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Deflagration characteristics of freely propagating flames in magnesium hydride dust clouds

Defence technology（防务技术） 2024年第1期31卷 471-483页

作者： Qiwei Zhang Yangfan Cheng Beibei Zhang Danyi Li Zhaowu Shen School of Chemical Engineering Anhui University of Science and TechnologyHuainan 232001AnhuiPR China School of Civil Engineering and Architecture Anhui University of Science and TechnologyHuainan 232001AnhuiPR China anhui Engineering Laboratory of Explosive Materials and technology Anhui University of Science and TechnologyHuainan 232001AnhuiPR China School of Engineering science University of Science and Technology of ChinaHefei 230027AnhuiPR China

The flame propagation processes of MgH_(2)dust clouds with four different particle sizes were recorded by a high-speed *** dynamic flame temperature distributions of MgH_(2)dust clouds were reconstructed by the two-color pyrometer technique,and the chemical composition of solid combustion residues were *** experimental results showed that the average flame propagation velocities of 23μm,40μm,60μm and 103μm MgH_(2)dust clouds in the stable propagation stage were 3.7 m/s,2.8 m/s,2.1 m/s and 0.9 m/s,*** dust clouds with smaller particle sizes had faster flame propagation velocity and stronger oscillation intensity,and their flame temperature distributions were more even and the temperature gradients were *** flame structures of MgH_(2)dust clouds were significantly affected by the particle sinking velocity,and the combustion processes were accompanied by micro-explosion of *** falling velocities of 23μm and 40μm MgH_(2)particles were 2.24 cm/s and 6.71 cm/s,*** the falling velocities of 60μm and 103μm MgH_(2)particles were as high as 15.07 cm/s and 44.42 cm/s,respectively,leading to a more rapid downward development and irregular shape of the ***,the dehydrogenation reaction had a significant effect on the combustion performance of MgH_(2)*** combustion of H_(2)enhanced the ignition and combustion characteristics of MgH_(2)dust,resulting in a much higher explosion power than the pure Mg *** micro-structure characteristics and combustion residues composition analysis of MgH_(2)dust indicated that the combustion control mechanism of MgH_(2)dust flame was mainly the heterogeneous reaction,which was affected by the dehydrogenation reaction.

关键词： Magnesium hydride dust Flame combustion mechanism Particle size Dust explosion Two-color pyrometer

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Manipulating photogenerated electron flow in nickel single‐atom catalysts for photocatalytic CO_(2)reduction into tunable syngas

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Carbon Energy 2024年第8期6卷 205-213页

作者： Yida Zhang Qingyu Wang Lihui Wu Haibin Pan Chengyuan Liu Yue Lin Gongming Wang Xusheng Zheng National Synchrotron Radiation Laboratory University of Science and Technology of ChinaHefeiAnhuiChina college of Chemistry and Materials science University of Science and Technology of ChinaHefeiAnhuiChina Department of Chemistry Hefei National Research Center for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefeiAnhuiChina

The key to designing photocatalysts is to orient the migration of photogenerated electrons to the target active sites rather than dissipate at inert ***,we demonstrate that the doping of phosphorus(P)significantly enriches photogenerated electrons at Ni active sites and enhances the performance for CO_(2)reduction into *** photocatalytic CO_(2)reduction,Ni single‐atom‐anchored P‐modulated carbon nitride showed an impressive syngas yield rate of 85μmol gcat^(−1)h^(−1)and continuously adjustable CO/H_(2)ratios ranging from 5:1 to 1:2,which exceeded those of most of the reported carbon nitride‐based single‐atom *** studies reveal that P doping improves the conductivity of catalysts,which promotes photogenerated electron transfer to the Ni active sites rather than dissipate randomly at low‐activity nonmetallic sites,facilitating the CO_(2)‐to‐syngas photoreduction process.

关键词： carbon nitride CO_(2)photoreduction electron flow Ni single atoms syngas

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Double quantum images encryption scheme based on chaotic system

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Chinese Physics B 2024年第4期33卷 305-320页

作者：蒋社想李杨石锦张茹 School of Computer science and Engineering Anhui University of Science and TechnologyHuainan 232001China anhui Key Laboratory of Mine Intelligent Equipment and technology Anhui University of Science&TechnologyHuainan 232001China

This paper explores a double quantum images representation(DNEQR)model that allows for simultaneous storage of two digital images in a quantum superposition ***,a new type of two-dimensional hyperchaotic system based on sine and logistic maps is investigated,offering a wider parameter space and better chaotic behavior compared to the sine and logistic *** on the DNEQR model and the hyperchaotic system,a double quantum images encryption algorithm is ***,two classical plaintext images are transformed into quantum states using the DNEQR ***,the proposed hyperchaotic system is employed to iteratively generate pseudo-random *** chaotic sequences are utilized to perform pixel value and position operations on the quantum image,resulting in changes to both pixel values and ***,the ciphertext image can be obtained by qubit-level diffusion using two XOR operations between the position-permutated image and the pseudo-random *** corresponding quantum circuits are also *** results demonstrate that the proposed scheme ensures the security of the images during transmission,improves the encryption efficiency,and enhances anti-interference and anti-attack capabilities.

关键词： double quantum images encryption chaotic system pixel scrambling XOR operation

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Effects of content and particle size of TiH2 powders on the energy output rules of RDX composite explosives

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Defence technology（防务技术） 2024年第2期32卷 297-308页

作者： Hao Wang Yangfan Cheng Shoujun Zhu Zihan Li Zhaowu Shen School of Chemical Engineering Anhui University of Science and TechnologyHuainan 232001China anhui Engineering Laboratory of Explosive Materials and technology Anhui University of Science and TechnologyHuainan 232001China School of Engineering science University of Science and Technology of ChinaHefei 230027China

In order to improve the detonation characteristics of RDX,a RDX-based composite explosive with TiH_(2)powders was *** effects of content and particle size of TiH_(2)powders on thermal safety,shock wave parameters and thermal damage effects of RDX-based composite explosive were studied with the C80 microcalorimeter,air blast experiment system and colorimetric thermometry *** results showed that TiH_(2)powders could enhance the thermal stability of RDX-based composite explosive and increase its ultimate decomposition *** content and particle size of TiH_(2)powders also had significant effects on the thermal safety,detonation velocity,shock wave parameters,fireball temperature and duration of RDX-based composite ***,the differences of TiH_(2)and Ti powders on the detonation energy output rules of RDX-based composite explosives were also compared,showing that TiH_(2)powders had better influences on improving the explosion power and thermal damage effect of RDX-based composite explosives than Ti powders,for the participation of free H_(2)released by TiH_(2)powders in the detonation ***_(2)powders have important research values as a novel energetic additive in the field of military composite explosives.

关键词： RDX Hydrogen storage alloy Air blast After-burn reaction Colorimetric thermometry

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A strategy to synthesize phosphorus-containing nickel phyllosilicate whiskers to enhance the flame retardancy of epoxy composites with excellent mechanical and dry-friction properties

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Frontiers of Chemical science and Engineering 2024年第3期18卷 39-50页

作者： Shibin Nie Zongquan Zhao Yuxuan Xu Wei He Wenli Zhai Jinian Yang School of Public Security and Emergency Management Anhui University of Science and TechnologyHefei231131China School of Safety science and Engineering Anhui University of Science and TechnologyHuainan232001China School of Materials science and Engineering Anhui University of Science and TechnologyHuainan232001China Institute of Energy Hefei Comprehensive National Science CenterHefei230000China

To enhance the fire safety and wear resistance of epoxy,phosphorus-containing nickel phyllosilicate whiskers(FP-NiPS)were synthesized using a facile hydrothermal technology,with 9,10-dihydro-9-oxa-10-phosphaphenanthrene as the organic *** impacts of FP-NiPS on the thermal stability,flame retardancy,and mechanical and tribological properties of EP composites were *** findings demonstrated that 5 wt%FP-NiPS elevated the limiting oxygen index of the EP composite from 23.8%to 28.4%,achieving a V-0 rating during vertical burning ***-NiPS could enhance the thermal stability of epoxy resin(EP)and facilitate the development of a dense and continuous carbon layer,thereby significantly improving the fire safety of the EP *** FP-NiPS led to an 8.2%increase in the tensile strength and a 38.8%increase in the elastic modulus of the EP composite,showing outstanding mechanical ***,FP-NiPS showed remarkable potential in enhancing the wear resistance of *** wear rate of 1 wt%FP-NiPS is 2.34×10^(−5) mm^(3)·N^(−1)·m^(−1),a decrease of 66.7%compared to *** work provides a novel promising modification method to enhance the fire safety,mechanical and wear resistance properties of EP.

关键词： nickel phyllosilicate epoxy resin flame retardant wear resistance mechanical property

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Real-Time Detection and Instance Segmentation of Strawberry in Unstructured Environment

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Computers, Materials & Continua 2024年第1期78卷 1481-1501页

作者： Chengjun Wang Fan Ding Yiwen Wang Renyuan Wu Xingyu Yao Chengjie Jiang Liuyi Ling School of Artificial Intelligence Anhui University of Science and TechnologyHuainan232001China School of Mechanical Engineering Anhui University of Science and TechnologyHuainan232001China

The real-time detection and instance segmentation of strawberries constitute fundamental components in the development of strawberry harvesting ***-time identification of strawberries in an unstructured envi-ronment is a challenging *** instance segmentation algorithms for strawberries suffer from issues such as poor real-time performance and low *** this end,the present study proposes an Efficient YOLACT(E-YOLACT)algorithm for strawberry detection and segmentation based on the YOLACT *** key enhancements of the E-YOLACT encompass the development of a lightweight attention mechanism,pyramid squeeze shuffle attention(PSSA),for efficient feature ***,an attention-guided context-feature pyramid network(AC-FPN)is employed instead of FPN to optimize the architecture’s ***,a feature-enhanced model(FEM)is introduced to enhance the prediction head’s capabilities,while efficient fast non-maximum suppression(EF-NMS)is devised to improve non-maximum *** experimental results demonstrate that the E-YOLACT achieves a Box-mAP and Mask-mAP of 77.9 and 76.6,respectively,on the custom ***,it exhibits an impressive category accuracy of 93.5%.Notably,the E-YOLACT also demonstrates a remarkable real-time detection capability with a speed of 34.8 *** method proposed in this article presents an efficient approach for the vision system of a strawberry-picking robot.

关键词： YOLACT real-time detection instance segmentation attention mechanism strawberry

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Sequence structure controllable polymerization-induced self-assembly

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science China Chemistry 2024年第1期67卷 390-397页

作者： Zi-Xuan Chang Ren-Man Zhu Chun-Yan Hong Wen-Jian Zhang Department of Polymer science and Engineering University of Science and Technology of ChinaHefei 230026China Institute of Physical science and Information technology Anhui UniversityHefei 230601China Key Laboratory of Environment-Friendly Polymeric Materials of anhui Province Anhui UniversityHefei 230601China

Polymerization-induced self-assembly(PISA)combines synthesis and self-assembly of artificial polymers in one-pot,which brings us one step closer to emulating ***,the reported PISA formulations primarily focus on developing nano-objects with new chemical compositions and rarely on structural regulation of polymers with specific ***,sequence structure controllable polymerization-induced self-assembly(SCPISA)is reported by using 7-(2-methacryloyloxyethoxy)-4-methylcoumarin(CMA)as a *** the copolymerization of 2-hydroxyethyl methacrylate(HEMA)and CMA,controlled incorporation of CMA units into the polymer chains can be realized by programmable light/heat ***-based P(HEMA-co-CMA)copolymers with the same composition but different sequence structures generate a range of ***,the morphologies of the resultant nano-objects can also be controlled by regulating the feed molar ratio of CMA and HEMA,which is similar to the conventional PISA,but the synthesis procedure is obviously simplified in *** versatility of the methodology is further demonstrated by the fabrication of different functional nano-objects with sequence structure-dependent morphologies in SCPISA systems with different functional monomers.

关键词： polymerization-induced self-assembly sequence-controlled polymers PET-RAFT polymerization

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Physics-based battery SOC estimation methods:Recent advances and future perspectives

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Journal of Energy Chemistry 2024年第2期89卷 27-40,I0003页

作者： Longxing Wu Zhiqiang Lyu Zebo Huang Chao Zhang Changyin Wei college of Mechanical Engineering Anhui Science and Technology UniversityChuzhou 233100AnhuiChina Hubei Key Laboratory of Power System Design and Test for Electrical Vehicle Hubei University of Arts and ScienceXiangyang 441053HubeiChina School of Internet Anhui UniversityHefei 230039AnhuiChina School of Mechanical and Electrical Engineering Guilin University of Electronic TechnologyGuilin 541004GuangxiChina

The reliable prediction of state of charge(SOC)is one of the vital functions of advanced battery management system(BMS),which has great significance towards safe operation of electric *** far,the empirical model-based and data-driven-based SOC estimation methods of lithium-ion batteries have been comprehensively discussed and reviewed in various ***,few reviews involving SOC estimation focused on electrochemical mechanism,which gives physical explanations to SOC and becomes most attractive candidate for advanced *** this reason,this paper comprehensively surveys on physics-based SOC algorithms applied in advanced ***,the research progresses of physical SOC estimation methods for lithium-ion batteries are thoroughly discussed and corresponding evaluation criteria are carefully ***,future perspectives of the current researches on physics-based battery SOC estimation are *** insights stated in this paper are expected to catalyze the development and application of the physics-based advanced BMS algorithms.

关键词： Lithium-ion batteries State of charge Electrochemical model Battery management system

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Thermal runaway evolution of a 280 Ah lithium-ion battery with LiFePO_(4) as the cathode for different heat transfer modes constructed by mechanical abuse

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Journal of Energy Chemistry 2024年第6期93卷 32-45,I0002页

作者： Zhixiang Cheng Chengdong Wang Wenxin Mei Peng Qin Junyuan Li Qingsong Wang State Key Laboratory of Fire science University of Science and Technology of ChinaHefei 230026AnhuiChina

Lithium iron phosphate batteries have been increasingly utilized in recent years because their higher safety performance can improve the increasing trend of recurring thermal runaway ***,the safety performance and mechanism of high-capacity lithium iron phosphate batteries under internal short-circuit challenges remain to be *** work analyzes the thermal runaway evolution of high-capacity LiFePO_(4) batteries under different internal heat transfer modes,which are controlled by different penetration *** penetration cases involving complete penetration and incomplete penetration were detected during the test,and two modes were performed incorporating nails that either remained or were removed after penetration to comprehensively reveal the thermal runaway mechanism.A theoretical model of microcircuits and internal heat conduction is also *** results indicated three thermal runaway evolution processes for high-capacity batteries,which corresponded to the experimental results of thermal equilibrium,single thermal runaway,and two thermal runaway *** difference in heat distribution in the three phenomena is determined based on the microstructure and material structure near the *** controlling the heat dissipation conditions,the time interval between two thermal runaway events can be delayed from 558 to 1417 s,accompanied by a decrease in the concentration of in-situ gas production during the second thermal runaway event.

关键词： Lithium-ion battery safety Micro short-circuit cell Heat transfer modes Internal short circuit Nail-penetration test

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Structure,electronic,and nonlinear optical properties of superalkaline M_(3)O(M=Li,Na)doped cyclo[18]carbon

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Chinese Physics B 2024年第2期33卷 311-317页

作者：刘晓东卢其亮罗其全 School of Physics and Material science Anhui UniversityHefei 230601China Institute of Physical science and Information technology Anhui UniversityHefei 230601China Department of Chemical Physics University of Science and Technology of ChinaHefei 230026China

Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic *** have low ionization *** a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer *** this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not *** C_(18) ring still exhibits alternating long and short *** charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.

关键词： superalkaline doped cyclocarbon structure and electronic properties nonlinear optical properties density functional theory(DFT)

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