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Rare earth-doped mixed Ni-Cu-Zn ferrites as an effective photocatalytic agent for active degradation of Rhodamine B dye

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Journal of Rare Earths 2024年第3期42卷 488-496,I0003页

作者： Swapnil A.Jadhav Sandeep B.Somvanshi Sudarshan S.Gawali Kranti Zakde K.M.Jadhav department of {1. Dr.Babasaheb Ambedkar Marathwada UniversityAurangabad431004MaharashtraIndia School of Materials Engineering Purdue UniversityWest Lafayette 47906USA University department of Basic and {1. Sciences MGM UniversityAurangabad431003MaharashtraIndia

In this study, a series of Gd^(3+)-doped mixed Ni-Cu-Zn ferrites with composition of Zn_(0.5)Ni_(0.3)Cu_(0.2)Fe_(2-x)Gd_(x)O_(4)(x = 0, 0.025, 0.05, 0.075, 0.1. was prepared using self-ignition sol-gel method. The prepared nanoparticles with an average size ranging from 22 to 26 nm show a single-phase cubic structure belonging to the spinel matrix. A rise in the Gd^(3+)concentration leads to an increase in crystallite size and lattice parameter. In Fourier transform infrared spectra, two main absorption bands belonging to the spinel structure are observed. The high-frequency bands(v_(1.) represent the tetrahedral complex, while the lowfrequency bands(v_(2)) signify the octahedral complex. The optical bandgap of the nanoferrites is found within the range of 2.91.to 2.41.eV, depending on their size. The magnetic characteristics of the material,such as saturation magnetization and coercivity are significantly altered with the concentration of Gd^(3+)in the solution. Using Rhodamine B(RhB) as a model organic pollutant, an in-depth investigation of the photocatalytic activity of the compounds was carried out. The present outcomes show that adding an adequate amount of Gd^(3+)significantly enhances the number of hydroxyl radicals produced by the ferrite,in turn, increasing the photocatalytic activity of the material. Mechanism elucidated by scavenger studies reveals that ·OH and holes are the primary reactive radicals responsible for the degradation *** photocatalysts show an insignificant performance loss in five consecutive cycles. Thus, it is concluded that these photocatalysts are highly suitable for the remediation of dye-contaminated wastewater.

关键词： Gd^(3+)substitution Spinel ferrite Structural properties Magnetic properties Photocatalysis Rare earths

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Stabilized Nickel-Rich-Layered Oxide Electrodes for High-Performance Lithium-Ion Batteries

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Energy & Environmental Materials 2024年第6期7卷 60-73页

作者： Zahra Ahaliabadeh Ville Miikkulainen Miia Mäntymäki Mattia Colalongo Seyedabolfazl Mousavihashemi Lide Yao Hua Jiang Jouko Lahtinen Timo Kankaanpää Tanja Kallio department of Chemistry and Materials Science(CMAT) School of Chemical EngineeringAalto University02150 EspooFinland department of Chemistry University of Helsinki00014 HelsinkiFinland department of {1. physics School of ScienceAalto University02150 EspooFinland Umicore Finland Oy 67101 KokkolaFinland

This work made use of the Aalto University Otanano-Nanomicroscopy Center and RAMI *** support from Business Finland NextGenBat[grant number 21.849]is greatly *** tomography experiment was performed at the beamline ID1.B of the European Synchrotron Radiation Facility(ESRF),Grenoble,France,in the frame of proposal *** patent titled“Stabilized Positive Electrode Material to Enable High Energy and Power Density Lithium-Ion Batteries”(IPD31.3)is pertinent to this *** was filed by Zahra Ahaliabadeh and Tanja Kallio,and the patent rights are held by Aalto University.

关键词： degradation mechanisms electrolyte decomposition hybrid coatings lithium-ion battery lithium-ion kinetics molecular layer deposition NMC81.

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A deep learning interatomic potential suitable for simulating radiation damage in bulk tungsten

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Tungsten 2024年第2期6卷 304-322页

作者： Chang-Jie Ding Ya-Wei Lei Xiao-Yang Wang Xiao-Lin Li Xiang-Yan Li Yan-Ge Zhang Yi-Chun Xu Chang-Song Liu Xue-Bang Wu Key Laboratory of Materials physics Institute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China Science Island University of Science and Technology of ChinaHefei 230026China Laboratory of Computational physics Institute of Applied Physics and Computational MathematicsBeijing 100088China

So far, it has been a challenge for existing interatomic potentials to accurately describe a wide range of physical properties and maintain reasonable efficiency. In this work, we develop an interatomic potential for simulating radiation damage in body-centered cubic tungsten by employing deep potential, a neural network-based deep learning model for representing the potential energy surface. The resulting potential predicts a variety of physical properties consistent with first-principles calculations, including phonon spectrum, thermal expansion, generalized stacking fault energies, energetics of free surfaces, point defects, vacancy clusters, and prismatic dislocation loops. Specifically, we investigated the elasticity-related properties of prismatic dislocation loops, i.e., their dipole tensors, relaxation volumes, and elastic interaction energies. This potential is found to predict the maximal elastic interaction energy between two 1.2 1.1.1. loops better than previous potentials, with a relative error of only 7.6%. The predicted threshold displacement energies are in reasonable agreement with experimental results, with an average of 1.8 eV. The efficiency of the present potential is also comparable to the tabulated gaussian approximation potentials and modified embedded atom method potentials, meanwhile, can be further accelerated by graphical processing units. Extensive benchmark tests indicate that this potential has a relatively good balance between accuracy, transferability, and efficiency.

关键词： Machine learning Deep learning Interatomic potential Radiation damage Tungsten

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Research on Multi-Scale Feature Fusion Network Algorithm Based on Brain Tumor Medical Image Classification

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Computers, Materials & Continua 2024年第6期79卷 5313-5333页

作者： Yuting Zhou Xuemei Yang Junping Yin Shiqi Liu Graduate School China Academy of Engineering PhysicsBeijing100000China department of Computational Mathematics Beijing Institute of Applied Physics and Computational MathematicsBeijing100000China National Key Laboratory of Computational physics Beijing100088China Shanghai Zhangjiang Institute of Mathematics Shanghai201203China

Gliomas have the highest mortality rate of all brain *** classifying the glioma risk period can help doctors make reasonable treatment plans and improve patients’survival *** paper proposes a hierarchical multi-scale attention feature fusion medical image classification network(HMAC-Net),which effectively combines global features and local *** network framework consists of three parallel layers:The global feature extraction layer,the local feature extraction layer,and the multi-scale feature fusion layer.A linear sparse attention mechanism is designed in the global feature extraction layer to reduce information *** the local feature extraction layer,a bilateral local attention mechanism is introduced to improve the extraction of relevant information between adjacent *** the multi-scale feature fusion layer,a channel fusion block combining convolutional attention mechanism and residual inverse multi-layer perceptron is proposed to prevent gradient disappearance and network degradation and improve feature representation *** double-branch iterative multi-scale classification block is used to improve the classification *** the brain glioma risk grading dataset,the results of the ablation experiment and comparison experiment show that the proposed HMAC-Net has the best performance in both qualitative analysis of heat maps and quantitative analysis of evaluation *** the dataset of skin cancer classification,the generalization experiment results show that the proposed HMAC-Net has a good generalization effect.

关键词： Medical image classification feature fusion transformer

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Synergistic enhancement of ultrasound therapy for tumors using hypoxia-activated 6-diazo-5-oxo-L-norleucine(DON)prodrug nanoparticles

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Nano Research 2024年第7期17卷 6323-6331页

作者： Mengfei Zheng Zhilin Liu Hang Xu Daping Ye Linjie Cui Chenguang Yang Lili Ma Kun Wang Kazuo Sakurai Zhaohui Tang Key Laboratory of Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China Jilin Biomedical Polymers Engineering Laboratory Changchun 130022China department of Chemistry and Biochemistry The University of Kitakyushu1-1 HibikinoKitakyushu 808-0135Japan

Ultrasound(US)has been applied in clinical practice for its non-invasive and high ***,it is difficult to achieve a satisfactory anti-tumor effect with US ***,the use of US therapy alone can exacerbate tumor *** this study,we prepared hypoxia-activated 6-diazo-5-oxo-L-norleucine(DON)prodrug nanoparticles(HDON-NPs)to improve US therapeutic *** an H22 murine liver cancer model,US therapy selectively disrupted tumor blood vessels,leading to increased tumor hypoxia and a 1.67-fold increase in the expression of nitroreductase(NTR).The combination therapy of US and HDON-NPs demonstrated a synergistic effect,resulting in a tumor suppression rate(TSR)of 90.2%±6.4%,which was 5.93-fold higher than that of US therapy *** combined treatment selectively blocked the glutamine metabolism of the tumor cells while simultaneously activating the T cells in the tumor microenvironment,thereby exerting a robust anti-tumor effect.

关键词： ultrasound therapy hypoxia-activated prodrug nanoparticles 6-diazo-5-oxo-L-norleucine(DON) glutamine antagonist starvation therapy

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Point-symmetry in SNR G1.9+0.3:A Supernova that Destroyed its Planetary Nebula Progenitor

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Research in Astronomy and Astrophysics 2024年第1期24卷 165-172页

作者： Noam Soker department of {1. TechnionHaifa3200003Israel

I analyze a new X-ray image of the youngest supernova remnant(SNR)in the Galaxy,which is the type Ia SNR G1.9+0.3,and reveal a very clear point-symmetrical *** explosion models of type Ia supernovae(SNe Ia)do not form such morphologies,the point-symmetrical morphology must come from the circumstellar material(CSM)into which the ejecta *** large-scale point-symmetry that I identify and the known substantial deceleration of the ejecta of SNR G1.9+0.3 suggest a relatively massive CSM of■1.⊙.I argue that the most likely explanation is the explosion of this SN Ia into a planetary *** scenario that predicts a large fraction of SN Ia inside PNe(SNIPs)is the core degenerate *** SN Ia scenarios might lead to only a very small fraction of SNIPs or none at all.

关键词： (stars:)supernovae:general ISM:supernova remnants (stars:)binaries(including multiple):close (ISM:)planetary nebulae:general stars:jets

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Ultrahigh-brightness 50 MeV electron beam generation from laser wakefield acceleration in a weakly nonlinear regime

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Matter and Radiation at Extremes 2024年第3期9卷 4-10页

作者： Zhongtao Xiang Changhai Yu Zhiyong Qin Xuhui Jiao Jiahui Cheng Qiaoxuan Zhou Gatie Axi Jianghua Jie Ya Huang Jintan Cai Jiansheng Liu department of {1. Shanghai Normal UniversityShanghai 200234China

We propose an efficient scheme to produce ultrahigh-brightness tens of MeV electron beams by designing a density-tailored plasma to induce a wakefield in the weakly nonlinear regime with a moderate laser energy of 1.0 *** this scheme,the second bucket of the wakefield can have a much lower phase velocity at the steep plasma density down-ramp than the first bucket and can be exploited to implement longitudinal electron injection at a lower laser intensity,leading to the generation of bright electron beams with ultralow emittance together with low energy ***-dimensional particle-in-cell simulations are carried out and demonstrate that high-quality electron beams with a peak energy of 50 MeV,ultralow emittance of28 nm rad,energy spread of 1.,charge of 4.4 pC,and short duration less than 5 fs can be obtained within a 1.mm-long tailored plasma density,resulting in an ultrahigh six-dimensional brightness B6D,n of2×1.1. A/m2/0.1..By changing the density parameters,tunable bright electron beams with peak energies ranging from 5 to 70 MeV,a small emittance of B0.1.mm mrad,and a low energy spread at a few-percent level can be *** bright MeV-class electron beams have a variety of potential applications,for example,as ultrafast electron probes for diffraction and imaging,in laboratory astrophysics,in coherent radiation source generation,and as injectors for GeV particle accelerators.

关键词： weakly nonlinear acceleration

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Effect of Eu3+,Bi3+,and Li+ doping on luminescent property of GdNbO4

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Journal of Rare Earths 2024年第1期42卷 66-75页

作者： S.W.Wi Y.S.Lee department of {1. and Integrative Institute of Basic Sciences Soongsil University

We investigated the emission properties of Eu3+-doped GdNbO4-based oxide phosphors,aiming at improving the Eu3+emission by codoping of Bi3+and Li+.Eu3+singly doped,Eu3+and Bi3+doubly doped,and Eu3+,Bi3+,and Li+triply doped GdNbO4were prepared using a high-temperature solid-state reaction *** red-orange emissions from Eu3+in the singly doped samples are significantly improved by the codoping of Bi3+,mainly due to the energy transfer from Bi3+to Eu3+.The additional codoping of Li+is found to increase the Eu3+emission *** improvement might be attributed to the increase in the photoluminescent quantum yield originating from larger grain sizes and better crystallinity.A detailed analysis of the X-ray diffraction pattern and the asymmetric ratio estimated from the photoluminescence spectra show that the local lattice environment around Eu3+in GdNbO4does not change significantly with the codoping of Bi3+and Li+.Our results indicate that Li+doping is a promising way to improve the emission properties of rare-earth ion-doped GdNbO4phosphors.

关键词： Eu 3+ GdNbO 4 Codoping of Li + Photoluminescence Sensitizer Rare earths

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Nondegenerate Soliton Solutions of(2+1.-Dimensional Multi-Component Maccari System

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Chinese physics Letters 2024年第6期41卷 11-17页

作者：孟勇方乒乒林机 department of {1. Zhejiang Normal UniversityJinhua 321004China

For a multi-component Maccari system with two spatial dimensions,nondegenerate one-soliton and two-soliton solutions are obtained with the bilinear *** can be seen by drawing the spatial graphs of nondegenerate solitons that the real component of the system shows a cross-shaped structure,while the two solitons of the complex component show a multi-solitoff *** the same time,the asymptotic analysis of the interaction behavior of the two solitons is conducted,and it is found that under partially nondegenerate conditions,the real and complex components of the system experience elastic collision and inelastic collision,respectively.

关键词： structure. degenerate soliton

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Parametric“non-nested”discriminants for multiplicities of univariate polynomials

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Science China Mathematics 2024年第8期67卷 1911-1932页

作者： Hoon Hong Jing Yang department of Mathematics North Carolina State UniversityRaleighNC 27695USA SMS-HCIC-School of Mathematics and physics Center for Applied Mathematics of GuangxiGuangxi Minzu UniversityNanning 530006China

We consider the problem of complex root classification,i.e.,finding the conditions on the coefficients of a univariate polynomial for all possible multiplicity structures on its complex *** is well known that such conditions can be written as conjunctions of several polynomial equalities and one inequality in the *** polynomials in the coefficients are called discriminants for *** is also known that discriminants can be obtained using repeated parametric greatest common *** resulting discriminants are usually nested determinants,i.e.,determinants of matrices whose entries are determinants,and so *** this paper,we give a new type of discriminant that is not based on repeated greatest common *** new discriminants are simpler in the sense that they are non-nested determinants and have smaller maximum degrees.

关键词： parametric polynomial complex roots discriminant multiplicity resultant

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