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Architecture Design and Interface Engineering of Self-assembly VS_(4)/rGO Heterostructures for Ultrathin Absorbent

Nano-Micro Letters 2022年第4期14卷 222-237页

作者： Qi Li Xuan Zhao Zheng Zhang Xiaochen Xun Bin Zhao Liangxu Xu Zhuo Kang Qingliang Liao Yue Zhang Academy for Advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringBeijing Key Laboratory for Advanced Energy Materials and TechnologiesSchool of Materials Science and EngineeringUniversity of Science

The employment of microwave absorbents is highly desirable to address the increasing threats of electromagnetic pollution.Importantly,developing ultrathin absorbent is acknowledged as a linchpin in the design of lightweight and flexible electronic devices,but there are remaining unprecedented challenges.Herein,the self-assembly VS_(4)/rGO heterostructure is constructed to be engineered as ultrathin microwave absorbent through the strategies of architecture design and interface engineering.The microarchitecture and heterointerface of VS_(4)/rGO heterostructure can be regulated by the generation of VS_(4) nanorods anchored on rGO,which can effectively modulate the impedance matching and attenuation constant.The maximum reflection loss of 2VS_(4)/rGO40 heterostructure can reach−43.5 dB at 14 GHz with the impedance matching and attenuation constant approaching 0.98 and 187,respectively.The effective absorption bandwidth of 4.8 GHz can be achieved with an ultrathin thickness of 1.4 mm.The far-reaching comprehension of the heterointerface on microwave absorption performance is explicitly unveiled by experimental results and theoretical calculations.Microarchitecture and heterointerface synergistically inspire multi-dimensional advantages to enhance dipole polarization,interfacial polarization,and multiple reflections and scatterings of microwaves.Overall,the strategies of architecture design and interface engineering pave the way for achieving ultrathin and enhanced microwave absorption materials.

关键词： Architecture design Interface Self-assembly Microwave absorption

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Bayesian Deep Learning for Dynamic Power System State Prediction Considering Renewable Energy Uncertainty

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Journal of Modern Power Systems and Clean Energy 2022年第4期10卷 913-922页

作者： Shiyao Zhang James J.Q.Yu academy for advanced interdisciplinary Studies Southern University of Science and TechnologyShenzhen 518055China Department of Computer science and Engineering Southern University of Science and TechnologyShenzhen 518055China

Modern power systems are incorporated with distributed energy sources to be environmental-friendly and costeffective.However,due to the uncertainties of the system integrated with renewable energy sources,effective strategies need to be adopted to stabilize the entire power systems.Hence,the system operators need accurate prediction tools to forecast the dynamic system states effectively.In this paper,we propose a Bayesian deep learning approach to predict the dynamic system state in a general power system.First,the input system dataset with multiple system features requires the data pre-processing stage.Second,we obtain the dynamic state matrix of a general power system through the Newton-Raphson power flow model.Third,by incorporating the state matrix with the system features,we propose a Bayesian long short-term memory(BLSTM)network to predict the dynamic system state variables accurately.Simulation results show that the accurate prediction can be achieved at different scales of power systems through the proposed Bayesian deep learning approach.

关键词： Bayesian deep learning data analytics NewtonRaphson power flow renewable energy source system state

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Service behavior of triboelectric nanogenerators:Bridging the gap between prototypes and applications

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Nano Research 2023年第9期16卷 11731-11752页

作者： Fangfang Gao Xiaochen Xun Xuan Zhao Liangxu Xu Qi Li Bin Zhao Tian Ouyang Qingliang Liao Yue Zhang Academy for Advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory for advanced Energy Materials and Technologies School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

The triboelectric nanogenerators(TENGs),suppling power for freely mobile and distributed electronic equipment from Internet of Things,have been considered as“the energy for the new era”.Research on the service behavior has become increasingly important for achieving the reliability evaluation and life prediction of TENGs,as TENGs advance from prototypes to practical applications.Due to the wide selection of materials,the diversity of device structures,and the complexity of working environment,TENGs show unique characteristics in the service behavior.These dilemmas lead to the fact that systematical summary of service behavior for TENGs is still in its infancy.Here,the progresses of the service behavior for TENGs are comprehensively reviewed from the influence of environmental factors on the service performance of TENGs to the impact of TENGs during the service on their surroundings.We summed up the performance evolution of TENGs in the real environment and the reproducibility of TENGs of which the electrical output will be restored after failure.Then,the service adaptability of TENG is systematically discussed,including the biological and environmental compatibility.Finally,the challenges and opportunities that the related research faced are proposed to promote the emerging technology from laboratory to factory.

关键词： triboelectric nanogenerator self-powered sensor service behavior environmental influence

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Dynamic behavior of tunneling triboelectric charges in two-dimensional materials

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International Journal of Minerals,Metallurgy and Materials 2023年第9期30卷 1801-1808页

作者： Xuan Zhao Liangxu Xu Xiaochen Xun Fangfang Gao Qingliang Liao Yue Zhang Academy for Advanced Interdisciplinary Science and Technology School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China Beijing advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory for Advanced Energy Materials and TechnologiesUniversity of Science and Technology BeijingBeijing 100083China

Although the research history of triboelectrification has been more than 2000 years, there are still many problems to be solved so far.The use of scanning probe microscopy provides an important way to quantitatively study the transfer, accumulation, and dissipation of triboelectric charges in the process of triboelectrification. Two-dimensional materials are considered to be key materials for new electronic devices in the post-Moore era due to their atomic-scale size advantages. If the electrostatic field generated by triboelectrification can be used to replace the traditional gate electrostatic field, it is expected to simplify the structure of two-dimensional electronic devices and reconfigure them at any time according to actual needs. Here, we investigate the triboelectrification process of various two-dimensional materials such as MoS_(2), WSe_(2),and ZnO. Different from traditional bulk materials, after two-dimensional materials are rubbed, the triboelectric charges generated may tunnel through the two-dimensional materials to the underlying substrate surface. Because the tunneling triboelectric charge is protected by the twodimensional material, its stable residence time on the substrate surface can reach more than 7 days, which is more than tens of minutes for the traditional triboelectric charge. In addition, the electrostatic field generated by the tunneling triboelectric charge can effectively regulate the carrier transport performance of two-dimensional materials, and the source–drain current of the field effect device regulated by the triboelectric floating gate is increased by nearly 60 times. The triboelectric charge tunneling phenomenon in two-dimensional materials is expected to be applied in the fields of new two-dimensional electronic devices and reconfigurable functional circuits.

关键词： two-dimensional materials triboelectric charge dynamic behavior reconfigurable electronics

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用于高性能二维范德华器件和规模化集成的无机分子晶体介电薄膜

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science Bulletin 2022年第10期67卷 1010-1012页

作者：张跃 Academy for Advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory for advanced Energy Materials and Technologies School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Two-dimensional(2D)materials,such as graphene,h-BN,and MoS_(2),and their van der Waals(vdW)heterostructures attracted tremendous research interests in the past decade for their intriguing properties at atomic thinness.2D materials not only offered a great platform for the fundamental research,but also brought promising application potentials in novel van der Waals electronic and optoelectronic[1-5].

关键词：介电薄膜 electronic graphene

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Flexible electronics and optoelectronics of 2D van der Waals materials

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International Journal of Minerals,Metallurgy and Materials 2022年第4期29卷 671-690页

作者： Huihui Yu Zhihong Cao Zheng Zhang Xiankun Zhang Yue Zhang Academy for Advanced Interdisciplinary Science and Technology School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China Beijing advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory for Advanced Energy Materials and TechnologiesUniversity of Science and Technology BeijingBeijing 100083China

Flexible electronics and optoelectronics exhibit inevitable trends in next-generation intelligent industries,including healthcare and wellness,electronic skins,the automotive industry,and foldable or rollable displays.Traditional bulk-material-based flexible devices considerably rely on lattice-matched crystal structures and are usually plagued by unavoidable chemical disorders at the interface.Two-dimensional van der Waals materials(2D VdWMs)have exceptional multifunctional properties,including large specific area,dangling-bond-free interface,plane-to-plane van der Waals interactions,and excellent mechanical,electrical,and optical properties.Thus,2D VdWMs have considerable application potential in functional intelligent flexible devices.To utilize the unique properties of 2D VdWMs and their van der Waals heterostructures,new designs and configurations of electronics and optoelectronics have emerged.However,these new designs and configurations do not consider lattice mismatch and process incompatibility issues.In this review,we summarized the recently reported 2D VdWM-based flexible electronic and optoelectronic devices with various functions thoroughly.Moreover,we identified the challenges and opportunities for further applications of 2D VdWM-based flexible electronics and optoelectronics.

关键词： two-dimensional van der Waals material two-dimensional van der Waals heterostructure flexible electronics flexible optoelectronics

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Design and tailoring of patterned ZnO nanostructures for perovskite light absorption modulation

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International Journal of Minerals,Metallurgy and Materials 2024年第5期31卷 855-861页

作者： Haonan Si Xuan Zhao Qingliang Liao Yue Zhang Academy for Advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China Key Laboratory of advanced Materials and Devices for Post-Moore Chips Ministry of EducationBeijing Key Laboratory for Advanced Energy Materials and TechnologiesSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Lithography is a pivotal micro/nanomanufacturing technique,facilitating performance enhancements in an extensive array of devices,encompassing sensors,transistors,and photovoltaic devices.The key to creating highly precise,multiscale-distributed patterned structures is the precise control of the lithography process.Herein,high-quality patterned ZnO nanostructures are constructed by systematically tuning the exposure and development times during lithography.By optimizing these parameters,ZnO nanorod arrays with line/hole arrangements are successfully prepared.Patterned ZnO nanostructures with highly controllable morphology and structure possess discrete three-dimensional space structure,enlarged surface area,and improved light capture ability,which achieve highly efficient energy conversion in perovskite solar cells.The lithography process management for these patterned ZnO nanostructures provides important guidance for the design and construction of complex nanostructures and devices with excellent performance.

关键词： lithography patterned ZnO nanorod arrays light absorption perovskite solar cell

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Application of neutron imaging in observing various states of matter inside lithium batteries

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National science Review 2023年第11期10卷 192-208页

作者： Lei Gao Songbai Han Haijin Ni Jinlong Zhu Liping Wang Song Gao Yonggang Wang Dubin Huang Yusheng Zhao Ruqiang Zou School of Materials science and Engineering Peking University academy for advanced interdisciplinary Studies Southern University of Science and Technology Department of Physics Southern University of Science and Technology Eastern Institute for advanced Study

Lithium batteries have been essential technologies and become an integral part of our daily lives, powering a range of devices from phones to electric vehicles. To fully understand and optimize the performance of lithium batteries, it is necessary to investigate their internal states and processes through various characterization methods. Neutron imaging has been an indispensable complementary characterization technique to X-ray imaging or electron microscopy because of the unique interaction principle between neutrons and matter. It provides particular insights into the various states of matter inside lithium batteries,including the Li+concentration in solid electrodes, the Li plating/stripping behavior of Li-metal anodes,the Li+diffusion in solid ionic conductors, the distribution of liquid electrolytes and the generation of gases.This review aims to highlight the capabilities and advantages of neutron imaging in characterizing lithium batteries, as well as its current state of application in this field. Additionally, we discuss the potential of neutron imaging to contribute to the ongoing development of advanced batteries through its ability to visualize internal evolution.

关键词： lithium battery neutron imaging electrodes electrolytes

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A historical overview of nano-optics:From near-field optics to plasmonics

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Chinese Physics B 2024年第5期33卷 134-145页

作者：邓妙怡朱星 Department of History of science Technology and MedicineAcademy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100871China School of Physics Peking UniversityBeijing 100871China

Nano-optics is an emergent research field in physics that appeared in the 1980s,which deals with light–matter optical interactions at the nanometer scale.In early studies of nano-optics,the main concern focus is to obtain higher optical resolution over the diffraction limit.The researches of near-field imaging and spectroscopy based on scanning near-field optical microscopy(SNOM)are developed.The exploration of improving SNOM probe for near-field detection leads to the emergence of surface plasmons.In the sense of resolution and wider application,there has been a significant transition from seeking higher resolution microscopy to plasmonic near-field modulations in the nano-optics community during the nano-optic development.Nowadays,studies of nano-optics prefer the investigation of plasmonics in different material systems.In this article,the history of the development of near-field optics is briefly reviewed.The difficulties of conventional SNOM to achieve higher resolution are discussed.As an alternative solution,surface plasmons have shown the advantages of higher resolution,wider application,and flexible nano-optical modulation for new devices.The typical studies in different periods are introduced and characteristics of nano-optics in each stage are analyzed.In this way,the evolution progress from near-field optics to plasmonics of nano-optics research is presented.The future development of nano-optics is discussed then.

关键词： nano-optics near-field optics surface plasmon plasmonic modulation

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Silicon-processes-compatible contact engineering for twodimensional materials integrated circuits

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Nano Research 2023年第11期16卷 12471-12490页

作者： Li Gao Zhangyi Chen Chao Chen Xiankun Zhang Zheng Zhang Yue Zhang Academy for Advanced Interdisciplinary Science and Technology Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China School of Materials science and Engineering Peking UniversityBeijing 100871China Key Laboratory of advanced Materials and Devices for Post-Moore Chips Ministry of EducationUniversity of Science and Technology BeijingBeijing 100083China

Two-dimensional(2D)semiconductors,especially transition metal dichalcogenides(TMDCs),have been proven to be excellent channel materials for the next-generation integrated circuit(IC).However,the contact problem between 2D TMDCs and metal electrodes has always been one of the main factors restricting their development.In this review,we summarized recent work on 2D TMDCs contact from the perspective of compatible integration with silicon processes and practical application requirements,including the contact performance evaluation indicators,special challenges encountered in 2D TMDCs,and recent optimization methods.Specifically,we sorted out and highlighted the performance indicators of 2D TMDCs contacts,including contact resistance(RC),contact scaling,contact stability,and contact electrical/thermal conductivity.Special challenges of 2D TMDCs and metal contact,such as severe Fermi level pinning,large RC,and difficult doping,are systematically discussed.Furthermore,typical methods for optimizing 2D TMDCs RC,edge contact strategies for scaling contact lengths,and solutions for improving contact stability are reviewed.Based on the current research and problems,the development direction of 2D TMDCs contacts that meet the silicon-based compatible process and application performance requirements is proposed.

关键词： two-dimensional(2D)semiconductors transition metal dichalcogenides field effect transistors contact engineering

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