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Synergistic enhancement of photocatalytic and antimicrobial efficacy of nitrogen and erbium co-doped ZnO nanoparticles

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Journal of Rare Earths 2024年第5期42卷 859-868,I0002页

作者： Sudipta Mondal Moniruzzaman Jamal Sikder Ashikuzzaman Ayon Md Jannatul Ferdous Anik Md Muktadir Billah department of Materials and Metallurgical {1. Bangladesh University of Engineering and TechnologyDhaka1000Bangladesh School of Materials engineering Purdue UniversityWest LafayetteIN47907USA department of Materials Science and {1. University of CaliforniaBerkeleyCA94720USA department of Materials Science and {1. Northwestern UniversityEvanstonI28USA

Using the chemical co-precipitation approach,a series of nitrogen(N) and erbium(Er) co-doped ZnO nanoparticles(NPs) was effectively synthesized to enhance the photocatalytic and antibacterial *** characterization techniques,including X-ray diffraction(XRD),X-ray photoelectron spectro scopy(XPS),scanning electron microscopy(SEM),UV-vis,and photoluminescence(PL) spectroscopy,were carried out to validate the evaluated photocatalytic and antibacterial *** analysis confirms the pure wurtzite ZnO phase without the presence of any secondary *** analysis confirms the succe ssful incorporation of nitrogen and erbium into the ZnO *** optical bandgap of ZnO calculated from UV-vis spectroscopy shows a redshift after Er-N co-doping,with the lowest bandgap of 3.21. eV calculated for Zn_(0.97)Er_(0.03)N_(0.01.O_(0.99) *** images demonstrate the formation of nanorods after N-Er co-doping,followed by gradually increase d rod diameter and length after N-Er ***,the photocatalytic activities of ZnO samples we re measured by their ability to facilitate the photodegradation of Rhodamine B under UV *** with 1.mol% N doping exhibits 88% photodegradation of RhB under UV light within 360 min,and the photodegradation and antibacterial activity are greatly improved with Er *** fact,3 mol% Er-1.mol% N doped ZnO NPs demonstrate the highest photocatalytic activity,with approximately 96% degradation after 360 min,as well as superior antibacterial activity against Staphylococcus aureus(Gram-positive bacteria) and Pseudomonas aeruginosa(Gram-negative bacteria) with the highest zone of inhibition(ZOI) of 1. nm,due to nanorod formation,increased reactive oxygen species(ROS),and decreased electron-hole recombination,as validated by SEM,XPS,and PL spectroscopy.

关键词： Chemical co-precipitation Co-doping Bandgap Photocatalysis Rare earths Antimicrobial

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An adaptive machine learning-based optimization method in the aerodynamic analysis of a finite wing under various cruise conditions

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Theoretical & Applied Mechanics Letters 2024年第1期14卷 27-34页

作者： Zilan Zhang Yu Ao Shaofan Li Grace X.Gu department of Mechanical {1. University of CaliforniaBerkeley 94720USA department of {1. Peking UniversityBeijing 100871China department of Civil and Environmental {1. University of CaliforniaBerkeley 94720USA

Conventional wing aerodynamic optimization processes can be time-consuming and imprecise due to the complexity of versatile flight *** of existing literature has considered two-dimensional infinite airfoil optimization,while three-dimensional finite wing optimizations are subject to limited study because of high computational *** we create an adaptive optimization methodology built upon digitized wing shape deformation and deep learning algorithms,which enable the rapid formulation of finite wing designs for specific aerodynamic performance demands under different cruise *** methodology unfolds in three stages:radial basis function interpolated wing generation,collection of inputs from computational fluid dynamics simulations,and deep neural network that constructs the surrogate model for the optimal wing *** has been demonstrated that the proposed methodology can significantly reduce the computational cost of numerical *** also has the potential to optimize various aerial vehicles undergoing different mission environments,loading conditions,and safety requirements.

关键词： Aerodynamic optimization Computational fluid dynamics Radial basis function Finite wing Deep learning neural network

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Machine learning-driven optimization of plasma-catalytic dry reforming of methane

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Journal of Energy Chemistry 2024年第9期96卷 153-163页

作者： Yuxiang Cai Danhua Mei Yanzhen Chen Annemie Bogaerts Xin Tu department of Electrical {1. and Electronics University of LiverpoolLiverpool L693GJUK Research Group PLASMANT Department of ChemistryUniversity of AntwerpUniversiteitsplein 1BE-2610 Wilrijk-AntwerpBelgium College of Electrical engineering and Control Science Nanjing Tech UniversityNanjing 211816JiangsuChina

This study investigates the dry reformation of methane(DRM)over Ni/Al_(2)O_(3)catalysts in a dielectric barrier discharge(DBD)non-thermal plasma reactor.A novel hybrid machine learning(ML)model is developed to optimize the plasma-catalytic DRM reaction with limited experimental *** address the non-linear and complex nature of the plasma-catalytic DRM process,the hybrid ML model integrates three well-established algorithms:regression trees,support vector regression,and artificial neural networks.A genetic algorithm(GA)is then used to optimize the hyperparameters of each algorithm within the hybrid ML *** ML model achieved excellent agreement with the experimental data,demonstrating its efficacy in accurately predicting and optimizing the DRM *** model was subsequently used to investigate the impact of various operating parameters on the plasma-catalytic DRM *** found that the optimal discharge power(20 W),CO_(2)/CH_(4)molar ratio(1.5),and Ni loading(7.8 wt%)resulted in the maximum energy yield at a total flow rate of∼51.mL/***,we investigated the relative significance of each operating parameter on the performance of the plasma-catalytic DRM *** results show that the total flow rate had the greatest influence on the conversion,with a significance exceeding 35%for each output,while the Ni loading had the least impact on the overall reaction *** hybrid model demonstrates a remarkable ability to extract valuable insights from limited datasets,enabling the development and optimization of more efficient and selective plasma-catalytic chemical processes.

关键词： Plasma catalysis Machine learning Process optimization Dry reforming of methane Syngas production

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Improved combustion stability of biogas at different CO_(2) concentrations using inhomogeneous partially premixed stratified flames

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Global Energy Interconnection 2024年第4期7卷 486-502页

作者： Mohy Saad Mansour Maged Kiriakos Lili Hao Mohamed Amr Serag-Eldin Mechanical Power engineering {1. Cairo University1 Gamaa StreetCairo Governorate 12613Egypt Mechanical engineering {1. The American University in CairoAUC AveCairo Governorate 11835Egypt College of Electrical engineering and Control Science Nanjing Tech UniversityNanjing 211816P.R.China

Biogas is a renewable and clean energy source that plays an important role in the current environment of lowcarbon *** high-content CO_(2) in biogas can be separated,transformed,and utilized,it not only realizes high-value utilization of biogas but also promotes carbon reduction in the biogas *** improve the combustion stability of biogas,an inhomogeneous,partially premixed stratified(IPPS)combustion model was adopted in this *** thermal flame structure and stability were investigated for a wide range of mixture inhomogeneities,turbulence levels,CO_(2) concentrations,air-to-fuel velocity ratios,and combustion energies in a concentric flow slot burner(CFSB).A fine-wire thermocouple is used to resolve the thermal flame *** flame size was reduced by increasing the CO_(2) concentration and the flames became lighter *** flame temperature also decreased with increase in CO_(2) *** stability was reduced by increasing the CO_(2) ***,at a certain level of mixture inhomogeneity,the concentration of CO_(2) in the IPPS mode did not affect the ***,the IPPS mode of combustion should be suitable for the combustion and stabilization of *** should support the design of highly stabilized biogas turbulent flames independent of CO_(2) *** data show that the lower stability conditions are partially due to the change in fuel combustion energy,which is characterized by the Wobbe index(WI).In addition,at a certain level of mixture inhomogeneity,the effect of the WI on flame stability becomes dominant.

关键词： Biogas Renewable energy Effect of CO_(2) Combustion stability Burner design Renewable fuels Partial premixed

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Special issue on electrochemical energy storage and conversion

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Frontiers in Energy 2024年第2期18卷 125-127页

作者： Yun ZHENG Gaixia ZHANG Sixu DENG Jiujun ZHANG Institute of New Energy Materials and engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China department of Electrical {1. École de Technologie Supérieure(ÉTS)Universitédu QuébecMontréalH3C 1K3Canada department of Chemical and Materials {1. Concordia UniversityMontrealQC H3G 1M8Canada

The escalating global consumption of fossil fuels has significantly elevated the levels of CO_(2)in the atmosphere,leading to an undesirable global energy crisis and environmental *** deployment of renewable energy resources is crucial to mitigate these *** recent years,there has been noteworthy progress in electrochemical energy storage and conversion techniques and devices,including hydrogen energy and fuel cells,advanced energy storage and power batteries,and CO_(2)electrochemical conversion and utilization.

关键词： electrochemical energy elevated

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Reinforcement Learning-Based Energy Management for Hybrid Power Systems:State-of-the-Art Survey,Review,and Perspectives

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Chinese Journal of Mechanical engineering 2024年第3期37卷 1-25页

作者： Xiaolin Tang Jiaxin Chen Yechen Qin Teng Liu Kai Yang Amir Khajepour Shen Li College of Mechanical and Vehicle engineering Chongqing UniversityChongqing 400044China School of Mechanical engineering Beijing Institute of TechnologyBeijing 100081China department of Mechanical and Mechatronics {1. University of WaterlooWaterlooON N2L 3G1Canada School of Civil engineering Tsinghua UniversityBeijing 100084China

The new energy vehicle plays a crucial role in green transportation,and the energy management strategy of hybrid power systems is essential for ensuring energy-efficient *** paper presents a state-of-the-art survey and review of reinforcement learning-based energy management strategies for hybrid power ***,it envisions the outlook for autonomous intelligent hybrid electric vehicles,with reinforcement learning as the foundational *** of all,to provide a macro view of historical development,the brief history of deep learning,reinforcement learning,and deep reinforcement learning is presented in the form of a ***,the comprehensive survey and review are conducted by collecting papers from mainstream academic *** most of the contributions based on three main directions—algorithm innovation,powertrain innovation,and environment innovation—provides an objective review of the research ***,to advance the application of reinforcement learning in autonomous intelligent hybrid electric vehicles,future research plans positioned as“Alpha HEV”are envisioned,integrating Autopilot and energy-saving control.

关键词： New energy vehicle Hybrid power system Reinforcement learning Energy management strategy

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Non-Hermitian polarization quantized by time-reversal symmetry

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Science China(Physics,Mechanics & Astronomy) 2024年

作者： Jing Cheng Jinbing Hu Zhigao Hu Lin Chen Minghui Lu Songlin Zhuang Technical Center for Multifunctional Magneto-optical Spectroscopy (Shanghai) Engineering Research Center of Nanophotonics & Advanced Instrument (Ministry of Education)Department of Physics and Electronic Science East of China Normal University College of optical-Electrical Information and Computer {1. University of Shanghai for Science and Technology Wuhan National Laboratory for Optoelectronics and School of optical and Electronic Information Huazhong University of Science and Technology National Laboratory of Solid State Microstructures Science and engineering Nanjing University

It is well known that in one-dimensional(1.) crystalline insulators, the electric polarization is a manifestation of Berry phase,which can not be quantized by time-reversal symmetry(TRS) as in Hermitian physics TRS does not induce any topological phase in one dimension. In this paper we report that even though associated with complex eigenenergies a 1. non-Hermitian insulator obeying only TRS is capable of presenting quantized bulk polarization. The underlying physical reason is unveiled: TRS guarantees the complex energies to come in pair(E, E*), and the corresponding decaying and amplifying wave functions also come in pair and have the same variation rate, hence, giving rise to a stable wannier center. The electron transport is performed by means of charge pumping process, which verifies the physical mechanism above. At last, we discuss the possible experimental implementation of the proposed model by means of twisted-π gauge flux.

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Organic polaritonic light-emitting diodes with high luminance and color purity toward laser displays

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Light(Science & Applications) 2024年第9期13卷 1956-1963页

作者： Jianbo De Ruiyang Zhao Fan Yin Chunling Gu Teng Long Han Huang Xue Cao Cunbin An Bo Liao Hongbing Fu Qing Liao Beijing Key Laboratory for optical Materials and Photonic Devices Department of ChemistryCapital Normal University100048 BeijingChina Beijing Special engineering Design and Research Institute 100028 BeijingChina Institute of Process engineering Chinese Academy of Sciences100190 BeijingChina Institute of Molecule Plus Tianjin University and Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)300072 TianjinChina School of Materials Science and engineering Hunan University of Science and Technology411201 XiangtanHunanChina

Achieving high-luminescence organic light-emitting devices(OLEDs)with narrowband emission and high color purity is important in various optoelectronic *** displays exhibit outstanding advantages in next-generation display technologies owing to their ultimate visual experience,but this remains a great ***,we develop a novel OLED based organic single *** strongly coupling the organic exciton state to an optical microcavity,we obtain polariton electroluminescent(EL)emission from the polariton OLEDs(OPLEDs)with high luminance,narrow-band emission,high color purity,high polarization as well as excellent optically pumped polariton ***,we evaluate the potential for electrically pumped polariton laser through theoretical analysis and provide possible *** work provides a powerful strategy with a material–device combination that paves the way for electrically driven organic single-crystal-based polariton luminescent devices and possibly lasers.

关键词： pumped laser polarization

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High-resolution photogrammetry to measure physical aperture of two separated rock fracture surfaces

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Journal of Rock Mechanics and Geotechnical engineering 2024年第8期16卷 2922-2934页

作者： Masoud Torkan Mateusz Janiszewski Lauri Uotinen Alireza Baghbanan Mikael Rinne department of Civil {1. Aalto UniversityEspooFinland department of Mining {1. Isfahan University of TechnologyIsfahanIran

Photogrammetry,reconstructing three-dimensional(3D)models from overlapping two-dimensional(2D)photos,finds application in rock mechanics and rock engineering to extract geometrical details of reconstructed objects,for example rock *** properties are important for determining the mechanical stability,permeability,strength,and shear behavior of the rock *** can be used to reconstruct detailed 3D models of two separated rock fracture surfaces to characterize fracture roughness and physical aperture,which controls the fluid flow,hydromechanical and shear behavior of the rock *** research aimed to determine the optimal number of scale bars required to produce high-precision 3D models of a fracture surface.A workflow has been developed to define the physical aperture of a fracture using *** blocks of Kuru granite(25 cm×25 cm×1. cm)with an artificially induced fracture,were *** scaling 3D models,321.markers were used as ground control points(GCPs)with predefined distances on each *** the samples were wellmatched in their original positions,the entire block was *** data of the GCPs were extracted from the 3D model of the *** half was surveyed separately and georeferenced by GCPs and merged into the same coordinate *** fracture surfaces were extracted from the 3D models and the vertical distance between the two surfaces was digitally calculated as physical *** assessment of the photogrammetric reconstruction showed a 20-30 mm digital control distance accuracy when compared to known distances defined between *** attain this accuracy,the study found that at least 200 scale bars were ***,photogrammetry was employed to measure changes in aperture under normal *** results obtained from this approach were found to be in good agreement with those obtained using linear variable displacement transducers(LVDTs),with differences ran

关键词： Photogrammetry Physical aperture Rock fracture Predefined distances Markers

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Reversibly sensitizing-storing-releasing ^(1.O_(2) within a single platinum(Ⅱ)-acetylide-based metallacycle molecule via laser power modulation

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Science China Chemistry 2024年第2期67卷 604-611页

作者： Ruyi Zhou Wen Lv Bo Li Bo Yu Sudi Zhang Yucheng Zhou Shujuan Liu Qiang Zhao State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced Materials(IAM)&Institute of Flexible Electronics(Future Technology)Nanjing University of Posts and Telecommunications(NUPT)Nanjing210023China College of Electronic and optical {1.&College of Flexible Electronics(Future Technology) Jiangsu Province Engineering Research Center for Fabrication and Application of Special Optical Fiber Materials and DevicesNanjing University of Posts and Telecommunications(NUPT)Nanjing210023China

Tumor hypoxia severely limits the therapeutic efficacy of photodynamic therapy(PDT) for solid tumors,which is highly dependent on tissue oxygen *** this study,we developed a platinum(Ⅱ)-acetylide-based metallacycle compound bearing six 1.4-dimethylnaphthalenes(DMN) groups,and controlled the photodynamic and photothermal effects of the compound by adjusting the power of 730 nm laser to achieve reversible sensitization,storage and release of 1.O_(2) within a single *** compound formed nanoparticles by self-assembly and exhibited good water solubility and *** laser irradiation,the strong spin-orbit coupling of platinum atoms in the metallacycle facilitated 1.O_(2) *** produced 1.O_(2) was captured by the DMN carriers and transported into the hypoxic tumor,where 1.O_(2) release was triggered owing to the good photothermal effect of the extended conjugation of the *** therapy,the metallacycle serving as a photosensitizer,1.O_(2) carrier,and photothermal reagent,achieved the synergistic therapy of PDT/PTT,demonstrating the versatility of the *** study proposes a new strategy to develop phototherapy agents that are suitable for hypoxic tumors.

关键词： metallacycles singlet oxygen endoperoxides near-infrared absorption synergistic treatment

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