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Magnetic nanoparticle-modified hollow double-shell SiC@C@FeCo with excellent electromagnetic wave absorption

Nano Research 2024年第4期17卷 3164-3174页

作者： Guiyu Peng Jintang Zhou Jiaqi Tao Weize Wang Jun Liu Junru Yao Yijie Liu Zhengjun Yao College of Materials science and technology Nanjing University of Aeronautics and AstronauticsNanjing 211100China key laboratory of Material Preparation and protection for Harsh environment(Nanjing University of Aeronautics and Astronautics) Ministry of Industry and Information TechnologyNanjing 211100China

Integrated micro and nanostructures,heterogeneous components,defects,and interfaces is the way to develop high-performance microwave absorbing ***,there still needs to be more precise experimental routes and effective *** this work,by a continuous process of vacuum sintering,hydrothermal,and carbon thermal reduction,magnetic FeCo nanoparticles were successfully embedded on the hollow double-shell mesoporous SiC@C surface,thus solving the challenges of a single component loss *** hollow double-shell nanostructure introduces air to enhance impedance matching while significantly reducing the density of the *** extensive defects and heterogeneous grain boundaries effectively enhance the polarization loss *** magnetic loss mechanism introduced by the magnetic particles effectively improves the impedance matching properties of the *** synergy of these multiple advantages has enabled the SCFC_(2)-8(here SiC@C@FeCo is abbreviated to SCFC,2 represents the initial metal ion content,and 8 represents the hydrothermal time)sample to achieve an adequate absorption bandwidth of 6.09 GHz at 2.0 *** a minimum reflection loss of-60.56 dB,the absorption bandwidth can cover the entire C,X,and Ku bands by adjusting the matching thickness(1.3–4.0 mm).This work provides a valuable paradigm for the deeper exploitation of microwave absorption potential and guides the development of other high-performance materials.

关键词： SiC@C@FeCo(SCFC)composites core–shell hollow structure microwave absorption

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Magneto-electric integrated design strategy of NiCo@C composites for synergistic absorption and conversion in mid-high frequency microwaves

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Nano Research 2024年第4期17卷 2205-2215页

作者： Yijie Liu Jintang Zhou Xiaoxuan He Lvtong Duan Yucheng Wang Zhenyu Cheng Zhengjun Yao College of Materials science and technology Nanjing University of Aeronautics and AstronauticsNanjing 211100China key laboratory of Material Preparation and protection for Harsh environment(Nanjing University of Aeronautics and Astronautics) Ministry of Industry and Information TechnologyNanjing 211100China

Achieving synergistic absorption of electromagnetic waves(EMWs)in the mid-high frequency and absorption band conversion is an urgent ***,the present solution is usually a straightforward mixture of magnetic component-carbon ***,we optimize the magnetic properties and electrical relaxation response from a chemical synthesis *** integrated design,the contents of carbon components and multi-dimensional morphology are controlled by retaining strong magnetic *** morphology design and the construction of heterogeneous interfaces will boost the intense response of charge in the surrounding to enhance the polarization *** multi-dimensional structure and electromagnetic(EM)properties of the sample after optimized engineering have an extremely powerful absorption conversion effect on EMW ***@C particles ultimately achieve synergistic absorption effects at low thickness(dhigh frequencies(10.5–18 GHz).Our work establishes a correlation mechanism between the physical and chemical properties of materials and EM *** also provides insight into the synergistic absorption of EMWs in the mid-high frequency and absorption band conversion strategies.

关键词： micro-nano composites NiCo@C hollow structure mid-high frequency absorption

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Multi-functional and multi-scenario applications for MXene aerogels with synergistically enhanced asymmetric modules

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Nano Research 2024年第4期17卷 3359-3368页

作者： Junru Yao Jintang Zhou Feng Yang Guiyu Peng Yijie Liu Zhengjun Yao Fan Wu Haibo Zeng College of Materials science and technology Nanjing University of Aeronautics and AstronauticsNanjing 211100China key laboratory of Material Preparation and protection for Harsh environment(Nanjing University of Aeronautics and Astronautics) Ministry of Industry and Information TechnologyNanjing 211100China School of Mechanical Engineering Nanjing University of Science and TechnologyNanjing 210094China

The development of multifunctional materials and synergistic applications of various functions are important conditions for integrated and miniaturized ***,we developed asymmetric MXene/aramid nanofibers/polyimides(AMAP)aerogels with different modules using an integrated molding *** asymmetric modules(layered MXene/aramid nanofibers section and porous MXene/aramid nanofibers/polyimides section)interactions are beneficial for enhanced performances,resulting in low reflection electromagnetic interference(EMI)shielding(specific shielding effectiveness of 2483(dB·cm^(3))/g and a low R-value of 0.0138),high-efficiency infrared radiation(IR)stealth(ultra-low thermal conductivity of 0.045 W/(m·K)and IR emissivity of 0.32 at 3–5μm and 0.28 at 8–14μm),and excellent thermal management performances of insulated Joule ***,these multifunctional AMAP aerogels are suitable for various application scenarios such as personal and building protection against electromagnetic pollution and cold,as well as military equipment protection against infrared detection and EMI.

关键词： multifunctional material electromagnetic interference shielding low reflection infrared radiation stealth thermal insulation Joule heating

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high-precision modeling of tide-induced 3-D magnetic field and analysis of geomagnetic satellite orbit requirements

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science China Earth sciences 2024年第1期67卷 165-178页

作者： Zhengyong REN Cong YANG Hongbo YAO Xu TANG Jingtian TANG Keke ZHANG key laboratory of Metallogenic Prediction of Nonferrous Metals and Geological environment Monitoring Ministry of Education Central South UniversityChangsha 410083China Hunan key laboratory of Nonferrous Resources and Geological Hazards Exploration Changsha 410083China School of Geosciences and Info-Physics Central South UniversityChangsha 410083China State key laboratory of Lunar and Planetary sciences Macao University of Science and TechnologyMacao 999078China

Ground-based magnetic observatories and geomagnetic satellites can observe the induced magnetic field generated by the motion of seawater containing sodium and chlorine *** the three-dimensional(3-D)spatial distribution of tide-induced magnetic fields(TIMF)is crucial for inverting the electrical conductivity structure of the oceanic *** also serves as an essential basis for designing optimal geomagnetic observatories and satellite ***,existing methods for simulating TIMF suffer from limitations in inaccurately modeling realistic coastlines,heterogeneous land and sea surface properties,and complex deep Earth structures,thereby the interpretational level of TIMF data is *** overcome this issue,we developed a tetrahedral-based finite element method for simulating TIMF,which can efficiently approximate realistic coastlines,heterogeneous land and sea surface properties,and complex deep Earth ***,we derived the boundary value problem for the seawater motion-induced electromagnetic field,which was solved using the vector finite element method based on tetrahedral ***,using the latest ocean depth and seafloor sediment layer models,we constructed a 3-D conductivity model of the Earth,which includes realistic coastlines,heterogeneous land and sea conductivity *** then computed the TIMF using the M_(2)tidal source as an example and validated our method by comparing it with results obtained from spherical harmonic finite element and integral equation ***,utilizing the computed high-precision M_(2),N_(2),and O1 TIMF signals,we marked global observatories capable of observing strong M_(2),N_(2),and O1 TIMF signals and predicted alternative stations suitable for tide signal ***,we calculated TIMF at heights of 450 and 200 km for the Macao science Satellite 1 and its subsequent *** results indicate that the amplitude of the tidal-induced magnetic field at

关键词： Ocean motional induction electromagnetic induction Ocean tides Geomagnetic satellite Macao science Satellite 1

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Heterogeneous MXene-based films with graded electrical conductivity towards highly efficient EMI shielding and electrothermal heating

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Nano Research 2024年第8期17卷 7264-7274页

作者： Yu Zhang Guangcheng Zhang Zhonglei Ma Jianbin Qin Xi Shen Department of Aeronautical and aviation Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Shaanxi key laboratory of Macromolecular science and technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Research Institute for Sports science and technology The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina

The increasing need for electromagnetic interference(EMI)shielding of electronics in cold environments such as those in aircraft,space exploration,and wearable heaters to avoid hazardous icing conditions or hypothermia requires the development of thin and lightweight EMI shielding materials preferably by absorbing rather than reflecting electromagnetic(EM)waves while also generating heat through energy-efficient electrothermal ***,it is challenging to achieve absorption-dominant EMI shielding and energy-efficient electrothermal heating simultaneously in a thin and lightweight ***,we develop a heterogeneous composite film comprising a porous multi-walled carbon nanotubes(MWCNTs)/bacterial cellulose(BC)film and an aligned MXene/Ag nanowires(NWs)backing via a sequential vacuum filtration *** porous film contains random conductive networks of MWCNTs with moderate conductivity while the aligned MXene sheets atop Ag NWs network affords high conductivity in the backing,giving rise to graded electrical conductivity for absorption-dominant EMI *** increasing Ag NW coverage leads to significantly increased electrical conductivity without increasing the EM wave reflection as well as the density and thickness of the film,yielding excellent specific EMI shielding effectiveness(>8500 dB/(g·cm^(2))),low driving voltage for energy-efficient electrothermal heating(163℃at 2.5 V),and fast response time(60 s)at a low areal density of 0.015 mg/cm^(2).Combining EMI shielding and electrothermal heating,the heterogeneous film developed here are promising contenders for the protection of electronic equipment in low-temperature environment.

关键词： heterogenous composite film MXene electromagnetic interference(EMI)shielding thermal management

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Fabricating bio-inspired high impact resistance carbon nanotube network films for multi-protection under an extreme environment

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Nano Research 2024年第9期17卷 7793-7802页

作者： Mingquan Zhu Kailu Xiao Wei Zhang Xudong Lei Yunxiang Bai Shijun Wang Peng Zhang Feng Gao Congying Wang Wenqiang Xu Huiyong Li Xianqian Wu Chao Wang Hui Zhang Luqi Liu Zhong Zhang CAS key laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China University of Chinese Academy of sciences Beijing 100049China Department of Materials science and Engineering Texas A&M UniversityCollege StationTexas 77840USA Institute of Mechanics Chinese Academy of SciencesBeijing 100190China School of Astronautics Harbin Institute of TechnologyHarbin150001China CAS key laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230027China

The fabrication of light-weight,highly impact-resistant,and energy-absorbent materials is urgently demanded in many facets of the society from body armor to aerospace engineering,especially under an extreme *** nanotubes(CNTs),one of the strongest and toughest materials ever found,also have good conductivity,chemical stability,and thermal stability,etc,making them a competitive candidate as building blocks to help achieve the above *** this work,a kind of CNT network was prepared by using chlorosulfonic acid(CSA)to release the internal stress of super-aligned carbon nanotube films(SA-CNTF)and dendritic polyamide amine(PAMAM)to further introduce multiple hydrogen bonds and interlocking *** fabricated bioinspired carbon nanotube network films(PAMAM@C-CNTF)have a high toughness of 45.97 MJ/m3,showing an increase of 420%compared to neat *** importantly,the anti-impact performance of the films(e.g.,with a maximum specific energy absorption of 1.40 MJ/kg under 80-100 m/s projectile impact)is superior to that of conventional protective materials from steel and Kevlar fiber,and also exceeds that of any other reported carbon-based *** hierarchical energy dissipation mechanism was further revealed through experiment and *** functions including intelligent heating/anti-icing,ultraviolet protection,as well as electromagnetic interference shielding properties make these network films have great potential in practical multi-protection applications,especially under an extreme environment.

关键词： carbon nanotubes composites mechanical properties multi-function

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MXene@c-MWCNT Adhesive Silica Nanofiber Membranes Enhancing electromagnetic Interference Shielding and Thermal Insulation Performance in Extreme environments

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Nano-Micro Letters 2024年第10期16卷 82-98页

作者： Ziyuan Han Yutao Niu Xuetao Shi Duo Pan Hu Liu Hua Qiu Weihua Chen Ben Bin Xu Zeinhom MEl-Bahy Hua Hou Eman Ramadan Elsharkawy Mohammed AAmin Chuntai Liu Zhanhu Guo key laboratory of Materials Processing and Mold(Zhengzhou University) Ministry of EducationNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002People's Republic of China School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026People's Republic of China key laboratory of Multifunctional Nanomaterials and Smart Systems Advanced Materials DivisionSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123People's Republic of China Shaanxi key laboratory of Macromolecular science and technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi'an 710072People's Republic of China College of Chemistry&Green Catalysis Center Zhengzhou UniversityZhengzhou 450001People's Republic of China Mechanical and Construction Engineering Faculty of Engineering and EnvironmentNorthumbria UniversityNewcastle Upon Tyne NE18UK Department of Chemistry Faculty of ScienceAl-Azhar UniversityNasr City 11884CairoEgypt Department of Chemistry Faculty of ScienceNorthern Border UniversityArarSaudi Arabia Department of Chemistry College of ScienceTaif UniversityP.O.Box 1109921944 TaifSaudi Arabia

A lightweight flexible thermally stable composite is fabricated by com-bining silica nanofiber membranes(SNM)with MXene@c-MWCNT hybrid *** flexible SNM with outstanding thermal insulation are prepared from tetraethyl orthosilicate hydrolysis and condensation by electrospinning and high-temperature calcination;the MXene@c-MWCNT_(x:y)films are prepared by vacuum filtration *** particular,the SNM and MXene@c-MWCNT_(6:4)as one unit layer(SMC_(1))are bonded together with 5 wt%polyvinyl alcohol(PVA)solution,which exhibits low thermal conductivity(0.066 W m^(-1)K^(-1))and good electromagnetic interference(EMI)shielding performance(average EMI SE_(T),37.8 dB).With the increase in func-tional unit layer,the overall thermal insulation performance of the whole composite film(SMC_(x))remains stable,and EMI shielding performance is greatly improved,especially for SMC_(3)with three unit layers,the average EMI SET is as high as 55.4 *** addition,the organic combination of rigid SNM and tough MXene@c-MWCNT_(6:4)makes SMC_(x)exhibit good mechanical tensile ***,SMC_(x)exhibit stable EMI shielding and excellent thermal insulation even in extreme heat and cold ***,this work provides a novel design idea and important reference value for EMI shielding and thermal insulation components used in extreme environmental protection equipment in the future.

关键词： SiO_(2)nanofiber membranes MXene@c-MWCNT Composite film Thermal insulation electromagnetic interference shielding

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Design of the high voltage isolation transmission module with low delay for ECRH system on J-TEXT

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Plasma science and technology 2018年第2期20卷 19-25页

作者：马海燕夏冬辉王之江崔芳泰余振雄金易坤刘昌海 State key laboratory of Advanced electromagnetic Engineering and technology Huazhong University of Science and Technology

As a flexible auxiliary heating method,the electron cyclotron resonance heating（ECRH） has been widely used in many tokamaks and also will be applied for the J-TEXT *** meet requirements of protection and fault analysis for the ECRH system on J-TEXT,signals of gyrotrons such as the cathode voltage and current,the anode voltage and current,etc should be transmitted to the control and data acquisition *** the high voltage environment of gyrotrons,isolation transmission module based on FPGA and optical fiber communication has been designed and *** test results indicate that the designed module has strong anti-noise ability,low error rate and high transmission *** delay of the module is no more than 5 μs which can fulfill the requirements.

关键词： J-TEXT tokamak electron cyclotron resonance heating high-voltage isolation

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Controllable and tunable plasma photonic crystals through a combination of photonic crystal and dielectric barrier discharge patterns

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Plasma science and technology 2023年第8期25卷 74-86页

作者：郭丽婷潘宇扬于广林王朝阳高匡雅范伟丽董丽芳 Department of Electrical Engineering Shanghai Jiao Tong UniversityShanghai 200240People's Republic of China aviation key laboratory of science and technology on high intensity electromagnetic environment protection Anhui Province Key Laboratory of Aircraft Lightning ProtectionHefei 230031People's Republic of China

We report five types of patterns with square symmetry,including three novel types obtained by inserting a specially designed grid photonic crystal(PC)into a dielectric barrier discharge *** are studied using an intensified charge-coupled device camera and photomultiplier *** three novel types of patterns are a square pattern with one structure,a square superlattice pattern with four sublattices and a(1/4)K_(grid)(K_(grid)is the basic wave vector of the grid),and another square pattern with a complex inversion discharge *** the application viewpoint,the five types of patterns can be used as plasma photonic crystals(PPCs).Their band diagrams under a transverse-magnetic wave simulated by the finite element method show that there are a large number of band *** with the original PC with only a unidirectional band gap,the five types of PPCs have tunable and omnidirectional band gaps,which is very important in controlling the propagation of electromagnetic waves in the mm-wave *** experimental results enrich the pattern types in the dielectric barrier discharge system and provide a method for obtaining PPCs with symmetry controllability and bandgap tunability.

关键词： dielectric barrier discharge plasma photonic crystal patterns electromagnetic waves

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Simulation analysis on microscopic discharge characteristics of the bipolar corona of a floating conductor

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Plasma science and technology 2023年第8期25卷 54-73页

作者：杨冬阳陈坚段泽民肖登明金之俭 Department of Electrical Engineering Shanghai Jiao Tong UniversityShanghai 200240People's Republic of China aviation key laboratory of science and technology on high intensity electromagnetic environment protection Anhui Province Key Laboratory of Aircraft Lightning ProtectionHefei 230031People's Republic of China

A floating conductor exhibits a bipolar corona phenomenon with microscopic discharge characteristics that are still *** this study,a plasma simulation model of the bipolar corona with 108 chemical reaction equations is established by combining hydrodynamics and plasma chemical *** evolution characteristics of electrons,positive ions,negative ions and neutral particles,as well as the distribution characteristics of space charges are analyzed,and the evolutionary flow of microscopic particles is *** results indicate that the positive end of the bipolar corona initiates discharge before the negative end,but the plasma chemistry at the negative end is more *** electron generation rate can reach 1240 mol(m^(3) s)^(-1),and the dissipation rate can reach 34 mol(m^(3) s)^(-1).The positive ion swarm is dominated by O_(4)^(+),and the maximum generation rate can reach 440 mol((m^(3) s)^(-1).The negative ion swarm is mainly O_(2) and O_(4).The O_(2) content is approximately 1.5-3 times that of O_(4),and the maximum reaction rate can reach 51 mol(m^(3) s)^(-1).The final destination of neutral particles is an accumulation in the form of O_(3) and NO,and the amount of O3 produced is approximately 4-6 times that of *** positive end of the bipolar corona is dominated by positive space charges,which continue to develop and spread outwards in the form of a pulse *** negative end exhibits a space charge distribution structure of concentrated positive charges and diffused negative *** validity of the microscopic simulation analysis is verified by the macroscopic discharge phenomenon.

关键词： bipolar corona evolution process floating conductor microscopic discharge characteristics space charge distribution

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