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Recent advances and perspectives of zinc metal-free anodes for zinc ion batteries

International Journal of Minerals,metallurgy and Materials 2024年第1期31卷 33-47页

作者： Jiabing Miao Yingxiao Du Ruotong Li Zekun Zhang Ningning Zhao Lei Dai Ling Wang Zhangxing He Science and Technology Innovation Center of Circular Economy Ha’erwusu Open-Pit Coal MineChina Shenhua Energy Co.Ltd.Ordos 010300China Research Center of Comprehensive Utilization of Coal Associated Resources National Energy GroupOrdos 010300China School of Chemical Engineering North China University of Science and TechnologyTangshan 063009China

zinc-ion batteries(ZIBs) are recognized as potential energy storage devices due to their advantages of low cost, high energy density, and environmental friendliness. However, zinc anodes are subject to unavoidable zinc dendrites, passivation, corrosion, and hydrogen evolution reactions during the charging and discharging of batteries, becoming obstacles to the practical application of ZIBs. Appropriate zinc metal-free anodes provide a higher working potential than metallic zinc anodes, effectively solving the problems of zinc dendrites, hydrogen evolution, and side reactions during the operation of metallic zinc anodes. The improvement in the safety and cycle life of batteries creates conditions for further commercialization of ZIBs. Therefore, this work systematically introduces the research progress of zinc metal-free anodes in “rocking chair” ZIBs. zinc metal-free anodes are mainly discussed in four categories: transition metal oxides,transition metal sulfides, MXene(two dimensional transition metal carbide) composites, and organic compounds, with discussions on their properties and zinc storage mechanisms. Finally, the outlook for the development of zinc metal-free anodes is proposed. This paper is expected to provide a reference for the further promotion of commercial rechargeable ZIBs.

关键词： zinc ion batteries anode zinc metal-free anode recent advances perspectives

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Research progress of“rocking chair”type zinc-ion batteries with zinc metal-free anodes

引用

Chinese Chemical Letters 2023年第12期34卷 42-52页

作者： Le Li Shaofeng Jia Minghui Cao Yongqiang Ji Hengwei Qiu Dan Zhang Shanxi Key Laboratory of Industrial Automation School of Mechanical EngineeringShaanxi University of TechnologyHanzhong 723001China Shaanxi Key Laboratory of Catalysis School of Chemistry and Environment ScienceShaanxi University of TechnologyHanzhong 723001China School of Electronic and Information Engineering Qingdao UniversityQingdao 266071China Department of Chemistry Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical BiologyTsinghua UniversityBeijing 100084China State Key Laboratory for Artifcial Microstructure and Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China

"Rocking chair"type lithium-ion batteries with lithium metal-free anodes have been successfully com-mercialized over the past few ***-ion batteries(zIBs)have gained increasing attention in recent years given their safety,greenness,ease of manufacture,and ***,the practical application of ZIBs is largely hindered by the dendritic growth of the Zn metal anode,low Coulombic eficiency,great harm,and existence of various side ***,this review provides a systematic overview of emerging"rocking chair"type ZIBs with zinc metal-free ***,the basic fundamen-tals,advantages,and challenges of“rocking chair”type ZIBs are ***,an overview of the design principles and recent progress of"rocking chair"type ZIBs with zinc metal-free anodes are ***,the key challenges and perspectives for future advancement of"rocking chair"type ZiBs with zinc metal-free anodes are *** review is anticipated to attracted increased focus to metal-free anodes"rocking chair"type metal-ion battery and provide new inspirations for the develop-ment of high-energy metal-ion batteries.

关键词： zinc ion batteries(ZIBs) "Rocking chair"type zinc metal-free anode Transition metal dichalcogenides Transition metal oxides Organic compounds

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