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Hydrogen bond-bridged phosphorene flexible film for photodynamic inhibiting Staphylococcus aureus

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Nano research 2024年第6期17卷 5461-5468页

作者： Ziyu Wei Wenting Li Zhifang Liu Yongfa Zhu Huaqiang Cao Department of Chemistry Engineering Research Center of Advanced Rare Earth MaterialsTsinghua UniversityBeijing 100084China

Antibiotics are a widely used and effective treatment for bacterial ***,bacteria can gradually evolve during infection,leading to developing resistance to antibiotics,which renders previously effective treatments *** a useful and convenient manner to treat bacterial infections is a great ***,we report a flexible hydrogen-bond-bridged phosphorene film with photodynamic antibacterial properties and excellent mechanical properties,fabricated from electrochemical exfoliation of black phosphorus(BP).When illuminated under 700 nm light,the hydrogen bond-bridged phosphorene flexible film is capable of converting ground-state triplet oxygen(O_(2))into excited-state singlet oxygen(^(1)O_(2)),destroying the structure of the membrane of Staphylococcus aureus,and eventually leading to bacterial death,via breaking the C=C of unsaturated fatty acids within the bacterial cell membrane after the reaction between^(1)O_(2)and unsaturated fatty acids,thus realizing a highly efficient antibacterial approach,which is supported by gas chromatography-mass spectrometry(GC-MS)*** work establishes an effective phototherapy platform for treating bacterial traumatic infections.

关键词： hydrogen bond-bridged phosphorene flexible film photodynamic Staphylococcus aureus

Nano-Ni-Induced Electronic Modulation of MoS2 Nanosheets Enables Energy-Saving H2 Production and Sulfide Degradation

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Energy & Environmental materials 2024年第3期7卷 232-239页

作者： Fan Liu Xinghong Cai Yang Tang Wenqian Liu Qianwei Chen Peixin Dong Maowen Xu Yangyang Tan Shujuan Bao Institute for Clean Energy & advanced materials School of Materials and EnergySouthwest University

Electrocatalytic hydrogen evolution and sulfion (S2-) recycling are promising strategies for boosting H2production and removing environmental ***,a nano-Ni-functionalized molybdenum disulfide （MoS2）nanosheet was assembled on steel mesh （Ni-MoS2/SM） for use in sulfide oxidation reaction-assisted,energy-saving *** and theoretical calculation results revealed that anchoring nano-Ni on highsurface-area slack MoS2 nanosheets not only optimized catalyst adsorption of polysulfides but also played an important role in promoting hydrogen evolution reaction kinetics by absorbing OHad,thereby greatly enhancing the catalytic performance toward sulfide oxidation reaction and hydrogen evolution ***,the Ni/MoS2-based hydrogen evolution reaction+sulfide oxidation reaction system achieved nearly 100%hydrogen production efficiency and only consumed 61%less power per kWh than the oxygen evolution reaction+hydrogen evolution reaction system,which suggested our proposed Ni-MoS2and novel hydrogen production system are promising for sustainable energy production.

关键词： hydrogen evolution reaction low energy consumption molybdenum disulfide sulfide oxidation reaction

Recent advances in molecular and nanoparticle probes for fluorescent bioanalysis

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Nano research 2024年第7期17卷 6443-6474页

作者： Haowen Luo Lejie Tian Yaoming Zhang Yang Wu Bin Li Jianxi Liu State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Yantai Zhongke research Institute of advanced materials and Green Chemical Engineering Shandong Laboratory of Advanced Materials and Green ManufacturingYantai 264006China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

With the increasing emphasis on ecological safety and physical health,the detection and treatment of harmful substances and diseases are becoming more and more ***,efficiently monitoring these biological behaviors with high accuracy and sensitivity in real-time has shown prominent research *** use of fluorescent probes to analyze organisms has gained momentum in recent years,especially in the field of organ imaging and assisted cancer therapy,where fluorescent bioanalysis demonstrates significant *** this review,we explored the latest advancements in fluorescent molecular probes(e.g.,small-molecule,macro-molecule,supramolecule)and fluorescent nanoparticle probes(e.g.,quantum dots or nanoclusters,metal-organic frameworks,polymers,complexes)used as bioanalytical tools in various assays over the last three *** also delved into their detective mechanisms,specific application areas,and characterization tools for responsive *** review aims to showcase the most recent and comprehensive research progress in fluorescent bioanalysis based on molecular and nanoparticle probes,offering guidance for future developments in the design and fabrication of fluorescent probes and their potential applications.

关键词： fluorescent biosensing bioimaging disease diagnosis tumor detection and treatment

Design and tailoring of patterned ZnO nanostructures for perovskite light absorption modulation

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International Journal of Minerals,Metallurgy and materials 2024年第5期31卷 855-861页

作者： Haonan Si Xuan Zhao Qingliang Liao Yue Zhang Academy for advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China Key Laboratory of advanced materials and Devices for Post-Moore Chips Ministry of EducationBeijing Key Laboratory for Advanced Energy Materials and TechnologiesSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Lithography is a pivotal micro/nanomanufacturing technique,facilitating performance enhancements in an extensive array of devices,encompassing sensors,transistors,and photovoltaic *** key to creating highly precise,multiscale-distributed patterned structures is the precise control of the lithography ***,high-quality patterned ZnO nanostructures are constructed by systematically tuning the exposure and development times during *** optimizing these parameters,ZnO nanorod arrays with line/hole arrangements are successfully *** ZnO nanostructures with highly controllable morphology and structure possess discrete three-dimensional space structure,enlarged surface area,and improved light capture ability,which achieve highly efficient energy conversion in perovskite solar *** lithography process management for these patterned ZnO nanostructures provides important guidance for the design and construction of complex nanostructures and devices with excellent performance.

关键词： lithography patterned ZnO nanorod arrays light absorption perovskite solar cell

High-temperature corrosion of sintered RE_(2)Si_(2)O_(7)(RE=Yb and Ho)environmental barrier coating materials by volcanic ash

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International Journal of Minerals,Metallurgy and materials 2024年第7期31卷 1628-1638页

作者： Ayahisa Okawa Son Thanh Nguyen Tadachika Nakayama Thi-Mai-Dung Do Hisayuki Suematsu Shu Yin Takuya Hasegawa Tsuneo Suzuki Takashi Goto Koichi Niihara Institute of Multidisciplinary research for advanced materials Tohoku UniversitySendai 980-8577Japan Department of Creative Engineering National Institute of TechnologyKushiro 084-0916Japan Extreme Energy-Density research Institute Nagaoka University of TechnologyNagaoka 940-2188Japan advanced Institute for materials research(WPI-AIMR) Tohoku UniversitySendai 980-8577Japan

Rare-earth silicates are promising environmental barrier coatings(EBCs)that can protect SiC_(f)/Si C_(m)substrates in next-genera tion gas turbine ***,RE_(2)Si_(2)O_(7)(RE=Yb and Ho)shows potential as an EBC due to its coefficient of thermal expansion(CTE)compatible with substrates and high resistance to water vapor *** target operating temperature for next-generation tur bine blades is 1400°*** is inevitable during adhesion to molten volcanic ash,and thus,understanding the corrosion behavior o the material is crucial to its *** study investigates the high-temperature corrosion behavior of sintered RE_(2)Si_(2)O_(7)(RE=Yb and Ho).Samples were prepared using a solid-state reaction and hot-press *** were then exposed to volcanic ash at 1400°C for 224,and 48 *** 48 h of exposure,volcanic ash did not react with Yb_(2)Si_(2)O_(7)but penetrated its interior,causing *** Ho_(2)Si_(2)O_(7)was partially dissolved in the molten volcanic ash,forming a reaction zone that prevented volcanic ash melts from penetrating the *** increasing heat treatment time,the reaction zone expanded,and the thickness of the acicular apatite grains increased The Ca:Si ratios in the residual volcanic ash were mostly unchanged for Yb_(2)Si_(2)O_(7)but decreased considerably over time for Ho_(2)Si_(2)O_(7).Th Ca in volcanic ash was consumed and formed apatite,indicating that RE^(3+)ions with large ionic radii(Ho>Yb)easily precipitated apatit from the volcanic ash.

关键词： environmental barrier coating volcanic ash rare-earth disilicate corrosion

Boosting high-rate Li-ion storage properties by La(Ⅲ)ion doping in spinel(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)high-entropy oxide anode

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Journal of advanced Ceramics 2024年第6期13卷 769-779页

作者： Shijie Chen Mengfan Bao Yanggang Jia Pengpeng Wang Dan Wei Yuhuan Guo Jie Tan Aiqin Mao advanced Ceramics research Center School of Materials Science and EngineeringAnhui University of TechnologyMa’anshan 243032China Key Laboratory of Green Fabrication and Surface Technology of advanced Metal materials(Anhui University of Technology) Ministry of EducationMa’anshan 243032China

The present work aims to create lattice distortion and optimize the surface oxygen vacancy(OV)concentration in a model spinel(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)high-entropy oxide(HEO)through a heteroatom La^(3+)doping *** demonstrated,La^(3+)with a large radius can be doped successfully into the spinel lattice of(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4),thereby not only causing lattice distortion to increase oxygen vacancies but also refining crystalline grains and improving the specific *** with the(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)anode,the(La_(0.01)CoCrFeMnNi)_(3/5.01)O_(4) anode with moderate doping exhibits excellent cycling performance(1228 mAh·g^(−1)after 400 cycles at 0.2 A·g^(−1))and yields an increase of 75%rate capability at 3 A·g^(−1)(420 mAh·g^(−1)at 3 A·g^(−1)).The desirable kinetic transport of electrons and diffusion of Li+within the moderately La^(3+)-doped anode and the synergistic interfacial pseudocapacitive behavior satisfy the redox reaction at a high rate,thus increasing rate capability.

关键词： lithium-ion battery(LIB) anode lattice distortion high-entropy oxide(HEO) high-rate performance La^(3+)doping oxygen vacancy(OV)

Phase-field simulation of precipitation kinetics and creep properties of Ni-Al-Cr/Ta superalloys

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Science China(Technological Sciences) 2024年第4期67卷 1139-1150页

作者： YANG ShuaiGe ZHANG Zan ZHUO JiCheng LONG HongLi LI YongSheng National Key Laboratory of advanced Casting Technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China

The precipitation kinetics ofγ'-Ni_(3)(Al,Ta)phase and creep properties of Ni-15Al-x Ta at.%superalloys are investigated by the crystal plasticity phase-field *** results show that the high Ta content brings a lower creep strain for the deceleration and steady creep stage,while the creep lifetime is *** large external strain intensifies the creep damage and shortens the creep life of Ni-15Al-3Ta at.%*** kinetics evolution and elements distribution are revealed in the quaternary Ni-10Al-8.5Cr-xT a(x=1.5 at.%,2.0 at.%,2.5 at.%)superalloys by the multi-component phase-field *** anti-phase boundary(APB)changes the coarsening mechanism ofγ'phase,and Ta promotes the precipitation ofγ'phase with an increasing volume fraction and particle *** composition difference betweenγ'andγphases increases with the rising of Ta content,the strong partitioning of Ta toγ'phase strengthens the partitioning of Ni and Cr toγmatrix,and Ta shows a superiority than Al in the lattice site occupation of L1_(2)-Ni_(3)(Al,X)*** an importantγ'phase forming element,the optimization of Ta content is essential for improving the mechanical properties of Ni-based superalloys.

关键词： Ni-Al-Ta alloys creep properties kinetics phase-field

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Congener-derived template to construct lithiophilic organic-inorganic layer/interphase for high volumetric capacity dendrite-free Li metal batteries

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Chinese Chemical Letters 2024年第3期35卷 453-460页

作者： Kang Yang Long Li Yuanbin Xiao Qiaoli Zhang Chenpeng Xi Borong Li Yan Yu Chengkai Yang Key Laboratory of advanced materials Technologies International(HongKong Macao and Taiwan)Joint Laboratory on Advanced Materials TechnologiesCollege of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China

The development of lithium-metal batteries(LMBs)is seriously restricted by the out-of-control dendrites growth and infinite volume ***,a pervasive organic-inorganic layer construction strategy is reported for the composite lithium metal anode with congener-derived organic-inorganic solid electrolyte interphase(SEI).In this strategy,the organic-inorganic Ag@polydopamine(Ag@PDA)layer is coated on the arbitrary substrates by a simple two-step *** thin and stable congener-derived SEI is insitu formed with fewer inorganic components and more organic components during charging/*** polydopamine with sufficient adhesion groups and lithiophilic Ag layer realize near-zero nucleation overpotential during lithium *** low interface resistance and stable lithium deposition are ***,the practical areal and volumetric capacities of the composite anode with three-dimensional copper(3DCu)as the substrate are 10 mAh/cm^(2)and 1538 mAh/cm^3(*** mass of anode).The symmetrical cell shows very low polarization voltage(10 mV)and more than 2500 h cycles life at 1 mA/cm^(2)(1 mAh/cm^(2)).The LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)-based full cells show improved capacity retention(82%)after 100 cycles at 0.5 *** modified lithiophilic anode with congener-derived interphase provides a promising strategy to realize the next-generation dendrite-free LMBs.

关键词： Lithium metal anode Congener-derived Lithiophilicity Volumetric capacity Organic-inorganic interphase

Highly responsive broadband Si-based MoS2 phototransistor on high-k dielectric

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Science China(Information Sciences) 2024年第6期67卷 180-189页

作者： Ali IMRAN Xin HE Jiwei LIU Qinghai ZHU Muhammad SULAMAN Fei XUE Mingsheng XU Deren YANG College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University ZJU-Hangzhou Global Scientific and Technological Innovation centre School of materials Science and Engineering State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of Technology

The demand for photodetectors and image sensors has grown exponentially in the past decade in biomedical, security surveillance, robotics, automotive, quality control, image recognition, and military applications, due to their superior quality, broadband detection, lower noise, and economic viability. Here,we report a MoS2channel-based phototransistor over an HfO2/n-Si substrate isolated by an h BN layer. The high photoresponse is achieved through the integration of the photoconduction, photogating, and mobility enhancement process by utilizing excellent features of MoS2, HfO2/Si, and h BN. The capacitive coupling of the photogenerated carriers by high-k dielectric HfO2leads to modulation of MoS2Fermi level due to electrostatic doping. Furthermore, the MoS2also contributes to the photogeneration of carriers due to its semiconducting nature, leading to additional photocurrent. Ultimately, the combination of photogating,photoconduction, and swift carrier extraction with remarkable mobility of 11.65 cm2· V-1· s-1results in high responsivity, external quantum efficiency, and detectivity of 4.5 × 10～8A · W-1, 0.72 × 10～6, and 6.20× 1016Jones at 266 nm illumination, respectively. The device also demonstrates broadband photoresponse from 266–1000 nm wavelengths. The high responsivity distinguishes the potential of our device for the future of optoelectronics and broadband image sensing applications.

关键词： photogating photoconduction two-dimensional materials high $~k$ dielectric carrier scattering phototransistor