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Enhancing multifunctional photocatalysis with acetate-assisted cesium doping and unlocking the potential of Z-scheme solar water splitting

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Carbon Energy 2024年第3期6卷 178-195页

作者： Mengmeng Ma Jingzhen Li Xiaogang Zhu Kong Liu Kaige Huang Guodong Yuan Shizhong Yue Zhijie Wang Shengchun Qu Key Laboratory of Semiconductor Materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijingChina Center of Materials Science and Optoelectronics engineering University of Chinese Academy of SciencesBeijingChina Department of physics College of Physical Science and TechnologyXiamen UniversityXiamenChina State Key Laboratory for Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijingChina

Graphitic carbon nitride(g-C_(3)N_(4))has been extensively doped with alkali metals to enlarge photocatalytic output,in which cesium(Cs)doping is predicted to be the most ***,the sluggish diffusion and doping kinetics of precursors with high melting points,along with imprecise regulation,have raised the debate on whether Cs doping could make *** this matter,we attempt to confirm the positive effects of Cs doping on multifunctional photocatalysis by first using cesium acetate with the character of easy *** optimized Csdoped g-C_(3)N_(4)(CCN)shows a 41.6-fold increase in visible-light-driven hydrogen evolution reaction(HER)compared to pure g-C_(3)N_(4) and impressive degradation capability,especially with 77%refractory tetracycline and almost 100%rhodamine b degradedwithin an *** penetration ofCs+is demonstrated to be a mode of interlayer doping,and Cs–N bonds(especially with sp^(2) pyridine N in C═N–C),along with robust chemical interaction and electron exchange,are *** atomic configuration triggers the broadened spectral response,the improved charge migration,and the activated photocatalytic ***,we evaluate the CCN/cadmium sulfide hybrid as a Z-scheme configuration,promoting the visible HER yield to 9.02 mmol g^(−1) h^(−1),which is the highest ever reported among all CCN *** work adds to the rapidly expanding field of manipulation strategies and supports further development of mediating served for photocatalysis.

关键词： acetate-assisted cesium doping multifunctional photocatalysis Z-scheme

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Recension of boron nitride phase diagram based on high-pressure and high-temperature experiments

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Chinese physics b 2024年第10期33卷 450-457页

作者： Ruike Zhang Ruiang Guo Qian Li Shuaiqi Li Haidong Long Duanwei He institute of Atomic and Molecular physics Sichuan UniversityChengdu 610065China College of physics and Electronic engineering Chongqing Normal UniversityChongqing 401331China Key Laboratory of High Energy Density physics and Technology of Ministry of Education Sichuan UniversityChengdu 610065China

Cubic boron nitride and hexagonal boron nitride are the two predominant crystalline structures of boron *** can interconvert under varying pressure and temperature ***,this transformation requires overcoming significant potential barriers in dynamics,which poses great difficulty in determining the c-bN/h-bN phase *** study used high-pressure in situ differential thermal measurements to ascertain the temperature of h-bN/c-bN conversion within the commonly used pressure range(3-6 GPa)for the industrial synthesis of c-bN to constrain the P-T phase boundary of h-bN/c-bN in the pressure-temperature range as much as *** on the analysis of the experimental data,it is determined that the relationship between pressure and temperature conforms to the following equation:P=a+1/***,P denotes the pressure(GPa)and T is the temperature(K).The coefficients are a=-3.8±0.8 GPa and b=229.8±17.1 GPa/*** findings call into question existing high-pressure and high-temperature phase diagrams of boron nitride,which seem to overstate the phase boundary temperature between c-bN and *** bN phase diagram obtained from this study can provide critical temperature and pressure condition guidance for the industrial synthesis of c-bN,thus optimizing synthesis efficiency and product performance.

关键词： hexagonal boron nitride phase diagram high temperature and high pressure cubic boron nitride phase transition differential thermal analysis

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Quantum control for time-dependent noise by inverse geometric optimization

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Science China(physics,Mechanics & Astronomy) 2024年第9期67卷 51-57页

作者： Xiaodong Yang Yingcheng Li Ran Liu Xinfang Nie Tao Xin Dawei Lu Jun Li institute of Quantum Precision Measurement State Key Laboratory of Radio Frequency Heterogeneous IntegrationCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China State Key Laboratory of Surface physics Department of PhysicsCenter for Field Theory and Particle Physicsand Institute for Nanoelectronic Devices and Quantum ComputingFudan UniversityShanghai 200433China Shenzhen institute for Quantum Science and engineering and Department of physics Southern University of Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Quantum Science and engineering Southern University of Science and TechnologyShenzhen 518055China Quantum Science Center of Guangdong-Hong Kong-Macao Greater bay Area(Guangdong) Shenzhen 518045China

Quantum systems are exceedingly difficult to engineer because they are sensitive to various types of *** particular,timedependent noises are frequently encountered in experiments but how to overcome them remains a challenging *** this work,we propose a flexible robust control technique to resist time-dependent noises based on inverse geometric optimization working in the filter-function *** basic idea is to parameterize the control filter function geometrically and minimize its overlap with the noise spectral *** then effectively reduces the noise susceptibility of the controlled system *** show that the proposed method can produce high-quality robust pulses for realizing desired quantum evolutions under realistic noise ***,we demonstrate this method in examples including dynamical decoupling and quantum sensing protocols to enhance their performances.

关键词： time-dependent noise robust control quantum gates and states dynamical decoupling quantum sensing

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Research of caged dynamics of clusters center atoms in Pd_(82)Si_(18) amorphous alloy

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Chinese physics b 2024年第4期33卷 623-629页

作者：邓永和陈贝祁清华李兵兵高明文大东王小云彭平 School of Computational Science and Electronics Hunan Institute of EngineeringXiangtan 411104China School of physics and Mechanical&Electrical engineering Jishou UniversityJishou 416000China School of Materials Science and engineering Hunan UniversityChangsha 410082China

To date,there is still a lack of a comprehensive explanation for caged dynamics which is regarded as one of the intricate dynamic behaviors in amorphous *** study focuses on Pd_(82)Si_(18)as the research object to further elucidate the underlying mechanism of caged dynamics from multiple perspectives,including the cage's lifetime,atomic local environment,and atomic potential *** results reveal that Si atoms exhibit a pronounced cage effect due to the hindrance of Pd atoms,resulting in an anomalous peak in the non-Gaussian *** in-depth investigation was conducted on the caged dynamics differences between fast and slow Si *** comparison to fast Si atoms,slow Si atoms were surrounded by more Pd atoms and occupied lower potential energy states,resulting in smaller diffusion displacements for the slow Si ***,slow Si atoms tend to be in the centers of smaller clusters with coordination numbers of 9 and *** the isothermal relaxation process,clusters with coordination numbers 9 and 10 have longer lifetimes,suggesting that the escape of slow Si atoms from their cages is more *** findings mentioned above hold significant implications for understanding the caged dynamics.

关键词： caged dynamics Pd_(82)Si_(18) amorphous alloy fast and slow atoms clusters lifetime

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Extending microwave-frequency electric-field detection through single transmission peak method

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Chinese physics b 2024年第5期33卷 417-423页

作者：刘青陈进湛王赫张杰阮伟民伍国柱郑顺元罗景庭宋振飞 College of physics and Optoelectronic engineering Shenzhen UniversityShenzhen 518060China Shenzhen institute for Technology Innovation National Institute of MetrologyShenzhen 518107China Center for Advanced Measurement Science National Institute of MetrologyBeijing 100029China

The strength of microwave(MW)electric field can be observed with high precision by using the standard electromagnetically induced transparency and Aulter–Towns(EIT-AT)technique,when its frequency is resonant or nearly-resonant with the Rydberg transition *** the detuning of MW field increases,one of the transmission peaks(single peak)is easier to measure due to its increased *** can be found that the central symmetry point of the two transmission peaks f_(1/2)is only related to the detuning of MW field△_(MW)and central symmetry point f_(0)of resonant MW field,satisfying the relation f_(1/2)=△_(MW)/2+f_(0).Thus,we demonstrate a single transmission peak method that the MW E-field can be determined by interval between the position of single peak and f_(1/2).We use this method to measure continuous frequencies in a band from-200 MHz to 200 MHz of the MW *** experimental results and theoretical analysis are presented to describe the effectiveness of this *** 50 MHzblem that the AT splitting cannot be measured by using the standard EIT-AT techniques or multiple atomic-level Rydberg atom schemes.

关键词： microwave electric field Rydberg atom electromagnetically induced transparency(EIT) Aulter-Towns splitting

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Polarization control of above-threshold ionization spectrum in elliptically polarized two-color laser fields

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Chinese physics b 2024年第4期33卷 136-144页

作者：金发成杨慧慧宋晓红李飞杜玲玲薛红杰魏丽敏白悦刘浩翔王兵兵杨玮枫 Faculty of Science Xi'an Aeronautical InstituteXi'an 710077China School of physics and Optoelectronic engineering Hainan UniversityHaikou 570288China Center for Theoretical physics Hainan UniversityHaikou 570288China Laboratory of Optical physics Beijing National Laboratory for Condensed Matter PhysicsInstitute of PhysicsChinese Academy of SciencesBeijing 100190China College of Science Shantou UniversityShantou 515063China University of Chinese Academy of Sciences Beijing 100049China

We study the above-threshold ionization(ATI)process of atoms exposed to fundamental and high-frequency lasers with arbitrary ellipticity by applying the frequency-domain *** is found that the angular-resolved ATI spectrum is sensitive to ellipticities of two lasers and emitted angles of the *** for the photon energy of the highfrequency laser more than atomic ionization potential,the width of plateau tends to a constant with increasing ellipticity of fundamental field,the dip structure disappears with increasing ellipticity of the high-frequency *** the help of the quantum channel analysis,it is shown that the angular distribution depends mainly on the ellipticity of high-frequency field in the case that its frequency is ***,one can see that the maximal and minimal energies in quantum numerical results are in good agreement with the classical *** investigation may provide theoretical support for experimental research on polarization control of ionization in elliptically polarized two-color laser fields.

关键词： above-threshold ionization two-color laser polarization control

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Molecular dynamics study of primary radiation damage in TiVTa concentrated solid-solution alloy

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Chinese physics b 2024年第3期33卷 530-535页

作者：赵永鹏豆艳坤贺新福曹晗王林枫邓辉球杨文 Reactor engineering Technology Research Division China Institute of Atomic EnergyBeijing 102413China School of physics and Electronics Hunan UniversityChangsha 410082China

The primary radiation damage in pure V and TiVTa concentrated solid-solution alloy(CSA)was studied using a molecular dynamics *** have performed displacement cascade simulations to explore the generation and evolution behavior of irradiation *** results demonstrate that the defect accumulation and agglomeration in TiVTa CSA are significantly suppressed compared to pure *** peak value of Frenkel pairs during cascade collisions in TiVTa CSA is much higher than that in pure V due to the lower formation energy of point ***,the longer lifetime of the thermal spike relaxation and slow energy dissipation capability of TiVTa CSA can facilitate the recombination of point *** defect agglomeration rate in TiVTa CSA is much lower due to the lower binding energy of interstitial clusters and reduced interstitial ***,the occurrence probability of dislocation loops in TiVTa CSA is lower than that in pure *** reduction in primary radiation damage may enhance the radiation resistance of TiVTa CSA,and the improved radiation tolerance is primarily attributed to the relaxation stage and long-term defect evolution rather than the ballistic *** results can provide fundamental insights into irradiation-induced defects evolution in refractory CSAs.

关键词： concentrated solid-solution alloy primary radiation damage molecular dynamics simulation

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Surface-modified Ag@Ru-P25 for photocatalytic CO_(2) conversion with high selectivity over CH_(4) formation at the solid–gas interface

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Carbon Energy 2024年第1期6卷 182-196页

作者： Chaitanya b.Hiragond Sohag biswas Niket SPowar Junho Lee Eunhee Gong Hwapyong Kim Hong Soo Kim Jin-Woo Jung Chang-Hee Cho bryan M.Wong Su-Il In Department of Energy Science&engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)DaeguRepublic of Korea Department of Chemical&Environmental engineering Materials Science&Engineering ProgramDepartment of ChemistryDepartment of Physics&AstronomyUniversity of California-RiversideRiversideCaliforniaUSA Department of physics and Chemistry Daegu Gyeongbuk Institute of Science and Technology(DGIST)DaeguRepublic of Korea NiceScience Corporation DaeguRepublic of Korea

Systematic optimization of the photocatalyst and investigation of the role of each component is important to maximizing catalytic activity and comprehending the photocatalytic conversion of CO_(2) reduction to solar fuels.A surface-modified Ag@Ru-P25 photocatalyst with H_(2)O_(2) treatment was designed in this study to convert CO_(2) and H_(2)O vapor into highly selective *** doping followed by Ag nanoparticles(NPs)cocatalyst deposition on P25(TiO_(2))enhances visible light absorption and charge separation,whereas H_(2)O_(2) treatment modifies the surface of the photocatalyst with hydroxyl(–OH)groups and promotes CO_(2) ***-resonance transmission electron microscopy,X-ray photoelectron spectroscopy,X-ray absorption near-edge structure,and extended X-ray absorption fine structure techniques were used to analyze the surface and chemical composition of the photocatalyst,while thermogravimetric analysis,CO_(2) adsorption isotherm,and temperature programmed desorption study were performed to examine the significance of H_(2)O_(2) treatment in increasing CO_(2) reduction *** optimized Ag1.0@Ru1.0-P25 photocatalyst performed excellent CO_(2) reduction activity into CO,CH4,and C2H6 with a~95%selectivity of CH4,where the activity was~135 times higher than that of pristine TiO_(2)(P25).For the first time,this work explored the effect of H_(2)O_(2) treatment on the photocatalyst that dramatically increases CO_(2) reduction activity.

关键词： gas-phase CO_(2) reduction H_(2)O_(2) treatment plasmonic nanoparticles solar fuel photocatalyst surface modification

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Exploration of microscopic physical processes of Z-pinch by a modified electrostatic direct implicit particle-in-cell algorithm

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Chinese physics b 2024年第9期33卷 433-442页

作者： Kaixuan Li Cheng Ning Ye Dong Chuang Xue institute of Applied physics and Computational Mathematics Beijing 100088China

For investigating efficiently the stagnation kinetic-process of Z-pinch,we develop a novel modified electrostatic implicit particle-in-cell algorithm in radial one-dimension for Z-pinch simulation in which a small-angle cumulative binary collision algorithm is *** our algorithm,the electric field in z-direction is solved by a parallel electrode-plate model,the azimuthal magnetic field is obtained by Ampere’s law,and the term for charged particle gyromotion is approximated by the cross product of the averaged velocity and magnetic *** simulation results of 2 MA deuterium plasma shell Zpinch,the mass-center implosion trajectory agrees generally with that obtained by one-dimensional MHD simulation,and the plasma current also closely aligns with the external *** phase space diagrams and radial-velocity probability distributions of ions and electrons are *** main kinetic characteristic of electron motion is thermal equilibrium and oscillation,which should be oscillated around the ions,while that of ion motion is implosion *** the region of stagnation radius,the radial-velocity probability distribution of ions transits from the non-equilibrium to equilibrium state with the current increasing,while of electrons is basically the equilibrium *** the initial ion density and current peak are not high enough,the ions may not reach their thermal equilibrium state through collisions even in its stagnation phase.

关键词： Z-pinch particle-in-cell ion heating charged particle collisions

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Electron kinetic effects in back-stimulated Raman scattering bursts driven by broadband laser pulses

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Matter and Radiation at Extremes 2024年第4期9卷 54-67页

作者： Q.K.Liu L.Deng Q.Wang X.Zhang F.Q.Meng Y.P.Wang Y.Q.Gao H.b.Cai S.P.Zhu Graduate School China Academy of Engineering PhysicsBeijing 100088China institute of Applied physics and Computational Mathematics Beijing 100094China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230026China Shanghai institute of Laser Plasma Shanghai 201800China HEDPS Center for Applied Physics and TechnologyPeking UniversityBeijing 100871China School of physics Zhejiang UniversityHangzhou 310027China

We examine electron kinetic effects in broadband-laser-driven back-stimulated Raman scattering(bSRS)bursts using particle-in-cell *** bursts occur during the nonlinear stage,causing reflectivity spikes and generating large numbers of hot ***-duration simulations are performed to observe burst events,and a simplified model is developed to eliminate the interference of the broadband laser’s random intensity *** the simplified model,we isolate and characterize the spectrum of electron plasma *** spectrum changes from a sideband structure to a turbulence-like structure during the burst.A significant asymmetry in the spectrum is *** asymmetry is amplified and transferred to electron phase space by high-intensity broadband laser pulses,leading to violent vortex-merging and generation of hot *** proportion of hot electrons increases from 6.76%to 14.7%during a single violent burst *** demonstrate that kinetic effects profoundly influence the bSRS evolution driven by broadband lasers.

关键词： scattering kinetic simplified

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