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Cu_(2)Se@C thin film with three-dimensional braided structure as a cathode material for enhanced Cu^(2+) storage

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Chinese Chemical Letters 2024年第5期35卷 523-528页

作者： Wenhao Chen Muxuan Wu Han Chen Lue Mo Yirong Zhu College of Materials and Advanced Manufacturing Hunan University of TechnologyZhuzhou 412007China Hunan Key of Laboratory of applied environmental Photocatalysis Changsha UniversityChangsha 410022China

In the face of multiple challenges brought by the changes of global climate and environment,developing clean energy and updating green energy storage equipment are important ways to achieve carbon peak and carbon *** batteries have become a research hotspot due to their advantages of using the multivalent charge carrier,high ionic conductivity,environmental friendliness and cost *** this work,the Cu_(2)Se@C(Cu_(2)Se coated on carbon clothes)thin film with a three-dimensional braided structure is fabricated by a simple electrochemical deposition method for Cu^(2+)storage for the first *** with the commercial Cu_(2)Se powder,the well-designed Cu_(2)Se@C film shows enhanced specific capacity(640 mAh/g at 0.5 A/g)and rate performance(542 mAh/g at 5 A/g)as well as superior cycling stability(82.7%capacity retention after 1000 cycles at 1 A/g).The Cu^(2+)storage mechanism of the Cu_(2)Se@C electrode is based on a reversible phase transition process of Cu_(2)Se←→Cu_(2-x)Se←→CuSe←→CuSe_(2).In kinetic characteristic analysis,the Cu_(2)Se@C electrode demonstrates faster Cu^(2+)diffusion in discharge process than charge process resulting from the phase transition and the variation of interplanar *** work highlights a facile one-piece design strategy and opens a new gateway for the exploration of advanced aqueous energy storage systems.

关键词： Cu_(2)Se@C Cu^(2+)storage Conversion mechanism Kinetic characteristic Flexible energy storage

Greenhouse gas emissions during the COVID-19 pandemic from agriculture in China

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Frontiers of Agricultural Science and Engineering 2024年第3期11卷 409-427页

作者： Jianing TIAN Chuanhui GU Yanchao BAI Division of Natural and applied Sciences Duke Kunshan University environmental Research Center Duke Kunshan University College of environmental Science and Engineering Yangzhou University

To study the impact of the COVID-19 pandemic on agricultural carbon emissions in China, the greenhouse gas emissions generated by crop and livestock production, and agricultural material and energy inputs in China from 2019 to 2021 were systematically calculated. It was found that from 2019 to 2021, Net greenhouse gas emissions（NGHGE） from agriculture in China had an increasing trend. Methane emissions ranked first in NGHGE, with an annual proportion exceeding 65% and an increasing annual trend. CH4emissions were primarily influenced by enteric fermentation and rice production. Nitrous oxide emissions accounted for around 22% of annual NGHGE and decreased from 2019 to 2021. The main sources of N2O emissions were the use of nitrogen fertilizers and manure management. Carbon dioxide emissions accounted for about 18% annually, with diesel and agricultural electricity use contributing to over 60% of CO2emissions. Soil carbon sequestration represented about a 6.1% lowering of NGHGE. The combined proportion of CH4emissions from enteric fermentation and rice production accounted for over 50% of total GHG emissions. The changes in NGHGE were mainly caused by disturbance of the livestock industry during the pandemic.

关键词： Agricultural systems emission factors greenhouse gases soil carbon sequestration

A2B7-type La-Mg-Ni alloys prepared by Mg thermal diffusion for improved hydrogen storage performance

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Rare Metals 2024年第7期43卷 3260-3272页

作者： Yong-Xi Zhang Guan-Jiu Wu Jing Gu Hong-Xing Kang Yuan Li Di Zhou Wen-Feng Wang Lu Zhang Shu-Min Han Hebei Key Laboratory of applied Chemistry School of Environmental and Chemical EngineeringYanshan University Department of Chemistry and Biochemistry San Diego State University State Key Laboratory of Metastable Materials Science and Technology Yanshan University

A novel approach based on thermal diffusion was used to achieve controllable Mg content in A2B7-type La-Mg-Ni-based *** formation mechanism of the A2B7-type phase as a result of the thermal diffusion process and the effect of Mg content on hydrogen storage performance were investigated.X-ray diffraction（XRD） patterns and Rietveld refinement results showed that increased Mg transformed the LaNi5phase in the La0.74Sm0.03Y0.23Ni4.32Al0.04precursor alloy into a superlattice *** electron microscopy（SEM） images showed that Mg was evenly distributed in the alloy *** in the superlattice significantly inhibited the phase decomposition of the superlattice structure during the hydrogen absorption/desorption *** A2B7-type La0.57Sm0.02Y0.18Mg0.23Ni3.38Al0.03alloy composed of Gd2Co7and Ce2Ni7phases was successfully *** pressure-composition isotherm profiles showed that the alloy had a hydrogen storage capacity as high as 1.73 wt%,with good cycling *** 50 cycles of hydrogen absorption/desorption,the alloy retained a hydrogen storage capacity of 1.45 wt%,with a capacity retention rate of up to 84.28%.The Mg thermal diffusion process thus provides a new approach for the controlled preparation of La-Mg-Ni-based alloys.

关键词： La–Mg–Ni-based hydrogen storage alloy A 2 B 7 -type superlattice alloy Mg thermal diffusion process Phase transformation Hydrogen storage property

Calcium-based polymers for suppression of soil acidification by improving acid-buffering capacity and inhibiting nitrification

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Journal of environmental Sciences 2024年第5期139卷 138-149页

作者： Fei Kang Yunshan Meng Yanning Ge Yun Zhang Haixiang Gao Xueqin Ren Jie Wang Shuwen Hu Beijing Key Laboratory of Farmland Soil Pollution Prevention-control and Remediation College of Resources and Environmental SciencesChina Agricultural UniversityBeijing 100193China Department of applied Chemistry China Agricultural UniversityBeijing 100193China

Soil acidification is a major threat to agricultural sustainability in tropical and subtropical *** and environmentally friendly materials,such as calcium lignosulfonate(CaLS),calcium poly(aspartic acid)(PASP-Ca),and calcium polyγ-glutamic acid(γ-PGA-Ca),are known to effectively ameliorate soil ***,their effectiveness in inhibiting soil acidification has not been *** study aimed to evaluate the effect of CaLS,PASP-Ca,andγ-PGA-Ca on the resistance of soil toward acidification as directly and indirectly(i.e.,via nitrification)caused by the application of HNO_(3)and urea,*** comparison,Ca(OH)_(2)and lignin were used as the inorganic and organic controls,*** the materials,γ-PGA-Ca drove the substantial improvements in the pH buffering capacity(pHBC)of the soil and exhibited the greatest potential in inhibiting HNO_(3)-induced soil acidification via protonation of carboxyl,complexing with Al~(3+),and cation exchange *** acidification induced by urea,CaLS was the optimal one in inhibiting acidification and increasing exchangeable acidity during ***,the sharp reduction in the population sizes of ammonia-oxidizing bacteria(AOB)and ammonia-oxidizing archaea(AOA)confirmed the inhibition of nitrification via CaLS ***,compared to improving soil pHBC,CaLS may play a more important role in suppressing indirect ***,γ-PGA-Ca was superior to PASP-Ca and CaLS in enhancing the soil pHBC and the its resistance to acidification induced by HNO_(3) addition,whereas CaLS was the best at suppressing urea-driven soil acidification by inhibiting *** conclusion,these results provide a reference for inhibiting soil re-acidification in intensive agricultural systems.

关键词： Calcium-based polymer Soil acidification pH buffering capacity Nitrification inhibition

Remaining Useful Life Prediction Method for Multi-Component System Considering Maintenance:Subsea Christmas Tree System as A Case Study

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China Ocean Engineering 2024年第2期38卷 198-209页

作者： WU Qi-bing CAI Bao-ping FAN Hong-yan WANG Guan-nan RAO Xi GE Weifeng SHAO Xiao-yan LIU Yong-hong CNOOC Safety Technology services Co. Ltd.Tianjin 300456China College of Mechanical and Electronic Engineering China University of PetroleumQingdao 266580China CNOOC EnerTech Safety&Environmental Protection BranchTianjin 300456China

Maintenance is an important technical measure to maintain and restore the performance status of equipment and ensure the safety of the production process in industrial production,and is an indispensable part of prediction and health ***,most of the existing remaining useful life(RUL)prediction methods assume that there is no maintenance or only perfect maintenance during the whole life cycle;thus,the predicted RUL value of the system is obviously lower than its actual operating *** complex environment of the system further increases the difficulty of maintenance,and its maintenance nodes and maintenance degree are limited by the construction period and working conditions,which increases the difficulty of RUL *** RUL prediction method for a multi-omponent system based on the Wiener process considering maintenance is *** performance degradation model of components is established by a dynamic Bayesian network as the initial model,which solves the uncertainty of insufficient data *** on the experience of experts,the degree of degradation is divided according to Poisson process simulation random failure,and different maintenance strategies are used to estimate a variety of condition maintenance *** example of a subsea tree system is given to verify the effectiveness of the proposed method.

关键词： remaining useful life Wiener process dynamic Bayesian networks maintenance subsea Christmas tree system

Regulating the crystal phase of bismuth-based semiconductors for promoted photocatalytic performance

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Science China Chemistry 2024年第6期67卷 1839-1864页

作者： Zhaohui Wu Mei-Chi Chong Shiying Zhang Junshan Li Yongfa Zhu Hunan Key Laboratory of applied environmental Photocatalysis Changsha UniversityChangsha410022China Department of Chemistry Tsinghua UniversityBeijing100084China Institute for Advanced Study Chengdu UniversityChengdu610106China

Numerous bismuth-based semiconductors(BBSs)with sophisticated and desirable structures used as photocatalysts for efficient photocatalytic degradation of water organic contaminants have attracted considerable ***,regulating the crystal phases and phase transition of BBSs for promoted photocatalytic performance is ***,the unique crystal structure and band structure features of each typical BBSs,and the vital roles on phase controlling of each phase were systematically presented based on the classification of ***,the critical factors for the phase transition of BBSs and intrinsic driving forces endowed by phases of BBSs for enhanced photocatalytic performance of organic contaminants removal were also *** review will provide systematical guidelines and horizons for regulating the crystal phase and phase transition of BBSs,promoting photocatalytic degradation and mineralization of organic contaminants.

关键词： bismuth-based semiconductors phase regulation photocatalytic performances organic contaminants

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A Comprehensive Systematic Review: Advancements in Skin Cancer Classification and Segmentation Using the ISIC Dataset

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Computer Modeling in Engineering & Sciences 2024年第9期140卷 2131-2164页

作者： Madiha Hameed Aneela Zameer Muhammad Asif Zahoor Raja Department of Computer Sciences Pakistan Institute of Engineering and Applied SciencesNilore50700Islamabad Future Technology Research Center National Yunlin University of Science and TechnologyDouliou64002Taiwan Directorate of IT services University of GujratGujrat50700Pakistan

The International Skin Imaging Collaboration(ISIC)datasets are pivotal resources for researchers in machine learning for medical image analysis,especially in skin cancer *** datasets contain tens of thousands of dermoscopic photographs,each accompanied by gold-standard lesion diagnosis *** challenges associated with ISIC datasets have spurred significant advancements,with research papers reporting metrics surpassing those of human *** cancers are categorized into melanoma and non-melanoma types,with melanoma posing a greater threat due to its rapid potential for metastasis if left *** paper aims to address challenges in skin cancer detection via visual inspection and manual examination of skin lesion images,processes historically known for their *** notable advancements in machine learning and deep learning models,persistent challenges remain,largely due to the intricate nature of skin lesion *** review research on convolutional neural networks(CNNs)in skin cancer classification and segmentation,identifying issues like data duplication and augmentation *** explore the efficacy of Vision Transformers(ViTs)in overcoming these challenges within ISIC dataset *** leverage their capabilities to capture both global and local relationships within images,reducing data duplication and enhancing model ***,ViTs alleviate augmentation issues by effectively leveraging original *** a thorough examination of ViT-based methodologies,we illustrate their pivotal role in enhancing ISIC image classification and *** study offers valuable insights for researchers and practitioners looking to utilize ViTs for improved analysis of dermatological ***,this paper emphasizes the crucial role of mathematical and computational modeling processes in advancing skin cancer detection methodologies,highlighting their significance in improving algorithmic

关键词： Medical image skin cancer classification skin cancer segmentation international skin imaging collaboration convolutional neural network deep learning

Biodegradability of bioplastics in different aquatic environments:A systematic review

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Journal of environmental Sciences 2024年第8期142卷 169-181页

作者： Maria Cristina Lavagnolo Valentina Poli Anna Maria Zampini Valentina Grossule Department of Civil Environmental and Architectural Engineering-Laboratory of Environmental EngineeringUniversity of PadovaLungargine Rovetta 8Padova 35100Italy

Bioplastics were first introduced as environmentally friendly materials,with properties similar to those of conventional plastics.A bioplastic is defined as biodegradable if it can be decomposed into carbon dioxide under aerobic degradation,or methane and CO_(2)under anaerobic conditions,inorganic compounds,and new cellular biomass,by the action of naturally occurring *** definition however does not provide any information on the environmental conditions,timescale and extent at which decomposition processes should *** regard to the aquatic environment,recognized standards have been established to assess the ability of plastics to undergo biodegradation;however,these standards fail to provide clear targets to be met to allow labelling of a bioplastic as ***,these standards grant the user an extensive leeway in the choice of process *** these reasons,the comparison of results deriving from different studies is *** authors analysed and discussed the degree of biodegradability of a series of biodegradable bioplastics in aquatic environments(both fresh and salt water)using the results obtained in the laboratory and from on-site testing in the context of different research *** Oxygen Demand(BOD),CO_(2)evolution,surface erosion and weight loss were the main parameters used by researchers to describe the percentage of *** results showed a large variability both in weight loss and BOD,even when evaluating the same type of *** confirms the need for a reference range of values to be established with regard to parameters applied in defining the biodegradability of bioplastics.

关键词： Biodegradation Bioplastic Plastic Natural environment Plastic waste

Oxidation of emerging organic contaminants by in-situ H_(2)O_(2) fenton system

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Green Energy & Environment 2024年第3期9卷 417-434页

作者： Yuqin Ni Chuxiang Zhou Mingyang Xing Yi Zhou State environmental Protection Key Lab of environmental Risk Assessment and Control on Chemical Processes School of Resources&Environmental EngineeringEast China University of Science and TechnologyShanghai200237China Key Laboratory for Advanced Materials and Institute of Fine Chemicals National Engineering Laboratory for Industrial Wastewater TreatmentSchool of Chemistry and Molecular EngineeringEast China University of Science and Technology130 Meilong RoadShanghai200237China Department of applied Natural Sciences Technische Hochschule LubeckMonkhofer Weg 23923562 LubeckGermany

The existence and risk of emerging organic contaminants(EOCs)have been under consideration and paid much effort to degrade these *** system is one of the most widely used technologies to solve this *** original Fenton system relies on the hydroxyl radicals produced by Fe(Ⅱ)/H_(2)O_(2) to oxidize the organic ***,the application of the Fenton system is limited by its low iron cycling efficiency and the high risks of hydrogen peroxide transportation and *** introduction of external energy(including light and electricity etc.)can effectively promote the Fe(Ⅲ)/Fe(Ⅱ)cycle and the reduction of oxygen to produce hydrogen peroxide in *** review introduces three in-situ Fenton systems,which are electro-Fenton,Photo-Fenton,and chemical *** mechanism,influencing factors,and catalysts of these three in-situ Fenton systems in degrading EOCs are discussed *** review strengthens the understanding of Fenton and in-situ Fenton systems in degradation,offering further insight into the real application of the in-situ Fenton system in the removal of EOCs.

关键词： In-situ H_(2)O_(2)production Fenton Emerging organic contaminants Photocatalysis Electrocatalysis