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Metal-to-insulator transitions in 3d-band correlated oxides containing Fe compositions

International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 48-59页

作者： Yiping Yu Yuchen Cui Jiangang He Wei Mao Jikun Chen Key Laboratory of Advanced Materials and Devices for Post-Moore Chips Ministry of EducationUniversity of Science and Technology BeijingBeijing 100083China School of Materials science and Engineering University of Science and Technology BeijingBeijing 100083China Institute of Industrial science The University of Tokyo4-6-1 KomabaMeguro-kuTokyo 153-8505Japan

Metal-to-insulator transitions (MITs),which are achieved in 3d-band correlated transitional metal oxides,trigger abrupt variations in electrical,optical,and/or magnetic properties beyond those of conventional *** such material families,iron(Fe:3d^(6)4s^(2))-containing oxides pique interest owing to their widely tunable MIT properties,which are associated with the various valence states of *** potential electronic applications also show promise,given the large abundance of Fe on *** MIT properties triggered by critical temperature (TMIT) were reported for ReFe_(2)O_(4)(Fe^(2.5+)),ReBaFe_(2)O_(5)(Fe^(2.5+)),Fe_(3)O_(4)(Fe^(2.67+)),Re_(1/3)Sr_(2/3)FeO_(3)(Fe^(3.67+)),Re Cu_(3)Fe_(4)O_(12)(Fe^(3.75+)),and Ca_(1-x)Sr_(x)FeO_(3)(Fe^(4+))(where Re represents rare-earth elements).The common feature of MITs of these Fe-containing oxides is that they are usually accompanied by charge ordering transitions or disproportionation associated with the valence states of ***,we review the material family of Fe-containing MIT oxides,their MIT functionalities,and their respective *** the perspective of potentially correlated electronic applications,the tunability of the TMITand its resultant resistive change in Fe-containing oxides are summarized and further compared with those of other materials exhibiting MIT *** particular,we highlight the abrupt MIT and wide tunability of TMITof Fe-containing quadruple perovskites,such as Re ***,their effective material synthesis still needs to be further explored to cater to potential applications.

关键词： metal-to-insulator transitions Fe-containing oxides charge ordering charge disproportionation

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Journal of Computer science & technology 2024年第1期39卷 63-81页

作者：陈章玉华宇左鹏飞孙园园郭云程 Wuhan National Laboratory for Optoelectronics School of Computer Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China

Image bitmaps,i.e.,data containing pixels and visual perception,have been widely used in emerging applica-tions for pixel operations while consuming lots of memory space and *** with legacy DRAM(dynamic ran-dom access memory),non-volatile memories(NVMs)are suitable for bitmap storage due to the salient features of high density and intrinsic ***,writing NVMs suffers from higher energy consumption and latency compared with read *** precise or approximate compression schemes in NVM controllers show limited performance for bitmaps due to the irregular data patterns and variance in *** observe the pixel-level similarity when writing bitmaps due to the analogous contents in adjacent *** exploiting the pixel-level similarity,we propose SimCom,an approximate similarity-aware compression scheme in the NVM module controller,to efficiently compress data for each write access *** idea behind SimCom is to compress continuous similar words into the pairs of base words with *** storage costs for small runs are further mitigated by reusing the least significant bits of base *** adaptively selects an appropriate compression mode for various bitmap formats,thus achieving an efficient trade-off be-tween quality and memory *** implement SimCom on GEM5/zsim with NVMain and evaluate the perfor-mance with real-world image/video *** results demonstrate the efficacy and efficiency of our SimCom with an efficient quality-performance trade-off.

关键词： approximate computing data compression memory architecture non-volatile memory

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WeldNet:A voxel-based deep learning network for point cloud annular weld seam detection

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science China(Technological sciences) 2024年第4期67卷 1215-1225页

作者： WANG Hui RONG YouMin XU JiaJun XIANG SongMing PENG YiFan HUANG Yu State Key Laboratory of Intelligent Manufacturing Equipment and technology Huazhong University of Science and TechnologyWuhan 430074China School of Mechanical science and Engineering Huazhong University of Science and TechnologyWuhan 430074China

Weld seam detection is an important part of automated *** present,few studies have been conducted on annular weld seams,and a lot of defects exist in the point cloud model of the tube sheet obtained by RGB-D cameras and photography *** at the above problems,this paper proposed an annular weld seam detection network named WeldNet where a voxel feature encoding layer was adaptively improved for annular weld seams,the sparse convolutional network and region proposal network(RPN)were used to detect annular weld seam position,and an annular weld seam detection loss function was ***,an annular weld seam dataset was established to train the *** with the random sampling consistency(RANSAC)method,WeldNet has a higher detection accuracy,as well as a higher detection success rate which has increased by 23%.Compared with U-Net,WeldNet has been proven to achieve a better detection result,and the intersection over the union of the weld seam detection is improved by 17.8%.

关键词： deep learning point cloud weld seam detection welding annular weld seam

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Research Progress on Bionic Water Strider Robots

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Journal of Bionic Engineering 2024年第2期21卷 635-652页

作者： Jianhao Liu Mingjun Shen Ziqiang Ma Xinping Zhou School of Mechanical science and Engineering Huazhong University of Science and TechnologyWuhan430074China State Key Laboratory of Intelligent Manufacturing Equipment and technology Huazhong University of Science and TechnologyWuhan430074China

Biological water striders have advantages such as flexible movement,low disturbance to the water surface,and low *** have developed a large number of biomimetic water strider robots based on their movement mechanism,which have broad application prospects in water quality testing,water surface reconnaissance,and *** article mainly reviews the research progress of biomimetic water strider ***,the biological and kinematic characteristics of water striders are outlined,and some mechanical parameters of biological water striders are *** basic equations of water strider movement are then ***,an overview is given of the past and current work on skating and jumping movements of biomimetic water strider robots based on surface tension and water pressure *** on the current research status of biomimetic water strider robots,the shortcomings of current research on biomimetic water striders are summarized,and the future development of biomimetic water strider robots is *** article provides new insights for the design of biomimetic water strider robots.

关键词： Bionics Water strider Robot Motion of robots on water surface

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A Li_(3)P nanoparticle dispersion strengthened ultrathin Li metal electrode for high energy density rechargeable batteries

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Nano Research 2024年第5期17卷 4031-4038页

作者： Lin Fu Xiancheng Wang Bao Zhang Zihe Chen Yuanjian Li Yongming Sun Provincial Guizhou Key Laboratory of Green Chemical and Clean Energy technology School of Chemistry and Chemical EngineeringGuizhou UniversityGuiyang 550025China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China School of Physical and Mathematical sciences Nanyang Technological UniversitySingapore 637371Singapore Institute of Materials Research and Engineering Agency for Science Technology and Research(A*STAR)Singapore 138634Singapore

Achievement of lithium(Li)metal anode with thin thickness(e.g.,≤30µm)is highly desirable for rechargeable high energy density ***,the fabrication and application of such thin Li metal foil electrode remain challenging due to the poor mechanical processibility and inferior electrochemical performance of metallic ***,mechanico-chemical synthesis of robust ultrathin Li/Li_(3)P(LLP)composite foils(~15µm)is demonstrated by employing repeated mechanical rolling/stacking operations using red P and metallic Li as raw *** in-situ formed Li+-conductive Li_(3)P nanoparticles in metallic Li matrix and their tight bonding strengthen the mechanical durability and enable the successful fabrication of free-standing ultrathin Li metal composite ***,it also reduces the electrochemical Li nucleation barrier and homogenizes Li plating/stripping *** matching to high-voltage LiCoO_(2),the full cell with a low negative/positive(N/P)capacity ratio of~1.5 offers a high energy density of~522 W·h·kg^(-1) at 0.5 C based on the mass of cathode and *** into account its facile manufacturing,potentially low cost,and good electrochemical performance,we believe that such an ultrathin composite Li metal foil design with nanoparticle-dispersion-strengthened mechanism may boost the development of high energy density Li metal batteries.

关键词： lithium metal anode high energy density battery mechanico-chemical synthesis ultrathin Li/Li_(3)P composite foil low negative/positive capacity ratio

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Enhanced Differentiable Architecture Search Based on Asymptotic Regularization

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Computers, Materials & Continua 2024年第2期78卷 1547-1568页

作者： Cong Jin Jinjie Huang Yuanjian Chen Yuqing Gong School of Computer science and technology Harbin University of Science and TechnologyHarbin150006China School of Automation Harbin University of Science and TechnologyHarbin150006China

In differentiable search architecture search methods,a more efficient search space design can significantly improve the performance of the searched architecture,thus requiring people to carefully define the search space with different complexity according to various *** rationalizing the search strategies to explore the well-defined search space will further improve the speed and efficiency of architecture *** this in mind,we propose a faster and more efficient differentiable architecture search method,***,we introduce a more efficient search space enriched by the introduction of two redefined convolution ***,we utilize a more efficient architectural parameter regularization method,mitigating the overfitting problem during the search process and reducing the error brought about by gradient ***,we introduce a natural exponential cosine annealing method to make the learning rate of the neural network training process more suitable for the search ***,group convolution and data augmentation are employed to reduce the computational ***,through extensive experiments on several public datasets,we demonstrate that our method can more swiftly search for better-performing neural network architectures in a more efficient search space,thus validating the effectiveness of our approach.

关键词： Differentiable architecture search allegro search space asymptotic regularization natural exponential cosine annealing

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Laser-assisted synthesis of PtPd alloy for efficient ethanol oxidation

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Nano Research 2024年第7期17卷 6032-6037页

作者： Zihang Chen Tong Liu Huijuan Zhang Beibei Pang Yuanhua Sun Longfei Hu Qiquan Luo Xiaokang Liu Linlin Cao Tao Yao School of Nuclear science and technology National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029China Institutes of Physical science and Information technology Anhui UniversityHefei 230601China

The inefficiency of ethanol oxidation reaction(EOR)presents a significant obstacle in harnessing renewable biofuels with high energy density into *** efforts,most Pt-based catalysts still suffer from drawbacks such as poor activity and susceptibility to CO poisoning,particularly in acidic ***,we employed a physical laser-assisted approach to synthetize a PtPd alloy with a 1:1 atomic *** alloy demonstrates remarkable performance in acidic EOR,boasting a high mass activity of 1.86 A·mgPt^(−1)and competitive resistance to *** in situ synchrotron radiation infrared spectroscopy with theoretical calculations,we reveal that the synergic interaction between Pt and Pd enhances both the adsorption of OH*intermediate and the dehydrogenation ability of *** work will prove the feasibility of synthesizing bimetallic alloys by a physical laser-assisted strategy and promote the development of advanced alloy electrocatalysts.

关键词： laser-assisted strategy Pt-based alloy in situ synchrotron radiation infrared spectroscopy ethanol oxidation reaction synergic interaction

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A Dual Discriminator Method for Generalized Zero-Shot Learning

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Computers, Materials & Continua 2024年第4期79卷 1599-1612页

作者： Tianshu Wei Jinjie Huang School of Computer science and technology Harbin University of Science and TechnologyHarbin150006China School of Automation Harbin University of Science and TechnologyHarbin150006China

Zero-shot learning enables the recognition of new class samples by migrating models learned from semanticfeatures and existing sample features to things that have never been seen before. The problems of consistencyof different types of features and domain shift problems are two of the critical issues in zero-shot learning. Toaddress both of these issues, this paper proposes a new modeling structure. The traditional approach mappedsemantic features and visual features into the same feature space;based on this, a dual discriminator approachis used in the proposed model. This dual discriminator approach can further enhance the consistency betweensemantic and visual features. At the same time, this approach can also align unseen class semantic features andtraining set samples, providing a portion of information about the unseen classes. In addition, a new feature fusionmethod is proposed in the model. This method is equivalent to adding perturbation to the seen class features,which can reduce the degree to which the classification results in the model are biased towards the seen *** the same time, this feature fusion method can provide part of the information of the unseen classes, improvingits classification accuracy in generalized zero-shot learning and reducing domain bias. The proposed method isvalidated and compared with othermethods on four datasets, and fromthe experimental results, it can be seen thatthe method proposed in this paper achieves promising results.

关键词： Generalized zero-shot learning modality consistent discriminator domain shift problem feature fusion

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Gas film/regenerative composite cooling characteristics of the liquid oxygen/liquid methane (LOX/LCH4) rocket engine

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Journal of Zhejiang University-science A(Applied Physics & Engineering) 2024年第8期25卷 631-649页

作者： Xinlin LIU Jun SUN Zhuohang JIANG Qinglian LI Peng CHENG Jie SONG science and technology on Scramjet Laboratory College of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China

The thermal protection of rocket engines is a crucial aspect of rocket engine *** this paper,the gas film/regenerative composite cooling of the liquid oxygen/liquid methane(LOX/LCH4)rocket engine thrust chamber was investigated.A gas film/regenerative composite cooling model was developed based on the Grisson gas film cooling efficiency formula and the one-dimensional regenerative cooling *** accuracy of the model was validated through experiments conducted on a 6 kg/s level gas film/regenerative composite cooling thrust ***,key parameters related to heat transfer performance were *** results demonstrate that the model is sufficiently accurate to be used as a preliminary design *** temperature rise error of the coolant,when compared with the experimental results,was found to be less than 10%.Although the pressure drop error is relatively large,the calculated results still provide valuable guidance for heat transfer *** addition,the performance of composite cooling is observed to be superior to regenerative *** the gas film flow rate results in higher cooling efficiency and a lower gas-side wall ***,the position at which the gas film is introduced greatly impacts the cooling *** optimal introduction position for the gas film is determined when the film is introduced from a single row of *** optimal introduction position results in a more uniform wall temperature distribution and reduces the peak ***,it is observed that a double row of holes,when compared to a single row of holes,enhances the cooling effect in the superposition area of the gas film and further lowers the gas-side wall *** results provide a basis for the design of gas film/regenerative composite cooling systems.

关键词： Liquid oxygen/liquid methane(LOX/LCH4)rocket engine Gas film cooling Regenerative cooling Heat transfer characteristics

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Better engineering layered vanadium oxides for aqueous zinc‐ion batteries: Going beyond widening the interlayer spacing

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SmartMat 2024年第1期5卷 83-109页

作者： Yue Guo Hanmei Jiang Binbin Liu Xingyang Wang Yifu Zhang Jianguo Sun John Wang Department of Materials science and Engineering National University of SingaporeSingaporeSingapore State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyDalianChina Institute of Materials Research and Engineering(IMRE) Agency for ScienceTechnology and Research(A*STAR)SingaporeSingapore

Aqueous zinc‐ion batteries(ZIBs)are regarded as among the most promising candidates for large‐scale grid energy storage,owing to their high safety,low costs,and environmental *** the past decade,vanadium oxides,which are exemplified by V2O5,have been widely developed as a class of cathode materials for ZIBs,where the relatively high theoretical capacity and structural stability are among the main ***,there are considerable challenges in the construction of vanadium‐based ZIBs with high capacity,long lifespan,and excellent rate *** widenings of the interlayer spacing in the layered vanadium oxides by pre‐intercalations appear to have reached their limitations in improving the energy density and other key performance parameters of ZIBs,although various metal ions(Na+,Ca2+,and Al3+)and even organic cations/groups have been ***,we discuss the advances made more recently,and also the challenges faced by the high‐performance vanadium oxides(V2O5‐based)cathodes,where there are several strategies to improve their electrochemical performance ranging from the new structural designs down to sub‐nano‐scopic/molecular/atomic levels,including cation pre‐intercalation,structural water optimization,and defect engineering,to macroscopic structural *** key principles for an optimal structural design of the V2O5‐based cathode materials for high energy density and fast‐charging aqueous ZIBs are examined,aiming at paving the way for developing energy storage designed for those large scales,high safety,and low‐cost systems.

关键词： aqueous zinc‐ion batteries cations pre‐intercalation defect engineering structural water vanadium oxides

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