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Towards carbon neutrality:Sustainable recycling and upcycling strategies and mechanisms for polyethylene terephthalate via biotic/abiotic pathways

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Eco-Environment & Health 2024年第2期3卷 117-130页

作者： Jiaqi Yang Zhiling Li Qiongying Xu Wenzong Liu Shuhong Gao Peiwu Qin Zhenglin Chen Aijie Wang school of Civil&Environmental Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China State Key Laboratory of Urban Water Resources and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China Institute of Biopharmaceutical and Health Engineering Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Tsinghua-Berkeley shenzhen Institute Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China

Polyethylene terephthalate(PET),one of the most ubiquitous engineering plastics,presents both environmental challenges and opportunities for carbon neutrality and a circular *** review comprehensively addressed the latest developments in biotic and abiotic approaches for PET recycling/***,microbial depolymerization of PET,along with the biosynthesis of reclaimed monomers[terephthalic acid(TPA),ethylene glycol(EG)]to value-added products,presents an alternative for managing PET waste and enables CO_(2.***,thermal treatments(i.e.,hydrolysis,glycolysis,methanolysis,etc.)and photo/electrocatalysis,enabled by catalysis advances,can depolymerize or convert PET/PET monomers in a more flexible,simple,fast,and controllable *** abiotic/biotic catalysis offers great potential for PET upcycling to generate commodity chemicals and alternative materials,ideally at lower energy inputs,greenhouse gas emissions,and costs,compared to virgin polymer ***,over 2. types of upgraded PET products(e.g.,adipic acid,muconic acid,catechol,vanillin,and glycolic acid,etc.)have been identified,underscoring the potential of PET upcycling in diverse *** can be made to develop chemo-catalytic depolymerization of PET,improve microbial depolymerization of PET(e.g.,hydrolysis efficiency,enzymatic activity,thermal and pH level stability,etc.),as well as identify new microorganisms or hydrolases capable of degrading PET through computational and machine learning ***,this review provides a roadmap for advancing PET recycling and upcycling technologies,which hold the potential to shape the future of PET waste management and contribute to the preservation of our ecosystems.

关键词： PET depolymerization Monomers Recycling/upcycling Biocatalysis Photo/electrocatalysis

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Unraveling the role of NiSnPH@OOH/CC perovskite hydroxide for efficient electrocatalytic oxidation of methanol to formate

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Nano Research 2024年第4期17卷 2388-2399页

作者： Jing Shao Yusheng Fang Xiaobing Wu Muhammad Imran Abdullah Youkun Tao College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China school of Science Harbin Institute of TechnologyShenzhen 518055China

The sluggish kinetics of oxygen evolution reaction(OER)is the key tailback for hydrogen production from the water *** OER with thermodynamically auspicious methanol oxidation reaction(MOR)can significantly boost the H_(2. and value-added products ***,it is currently challenging to achieve a synergistic manipulation of product selectivity and performance for MOR ***,we report NiSnPH@OOH/CC(CC=carbon cloth)perovskite hydroxide nanosphere as an efficient MOR electrocatalyst with high activity,stability,and selectivity towards methanol oxidation to formate.A surface amorphous layer of defect rich NiOOH was generated in operando by selective Sn leaching with stable perovskite hydroxide bulk structure,which mitigates the oxidative power and optimizes the local coordination environment of the active NiOOH *** situ Raman combined with electrochemical studies further confirm the key active species,NiOOH,generated in operando enhance the MOR and blocking the over oxidation of methanol to CO_(2..As a result,NiSnPH@OOH/CC effectively masks the OER and attains>99%selectivity with 100%Faradic efficiency for *** results of this study show the advances of NiSnPH@OOH/CC as an efficient electrocatalyst for MOR and also suggest its potential applications for various small organic molecules oxidation.

关键词： perovskite hydroxide small organic molecules nickel oxy(hydroxide) value-added products methanol oxidation reaction

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Continuous near-complete photocatalytic degradation of toluene by V/N-doped TiO_(2.loade d on honeycomb ceramics under UV irradiation

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Journal of Materials Science & Technology 2024年第7期174卷 188-194页

作者： Gang Liu Lijuan Han Jingwei Wang Yongqiang Yang Zuoyan Chen Bilu Liu Xingcai An Gansu Natural Energy Institute Lanzhou 730046China shenzhen Geim Graphene Center Tsinghua-Berkeley Shenzhen Institute&Institute of Materials ResearchTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China

Photocatalytic degradation of volatile organic compounds(VOCs)is a significant applying aspect of *** the modulation of photocatalysts and the rational dispersion of them on supports are key for solar-driven VOC *** batch-type photoreactors have low efficiency while continuous-flow photoreactors suffer from the problem of incomplete removal of ***,aiming for continuous and complete degradation of toluene gas as the target contaminant,continuous-flow pho-tocatalytic degradation reactors were made by adhering the vanadium and nitrogen codoped TiO_(2.on honeycomb ceramics(V/N-TiO_(2.@HC)by a simple sol-gel *** such a reactor,the rich ordered pores in the HC accelerate mass transport of toluene,and the introduction of V/N dopants narrows the bandgap and widens the light absorption range of TiO_(2.,together resulting in continuous and nearly-complete pho-tocatalytic degradation of *** unique and stable structure of HC allows the photocatalysts to be *** degradation rate of toluene gas can reach 97.8%,and after 2. rounds of photocatalytic degra-dation,there is still a degradation rate of 96.7%.The impacts of loading times and gaseous flow rate on the photocatalytic performance of V/N-TiO_(2.@HC are studied in *** study provides a practical so-lution for the continuous and complete photocatalytic degradation of VOCs and opens a new application field for HC.

关键词： Honeycomb ceramics V/N co-doped TiO_(2. Photocatalytic degradation Toluene gas Continuous and complete degradation

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Reconstructing coherent dynamics of bound states induced by strong attosecond XUV pulses

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Chinese Optics Letters 2024年第2期22卷 56-63页

作者：贾利娟刘明清王新强徐龙闫培光姜维超傅立斌 Institute of Quantum Precision Measurement College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China Department of Physics Xiamen UniversityXiamen 361005China graduate school of China Academy of Engineering Physics Beijing 100193China

We propose a scheme that utilizes weak-field-induced quantum beats to investigate the electronic coherences of atoms driven by a strong attosecond extreme ultraviolet(XUV)*** technique involves using a strong XUV pump pulse to excite and ionize atoms and a time-delayed weak short pulse to probe the photoelectron *** theoretical analysis demonstrates that the information regarding the bound states,initiated by the strong pump pulse,can be precisely reconstructed from the weak-field-induced quantum beat *** examine this scheme,we apply it to the attosecond XUV laser-induced ionization of hydrogen atoms by solving a three-dimensional time-dependent Schr?dinger *** work provides an essential reference for reconstructing the ultrafast dynamics of bound states induced by strong XUV attosecond pulses.

关键词： attosecond pulse bound-state dynamics quantum beats

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Low cost and low density chloride solid electrolyte for all solid state cathode with high active material ratio

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Nano Research 2024年第10期17卷 8826-8833页

作者： Hao-Yuan Tan Mei-Yu Zhou Zhongyuan Huang Jin-Da Luo Jing-Tian Yang Jian-Ping Wang Ye-Chao Wu Xiao-Bin Cheng Zi-Wei Wang Xu-Dong Hao Linjun Wang Ke Gong Yi-Chen Yin Yinguo Xiao Hong-Bin Yao Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China Department of Applied Chemistry University of Science and Technology of ChinaHefei 230026China school of Advanced Materials Peking University Shenzhen Graduate SchoolShenzhen 518055China

Chloride solid electrolytes(SEs)have attracted widespread attention due to their high room-temperature ionic conductivity and excellent cathode ***,the conventionally selected central metal elements(e.g.,In,Y and Ta)are usually rare and heavy,inevitably causing the high cost and high density of the obtained chloride ***,by choosing abundant and light Mg and Al as central metal elements,we develop a cheap and low density Li_(1.2.Mg_(0.95)Al_(0.3)Cl_(4)SE for high active material ratio in all solid state *** replacement of Mg^(2.)by Al^(3+)in the framework yields vacancies and lowers the non-lithium metal ions occupancy at Mg/Li co-occupied 16d site,effectively relieving the blocking effects by Mg^(2.)in the pristine spinel Li_(2.2.)Mg_(1+x)Cl_(4).Thus,a significantly improved room-temperature conductivity of 3.08×10^(-4)S·cm^(-1)is achieved,two orders of magnitude higher than that of Li_(1.2.Mg_(1.4)Cl_(4).More attractively,its low density of only 1.98 g·cm-3 enables low SE mass ratio in cathodes(only 16 wt.%)with still effective electrolyte/cathode contact and lithium-ion conduction *** charged to potential of 4.30 V,the asfabricated Li_(1.2.Mg_(0.95)Al_(0.3)Cl_(4)-based solid lithium battery with uncoated NCM52. cathode can be cycled for over 100 cycles with a capacity retention of 86.68%at room temperature.

关键词： chloride solid electrolytes low cost low density Li+conductivities

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Wearable pressure sensors based on antibacterial and porous chitosan hydrogels for full-range human motion detection

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Science China(Technological Sciences) 2024年第8期67卷 2475-2484页

作者： ZHANG YingXin LIU HanGuang JIN ShunYu LI YaJuan ZHANG Wan ZHOU Hang NIE ZanXiang HUANG Yuan school of Microelectronics Science and Technology Sun Yat-sen UniversityGuangzhou 510275China Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230022China Department of Clinical Laboratory the First Affiliated Hospital of Anhui Medical UniversityHefei 230022China school of Electronic and Computer Engineering Peking University Shenzhen Graduate SchoolShenzhen 518055China Zinergy shenzhen Ltd. Shenzhen 518109China

Wearable pressure sensors made from conductive hydrogels hold significant potential in health ***,limited pressure range(Pa to hundreds of kPa)and inadequate antibacterial properties restrict their practical applications in diagnostic and health ***,a wearable high-performance pressure sensor was assembled using a facilely prepared porous chitosan-based hydrogel,which was constructed from commercial phenolphthalein particles as a sacrificial *** relationship between the porosity of hydrogels and sensing performance of sensors was systematically ***,the wearable pressure sensor,featuring an optimized porosity of hydrogels,exhibits an ultrawide sensing capacity from 4.83 Pa to 2.0 k Pa(range-to-limit ratio of 51,760)and high sensitivity throughout high pressure ranges(0.7 kPa~(-1),12.–2.0 kPa).The presence of chitosan endows these hydrogels with outstanding antibacterial performance against *** and ***,making them ideal candidates for use in wearable *** features allow for a practical approach to monitor full-range human motion using a single device with a simple structure.

关键词： porous hydrogels antibacterial performances wearable pressure sensors full-range human motion chitosan

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Audio-visual keyword transformer for unconstrained sentence-level keyword spotting

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CAAI Transactions on Intelligence Technology 2024年第1期9卷 142-152页

作者： Yidi Li Jiale Ren Yawei Wang Guoquan Wang Xia Li Hong Liu Key Laboratory of Machine Perception Peking UniversityShenzhen Graduate SchoolShenzhenChina College of Electronics and Information Engineering Sichuan UniversityChengduChina Department of Computer Science ETH ZurichZurichSwitzerland

As one of the most effective methods to improve the accuracy and robustness of speech tasks,the audio-visual fusion approach has recently been introduced into the field of Keyword Spotting(KWS).However,existing audio-visual keyword spotting models are limited to detecting isolated words,while keyword spotting for unconstrained speech is still a challenging *** this end,an Audio-Visual Keyword Transformer(AVKT)network is proposed to spot keywords in unconstrained video *** authors present a transformer classifier with learnable CLS tokens to extract distinctive keyword features from the variable-length audio and visual *** outputs of audio and visual branches are combined in a decision fusion *** humans can easily notice whether a keyword appears in a sentence or not,our AVKT network can detect whether a video clip with a spoken sentence contains a pre-specified ***,the position of the keyword is localised in the attention map without additional position ***-imental results on the LRS2.KWS dataset and our newly collected PKU-KWS dataset show that the accuracy of AVKT exceeded 99%in clean scenes and 85%in extremely noisy *** code is available at https://***/jialeren/AVKT.

关键词： artificial intelligence multimodal approaches natural language processing neural network speech processing

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Lift system optimization for hover-capable flapping wing micro air vehicle

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Frontiers of Mechanical Engineering 2024年第3期19卷 61-75页

作者： Shengjie XIAO Yongqi SHI Zemin WANG Zhe NI Yuhang ZHENG Huichao DENG Xilun DING Department of Mechanical Engineering and Automation Beihang UniversityBeijing 100191China Department of Mechanical Engineering Tsinghua UniversityBeijing 100084China shenzhen International graduate {2. Tsinghua UniversityShenzhen 518055China

A key challenge is using bionic mechanisms to enhance aerodynamic performance of hover-capable flapping wing micro air vehicle(FWMAV).This paper presented a new lift system with high lift and aerodynamic efficiency,which use a hummingbird as a bionic *** new lift system is able to effectively utilize the high lift mechanism of hummingbirds,and this study innovatively utilizes elastic energy storage elements and installs them at the wing root to help improve aerodynamic performance.A flapping angle of 154°is achieved through the optimization of the flapping mechanism *** optimized wing shape and parameters are obtained through experimental studies on the ***,the max net lift generated is 17.6%of the flapping wing vehicle’s ***,energy is stored and released periodically during the flapping cycle,by imitating the musculoskeletal system at the wing roots of hummingbirds,thereby improving the energy utilization rate of the FWMAV and reducing power consumption by 4.5%under the same ***,strength verification and modal analyses are conducted on the flapping mechanism,and the weight of the flapping mechanism is reduced through the analysis and testing of different *** results show that the lift system can generate a stable lift of 31.98 g with a wingspan of 175 mm,while the lift system weighs only 10.5 g,providing aerodynamic conditions suitable for high maneuverability flight of FWMAVs.

关键词： lift optimization flapping wing elastic energy hovering flapping mechanism

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ENERGY CONSERVATION FOR THE WEAK SOLUTIONS TO THE 3D COMPRESSIBLE NEMATIC LIQUID CRYSTAL FLOW

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Acta Mathematica Scientia 2024年第3期44卷 851-864页

作者：谭忠李心亮杨惠 school of Mathematical Sciences Xiamen UniversityXiamen361005China shenzhen Research Institute of Xiamen University Shenzhen518057China school of Mathematics and Statistics Shenzhen UniversityShenzhen518060China College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen518060China

In this paper,we establish some regularity conditions on the density and velocity fields to guarantee the energy conservation of the weak solutions for the three-dimensional compressible nematic liquid crystal flow in... 详细信息

关键词： compressible nematic liquid crystal flow weak solutions energy conservation

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Integrated interconnected porous and lamellar structures realized fast ion/electron conductivity in high-performance lithium-sulfur batteries

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Chinese Chemical Letters 2024年第6期35卷 161-167页

作者： Ya Song Mingxia Zhou Zhu Chen Huali Nie Jiao-Jing Shao Guangmin Zhou school of Materials and Metallurgy Guizhou UniversityGuiyang 550025China Medical College of Guizhou University Guiyang 550025China College of Biological Science and Medical Engineering Donghua UniversityShanghai 201620China shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China

The practical application of high-energy-density lithium-sulfur(Li-S)batteries have been highly praised for energy storage devices,while are largely hindered by the“shuttling effect”.Herein,core-shell carbon spheres composed of interlinked porous core and lamellar shell were designed to restrain the polysulfide *** microporous structure with pore size of around 1 nm effectively trap lithium ***,the interconnected porous core shortens the ion transfer distance and the lamellar carbon shell endows the carbon spheres with fast electron conduction,finally facilitating polysulfide conversion ***,the Li-S batteries with the carbon spheres as the interlayer show high discharge specific capacity of 1002.m Ah/g at 2.C with 574 m Ah/g remaining after 600 cycles,and high areal capacity of 5.48 m Ah/cm^(2. with sulfur loading of 4.67 mg/cm^(2. at 0.1 *** corresponding pouch cells also exhibit stable cycling stability with an initial discharge specific capacity of 1082.m Ah/g at 0.1 C.

关键词： Interlayer Shuttle effect Strong adsorption Porous carbon spheres Lithium-sulfur batteries

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