检索结果-南通市图书馆

Graphene effectively activating "dead" water molecules between manganese dioxide layers in potassium-ion battery

Journal of Energy Chemistry 2024年第6期93卷 306-315,I0008页

作者： Xinhai Wang Wensheng Yang Shengshang Lu Shangshu Peng Tong Guo Quan Xie Qingquan Xiao Yunjun Ruan institute of advanced Optoelectronic Materials and Technology College of Big Data and Information EngineeringGuizhou UniversityGuiyang 550025GuizhouChina

Aqueous potassium-ion batteries(APIBs),recognized as safe and reliable new energy devices,are considered as one of the alternatives to traditional *** MnO_(2),serving as the main cathode,exhibits a lower specific capacity in aqueous electrolytes compared to organic systems and operates through a different reaction *** application of highly conductive graphene may effectively enhance the capacity of APIBs but could complicate the potassium storage *** this study,a MnO_(2) cathode pre-intercalated with K~+ions and grown on graphene(KMO@rGO) was developed using the microwave hydrothermal method for ***@rGO achieved a specific capacity of 90 mA h g^(-1) at a current density of 0.1 A g^(-1),maintaining a capacity retention rate of>90% after 5000 cycles at 5 A g^(-1).In-situ and exsitu characterization techniques revealed the energy-storage mechanism of KMO@rGO:layered MnO_(2)traps a large amount of "dead" water molecules during K~+ions ***,the introduction of graphene enables these water molecules to escape during K~+ ions insertion at the *** galvanostatic intermittent titration technique and density functional theory confirmed that KMO@rGO has a higher K~+ions migration rate than MnO_(2).Therefore,the capacity of this cathode depends on the interaction between dead water and K~+ions during the energy-storage *** optimal structural alignment between layered MnO_(2) and graphene allows electrons to easily flow into the external *** charge compensation forces numerous low-solvent K~+ions to displace interlayer dead water,enhancing the *** unique reaction mechanism is unprecedented in other aqueous battery studies.

关键词： Graphene K-ion batteries Mn-based layered oxide Water molecules Density functional theory

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Weighted Probability Density Estimator with Updated Bandwidths

引用

Journal of Systems Science & Complexity 2024年第2期37卷 886-906页

作者： WU Yi YU Wei WANG Xuejun PRAKASA RAO B L S School of big data and Artificial Intelligence Chizhou UniversityChizhou 247000China School of big data and Statistics Anhui UniversityHefei 230601China CR Rao advanced institute of Mathematics Statistics and Computer ScienceHyderabad 500046India

In this paper,the authors study a class of weighted version of probability density *** is shown that the weighted estimator contains some existing estimators of probability density,no matter they are recursive or *** statistical results including weak consistency,strong consistency,rate of strong consistency,and asymptotic normality are established under some mild ***,the random weighted estimator is also *** numerical simulations and a real data analysis are presented to study the numerical performances of the estimators.

关键词： Asymptotic normality consistency numerical simulation probability density real data analysis updated bandwidths weighted estimator

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Perpendicular-Cutdepth:Perpendicular Direction Depth Cutting data Augmentation Method

引用

Computers, Materials & Continua 2024年第4期79卷 927-941页

作者： Le Zou Linsong Hu Yifan Wang Zhize Wu Xiaofeng Wang Anhui Provincial Engineering Laboratory of big data Technology Application forUrban Infrastructure School ofArtificial Intelligence and Big DataHefei UniversityHefei230601China institute of Applied Optimization School of Artificial Intelligence and Big DataHefei UniversityHefei230601China

Depth estimation is an important task in computer *** data at scale for monocular depth estimation is challenging,as this task requires simultaneously capturing RGB images and depth ***,data augmentation is crucial for this *** data augmentationmethods often employ pixel-wise transformations,whichmay inadvertently disrupt edge *** this paper,we propose a data augmentationmethod formonocular depth estimation,which we refer to as the Perpendicular-Cutdepth *** method involves cutting realworld depth maps along perpendicular directions and pasting them onto input images,thereby diversifying the data without compromising edge *** validate the effectiveness of the algorithm,we compared it with existing convolutional neural network(CNN)against the current mainstream data augmentation ***,to verify the algorithm’s applicability to Transformer networks,we designed an encoder-decoder network structure based on Transformer to assess the generalization of our proposed *** results demonstrate that,in the field of monocular depth estimation,our proposed method,Perpendicular-Cutdepth,outperforms traditional data *** the indoor dataset NYU,our method increases accuracy from0.900 to 0.907 and reduces the error rate from0.357 to *** the outdoor dataset KITTI,our method improves accuracy from 0.9638 to 0.9642 and decreases the error rate from 0.060 to 0.0598.

关键词： Perpendicular depth estimation data augmentation

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Effects of vacancy and external electric field on the electronic properties of the MoSi_(2)N_(4)/graphene heterostructure

引用

Chinese Physics B 2024年第3期33卷 542-550页

作者：梁前罗祥燕钱国林王远帆梁永超谢泉 College of big data and Information Engineering Institute of New Optoelectronic Materials and TechnologyGuizhou UniversityGuiyang 550025China

Recently,the newly synthesized septuple-atomic layer two-dimensional(2D)material MoSi_(2)N_(4)(MSN)has attracted attention *** work delves into the effect of vacancies and external electric fields on the electronic properties of the MSN/graphene(Gr)heterostructure using first-principles *** find that four types of defective structures,N-in,N-out,Si and Mo vacancy defects of monolayer MSN and MSN/Gr heterostructure are stable in ***,vacancy defects can effectively modulate the charge transfer at the interface of the MSN/Gr heterostructure as well as the work function of the pristine monolayer MSN and MSN/Gr ***,the application of an external electric field enables the dynamic switching between n-type and p-type Schottky *** work may offer the possibility of exceeding the capabilities of conventional Schottky diodes based on MSN/Gr heterostructures.

关键词： MoSi_(2)N_(4) vacancy defects external electric field Schottky contacts

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

An Improved Northern Goshawk Optimization Algorithm for Feature Selection

引用

Journal of Bionic Engineering 2024年第4期21卷 2034-2072页

作者： Rongxiang Xie Shaobo Li Fengbin Wu State Key Laboratory of Public big data College of Computer Science and TechnologyGuizhou UniversityGuiyang550025China State Key Laboratory of Public big data Guizhou UniversityGuiyang550025China

Feature Selection(FS)is an important data management technique that aims to minimize redundant information in a *** work proposes DENGO,an improved version of the Northern Goshawk Optimization(NGO),to address the FS *** NGO is an efficient swarm-based algorithm that takes its inspiration from the predatory actions of the northern *** order to overcome the disadvantages that NGO is prone to local optimum trap,slow convergence speed and low convergence accuracy,two strategies are introduced in the original NGO to boost the effectiveness of ***,a learning strategy is proposed where search members learn by learning from the information gaps of other members of the population to enhance the algorithm's global search ability while improving the population ***,a hybrid differential strategy is proposed to improve the capability of the algorithm to escape from the trap of the local optimum by perturbing the individuals to improve convergence accuracy and *** prove the effectiveness of the suggested DENGO,it is measured against eleven advanced algorithms on the CEC2015 and CEC2017 benchmark functions,and the obtained results demonstrate that the DENGO has a stronger global exploration capability with higher convergence performance and ***,the proposed DENGO is used for FS,and the 29 benchmark datasets from the UCL database prove that the DENGO-based FS method equipped with higher classification accuracy and stability compared with eight other popular FS methods,and therefore,DENGO is considered to be one of the most prospective FS ***'s code can be obtained at https://***/matlabcentral/fileexchange/158811-project1.

关键词： Northern goshawk optimization Learning strategy Hybrid differential strategy Numerical optimization Feature selection

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Blockchain-Based Key Management Scheme Using Rational Secret Sharing

引用

Computers, Materials & Continua 2024年第4期79卷 307-328页

作者： Xingfan Zhao Changgen Peng Weijie Tan Kun Niu State Key Laboratory of Public big data College of Computer Science and TechnologyGuizhou UniversityGuiyang550025China Guizhou big data Academy Guizhou UniversityGuiyang550025China

Traditional blockchain key management schemes store private keys in the same location,which can easily lead to security issues such as a single point of ***,decentralized threshold key management schemes have become a research focus for blockchain private key *** security of private keys for blockchain user wallet is highly related to user identity authentication and digital asset *** threshold blockchain private key management schemes based on verifiable secret sharing have made some progress,but these schemes do not consider participants’self-interested behavior,and require trusted nodes to keep private key fragments,resulting in a narrow application scope and low deployment efficiency,which cannot meet the needs of personal wallet private key escrow and recovery in public *** design a private key management scheme based on rational secret sharing that considers the self-interest of participants in secret sharing protocols,and constrains the behavior of rational participants through reasonable mechanism design,making it more suitable in distributed scenarios such as the public *** proposed scheme achieves the escrow and recovery of personal wallet private keys without the participation of trusted nodes,and simulate its implementation on smart *** to other existing threshold wallet solutions and keymanagement schemes based on password-protected secret sharing(PPSS),the proposed scheme has a wide range of applications,verifiable private key recovery,low communication overhead,higher computational efficiency when users perform one-time multi-key escrow,no need for trusted nodes,and personal rational constraints and anti-collusion attack capabilities.

关键词： Blockchain smart contract rational secret sharing key management

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Theoretical Exploration of Alloying Effects on Stabilities and Mechanical Properties ofγʹPhase in Novel Co–Al–Nb-Base Superalloys

引用

Acta Metallurgica Sinica(English Letters) 2024年第7期37卷 1238-1248页

作者： Guan-Cheng Gu Zhao-Jing Han Ze-Yu Chen Zhao-Xuan Li Sheng-Bao Xia Zheng-Ning Li Hua Jin Wei-Wei Xu Xing-Jun Liu Shenzhen Research institute of Xiamen University School of Aerospace EngineeringXiamen UniversityXiamen361005China institute of Materials Genome and big data Harbin Institute of TechnologyShenzhen518055China

The new developedγ/γʹCo–Al–Nb-base alloys show great potentials as high-temperature ***,finding appropriate compositions to improve performance of alloys still poses a great challenge to the development of Co–Al–Nb-base *** by the lack of alloying effects on fundamental properties of criticalγʹphase,we systematically performed a theoretical investigation on the effect of alloying elements TM(TM:Ti,V,Cr,Zr,Mo,Ta,W,Re,and Ru)on phase stabilities and mechanical properties of L1_(2)-typeγʹ(Co,Ni)_(3)(Al,Nb).By analyzing the stability ofγʹphase with respect to its competitive B2 and D0_(19) phases,the results shown that Ti,V,and Cr enhance the L1_(2) stability and widen the L1_(2)–D0_(19) energy barrier,in which V yields the maximum *** analysis of electronic structure indicated that the alternation of valence electrons at fermi level would be the atomic origin for doping TM inγʹ*** calculated results of mechanical properties shown that V and Cr are expected to be optimal dopant for enhancing the strength and the ductility ofγʹ*** addition of Ta is also beneficial for enhancing the strength at the slight expense of ductility ofγʹ*** drawing the mechanical maps,the preferred composition range for the phases with desired properties is roughly demarcated in theory for the multi-addition of V/Cr and V/Ta inγʹ*** findings would be useful for optimizing the performance of novelγ/γʹCo–Al–Nb-base superalloys.

关键词： Co-Al-Nb-base superalloys γ/γʹdual-phase Phase stability Mechanical properties First-principle methods

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

A Survey of LLM datasets:From Autoregressive Model to AI Chatbot

引用

Journal of Computer Science & Technology 2024年第3期39卷 542-566页

作者：杜非马新建杨婧如柳熠罗超然王学斌姜海鸥景翔 National Key Laboratory of data Space Technology and System Beijing 100195China advanced institute of big data Beijing 100195China Fu Foundation School of Engineering and Applied Science Columbia UniversityNY 10027U.S.A. School of Software and Microelectronics Peking UniversityBeijing 100091China CCF IEEE

Since OpenAI opened access to ChatGPT,large language models(LLMs)become an increasingly popular topic attracting researchers’attention from abundant ***,public researchers meet some problems when developing LLMs given that most of the LLMs are produced by industries and the training details are typically *** datasets are an important setup of LLMs,this paper does a holistic survey on the training datasets used in both the pre-train and fine-tune *** paper first summarizes 16 pre-train datasets and 16 fine-tune datasets used in the state-of-the-art ***,based on the properties of the pre-train and fine-tune processes,it comments on pre-train datasets from quality,quantity,and relation with models,and comments on fine-tune datasets from quality,quantity,and *** study then critically figures out the problems and research trends that exist in current LLM *** study helps public researchers train and investigate LLMs by visual cases and provides useful comments to the research community regarding data *** the best of our knowledge,this paper is the first to summarize and discuss datasets used in both autoregressive and chat *** survey offers insights and suggestions to researchers and LLM developers as they build their models,and contributes to the LLM study by pointing out the existing problems of LLM studies from the perspective of data.

关键词： large language model(LLM) autoregressive model AI chatbot natural language processing(NLP)corpora OpenAI

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Discriminatively Constrained Semi-Supervised Multi-View Nonnegative Matrix Factorization with Graph Regularization

引用

big data Mining and Analytics 2024年第1期7卷 55-74页

作者： Guosheng Cui Ye Li Jianzhong Li Jianping Fan Shenzhen institute of advanced Technology Chinese Academy of SciencesShenzhen 518055China Joint Engineering Research Center for Health big data Intelligent Analysis Technology Shenzhen 518055China University of Chinese Academy of Sciences Beijing 100049China School of Computer Science and Control Engineering Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Nonnegative Matrix Factorization(NMF)is one of the most popular feature learning technologies in the field of machine learning and pattern *** has been widely used and studied in the multi-view clustering tasks because of its *** study proposes a general semi-supervised multi-view nonnegative matrix factorization *** algorithm incorporates discriminative and geometric information on data to learn a better-fused representation,and adopts a feature normalizing strategy to align the different *** specific implementations of this algorithm are developed to validate the effectiveness of the proposed framework:Graph regularization based Discriminatively Constrained Multi-View Nonnegative Matrix Factorization(GDCMVNMF)and Extended Multi-View Constrained Nonnegative Matrix Factorization(ExMVCNMF).The intrinsic connection between these two specific implementations is discussed,and the optimization based on multiply update rules is *** on six datasets show that the effectiveness of GDCMVNMF and ExMVCNMF outperforms several representative unsupervised and semi-supervised multi-view NMF approaches.

关键词： multi-view semi-supervised clustering discriminative information geometric information feature normalizing strategy

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Time-sensitive prediction of NO_(2) concentration in China using an ensemble machine learning model from multi-source data

引用

Journal of Environmental Sciences 2024年第3期137卷 30-40页

作者： Chenliang Tao Man Jia Guoqiang Wang Yuqiang Zhang Qingzhu Zhang Xianfeng Wang Qiao Wang Wenxing Wang big data Research Center for Ecology and Environment Environment Research InstituteShandong UniversityQingdao 266237China Shandong Provincial Eco-environment Monitoring Center Jinan 250101China

Nitrogen dioxide(NO_(2))poses a critical potential risk to environmental quality and public health.A reliable machine learning(ML)forecasting framework will be useful to provide valuable information to support government *** on the data from1609 air quality monitors across China from 2014-2020,this study designed an ensemble ML model by integrating multiple types of spatial-temporal variables and three sub-models for time-sensitive prediction over a wide *** ensemble ML model incorporates a residual connection to the gated recurrent unit(GRU)network and adopts the advantage of Transformer,extreme gradient boosting(XGBoost)and GRU with residual connection network,resulting in a 4.1%±1.0%lower root mean square error over XGBoost for the test *** ensemble model shows great prediction performance,with coefficient of determination of 0.91,0.86,and 0.77 for 1-hr,3-hr,and 24-hr averages for the test results,*** particular,this model has achieved excellent performance with low spatial uncertainty in Central,East,and North China,the major site-dense *** the interpretability analysis based on the Shapley value for different temporal resolutions,we found that the contribution of atmospheric chemical processes is more important for hourly predictions compared with the daily scale predictions,while the impact of meteorological conditions would be ever-prominent for the *** with existing models for different spatiotemporal scales,the present model can be implemented at any air quality monitoring station across China to facilitate achieving rapid and dependable forecast of NO_(2),which will help developing effective control policies.

关键词： Air quality prediction Deep learning Ensemble method Nitrogen dioxide Spatiotemporal covariates

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：