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High-energy-density lithium manganese iron phosphate for lithium-ion batteries: Progresses, challenges, and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang Yan Li Libo Chen Handong Jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing Research Institute for Intelligent Wearable Systems The Hong Kong Polytechnic University Institute of Advanced Structure Technology Beijing Institute of Technology

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate (LiMnxFe1-xPO4) has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** LiMnxFe1-xPO4has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and Li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of LiMnxFe1-xPO4to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of LiMnxFe1-xPO4,including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable LiMnxFe1-xPO4materials,to achieve practical energy storage requirements.

关键词： Lithium manganese iron phosphate High energy density Lithium-ion batteries Reaction mechanism Tap density

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Effect of AlN coating on hydrogen permeability and surface structure of VT6 alloy by vacuum arc ion plating

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Chinese Physics B 2019年第10期28卷 546-549页

作者： Zi-Yi Ding national Research Tomsk polytechnic university

We study the absorption of hydrogen of metal by the permeability method. With the help of the gas reaction controller(GRC), the absorptive capacity of hydrogen, which is a function of time, temperature and pressure, can be recorded. The effect of the performance of the hydrogen permeability of AlN coating on the titanium alloy surface structure is *** the research, the AlN is selected to be added to the titanium alloy sample VT6, and the properties of the titanium alloy are investigated, and the hydrogen absorption rate of the coating is calculated by performing the hydrogen saturation of the test sample. The results show that under 600℃ the AlN film reduces the hydrogen absorption rate of titanium alloy and improves the surface properties of VT6 alloy.

关键词： titanium alloy ion plating aluminum nitride hydrogen

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Catalyst–Support Interaction in Polyaniline‑Supported Ni_(3)Fe Oxide to Boost Oxygen Evolution Activities for Rechargeable Zn‑Air Batteries

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Nano-Micro Letters 2025年第1期17卷 176-190页

作者： Xiaohong Zou Qian Lu Mingcong Tang Jie Wu Kouer Zhang Wenzhi Li Yunxia Hu Xiaomin Xu Xiao Zhang Zongping Shao Liang An Department of Mechanical Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and TechnologyNanjing University of Information Science and TechnologyNanjing 210044People’s Republic of China Department of Chemistry The Chinese University of Hong KongMa Lin BuildingShatinHong Kong SAR 999077People’s Republic of China WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia Research Institute for Advanced Manufacturing The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China

Catalyst–support interaction plays a crucial role in improving the catalytic activity of oxygen evolution reaction(OER).Here we modulate the catalyst–support interaction in polyaniline-supported Ni_(3)Fe oxide(Ni_(3)Fe oxide/PANI)with a robust hetero-interface,which significantly improves oxygen evolution activities with an overpotential of 270 mV at 10 mA cm^(-2)and specific activity of 2.08 mA cm_(ECSA)^(-2)at overpotential of 300 mV,3.84-fold that of Ni_(3)Fe *** is revealed that the catalyst–support interaction between Ni_(3)Fe oxide and PANI support enhances the Ni–O covalency via the interfacial Ni–N bond,thus promoting the charge and mass transfer on Ni_(3)Fe *** the excellent activity and stability,rechargeable Zn-air batteries with optimum Ni_(3)Fe oxide/PANI are assembled,delivering a low charge voltage of 1.95 V to cycle for 400 h at 10 mA cm^(-2).The regulation of the effect of catalyst–support interaction on catalytic activity provides new possibilities for the future design of highly efficient OER catalysts.

关键词： Catalyst-support interaction Supported catalysts Heterointerface Oxygen evolution reaction Zn-air batteries

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Determining absolute value of thermal neutron flux density based on monocrystalline silicon in nuclear reactors

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Nuclear Science and Techniques 2022年第7期33卷 133-138页

作者： V.A.Varlachev E.G.Emets Yu-Chen Mu E.A.Bondarenko V.A.Govorukhin national Research Tomsk polytechnic university Tomsk634050Russia

A new type of neutron detector based on monocrystalline Si is developed to measure the fluence and flux density of thermal and fast *** principle of this detector is based on the relationship between changes in electrical conductivity and neutron fluence during ***,the absolute values of thermal neutron fluence and flux density are measured in a facile manner with high *** with activation methods,our method not only possesses a similar accuracy,but also demonstrates superior application potential for the investigation of neutron fields in nuclear reactors owing to its suitable half-life.

关键词： Thermal neutron Neutron detector Neutron flux density Cadmium difference methods

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Effect of the high-power electromagnetic pulses on the reactivity of the coal-water slurry in hot environment

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Chinese Journal of Chemical Engineering 2020年第12期28卷 3145-3151页

作者： M.V.Belonogov R.I.Taburchinov R.I.Egorov national Research Tomsk polytechnic university TomskRussian Federation

An effect of the high-power electromagnetic pulses onto the droplet of coal-water slurry inside the furnace was *** contrary to the previously investigated laser-induced fuel atomization that occurs at the room temperature,the pre-heated(to 400 K)slurry becomes dry enough to prevent the explosion-like steam ***,fuel does not atomize and the ignition does not ***,the absorption of several laser pulses leads to evident sintering of irradiated surface with following increase of the ignition delay time for up to 24%.Variation of the pulse energy in range 48-118 mJ(corresponding intensity up to 2.4 J·cm^-2)leads to certain variation of the increase of ignition *** strong pulsed overheating of the coal water slurry which does not initiate the fine atomization of the fuel generally makes its ignition longer.

关键词： Waste-derived fuels Coal-water slurry Auto-ignition Ignition delay time High-power laser pulse

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Active control of friction by transverse oscillations

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Friction 2019年第1期7卷 74-85页

作者： J.BENAD K.NAKANO V.L.POPOV M.POPOV Technische Universit?t Berlin Yokohama national university national Research Tomsk polytechnic university national Research Tomsk State university

The present paper is devoted to a theoretical analysis of sliding friction under the influence of in-plane oscillations perpendicular to the sliding direction. Contrary to previous studies of this mode of active control of friction, we consider the influence of the stiffness of the tribological contact in detail and show that the contact stiffness plays a central role for small oscillation amplitudes. In the present paper we consider the case of a displacement-controlled system, where the contact stiffness is small compared to the stiffness of the measuring system. It is shown that in this case the macroscopic coefficient of friction is a function of two dimensionless parameters— a dimensionless sliding velocity and dimensionless oscillation amplitude. In the limit of very large oscillation amplitudes, known solutions previously reported in the literature are reproduced. The region of small amplitudes is described for the first time in this paper.

关键词： sliding friction in-plane oscillation contact stiffness coefficient of friction active control of friction

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Synthesis of large diamond crystals containing high-nitrogen concentration at high pressure and high temperature using Ni-based solvent by temperature gradient method

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Chinese Physics B 2010年第11期19卷 662-666页

作者：黄国锋贾晓鹏李尚升张亚飞李勇赵明马红安 national Lab of Superhard Materials Jilin University Henan polytechnic university

This paper reprots that with Ni-based catalyst/solvent and with a dopant of NAN3, large green single crystal diamonds with perfect shape are successfully synthesized by temperature gradient method under high pressure and high temperature in a China-type cubic anvil high-pressure apparatus （SPD-6 × 1200）, and the highest nitrogen concentration reaches approximately 121-1257 ppm calculated by infrared absorption spectra. The synthesis conditions are about 5.5 CPa and 1240-1300 ℃. The growth behaviour of diamond with high-nitrogen concentration is investigated in detail. The results show that, with increasing the content of NaN3 added in synthesis system, the width of synthesis temperature region for growth high-quality diamonds becomes narrower, and the morphology of diamond crystal is changed from cube-octahedral to octahedral at same temperature and pressure, the crystal growth rate is slowed down, nevertheless, the nitrogen concentration doped in synthetic diamond increases.

关键词： high temperature and high pressure nitrogen-doped diamond crystal temperature gra- dient method additive NaN3

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Influence of beam current on microstructure of electron beam melted Ti-6Al-4V alloy

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Progress in Natural Science:Materials International 2019年第4期29卷 440-446页

作者： Roman Laptev Natalia Pushilina Egor Kashkarov Maxim Syrtanov Ekaterina Stepanova Andrey Koptyug Andrey Lider national Research Tomsk polytechnic university Mid Sweden university

The defect microstructure of the samples manufactured from Ti-6A1-4V powder was studied using electron beam melting(EBM) in the beam current range of 17-13 *** hybrid digital complex combined positron lifetime spectroscopy and coincidence Doppler broadening spectroscopy was used to characterize the defect structure of the *** microstructure and defects were also analyzed by transmission electron *** has been established that the main type of the defects in the EBM manufactured samples is *** to the conducted measurements and calculations,the dislocation density in the EBM manufactured samples exceeds by two orders the similar value for the cast Ti-6Al-4 *** of Ti-Ti-Al nanoscale clusters has been found in the EBM manufactured samples.

关键词： Titanium alloy Additive technology Electron beam melting Positron spectroscopy Defects Transmission electron microscopy

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Analysis of recent Antarctic plate kinematics based on GNSS data

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Geodesy and Geodynamics 2023年第2期14卷 99-110页

作者： Ihor Savchyn Ivan Brusak Korneliy Tretyak Lviv polytechnic national university Institute of GeodesyUkraine

The research aims to study recent Antarctic plate kinematics based on Global Navigation Satellite System(GNSS)*** research covers 60 continuous GNSS stations located on the Antarctic plate during *** determine the components of horizontal displacement vectors of these GNSS stations and construct the schematic map of their *** results indicate that the direction of velocity vectors of horizontal displacements has a rotational nature in clockwise *** analysis of deformation processes shows that a gradual decrease in the horizontal strain rates,maximum shear strain and area strain is taking place from west to east,in the direction of West Antarctica-the Transantarctic Mountains-East *** absolute rotation pole of the Antarctic plate in the ITRF2014/IGS14 reference frame has been determined,and the obtained values are in good agreement with recent plate models.

关键词： Continuous GNSS station Horizontal velocity Strain rates Rotation pole The Antarctic plate

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Spontaneous Orientation Polarization of Anisotropic Equivalent Dipoles Harnessed by Entropy Engineering for Ultra‑Thin Electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： Honghan Wang Xinyu Xiao Shangru Zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao Che Junye Cheng Liaoning Key Lab of Lignocellulose Chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of Life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China Department of Mechanical Engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and Engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HEAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HEAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HEAs and construction of emblematic shell-core CCF/HEAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HEAs composite prepared by 35%molar ratio of Mn element(CCP/HEAs-Mn_(2.15))achieves efficient electromagnetic wave(EMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HEAs-based EMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes Emblematic shell-core heterointerfaces Ultra-thin thickness

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