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Chinese physics B 2024年第6期33卷 605-612页

作者：毛党新吴园燕涂育松 college of physics science and {3. Yangzhou UniversityYangzhou 225009China

The hydroxyl-terminated self-assembled monolayer(OH-SAM),as a surface resistant to protein adsorption,exhibits substantial potential in applications such as ship navigation and medical implants,and the appropriate strategies for designing anti-fouling surfaces are ***,we employ molecular dynamics simulations and alchemical free energy calculations to systematically analyze the factors influencing resistance to protein adsorption on the SAMs terminated with single or double OH groups at three packing densities(∑=2.0 nm^(-2),4.5 nm^(-2),and 6.5 nm^(-2)),*** the first time,we observed that the compactness and order of interfacial water enhance its physical barrier effect,subsequently enhancing the resistance of SAM to protein ***,the spatial hindrance effect of SAM leads to the embedding of protein into SAM,resulting in a lack of resistance of SAM towards ***,the number of hydroxyl groups per unit area of double OH-terminated SAM at ∑=6.5 nm^(-2) is approximately 2 to 3.times that of single OH-terminated SAM at ∑=6.5 nm^(-2) and 4.5 nm^(-2),consequently yielding a weaker resistance of double OH-terminated SAM towards ***,due to the structure of SAM itself,i.e.,the formation of a nearly perfect ice-like hydrogen bond structure,the SAM exhibits the weakest resistance towards *** study will complement and improve the mechanism of OH-SAM resistance to protein adsorption,especially the traditional barrier effect of interfacial water.

关键词： molecular dynamics simulation self-assembled monolayer resistance to protein adsorption hydrogen bond interfacial water

A review on covalent organic frameworks for rechargeable zinc-ion batteries

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Chinese Chemical Letters 2024年第7期35卷 107-120页

作者： Yunyu Zhao Chuntao Yang Yingjian Yu college of physics science and {3. Kunming UniversityKunming 650214China

In recent years,rechargeable zinc-ion batteries(ZIBs)are considered to be a promising alternative to lithium-ion batteries owing to their high safety and theoretical capacity with low ***,the in-depth development of rechargeable zinc-ion batteries is restricted by a sequence of issues,such as the dissolution and structure collapse of cathode materials,the formation of by-products,severe anode corrosion,passivation,and the growth of zinc *** covalent organic frameworks(COFs)can solve the above problems to a certain extent owing to their ideal characteristics,such as rigid structure,insolubility,high porosity,and abundant active ***,as advanced materials for ZIBs,have attracted researchers'*** this review,we systematically summarized the synthesis methods of COFs and discussed the application of several advanced characterization technologies in COFs,which would provide a reference for the in-depth research of *** addition,we elucidated the use of COFs as cathode materials and anode protective layers in rechargeable ***,we discussed the challenges and solutions in the development of COF materials,which would provide constructive insights into the future direction of COFs.

关键词： Covalent organic framework Zn-ion battery Zinc dendrite Anode Cathode

Single-atomic activation on ZnIn_(2)S_(4)basal planes boosts photocatalytic hydrogen evolution

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Nano Research 2024年第7期17卷 5949-5955页

作者： Jianpeng Cui Ying Wang Luxue Lin Xiaotian Yang Xuyu Luo Shiying Guo Xiaoyong Xu college of physics science and {3. and Center for Interdisciplinary ResearchYangzhou UniversityYangzhou 225002China

The use of single-atom cocatalysts plays a crucial role in enhancing artificial photocatalysis,where the precise construction of stable and efficient single-atom configuration is essential but remains ***,we report a simple one-step hydrothermal method for preparing single-atomic Mo modified ZnIn_(2)S_(4)(Mo-ZIS)nanosheets as a highly active photocatalytic hydrogen evolution(PHE)*** Mo substituting for portion of In atoms in ZIS nanosheets induces the spatial charge redistribution,which not only promotes the separation of photogenerated charge carriers but also optimizes the Gibbs free energy of adsorbing H*on S atoms at basal *** a result,Mo-ZIS exhibits an impressive PHE rate as high as 6.71 mmol·g^(−1)·h^(−1),over 10 times that of the pristine ZIS,with an apparent quantum efficiency(AQE)up to 3..8%at 420 *** study gains insights into the coordination configuration and electronic modulation resulting from single-atomic decoration,providing mechanistic cognitions for the development of advanced photocatalysts via non-precious metal atomic modification.

关键词： photocatalytic hydrogen evolution ZnIn_(2)S_(4) single-atom activation Gibbs free energy

Light-assisted rechargeable zinc-air battery:Mechanism,progress,and prospects

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Journal of Energy Chemistry 2024年第4期91卷 178-193页

作者： Jiangchang Chen Jinlong Luo Youlin Xiang Yingjian Yu college of physics science and {3. Kunming UniversityKunming 650214YunnanChina

Exploring effective energy storage systems is critical to alleviate energy *** zinc-air batteries are promising energy storage ***,conventional rechargeable zinc-air battery systems face many challenges associated with electrolytes and electrodes,causing inferior electrochemistry *** light-assisted strategy represents a novel and innovative approach to conventional zinc-air battery technology that uses only electrical *** strategy effectively combines both light and electrical energy conversion/storage *** addition,light-assisted rechargeable zinc-air batteries can achieve photocharging with or without applied electrical bias by partially using solar energy and the acceleration of oxygen reduction/evolution reaction *** this paper,the working mechanism and structural design of the light-assisted rechargeable zinc-air batteries are introduced based on the theory of photoelectrochemistry and its ***,the latest advances in electrolyte and photocathode design strategies are discussed in *** performance enhancement of aqueous light-assisted rechargeable zinc-air batteries using photoelectric materials is ***,a summary and outlook on the further modification of properties of light-assisted rechargeable zinc-air batteries,especially the photovoltaic electrode catalyst design strategies,are *** review provides insights and guidance for the design of high-performance light-assisted rechargeable Zn-air batteries for next-generation energy storage devices.

关键词： Zn-air battery Light-assisted Electrolyte Catalyst Semiconductor

Enhancing I0/I-Conversion Efficiency by Starch Confinement in Zinc-Iodine Battery

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Energy & Environmental Materials 2024年第1期7卷 118-124页

作者： Danyang Zhao Qiancheng Zhu Qiancheng Zhou Wenming Zhang Ying Yu Shuo Chen Zhifeng Ren Institute of Nanoscience and Nanotechnology College of Physical Science and Technology Central China Normal University National & Local Joint Engineering Laboratory of New Energy Photoelectric Devices College of Physics Science and Technology Hebei University Department of physics and Tc SUH University of Houston

The redox couple of I0/I-in aqueous rechargeable iodine-zinc（I2-Zn）batteries is a promising energy storage resource since it is safe and costeffective,and provides steady output ***,the cycle life and efficiency of these batteries remain unsatisfactory due to the uncontrolled shuttling of polyiodide（I3.and I5-） and side reactions on the Zn anode.

关键词： aqueous battery conversion efficiency iodine–zinc battery starch confinement

Fully spin-polarized, valley-polarized and spin-valley-polarized electron beam splitters utilizing zero-line modes in a three-terminal device

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Chinese physics B 2024年第6期33卷 596-603页

作者：吕小龙杨加恩谢航 college of science Guangxi University of Science and TechnologyLiuzhou 545006China college of physics Chongqing UniversityChongqing 401331China Chongqing Key Laboratory for Strongly-Coupled physics Chongqing UniversityChongqing 401331China

Topological zero-line modes(ZLMs) with spin and valley degrees of freedom give rise to spin, valley and spinvalley transport, which support a platform for exploring quantum transport physics and potential applications in spintronic/valleytronic devices. In this work, we investigate the beam-splitting behaviors of the charge current due to the ZLMs in a three-terminal system. We show that with certain combinations of ZLMs, the incident charge current along the interface between different topological phases can be divided into different polarized currents with unit transmittance in two outgoing terminals. As a result, fully spin-polarized, valley-polarized and spin-valley-polarized electron beam splitters are generated. The mechanism of these splitters is attributed to the cooperative effects of the distribution of the ZLMs and the intervalley and intravalley scatterings that are modulated by the wave-vector mismatch and group velocity mismatch. Interestingly, half-quantized transmittance of these scatterings is found in a fully spin-valley-polarized electron beam ***, the results indicate that these splitters can be applicable to graphene, silicene, germanene and stanene due to their robustness against the spin–orbit coupling. Our findings offer a new way to understand the transport mechanism and investigate the promising applications of ZLMs.

关键词： topological zero-line modes spin polarization valley polarization quantum transport

Infrared imaging of magnetic octupole domains in non-collinear antiferromagnets

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National science Review 2024年第06期11卷 197-205页

作者： Peng Wang Wei Xia Jinhui Shen Yulong Chen Wenzhi Peng Jiachen Zhang Haolin Pan Xuhao Yu Zheng Liu Yang Gao Qian Niu Zhian Xu Hongtao Yang Yanfeng Guo Dazhi Hou International Center for Quantum Design of Functional Materials(ICQD) School of Emerging TechnologyUniversity of Science and Technology of China college of Mathematics and physics Qingdao University of Science and Technology School of Physical science and technology Shanghai Tech University Shanghai Tech Laboratory for Topological physics Shanghai Tech University Department of physics University of Science and Technology of China CAS Key Laboratory of Strongly-Coupled Quantum Matter physics University of Science and Technology of China Xi'an Institute of Optics and Precision Mechanics of Chinese Academy of sciences

Magnetic structure plays a pivotal role in the functionality of antiferromagnets（AFMs）, which not only can be employed to encode digital data but also yields novel phenomena. Despite its growing significance,visualizing the antiferromagnetic domain structure remains a challenge, particularly for non-collinear AFMs. Currently, the observation of magnetic domains in non-collinear antiferromagnetic materials is feasible only in Mn3.n, underscoring the limitations of existing techniques that necessitate distinct methods for in-plane and out-of-plane magnetic domain imaging. In this study, we present a versatile method for imaging the antiferromagnetic domain structure in a series of non-collinear antiferromagnetic materials by utilizing the anomalous Ettingshausen effect（AEE）, which resolves both the magnetic octupole moments parallel and perpendicular to the sample surface. Temperature modulation due to AEE originating from different magnetic domains is measured by lock-in thermography, revealing distinct behaviors of octupole domains in different antiferromagnets. This work delivers an efficient technique for the visualization of magnetic domains in non-collinear AFMs, which enables comprehensive study of the magnetization process at the microscopic level and paves the way for potential advancements in applications.

关键词： non-collinear antiferromagnet domain structure infrared imaging anomalous Ettingshausen effect

STDNet: A Spatio-Temporal Decomposition Neural Network for Multivariate Time Series Forecasting

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Tsinghua science and technology 2024年第4期29卷 1232-1247页

作者： Zhuolun Jiang Zefei Ning Hao Miao Li Wang college of Computer science and technology(college of Data science) Taiyuan University of TechnologyJinzhong 030600China

Long-term multivariate time series forecasting is an important task in engineering applications. It helps grasp the future development trend of data in real-time, which is of great significance for a wide variety of fields. Due to the non-linear and unstable characteristics of multivariate time series, the existing methods encounter difficulties in analyzing complex high-dimensional data and capturing latent relationships between multivariates in time series, thus affecting the performance of long-term prediction. In this paper, we propose a novel time series forecasting model based on multilayer perceptron that combines spatio-temporal decomposition and doubly residual stacking, namely Spatio-Temporal Decomposition Neural Network (STDNet). We decompose the originally complex and unstable time series into two parts, temporal term and spatial term. We design temporal module based on auto-correlation mechanism to discover temporal dependencies at the sub-series level, and spatial module based on convolutional neural network and self-attention mechanism to integrate multivariate information from two dimensions, global and local, respectively. Then we integrate the results obtained from the different modules to get the final forecast. Extensive experiments on four real-world datasets show that STDNet significantly outperforms other state-of-the-art methods, which provides an effective solution for long-term time series forecasting.

关键词： time series forecasting multivariate time series spatio-temporal decomposition

Superconducting ternary hydrides: progress and challenges

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National science Review 2024年第7期11卷 47-61页

作者： Wendi Zhao Xiaoli Huang Zihan Zhang Su Chen Mingyang Du Defang Duan Tian Cui Institute of High Pressure physics School of Physical Science and Technology Ningbo University State Key Laboratory of Superhard Materials College of Physics Jilin University

Since the discovery of the high-temperature superconductors H3. and LaH10under high pressure,compressed hydrides have received extensive attention as promising candidates for room-temperature superconductors. As a result of current high-pressure theoretical and experimental studies, it is now known that almost all the binary hydrides with a high superconducting transition temperature（Tc） require extremely high pressure to remain stable, hindering any practical application. In order to further lower the stable pressure and improve superconductivity, researchers have started exploring ternary hydrides and had many achievements in recent years. Here, we discuss recent progress in ternary hydrides, aiming to deepen the understanding of the key factors regulating the structural stability and superconductivity of ternary hydrides, such as structural motifs, bonding features, electronic structures, electron–phonon coupling, ***, the current issues and challenges of superconducting ternary hydrides are presented, together with the prospects and opportunities for future research.

关键词： high pressure ternary hydrides conventional superconductivity electron–phonon coupling

Exploration of heavy Higgs bosons at a 100 TeV hadron collider within the semi-constrained next-to-minimal supersymmetric standard model

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Chinese physics C 2024年第9期48卷 107-117页

作者： Kun Wang Pengfu Tian Jingya Zhu college of science University of Shanghai for Science and TechnologyShanghai 200093China School of physics and technology Wuhan UniversityWuhan 430072China School of physics and Electronics Henan UniversityKaifeng 475004China

In this study,we explore the detectability of heavy Higgs bosons in the pp→bbH/A→bbtt channel at a100 TeV hadron collider within the semi-constrained next-to-minimal supersymmetric standard *** calculate their production cross sections and decay branching ratios and compare them with simulation results from *** focus on the heavy doublet-dominated CP-even Higgs H and CP-odd Higgs A,with mass limits set below 10TeV to ensure *** a collider with an integrated luminosity of 3.ab^(-1),the potential for detecting heavy Higgs bosons varies significantly with their mass and tanβ.Heavy Higgs bosons with masses below 2 TeV are within the testable range,while those heavier than 7 TeV are below the exclusion and discovery thresholds,rendering them *** masses between 2 and 7 TeV,heavy Higgs bosons with tanβ smaller than 20 can be detected,whereas those with tanβ larger than 20 are beyond the current discovery or exclusion capabilities.

关键词： next-to-minimal supersymmetric standard model heavy Higgs boson 100 TeV hadron collider