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Effect of Y substitution on the microstructure,magneto-optical,and thermal properties of(Tb_(1−x)Y_(x))_(3)Al_(5)O_(12)transparent ceramics

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Journal of Advanced Ceramics 2024年第4期13卷 529-538页

作者： Lixuan Zhang Dianjun Hu Xiao Li Ziyu Liu Chen Hu Lexiang Wu Tingsong Li Dariusz Hreniak Jiang Li Transparent Ceramics research Center Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 201899China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou 341000China institute of low temperature and structure research Polish Academy of SciencesWroclaw 50-422Poland

Faraday isolators can prevent the front-end system from disturbance and damage caused by a back-reflected beam,so they are important elements in laser *** magneto-optical materials are the most important component in Faraday isolators,the studies on magneto-optical materials have attracted much attention these ***_(3)Al_(5)O_(12)(TAG)ceramics are considered to be one of the most promising magneto-optical materials for visible to near-infrared wavelength band application because of their outstanding comprehensive magneto-optical ***,the optical quality of TAG ceramics needs further optimization to meet the application *** this work,high optical quality(Tb_(1−x)Y_(x))_(3)Al_(5)O_(12)(x=0,0.05,0.1,0.2,and 0.3)magneto-optical ceramics were fabricated successfully by solid-state reaction sintering combined with hot isostatic pressing(HIP)*** the ceramics obtained showed a single garnet phase for different values of x in the range *** addition of Y_(2)O_(3) was found to suppress the secondary phase and improve optical quality *** ceramic samples obtained had clear grain boundaries and possessed the in-line transmittance values of 82.9%at 1064 nm and 82.2%at 633 nm,*** Verdet constants of(Tb_(1−x)Y_(x))_(3)Al_(5)O_(12)ceramics with x=0,0.05,0.1,0.2,and 0.3 were−188.1,−175.4,−168.5,−143.0,and−119.9 rad/(T·m),*** thermal conductivity of TAG ceramics was found to be 5.23 W/(m·K)at 25℃,and when 20%Y was substituted in place of Tb,the thermal conductivity decreased by only 9.4%.

关键词： (Tb_(1−x)Y_(x))_(3)Al_(5)O_(12)ceramics magneto-optical materials optical quality thermal properties

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Overcoming side reaction effects in the colloidal synthesis of ZnSe/ZnS core/shell quantum dots with an etching strategy

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Nano research 2024年第8期17卷 7020-7026页

作者： Jinhua He Chenhui Wang Mingrui Liu Muhammad Ramzan Zhiwei Long Xian-gang Wu Yu Chen Haizheng Zhong MIIT Key Laboratory for low-Dimensional Quantum structure and Devices School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Engineering research Center for Mixed Reality and Advanced Display Technology School of Optics and PhotonicsBeijing Institute of TechnologyBeijing 100081China

The potential use of large-size ZnSe quantum dots as blue emitters for display applications has greatly inspired the colloidal ***,we report the negative effects of side reactions of large-size ZnSe quantum *** side reactions between oleic acid and oleylamine generated amidation products and H_(2)O,which led to the hydrolysis of Zn(OA)2 to Zn(OH)2 and the subsequent formation of zinc oxide(ZnO)and zinc bis[diphenylphosphinate](Zn(DPPA)2)*** side reactions resulted in the formation of a defective surface including a Se-rich surface and oxygen-related *** negative effects can be overcome by adopting an etching strategy using potassium fluoride and myristic acid in *** overcoating a ZnS shell,blue emissive ZnSe/ZnS quantum dots with a maximum photoluminescence quantum yield of up to 91%were *** further fabricated ZnSe quantum dots-based blue light-emitting diodes with an emission peak at 456 *** device showed a turn-on voltage of 2.7 V with a maximum external quantum efficiency of 4.2%and a maximum luminance of 1223 cd·m^(−2).

关键词： quantum dots ZnSe side reactions surface etching light-emitting diodes

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Heat distribution model under hydrogen-rich low-carbon conditions in blast furnace

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Journal of Iron and Steel research International 2024年第3期31卷 584-594页

作者： Gang Wang Jun Xu Kun He Zhong-ping Zou Hao Bai School of Metallurgy and Ecological Engineering University of Science and Technology BeijingBeijing 100083China CISDI low-Carbon Blast Furnace research Office MCC Low-Carbon Technology Research InstituteChongqing 401122China

low carbon development of blast furnaces is one of the key technological directions in the current development of *** to the differences in the physical and chemical properties of hydrogen and carbon,hydrogen-rich media entering a blast furnace will change the heat distribution,thus affecting the stability of ***,a heat distribution model was proposed to study the temperature distribution in a blast furnace,simultaneously considering gas-solid heat exchange,slag and iron melting,and chemical *** model was used to analyze the temperature distribution of a 2300 m^(3) blast furnace and was verified via comparison with actual production ***,the effects of the injection rate of hydrogen-rich media,H2 concentration,and oxygen enrichment rate of the blast on the temperature distribution were *** indicated that the increase in the injection rate of the hydrogen-rich media decreased the amount of direct reduction and led to an increase in the furnace ***,an increase in the oxygen enrichment rate led to a decrease in the furnace temperature,but could reduce the solid fuel ratio,while the change in H2 concentration had less effect on the temperature *** combination of hydrogen-rich media injection and the increase in the oxygen enrichment rate would help to adjust the temperature distribution to the same level as the conventional blast furnace conditions.

关键词： Heat distribution Blast furnace low-carbon condition Hydrogen enrichment Calculation model

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High recorded color rendering performance of single-structured Ce,Mn:Y_(3)(Al,Sc)_(2)Al_(3)O_(12)phosphor ceramics for high-power white LEDs/LDs

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Journal of Advanced Ceramics 2024年第6期13卷 810-820页

作者： Xuanchu Liu Congcong Yang Yanbin Li Chang Min Jian Kang Tianyuan Zhou Chunming Zhou Chaofan Shi Cen Shao Bingheng Sun Wieslaw Strek Hao Chen Le Zhang Jiangsu Key Laboratory of Advanced Laser Materials and Devices School of Physics and Electronics EngineeringJiangsu Normal UniversityXuzhou 221116China Jiangsu Xiyi Advanced Materials research institute of Industrial Technology Xuzhou 221400China Xuzhou EAGLED Technology Co. Ltd.Xuzhou 221116China Xuzhou Kangna Advanced Materials Technology Co. Ltd.Xuzhou 221116China Shanghai institute of Optics Fine Mechanics Chinese Academy of SciencesShanghai 201800China institute of low temperature and structure research Polish Academy of SciencesWroclaw 50-422Poland State Key Laboratory of Crystal Materials Shandong UniversityJinan 250100China

Achieving a high color rendering index(CRI)and luminous stability in single-structured Ce:Y_(3)Al_(5)O_(12)(Ce:YAG)phosphor ceramics(PCs)is crucial for high-power white light-emitting diodes or laser diodes(LEDs/LDs).However,cyan valleys and insufficient amounts of the red component in the Ce:YAG emission spectra significantly limit their real *** this work,a series of Ce,Mn:Y_(3)(Al,Sc)_(2)Al_(3)O_(12)(Ce,Mn:YSAG)PCs were fabricated by vacuum sintering,and efficient spectral regulation was realized for full-color *** cyan valley was filled by the blueshifted emission peak of Ce^(3+)via Sc^(3+)*** orange‒red emission at approximately 580 nm was effectively supplemented via Mn^(2+)*** particular,CRI of Ce,Mn:YSAG increased from 56.4 to 85.8,a 52%increase compared with that of Ce:YAG under high-power LED excitation,and the operating temperature was stable at approximately 50℃for long working ***,CRI of 80.9 could still be obtained for PC-based white *** results indicated that Ce,Mn:YSAG PC,which has excellent CRI and luminous stability,is an extremely promising color convertor for high-power white LEDs/LDs.

关键词： color rendering index(CRI) color converter Ce:Y_(3)Al_(5)O_(12)(Ce:YAG)phosphor ceramics(PCs) high-power white light-emitting diodes or laser diodes(LEDs/LDs) luminous stability

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Microstructural evolution,mechanical properties and degradation mechanism of PS-PVD quasi-columnar thermal barrier coatings exposed to glassy CMAS deposits

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Rare Metals 2024年第7期43卷 3329-3340页

作者： Zi-Yue Yu Liang-Liang Wei Xing-Ye Guo Bao-Peng Zhang Qing He Hong-Bo Guo School of Materials Science and Engineering Beihang UniversityBeijing100191China Key Laboratory of High-temperature structure Materials and Protective Coatings(Ministry of Industry and Information Technology) Beihang UniversityBeijing 100191China Surface Engineering research institute Chinese Academy of Agricultural Mechanization SciencesBeijing 100083China

Thermal barrier coatings(TBCs) applied in aeroengines tend to be attacked by molten calcia-magnesiaalumino-silicate(CMAS) at high operating ***-stabilized zirconia(YSZ) coatings with quasicolumnar microstructure were fabricated by plasma spray physical vapor deposition(PS-PVD) *** chemic al changes,micros tructural transform ation,mechanical properties and degradation mechanisms of the CM AS-interacted TBCs in the thermal cycling tests were *** YSZ grains were dissolved in the CMAS melts,and then the ZrO_(2) grains were reprecipitated with spherical shape,accompanying with phase transformation from tetragonal(t) to monoclinic(m).The thermal cycling tests reveal that the YSZ coating fails at the early stage due to the attack of *** fractures in intracolumns lead to partial spallation of the *** failure of the coating occurs at the interfaces between thermally grown oxides(TGO) layer and YSZ topcoat;especially,the hardness and Young's modulus of the YSZ coatings increase intensively,as the coatings were infiltrated by the CMAS for a long time.

关键词： CMAS Thermal barrier coatings Young's modulus Thermal cycling behavior PS-PVD

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Process metallurgy and data-driven prediction and feedback of blast furnace heat indicators

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1228-1240页

作者： Quan Shi Jue Tang Mansheng Chu School of Metallurgy Northeastern UniversityShenyang 110819China institute for Frontier Technologies of low-carbon Steelmaking Northeastern UniversityShenyang 110819China Engineering research Center of Frontier Technologies for low-carbon Steelmaking(Ministry of Education) Shenyang 110819China

The prediction and control of furnace heat indicators are of great importance for improving the heat levels and conditions of the complex and difficult-to-operate hour-class delay blast furnace(BF)*** this work,a prediction and feedback model of furnace heat indicators based on the fusion of data-driven and BF ironmaking processes was *** data on raw and fuel materials,process op-eration,smelting state,and slag and iron discharge during the whole BF process comprised 171 variables with 9223 groups of data and were comprehensively analyzed.A novel method for the delay analysis of furnace heat indicators was *** extracted delay variables were found to play an important role in *** method that combined the genetic algorithm and stacking efficiently im-proved performance compared with the traditional machine learning algorithm in improving the hit ratio of the furnace heat prediction *** hit ratio for predicting the temperature of hot metal in the error range of±10℃ was 92.4%,and that for the chemical heat of hot metal in the error range of±0.1wt%was 93.3%.On the basis of the furnace heat prediction model and expert experience,a feedback model of furnace heat operation was established to obtain quantitative operation suggestions for stabilizing BF heat *** sugges-tions were highly accepted by BF ***,the comprehensive and dynamic model proposed in this work was successfully ap-plied in a practical BF *** improved the BF temperature level remarkably,increasing the furnace temperature stability rate from 54.9%to 84.9%.This improvement achieved considerable economic benefits.

关键词： blast furnace furnace heat genetic algorithm stacking prediction and feedback

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Fundamentals and progress of the manifold method based on independent covers

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Science China(Technological Sciences) 2024年第4期67卷 966-991页

作者： SU HaiDong LIN ShaoZhong XIE ZhiQiang GONG YaQi QI YongFeng Material and Engineering structure Department Yangtze River Scientific Research InstituteWuhan 430010China research Center of Water Engineering Safety and Disaster Prevention of Ministry of Water Resources Wuhan 430010China

Aiming to solve mesh generation,computational stability,accuracy control,and other problems encountered with existing numerical methods,such as the finite element method and the finite volume method,a new numerical computational method for continuum mechanics,namely the manifold method based on independent covers(MMIC),is proposed based on the concept of mathematical manifolds,to form partitioned series solutions of partial differential *** partitions,the cover meshes have the characteristics of arbitrary shape,arbitrary connection,and arbitrary *** are expected to fundamentally solve the mesh generation problem and can also simulate the precise geometric boundaries of the CAD model and strictly impose boundary *** the selection of series solutions,local analytical solutions(such as series solutions at crack tips and series solutions in infinite domains)or proper forms of complete series can be used to reflect the local or global characteristics of the physical field to accelerate *** applications are presented.A new method of beam,plate,and shell analysis is *** deformation characteristics of beams,plates,and shells are simulated with polynomial series of suitable forms,and the analysis of curved beams and shells with accurate geometric representation is *** the static elastic analysis of two-dimensional structures,a mesh splitting algorithm is proposed,and h-p version adaptive analysis is carried out with error ***,automatic computation integrated with CAD is *** analysis is also attempted for the solution of differential equations of *** the one-dimensional convection-diffusion equation and Burgers equation,calculation results with high precision are obtained in strong convection and shock wave simulations,avoiding nonphysical *** solving the two-dimensional incompressible Navier-Stokes equation is also *** series solution formula is used to o

关键词： series solutions mesh generation adaptive analysis fixed meshes numerical manifold method

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Overview of coals as carbon anode materials for sodium-ion batteries

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Clean Energy 2024年第4期8卷 197-218页

作者： Junli Kong Zhijiang Su Chunwei Dong Quanbin Chen Guanghong Pan National institute of Clean-and-low-Carbon Energy Beijing 102211China

Energy storage is an important technology in achieving carbon-neutrality *** with lithium-ion batteries,the raw materials of sodium-ion batteries are abundant,low-cost,and highly ***,their costs are expected to be further reduced as large-scale applications take off,making them viable for energy storage *** primary anode material for sodium-ion batteries is hard carbon,which has a high sodium-ion storage capacity but is relatively expensive,limiting its applications in energy *** order to widen the applications of sodium-ion batteries in energy storage and other fields,it is particularly important to develop anode materials that have both high performance and low ***,with abundant reserves and worldwide availability,can serve as low-cost carbon sources for anode ***,coals of different grades of metamorphism have different structural characteristics that can be tailored for the structural characteristics of coal-based anode materials for sodium-ion bat*** research on tailoring coals as the anode materials for sodium-ion batteries is summarized and the recent progress made towards mitigating the existing issues is analysed in this ***,the impacts of different grades of metamorphism on the sodium-ion storage performance of coal-based anode materials prepared using direct carbonization are discussed in *** on improving the electrochemical performances of coal-based anode materials through pore and microcrystalline structure controls and surface as well as interface modifications are ***,the advantages and disadvantages of different preparation methods are *** make the industrial applications of coal-based anode materials for sodium-ion batteries more viable,the importance of the de-ashing process is introduced.

关键词： coals sodium-ion batteries anodes structure controls de-ashing process

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Fabrication and characterization of multi-scale coated boron powders with improved combustion performance:A brief review

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Defence Technology（防务技术） 2024年第1期31卷 27-40页

作者： Rui Liu Danfeng Yang Kunyu Xiong Ying-Lei Wang Qi-Long Yan Science and Technology on Combustion Internal Flow and Thermo-structure LaboratoryNorthwestern Polytechnical UniversityXi'an710072China Xi'an Modern Chemistry research institute Xi'an710065China

Boron has high mass and volume calorific values,but it is difficult to ignite and has low combustion *** literature review summarizes the strategies that are used to solve the above-mentioned problems,which include coatings of boron by using fluoride compounds,energetic composites,metal fuels,and metal *** techniques include recrystallization,dual-solvent,phase transfer,electrospinning,*** one of the effective coating agents,the fluorine compounds can react with the oxide shell of boron *** comparison,the energetic composites can effectively improve the flame temperature of boron powder and enhance the evaporation efficiency of oxide film as a condensed *** and metal oxides would react with boron powder to form metal borides with a lower ignition point,which could reduce its ignition temperature.

关键词： Boron powder coating structure and morphology Condensed phase thermal reaction Ignition and combustion

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Exploring centimeter-sized crystals of bismuth-iodide perovskite toward highly sensitive X-ray detection

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Chinese Chemical Letters 2024年第6期35卷 185-188页

作者： Xin Dong Jing Liang Zhijin Xu Huajie Wu Lei Wang Shihai You Junhua Luo Lina Li College of Chemistry Fuzhou UniversityFuzhou 350116China State Key Laboratory of structure Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China University of Chinese Academy of Sciences Beijing 100049China

Lead-halide perovskites exhibit outstanding performance in X-ray detection due to their intrinsic features such as high charge carrier mobility,large atomic number,and long carrier lifetime,but the toxicity of lead is regarded as the major factor hindering their ***,we introduce organic molecule(R)-(-)-2-methylpiperazine(R-MPz)into the bismuth-based structure to synthesize lead-free(R)-(H_(2)MPz)BiI_(5)(R-MBI).The high-quality centimeter-sized single crystals have been obtained,which show a low dark current and superior environmental ***,the single-crystal device of R-MBI exhibits a highμτproduct up to 1.88×10^(-4)cm^(2)/V and a low trap density of 1.21×10^(10)cm^(-3).Further,the detector displays excellent detection sensitivity of 263.58μC Gy_(air)^(-1)cm^(-2)and a favorable low detection limit of 4.35μGyair/s,both of which meet the requirement for medical *** findings shed light on the exploration of innovative bismuth-based hybrid perovskites for high-performance X-ray detection.

关键词： Perovskite Lead-free Bismuth-based X-ray detection Sensitivity

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