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Exploring one material for dual applications:A red-emitting mg2GeO4:Eu3+ nanophosphor for future generation energy efficient WLEDs and dosimetric applications

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Journal of Rare Earths 2024年第10期42卷 1835-1845页

作者： Akshay Arjun G.P.Darshan s.C.sharma H.Nagabhushana D.V.sunitha H.B.Premkumar department of physics Faculty of Mathematical and Physical SciencesM.S.Ramaiah University of Applied Sciences Jain university C.N.R.Rao Centre for Advanced materials Tumkur University school of applied sciences (physics) REVA University

The envisaged design and developme nt of individual mate rials to excavate a broader spectrum of desired properties and offer multiple applications are highly *** this in mind,a series of forsterite-structured mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was synthesized via a solution combustion method using oxalyl dihydrazide as a *** X-ray diffraction patterns confirm the orthorhombic crystal system with a Puma space *** results clearly show irregularly shaped cluster-like structures with aggregation of the *** diffuse reflectance spectra,the optical energy band gap of the mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was estimated and obtained to be～4.12-4.32 *** photoluminescence emission spectra exhibit intense peaks at ～579,589,610,661,and 707 nm,which are due to characteristic5D0→7F0,5D0→7F1,5Do→7F2,5D0→7F3and5D0→7F4transitions of Eu3+ions,*** Commission International de L'Eclairage color coordinates are gradually tuned from pale red（0.5980,0.4012） to a pure red（0.6385,0.3611） *** glow peaks showcase excellent super-linear response at low doses of γ-irradiations,indicating that the prepared phosphor can be used in thermoluminescent personal dosimetry which is a biological tissue *** aforementioned results demonstrate that the prepared mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors are considered an excellent candidate for dual applications,i.e.,red component in future generation white-light-emitting diodes（WLEDs） and personal dosimetric applications.

关键词： Dosimetry Nanophosphors Photoluminescence Photometric properties Rare earths Thermoluminescence

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Optoelectronic and thermoelectric properties of spinel chalcogenides HgLa2X4（X=s and se）:A first-principles study

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Journal of Rare Earths 2024年第10期42卷 1927-1936页

作者： Aparna Dixit Inas A.Ahmed Jisha Annie Abraham Zeinhom m.El-Bahy mumtaz manzoor sajad Ahmad Dar Ramesh sharma department of Basic science and Humanities Pranveer Singh Institute of Technology department of Chemistry Faculty of ScienceKing Khalid University department of physics National Defence Academy department of Chemistry Faculty of ScienceAl-Azhar University Institute of physics Slovak Academy of Sciences department of physics Motilal Vigyan Mahavidyalya College department of applied science Feroze Gandhi Institute of Engineering and Technology

We investigated spinel chalcogenides HgLa2（s/se）4by using density function theory,and scrutinized the structural,optical,electrical,mechanical and thermoelectric transport characteristics of HgLa2（s/se）4spinel *** enthalpy of formation,energy of cohesion,and energy volume optimum plots were used to obtain the stability as well as the perfect ground state of these *** ductility of these materials was the best illustrated with the help of Poisson's and Pugh's *** band gap results were obtained using Trans and Blaha modified Becke-Johanson potential（TB-mBJ）.Both the materials present semi-conducting nature with direct band gap equal to 1.449 and 0.892 eV respectively for HgLa2s4and *** were also made for optical characteristics with the values of dielectric function,absorption coefficient,optical conductivity,reflectivity,and refractive *** to the findings,both of these materials are suitable for infrared optoelectronic *** materials were found to have promising optoelectronic and thermoelectric applications after their optical properties and transport aspects were *** tiny levels of temperature conductivities,substantial am ounts of power conductivities,the figure of merit（more than unity）,as well as seebecs coefficients all point to the potential use of both the materials in thermoelectric power generators.

关键词： Density functional theory Direct band gap Optoelectronic Power factor semiconductors Thermoelectric

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Enhancing the Performance of Perovskite Light-Emitting Diodes via synergistic Effect of Defect Passivation and Dielectric screening

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Nano-micro Letters 2024年第10期16卷 244-256页

作者： Xuanchi Yu Jia Guo Yulin mao Chengwei shan Fengshou Tian Bingheng meng Zhaojin Wang Tianqi Zhang Aung Ko Ko Kyaw shuming Chen Xiaowei sun Kai Wang Rui Chen Guichuan Xing Institute of applied physics and materials engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078People's Republic of China department of Electrical and Electronic engineering Southern University of Science and TechnologyShenzhen 518055People's Republic of China

metal halide perovskites,particularly the quasi-two-dimensional perovskite subclass,have exhibited considerable potential for next-generation electroluminescent materials for lighting and ***,the presence of defects within these perovskites has a substantial influence on the emission efficiency and durability of the *** this study,we revealed a synergistic passivation mechanism on perovskite films by using a dual-functional compound of potassium *** dual functional potassium bromide on the one hand can passivate the defects of halide vacancies with bromine anions and,on the other hand,can screen the charged defects at the grain boundaries with potassium *** approach effectively reduces the probability of carriers quenching resulting from charged defects capture and consequently enhances the radiative recombination efficiency of perovskite thin films,leading to a significant enhancement of photoluminescence quantum yield to near-unity values(95%).meanwhile,the potassium bromide treatment promoted the growth of homogeneous and smooth film,facilitating the charge carrier injection in the ***,the perovskite light-emitting diodes based on this strategy achieve a maximum external quantum efficiency of~21%and maximum luminance of~60,000 cd m^(-2).This work provides a deeper insight into the passivation mechanism of ionic compound additives in perovskite with the solution method.

关键词： synergistic passivation strategy Defects passivation Dielectric screening Perovskite light-emitting diodes

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Electrochemical performance of a symmetric supercapacitor device designed using laser-induced multilayered graphene

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新型炭材料(中英文) 2024年

作者： Gargi Dhiman Kavita Kumari Bon-Heun Koo Faheem Ahmed Nagih m.shaalan saurabh Dalela Parvez A.Alvi Ranjeet Kumar Brajpuriya shalendra Kumar department of physics School of Advanced EngineeringUPES Industrial technology Research Institute Changwon National University Changwon department of applied sciences and Humanities Faculty of Engineering and Technology Jamia Millia Islamia department of physics College of Science King Faisal University physics department Faculty of Science Assiut University department of Pure & applied physics University of Kota department of Physical science

This study demonstrates a facile and economical approach for fabricating laser-induced graphene（LIG）, which results in improved electrochemical performance. Polyimide polymer was used as a starting material for LIG synthesis and irradiated under ambient conditions using a CO2laser. The prepared LIG samples were characterized by Raman spectroscopy and FTIR, which validated the formation of multilayered graphene containing sp2 hybridized C=C bonds. The FE-sEm revealed three-dimensional sheetlike structures, while HR-TEm images displayed lattice planes with an interplanar spacing of approximately 0.33 nm, corresponding to the（002） plane of graphene. The electrochemical performance of the as-prepared LIG samples demonstrated a remarkable areal specific capacitance（CA） of 51 mF cm-2(170 F g-1) at 1 mA cm-2(3.3 A g-1) in a three-electrode configuration with 1m KOH as the aqueous electrolyte. The LIG electrodes produced an energy density of ～3.5 μWh cm-2and a power density of ～350 μW cm-2,demonstrating significant energy storage capabilities. Additionally, the electrodes exhibited excellent cyclic stability, retaining 87%of their specific capacitance after 3 000 cycles at 1 mA/cm2. The symmetric supercapacitor fabricated with LIG electrodes and the tested 1m KOH electrolyte showed a specific capacitance of 23 mF cm-2and maintained excellent retention after 10,000 cycles,showing LIG's potential for supercapacitor applications.

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mixed convectional and chemical reactive flow of nanofluid with slanted mHD on moving permeable stretching/shrinking sheet through nonlinear radiation,energy omission

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Chinese physics B 2024年第5期33卷 193-202页

作者： saleem Nasir sekson sirisubtawee Pongpol Juntharee Taza Gul department of mathematics Faculty of Applied ScienceKing Mongkut's University of Technology North BangkokBangkok 10800Thailand department of mathematics City University of Science and Information TechnologyPeshawarPakistan

Hybrid nanofluids are remarkable functioning liquids that are intended to reduce the energy loss while maximizing the heat *** the involvement of suction and nonlinear thermal radiation effects,this study attempted to explore the energy transmission features of the inclined magnetohydrodynamic(mHD)stagnation flow of CNTs-hybrid nanofluid across the nonlinear permeable stretching or shrinking *** work also included some noteworthy features like chemical reactions,variable molecular diffusivity,quadratic convection,viscous dissipation,velocity slip and heat omission *** appropriate similarity components,the model equations were modified to ODEs and computed by using the HAm *** impact of various relevant flow characteristics on movement,heat and concentration profiles was investigated and plotted on a *** various model factors,the significance of drag friction,heat and mass transfer rate were also computed in tabular and graphical *** leads to the conclusion that such factors have a considerable impact on the dynamics of fluid as well as other engineering measurements of ***,viscous forces are dominated by increasing the values ofλ_(p),δ_(m)andδ_(q),and as a result,F(ξ)accelerates while the opposite trend is observed for m andφ.The drag friction is boosted by the augmentation m,λ_(p)andφ,but the rate of heat transfer *** to our findings,hybrid nanoliquid effects dominate that of ordinary nanofluid in terms of F(ξ),Θ(ξ)andφ(ξ)*** HAm and the numerical technique(shooting method)were found to be in good agreement.

关键词： hybrid nanofluid(sWCNT+mWCNT/H_(2)O) velocity slip conditions nonlinear thermal radiation exponential stretching/shrinking sheet inclined magnetohydrodynamic(mHD)stagnation flow

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Analysis of application range of simplified models for field to thermo-field to thermionic emission processes from the cathode

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Plasma science and technology 2024年第9期26卷 51-60页

作者： Li sUN Zhuo DAI ming XU Wei WANG Zengyao LI applied physics department Xi’an University of TechnologyXi’an 710048People’s Republic of China Key Laboratory of Thermo-Fluid science and engineering Ministry of EducationSchool of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049People’s Republic of China

Electron emission plays a dominant role in plasma-cathode interactions and is a key factor in many plasma phenomena and industrial *** is necessary to illustrate the various electron emission mechanisms and the corresponding applicable description models to evaluate their impacts on discharge *** this study,detailed expressions of the simplified formulas valid for field emission to thermo-field emission to thermionic emission typically used in the numerical simulation are proposed,and the corresponding application ranges are determined in the framework of the murphy-Good theory,which is commonly regarded as the general model and to be accurate in the full range of conditions of the validity of the *** parameterization was used to evaluate the emission current density of the murphy-Good formula,and a deviation factor was defined to obtain the application ranges for different work functions(2.5‒5 eV),cathode temperatures(300‒6000 K),and emitted electric fields(10^(5) to 10^(10) V·m^(-1)).The deviation factor was shown to be a nonmonotonic function of the three parameters.A comparative study of particle number densities in atmospheric gas discharge with a tungsten cathode was performed based on the one-dimensional implicit particle-in-cell(PIC)with the monte Carlo collision(mCC)method according to the aforementioned application *** was found that small differences in emission current density can lead to variations in the distributions of particle number density due to changes in the collisional *** study provides a theoretical basis for selecting emission models for subsequent numerical simulations.

关键词： electron emission processes application range murphy-Good theory implicit particlein-cell monte Carlo collision method

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Bridging the Fabry–Perot cavity and asymmetric Berreman mode for long-wave infrared nonreciprocal thermal emitters

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science China Technological sciences 2024年第10期67卷 3285-3293页

作者： CHEN ZiHe YU shiLv HU Run school of Energy and Power engineering Huazhong University of Science and Technology Wuhan National Laboratory for Optoelectronics Huazhong University of Science and Technology department of applied physics Kyung Hee University

The long-wave infrared band(8–14 μm) is essential for several applications, such as infrared detection, radiative cooling, and near-field heat transfer. However, according to Kirchhoff's law, the intrinsic balance between thermal absorption and emission limits the further improvement of photon energy conversion and thermal management. Thus, breaking Kirchhoff's balance and achieving nonreciprocal thermal radiation in the long-wave infrared band are necessary. most existing designs for nonreciprocal thermal emitters rely on grating or photonic crystal structures to achieve nonreciprocal thermal radiation at narrow peaks, which are relatively complex and typically realize bands larger than 14 μm. Here, a sandwich structure consisting of an epsilon-nearzero(ENZ) magneto-optical layer(mOL), a dielectric layer(DL), and a metal layer is proposed to achieve a strong nonreciprocal effect in the long-wave infrared band, which is mainly attributed to the strengthening of the asymmetric Berreman mode by the Fabry–Perot cavity. In addition, the impact of the incident angle, DL thickness, and DL refractive index on the nonreciprocal thermal radiation has been investigated. moreover, by replacing the ENZ mOL with the gradient ENZ mOL, the existence of the DL can further improve the nonreciprocity of the broadband nonreciprocal thermal radiation. The proposed work promotes the development and application of nonreciprocal energy devices.

关键词： long-wave infrared band nonreciprocal thermal radiation sandwich structure Fabry–Perot cavity asymmetric berreman mode

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Emerging direct current triboelectric nanogenerator for high-entropy mechanical energy harvesting

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science China(Technological sciences) 2024年第5期67卷 1297-1316页

作者： CHEN Jie GUO RuiLong GUO HengYu College of physics and Electronic engineering Chongqing Normal UniversityChongqing 401331China department of applied physics Chongqing UniversityChongqing 401331China

In the era of the Internet of Things(IoT),the provision of sustainable power to distributed,mobile,and low-power-consumption electronic devices is a critical *** overcome this challenge,the triboelectric nanogenerator(TENG),a highly efficient high-entropy mechanical energy harvesting device,was developed in *** device enables the direct conversion of irregular and low-frequency mechanical energy into pulsed alternating current(AC)***,the incompatibility of most electronic devices with AC signals necessitates rectifier circuits or generators that deliver direct current(DC)*** recent years,DC-TENGs have undergone extensive development,achieving significant milestones in various application fields while also facing crucial challenges that require *** this review,three categories of DC-TENG devices with distinct operating mechanisms are comprehensively explored:multiphase coupling,mechanical rectification,and air *** typical structures and working mechanisms are thoroughly discussed,and specific output performance limitations,along with corresponding optimization strategies,are ***,the applications of DC-TENGs in various scenarios are ***,the challenges faced by DC-TENGs and potential solutions are analyzed to guide further advancements in this technology.

关键词： TENG direct current working mechanisms output performance limitations optimization strategies

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microstructure and magnetocaloric properties of melt-extracted smGdDyCoAl high-entropy amorphous microwires

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Rare metals 2024年第3期43卷 1234-1242页

作者： shi-Jie Wei Hong-Xian shen Lun-Yong Zhang Lin Luo Xin-Xing Tang Jian-Fei sun Xiao-Qing Li school of materials science and engineering Harbin Institute of TechnologyHarbin150001China applied materials physics Department of Materials Science and EngineeringKTH-Royal Institute of Technology10044StockholmSweden

This paper presents a systematic investigation of the microstructure and magnetocaloric properties of melt-extracted sm_(20)Gd_(20)Dy_(20)Co_(20)Al_(20)high-entropy *** fabricated wires exhibited an amorphous structure,and the temperature interval of the undercooled liquid AT was 45 *** microwires underwent a second-order magnetic transition from a ferromagnetic to a paramagnetic state near the Curie temperature(T_(C)=52 K),The maximum magnetic entropy change(-Δs_m^(max)),the relative cooling power and the refrigeration capacity reached 6.34 J·kg^(-1)·K^(-1).422.09 J·kg^(-1)and 332.94 J·kg^(-1),respectively,under a magnetic field change of 5 *** addition,the temperature-averaged entropy changes with two temperature lifts(3 and 10 K)were 6.32 and 6.27 J·kg^(-1)·K^(-1),*** good magnetocalorie performance highlights the significant potential for the sm_(20)Gd_(20)Dy_(20)Co_(20)Al_(20)microwires to be used as magnetic refrigerant materials in low-temperature region *** work will serve as a valuable reference for future investigations on low-temperature high-entropy magnetocaloric materials.

关键词： melt-extraction High-entropy amorphous microwires magnetocaloric effect magnetic refrigeration

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High Density 3D Carbon Tube Nanoarray Electrode Boosting the Capacitance of Filter Capacitor

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Nano-micro Letters 2024年第11期16卷 242-254页

作者： Gan Chen Fangming Han Huachun ma Pei Li Ziyan Zhou Pengxiang Wang Xiaoyan Li Guowen meng Bingqing Wei Key Laboratory of materials physics and Anhui Key Laboratory of Nanomaterials and NanotechnologyInstitute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031People’s Republic of China department of materials science and engineering University of Science and Technology of ChinaHefei 230026People’s Republic of China department of mechanical engineering University of DelawareNewarkDE 19716USA mechano‑X Institute Applied Mechanics LaboratoryDepartment of Engineering MechanicsTsinghua UniversityBeijing 100084People’s Republic of China

Electric double-layer capacitors(EDLCs)with fast frequency response are regarded as small-scale alternatives to the commercial bulky aluminum electrolytic *** carbon-based nanoarray electrodes with precise alignment and smooth ion channels is crucial for enhancing EDLCs’***,controlling the density of macropore-dominated nanoarray electrodes poses challenges in boosting the capacitance of line-filtering ***,a simple technique to finely adjust the vertical-pore diameter and inter-spacing in three-dimensional nanoporous anodic aluminum oxide(3D-AAO)template is achieved,and 3D compactly arranged carbon tube(3D-CACT)nanoarrays are created as electrodes for symmetrical EDLCs using nanoporous 3D-AAO template-assisted chemical vapor deposition of *** 3D-CACT electrodes demonstrate a high surface area of 253.0 m^(2) g^(−1),a D/G band intensity ratio of 0.94,and a C/O atomic ratio of *** a result,the high-density 3D-CT nanoarray-based sandwich-type EDLCs demonstrate a record high specific areal capacitance of 3.23 mF cm^(-2) at 120 Hz and exceptional fast frequency response due to the vertically aligned and highly ordered nanoarray of closely packed CT *** 3D-CT nanoarray electrode-based EDLCs could serve as line filters in integrated circuits,aiding power system miniaturization.

关键词： Compactly arranged Three-dimensional carbon tube nanoarray Dimensional carbon tube nanoarray Fast frequency response Electric double-layer capacitors Layer capacitors AC line-filtering Filtering

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