of EngineeringUniversity of GuilanRashtIran Department of Water and Environmental Engineering Caspian Sea Basin Research CenterUniversity of GuilanRashtIran

Graphitic carbon nitride with nanorod structure(Nr-GCN)was synthesized using melamine as a precursor without any other reagents by hydrothermal pretreatment ***,FTIR,SEM,N_(2)adsorption-desorption from BET,UV-Vis DRS spectroscopy,and photoluminescence were used to characterize the prepared ***,the photoelectrochemical behavior of nanoparticles was studied by photocurrent transient response and cyclic voltammetry ***(PS)fibrous mat was fabricated by electrospinning technique and used as a support for the stabilization of the *** performance of the synthesized nanoparticles and photocatalytic fibers(PS/Nr-GCN)was evaluated in oilfield-produced water treatment under visible light *** this process,oil contaminants were adsorbed by hydrophobic polystyrene fibers and simultaneously degraded by *** removal efficiency of chemical oxygen demand(COD)has been obtained 96.6%and 98.4%by Nr-GCN and PS/Nr-GCN,respectively,at the optimum conditions of pH4,photocatalyst dosage 0.5 g/L,COD initial concentration 550 mg/L,and illumination time 150 *** gas chromatography-mass spectroscopy analysis results showed 99.3%removal of total petroleum hydrocarbons using photocatalytic fibers of PS/*** results demonstrated that the GCN has outstanding features like controllable morphology,visible-light-driven,and showing high potential in oily wastewater ***,the synergistic effect of adsorption and photocatalytic degradation is an effective technique in oilfield-produced water treatment.

关键词： Graphitic carbon nitride(GCN) Nanorod structure Polystyrene fibrous mat Photocatalytic fibers Oilfield-produced water(OPW)

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Ultrathin organic solvent nanofiltration membrane with polydopamine-HKUST-1 interlayer for organic solvent separation

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Journal of Environmental Sciences 2024年第7期141卷 182-193页

作者： Haike Li Xindong Li Guozai Ouyang Lijinhong Huang Lang Li Wenhao Li Wanfu Huang Duokun Li Ganzhou Key Laboratory of basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou 341000China Innovation center for Water Quality Security Technology at Ganjiang River basin Jiangxi University of Science and TechnologyGanzhou 341000China School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou 341000China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityWA 6845Australia School of Materials Science and Engineering Tiangong UniversityTianjin 300387China

Polydopamine(PDA)and metal-organic skeleton HKUST-1 were co-deposited on the base membrane of hexamethylenediamine(HDA)-crosslinked polyetherimide(PEI)ultrafiltration membrane as the interlayer,and high-throughput organic solvent nanofiltration membrane(OSN)was prepared by interfacial polymerization and solvent activation *** polyamide(PA)layer surface roughness from 28.4 nm in PA/PEI to 78.3 nm in PA/PDA-HKUST-10.6/PEI membrane,reduced the thickness of the separation layer from 79 to 14 nm,and significantly improved the hydrophilic,thermal and mechanical *** flux of the PA/PDA-HKUST-10.6/PEI membrane in a 0.1 g/L Congo Red(CR)ethanol solution at 0.6 MPa test pressure reached 21.8 L/(m^(2)·hr)and the rejection of CR was 92.8%.Solvent adsorption test,N,N-dimethylformamide(DMF)immersion experiment,and long-term operation test in ethanol showed that the membranes had high solvent *** solvent flux test demonstrated that,under the test pressure of 0.6 MPa,the flux of different solvents ranked as follows:methanol(56.9 L/(m^(2)·hr))>DMF(39.6 L/(m^(2)·hr))>ethanol(31.2 L/(m^(2)·hr))>IPA(4.5 L/(m^(2)·hr))>N-hexane(1.9 L/(m^(2)·hr)).The ability of the membranes to retain dyes in IPA/water dyes solution was also *** flux of the membrane was 30.4 L/(m^(2)·hr)and the rejection of CR was 91.6%when the IPA concentration reached 50%.This OSN membrane-making strategy is economical,environment-friendly and efficient,and has a great application prospect in organic solvent separation systems.

关键词： Interfacial polymerization Organic solvent nanofiltration Interlayer Metal-organic frameworks Polydopamine

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Seismic attribute and well-log analysis for channel characterization in the upper San Andres and Grayburg formations of the Midland basin,Texas

Energy Geoscience

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Energy Geoscience 2024年第2期5卷 263-278页

作者： Sumit Verma Esra Yalçın Yılmaz Laura Ortiz Sanguino Justin Yandell Miles A.Henderson Robert C.Trentham Department of Geosciences The University of Texas Permian BasinOdessaTXUSA School of Geosciences The University of OklahomaNormanOKUSA

The Permian basin is one of the most prolific,and currently one of the most active,oil and gas basins in the *** Lower Permian strata in the Permian basin have produced more than 14 billion barrels of oil(BBO),making it the largest volume of hydrocarbon in the *** in the Midland basin during late Leonardian through early Guadalupian(ca.272e269 Ma)resulted in progradation of shelf edge and ultimately closure of the basin by Middle Permian *** analyzed a merged seismic survey covering parts of the Permian basin(i.e.,Central basin Platform and Midland basin)in Andrews,Ector,and Midland Counties,*** seismic survey and well logs show the presence of gently dipping(ca.1°)clinoforms in the Upper San Andres and Grayburg Formations on the eastern edge of the Central basin Platform and western Midland *** seismic attributes,curvature,and spectral decomposition identify low sinuosity slope channels oriented north-south,but such channels do not appear beyond the *** shelf edge shifts from north to south during deposition of the Upper San Andres and Grayburg *** identify five basinward shifts noted by the migration of the shelf edge toward the basin center and the presence of channel features along the depositional *** petrophysical analysis indicates that channels cut into carbonate rocks and are filled by siliciclastic sediments;this interpretation is supported by the most negative curvature anomalies along the channel axes caused by the differential compaction between the carbonate and siliciclastic *** are a few channels with a northwest-southeast strike,which matches the direction of the Concho Lineament observed by satellite *** observations are consistent with previous interpretations of the northern Midland basin closure during Middle-Late Permian time.

关键词： Permian shelf carbonate

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River width and depth as key factors of diurnal activity energy expenditure allocation for wintering Spot-billed Ducks in the Xin'an River basin

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Avian Research 2024年第1期15卷 116-122页

作者： Chao Yu Xuying Lu Deli Sun Mengnan Chu Xueyun Li Qun Li College of Life and Environmental Sciences Huangshan UniversityHuangshan245021China Environment Conservation Research Centre of Xin’an River basin Huangshan UniversityHuangshan 245021China Department of Resources Conservation Southern Anhui National Wildlife Rescue CenterXiuning 245400China

Rivers are important habitats for wintering ***,they are easily influenced by natural and human *** important approach for waterbirds to adapt to habitats is adjusting the activity time and energy expenditure allocation of diurnal *** compensatory foraging hypothesis predicts that increased energy expenditure leads to longer foraging time,which in turn increases food intake and helps maintain a constant energy ***,it is unclear whether human-disturbed habitats result in increased energy expenditure related to safety or *** this study,the scan sample method was used to observe the diurnal behavior of the wintering Spot-billed Duck(Anas poecilorhyncha) in two rivers in the Xin’an River basin from October 2021 to March *** allocation of time and energy expenditure for activity in both normal and disturbed environments was *** results showed that foraging accounted for the highest percentage of time and energy ***,foraging decreased in the disturbed environment than that in the normal *** behavior showed the opposite trend,while other behaviors were similar in both *** total diurnal energy expenditure of ducks in the disturbed environment was greater than that in the normal environment,with decreased foraging and resting time percentage and increased behaviors related to immediate safety(swimming and alert) and *** results oppose the compensatory foraging hypothesis in favor of increased *** optimal diurnal energy expenditure model included river width and water depth,which had a positive relationship;an increase in either of these two factors resulted in an increase in energy *** study provides a better understanding of energy allocation strategies underlying the superficial time allocation of wintering waterbirds according to environmental *** these changes can help understand the maximum fitness of wi

关键词： Diurnal behavior activities River factors Time and energy expenditure allocation Wintering Spot-billed Duck Xin’an River basin

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Water-soluble chitosan promotes remediation of Pb-contaminated soil by Hylotelephium spectabile

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 109-122页

作者： Bingxin Guo Yiwei Zhang Junxing Yang Tianwei Qian Junmei Guo Xiaona Liu Yuan Jiao Tongbin Chen Guodi Zheng Wenjun Li Fei Qi College of Environmental Science and Engineering Taiyuan University of TechnologyShanxi Key Laboratory of Earth Surface Processes and Resource Ecological Security in Fenhe River BasinShanxi Engineering Research Center of Low Carbon Remediation for Water and Soil Pollution in Yellow River BasinJinzhong 030600China center for Environmental Remediation Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China Shanxi Transportation Holding Ecological Environment Co. Ltd.Shanxi 030000China Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Water-soluble chitosan(WSC)has been studied for its ability to mobilize soil Pb and promote the phytoremediation by Hylotelephium spectabile in Pb-contaminated *** aimed to clarify the internal mechanism by which wSC impacts phytoremediation by examining plant growth and Pb accumulation performance of *** as well as the Pb form,functional groups,and mineral phases of Pb-contaminated *** effectively decreased soil pH and activated Pb migration in rhizosphere soils,with a considerable increase in water-soluble and acid-extractable Pb by 29%-102%and 9%-65%,respectively,and a clear decreasing trend in reducible and oxidizable ***-transform infrared spectroscopy revealed a significant increase in amino and hydroxyl groups in the soil generated by *** coordination of Pb with amino and hydroxyl groups may play an important role in the formation of Pb complexes and activation of Pb in *** field trials,the application of WSC significantly increased Pb accumulation in *** by 125.44%,reaching 92 g/hm^(2).Moreover,the organic matter and nitrogen in the soils were increased by WSc,which improved the growth conditions of *** obvious growth inhibition was observed in either the pot or field ***,WSC is a promising chelating agent for mobilizing Pb in ***,WSC can be potentially used to boost ***-mediated phytoremediation of Pb-contaminatedfarmland.

关键词： Phytoremediation Pb-contaminated soil Water-soluble chitosan Hylotelephium spectabile Fourier transform infrared spectroscopy

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Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao Li Lijinhong Huang Bin Xiao Xiaoguang Duan Haike Li Lang Li Wanfu Huang Ganzhou Key Laboratory of basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation center for Water Quality Security Technology at Ganjiang River basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the Langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

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Exploring the blindspot:The soil plastisphere

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Soil Ecology Letters 2024年第2期6卷 1-4页

作者： Xiaoxuan Su Kai Yang Interdisciplinary Research center for Agriculture Green Development in Yangtze River basin Southwest UniversityChongqing400715China Key Laboratory of Urban Environment and Health Institute of Urban EnvironmentChinese Academy of SciencesXiamen361021China

Plastic pollution is a growing concern in soil ecosystems *** accumulation of(micro)plastic debris leads to a unique microenvironment,termed the“plastisphere.”Notably,the dynamics and behaviors of the soil plastisphere diverge from its marine counterpart,where it is initially defined,thereby likely exhibiting an uncharacterized feature in ecological effects and *** understanding of the soil plastisphere holds significant implications for environmental science and practical applications in pollution management and agricultural *** with the oceanic plastisphere,research on the soil plastisphere is still in its infancy with limited but significant studies contributing to current knowledge.A recent seminal work by Rillig et al.(Rillig et al.,*** Reviews ***:10.1038/s41579-023-00967-2)has inspired us and provided comprehensive insights into the characteristics and function of the soil *** this commentary,we present core aspects of the soil plastisphere,encompassing its microbial communities,biogeochemical processes,and ecological implications,as well as highlight current methodologies probing this domain.

关键词： soil pollution thereby

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Mechanism of Diabatic Heating on Precipitation and the Track of a Tibetan Plateau Vortex over the Eastern Slope of the Tibetan Plateau

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Advances in Atmospheric Sciences 2024年第1期41卷 155-172页

作者： Yuanchang DONG Guoping LI Xiaolin XIE Long YANG Peiwen ZHANG Bo ZENG Institute of Plateau Meteorology China Meteorological Administration(CMA)/Heavy Rain and Drought-Flood Disaster in Plateau and Basin Key Laboratory of Sichuan ProvinceChengdu 610072China School of Atmospheric Sciences Chengdu University of Information TechnologyChengdu 610225China Meteorological Observation Data center of Sichuan Province Chengdu 610072China Sichuan Branch of Meteorologist Training Institute CMAChengdu 610072China

Existing studies contend that latent heating(LH)will replace sensible heating(SH)to become the dominant factor affecting the development of the Tibetan Plateau vortex(TPV)after it moves off the Tibetan Plateau(TP).However,in the process of the TPV moving off the TP requires that the airmass traverse the eastern slope of the Tibetan Plateau(ESTP)where the topography and diabatic heating(DH)conditions rapidly *** LH gradually replaces SH to become the dominant factor in the development of the TPV over the ESTP is still not very *** this paper,an analysis of a typical case of a TPV with a long life history over the ESTP is performed by using multi-sourced meteorological data and model *** results show that SH from the TP surface can change the TPV-associated precipitation distribution by temperature advection after the TPV moves off the *** LH can then directly promote the development of the TPV and has a certain guiding effect on the track of the *** SH can control the active area of LH by changing the falling area of the TPV-associated precipitation,so it still plays a key role in the development and tracking of the TPV even though it has moved out of the main body of the TP.

关键词： eastern slope of the Tibetan Plateau diabatic heating Tibetan Plateau vortex precipitation distribution track

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A study on the impact of heritage protection on urban carbon emissions

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Science China Technological Sciences 2024年第9期67卷 2675-2692页

作者： WANG Fang XUE PengCheng WANG ShunYi LIU YunHuai River basin Habitats Research center College of Architecture and Landscape ArchitecturePeking University Shanxi Key Laboratory of Watershed Built Environment with Locality (Peking University) Peking University College of Urban and Environmental Sciences Peking University School of Computer Science Peking University

A major goal of current international urban development and construction is to lower carbon emissions. Synergies exist between the preservation of historic cities and the development of low-carbon cities; however, the relationship between preservation of historic cities and carbon emissions remains unclear. This study focuses on the cities in the “Yellow-Canal-Yangtze” watershed community, which includes the Yellow River basin, Yangtze River basin, and the Grand Canal region, and aims to verify the differences in CO2emissions（CE） between historic and non-historic cities through multiple comparisons after ***, Ridge Regression was used to determine the impact and dimensions of the relevant variables associated with the preservation of historic cities on CE. Combined with national development goals, this study predicts changes in the CE of historic city preservation under different scenarios. This study found significant differences between historic and non-historic cities, as the total CE of historic cities is 2.42 times higher than that of non-historic cities. The dimension with the largest difference was the CE related to transportation, with aviation emissions of historic cities reaching 15.22 times higher than that of non-historic cities. Although the preservation of historic cities has led to an overall increase in the CE, there is significant potential for CE reduction in land use, transportation infrastructure, and tourism development related to historic city preservation. In the future, historic cities can contribute to China's carbon neutrality and the United Nation's development goals through the creation of larger historical preservation areas, more convenient public transportation, and more vibrant tourism.

关键词： CO2 emissions urban planning cultural heritage historic city “Yellow-Canal-Yangtze” watershed community

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Ecological problems and ecological restoration zoning of the Aral Sea

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Journal of Arid Land 2024年第3期16卷 315-330页

作者： BAO Anming YU Tao XU Wenqiang LEI Jiaqiang JIAPAER Guli CHEN Xi Tojibaev KOMILJON Shomurodov KHABIBULLO Xabibullaev B SAGIDULLAEVICH Idirisov KAMALATDIN State Key Laboratory of Desert and Oasis Ecology Xinjiang Institute of Ecology and GeographyChinese Academy of SciencesUrumqi 830011China Key Laboratory of GIS&RS Application Xinjiang Uygur Autonomous RegionUrumqi 830011China University of Chinese Academy of Sciences Beijing 100049China CAS Research center for Ecology and Environment of Central Asia Urumqi 830011China Institute of Botany of the Academy of Sciences of the Republic of Uzbekistan Tashkent 100125Uzbekistan International Innovation center for Aral Sea basin under the President of the Republic of Uzbekistan Nukus 230100Uzbekistan

The Aral Sea was the fourth largest lake in the world but it has shrunk dramatically as a result of irrational human activities, triggering the "Aral Sea ecological crisis". The ecological problems of the Aral Sea have attracted widespread attention, and the alleviation of the Aral Sea ecological crisis has reached a consensus among the five Central Asian countries(Kazakhstan, Uzbekistan, Tajikistan, Kyrgyzstan, and Turkmenistan). In the past decades, many ecological management measures have been implemented for the ecological restoration of the Aral Sea. However, due to the lack of regional planning and zoning, the results are not ideal. In this study, we mapped the ecological zoning of the Aral Sea from the perspective of ecological restoration based on soil type, soil salinity, surface water, groundwater table, Normalized Difference Vegetation Index(NDVI), land cover, and aerosol optical depth(AOD) data. Soil salinization and salt dust are the most prominent ecological problems in the Aral Sea. We divided the Aral Sea into 7 first-level ecological restoration subregions(North Aral Sea catchment area in the downstream of the Syr Darya River(Subregion Ⅰ);artificial flood overflow area in the downstream of the Aral Sea(Subregion Ⅱ);physical/chemical remediation area of the salt dust source area in the eastern part of the South Aral Sea(Subregion Ⅲ);physical/chemical remediation area of severe salinization in the central part of the South Aral Sea(Subregion Ⅳ);existing water surface and potential restoration area of the South Aral Sea(Subregion Ⅴ);Aral Sea vegetation natural recovery area(Subregion Ⅵ);and vegetation planting area with slight salinization in the South Aral Sea(Subregion Ⅶ)) and 14 second-level ecological restoration subregions according to the ecological zoning principles. Implementable measures are proposed for each ecological restoration subregion. For Subregion Ⅰ and Subregion Ⅱ with lower elevations, artificial flooding should be carried out to re

关键词： ecological restoration zoning salt and dust storms soil salinization ecological crisis Aral Sea Central Asia

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