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Recent advances and perspectives of zinc metal-free anodes for zinc ion batteries

International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 33-47页

作者： Jiabing Miao Yingxiao Du Ruotong Li Zekun Zhang Ningning Zhao Lei Dai Ling Wang Zhangxing He Science and Technology Innovation Center of Circular Economy Ha’erwusu Open-Pit Coal MineChina Shenhua Energy Co.Ltd.Ordos 010300China Research Center of Comprehensive Utilization of Coal Associated Resources National Energy GroupOrdos 010300China School of Chemical Engineering North China University of Science and TechnologyTangshan 063009China

zinc-ion batteries(ZIBs) are recognized as potential energy storage devices due to their advantages of low cost, high energy density, and environmental friendliness. However, zinc anodes are subject to unavoidable zinc dendrites, passivation, corrosion, and hydrogen evolution reactions during the charging and discharging of batteries, becoming obstacles to the practical application of ZIBs. Appropriate zinc metal-free anodes provide a higher working potential than metallic zinc anodes, effectively solving the problems of zinc dendrites, hydrogen evolution, and side reactions during the operation of metallic zinc anodes. The improvement in the safety and cycle life of batteries creates conditions for further commercialization of ZIBs. Therefore, this work systematically introduces the research progress of zinc metal-free anodes in “rocking chair” ZIBs. zinc metal-free anodes are mainly discussed in four categories: transition metal oxides,transition metal sulfides, MXene(two dimensional transition metal carbide) composites, and organic compounds, with discussions on their properties and zinc storage mechanisms. Finally, the outlook for the development of zinc metal-free anodes is proposed. This paper is expected to provide a reference for the further promotion of commercial rechargeable ZIBs.

关键词： zinc ion batteries anode zinc metal-free anode recent advances perspectives

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Recent advances in interfacial modification of zinc anode for aqueous rechargeable zinc ion batteries

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能源化学:英文版 2023年第8期83卷 287-303,I0009页

作者： Qing Wen Hao Fu Ru-de Cui He-Zhang Chen Rui-Han Ji Lin-Bo Tang Cheng Yan Jing Mao Ke-Hua Dai Xia-Hui Zhang Jun-Chao Zheng School of Metallurgy and Environment Central South UniversityChangsha 410083HunanChina Engineering Research Center of the Ministry of Education for Advanced Battery Materials Central South UniversityChangsha 410083HunanChina School of Chemistry and Chemical Engineering Hunan University of Science and TechnologyXiangtan 411201HunanChina School of Mechanical Medical and Process EngineeringQueensland University of TechnologyBrisbaneQueensland 4001Australia School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001HenanChina College of Chemistry Tianjin Normal UniversityTianjin 300387China School of Mechanical and Materials Engineering Washington State UniversityPullman 99164WashingtonUnited States

To tackle energy crisis and achieve sustainable development, aqueous rechargeable zinc ion batteries have gained widespread attention in large-scale energy storage for their low cost, high safety, high theoretical capacity, and environmental compatibility in recent years. However, zinc anode in aqueous zinc ion batteries is still facing several challenges such as dendrite growth and side reactions(e.g., hydrogen evolution), which cause poor reversibility and the failure of batteries. To address these issues, interfacial modification of Zn anodes has received great attention by tuning the interaction between the anode and the electrolyte. Herein, we present recent advances in the interfacial modification of zinc anode in this review. Besides, the challenges of reported approaches of interfacial modification are also ***, we provide an outlook for the exploration of novel zinc anode for aqueous zinc ion *** hope that this review will be helpful in designing and fabricating dendrite-free and hydrogenevolution-free Zn anodes and promoting the practical application of aqueous rechargeable zinc ion batteries.

关键词： zinc ion batteries zinc anode Interfacial modification Functional coating

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Oxide-based cathode materials for rechargeable zinc ion batteries:Progresses and challenges

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Journal of Energy Chemistry 2021年第6期30卷 516-542,I0013页

作者： Yingze Zhou Fandi Chen Hamidreza Arandiyan Peiyuan Guan Yunjian Liu Yuan Wang Chuan Zhao Danyang Wang Dewei Chu School of Materials Science and Engineering The University of New South WalesSydney 2052Australia Laboratory of Advanced Catalysis for Sustainability School of ChemistryThe University of SydneySydney 2006Australia The University of Sydney Nano Institute(Sydney Nano) The University of SydneyNSW 2006Australia School of Material Science and Technology Jiangsu UniversityZhenjiang 212013JiangsuChina School of Chemistry The University of New South WalesSydneyNew South Wales 2052Australia

With the increasing demands for electrical energy storage technologies,rechargeable zinc ion batteries(ZIBs)have been rapidly developed in recent years owing to their high safety,low cost and high energy storage *** cathode is an essential part of ZIBs,which hosts zinc ions and determines the capacity,rate and cycling performance of the *** mainstream cathodes for ZIBs are oxidebased materials with tunnel,layer or 3 D crystal *** this review,we mainly focus on the latest advanced oxide-based cathode materials in ZIBs,including manganese oxides,vanadium oxides,spinel compounds,and other metal oxide based *** addition,the mechanisms of zinc storage and recent development in cathode design have been discussed in ***,current challenges and perspectives for the future research directions of oxide-based cathodes in ZIBs are presented.

关键词： zinc ion batteries Oxide-based cathode Manganese oxides cathode Vanadium oxides cathode

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Recent advances and perspectives on vanadium-and manganese-based cathode materials for aqueous zinc ion batteries

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Journal of Energy Chemistry 2021年第8期30卷 134-159,I0004页

作者： Na Liu Bin Li Zhangxing He Lei Dai Haiyan Wang Ling Wang School of Chemical Engineering North China University of Science and TechnologyTangshan 063009China Hunan Provincial Key Laboratory of Chemical Power Sources Hunan Provincial Key Laboratory of Efficient and Clean Utilization of Manganese ResourcesCollege of Chemistry and Chemical EngineeringCentral South UniversityChangsha 410083China

The growing demand for energy storage has inspired researchers’exploration of advanced *** zinc ion batteries(ZIBs)are promising secondary chemical battery system that can be selected and *** ZIBs possess merits of high security,low cost,environmental friendliness,and competitive performance,and they are received a lot of ***,the development of suitable zinc ion intercalation-type cathode materials is still a big challenge,resulting in failing to meet the commercial needs of *** vanadium-based and manganese-based compounds are representative of the most advanced and most widely used rechargeable ZIBs *** valence state of vanadium is+2~+5,which can realize multi-electron transfer in the redox reaction and has a high specific *** of the manganese-based compounds have tunnel structure or three-dimensional space frame,with enough space to accommodate zinc *** order to understand the energy storage mechanism and electrochemical performance of these two materials,a specialized review focusing on state-of-the-art developments is *** review offers access for researchers to keep abreast of the research progress of cathode materials for *** latest advanced researches in vanadium-based and manganese-based cathode materials applied in aqueous ZIBs are *** article will provide useful guidance for future studies on cathode materials and aqueous ZIBs.

关键词： zinc ion batteries Cathode Vanadium-based materials Manganese-based materials Recent advances

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Plasma-inducedε-MnO_(2)based aqueous zinc-ion batteries and their dissolution-deposition mechanism

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Journal of Materials Science & Technology 2022年第32期127卷 206-213页

作者： Le Zhang Shuhua Yang Wenqing Fu Yanwei Cui Jieqiang Wang Degang Zhao Chao Yang Xiutong Wang Bingqiang Cao Materials Center for Energy and Photoelectrochemical Conversion School of Material Science and EngineeringUniversity of JinanJinan 250022China School of Physics and Physical Engineering Qufu Normal UniversityQufu 273165China Key Laboratory of Marine Environmental Corrosion and Bio-fouling Institute of Oceanology and Center for Ocean Mega-ScienceChinese Academy of SciencesQingdao 266071China

MnO_(2)has attracted great interest in working as the cathode of zinc ion ***,the development of high-capacity,high-energy-density,and durable manganese-based cathodes with an easy synthesis strategy and proper energy storage mechanism remains an ongoing ***,a facile plasmainduced strategy was demonstrated to introduce oxygen vacancies into theε-MnO_(2),and the obtained oxygen vacancies-richε-MnO_(2)nanosheets(ε-MnO_(2-x))show satisfactory electrochemical ***,an appropriate energy storage mechanism for dissolution/deposition was *** to a synergistic effect of the oxygen vacancies inε-MnO_(2)nanosheets and the exposed free-standing collector for Mn^(2+) dissolution/deposition,theε-MnO_(2-x) nanosheets electrode delivers a remarkable capacity(337 mAh g^(-1)at 0.1 A g^(-1))and exhibits an ultrahigh energy density of 462 Wh kg^(-1)(based on the weights of the cathode active material).Furthermore,impressive durability with 85.9%capacity retention after 1000 cycles was *** superior electrochemical performance makes the plasma-induced strategy promising for designing advanced metal oxide electrode materials for high-performance aqueous zinc ion batteries.

关键词： Plasma-induced strategy ε-MnO_(2) Oxygen vacancies Dissolution/deposition zinc ion batteries

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In-situ formation of hierarchical solid-electrolyte interphase for ultra-long cycling of aqueous zinc-ion batteries

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Nano Research 2023年第1期16卷 449-457页

作者： Shaojie Zhang Jiajia Ye Huaisheng Ao Mingying Zhang Xilong Li Zhibin Xu Zhiguo Hou Yitai Qian School of Chemistry and Chemical Engineering Shandong UniversityJinan 250100China School of Chemistry and Material Science University of Science and Technology of ChinaHefei 230026China

Aqueous rechargeable zinc ion batteries have received widespread attention due to their high energy density and low ***,zinc metal anodes face fatal dendrite growth and detrimental side reactions,which affect the cycle stability and practical application of zinc ion ***,an in-situ formed hierarchical solid-electrolyte interphase composed of InF3,In,and ZnF2 layers with outside-in orientation on the Zn anode(denoted as Zn@InF3)is developed by a sample InF3 *** inner ultrathin ZnF2 interface between Zn anode and InF3 layer formed by the spontaneous galvanic replacement reaction between InF3 and Zn,is conductive to achieving uniform Zn deposition and inhibits the growth of zinc dendrites due to the high electrical resistivity and Zn2+***,the middle uniformly generated metallic In and outside InF3 layers functioning as corrosion inhibitor suppressing the side reaction due to the waterproof surfaces,good chemical inactivity,and high hydrogen evolution ***,the as-prepared zinc anode enables dendrite-free Zn plating/stripping for more than 6,000 h at nearly 100%coulombic efficiency(CE).Furthermore,coupled with the MnO2 cathode,the full battery exhibits the long cycle of up to 1,000 cycles with a low negative-to-positive electrode capacity(N/P)ratio of 2.8.

关键词： zinc ion batteries solid-electrolyte interphase in-situ formation hierarchical coating

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Tuning the layer structure of molybdenum trioxide towards high-performance aqueous zinc-ion batteries

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Chinese Chemical Letters 2023年第4期34卷 489-494页

作者： Yu Tan Jinjun He Bo Wang Cheng Chao Li Taihong Wang College of Materials Science and Engineering Hunan UniversityChangsha 410082China School of Chemical Engineering and Light Industry Guangdong University of TechnologyGuangzhou 510006China School of Chemistry Sun Yat-sen UniversityGuangzhou 510275China Department of Electrical and Electronic Engineering Southern University of Science and TechnologyShenzhen 518055China College of Chemistry and Materials Science Hunan Agriculture UniversityChangsha 410128China

Aqueous zinc-ion batteries(ZIBs) have attracted significant attentions because of low cost and high reliability. However, conventional ZIBs are severely limited by the development of high energy density cathode materials with reversible Zn^(2+)insertion/extraction. Herein, a conducting polymer intercalated MoO_(3)(PMO) with extensively extended interlayer spacing is developed as a high-performance ZIBs cathode material. The interlayer spacing of PMO is prominently increased which results in an improved Zn^(2+)mobility during charge and discharge process. More significantly, the electrochemical results reveals that the intercalation of PANI facilitates the charge storage and reinforces the layered structure of MoO_(3), leading to a high capacity and good cycling stability. DFT calculation further reveals the intercalation of PANI into MoO_(3)significantly lower Zn^(2+)diffusion barrier. Benefit from these advantages, the ZIBs based on PMO electrode delivers a considerable capacity of 157 m Ah/g at 0.5 A/g and ameliorative stability with 63.4%capacity retention after 1000 cycles.

关键词： Molybdenum trioxide Cathode zinc ion batteries Polyaniline intercalation Layered structure

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Charge storage mechanism of MOF-derived Mn2O3 as high performance cathode of aqueous zinc-ion batteries

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Journal of Energy Chemistry 2021年第1期30卷 277-283,I0009页

作者： Min Mao Xingxing Wu Yi Hu Qunhui Yuan Yan-Bing He Feiyu Kang Tsinghua Shenzhen International Graduate School Division of Energy&EnvironmentTsinghua UniversityShenzhen 518055GuangdongChina Laboratory of Advanced Materials Department of Materials Science and EngineeringTsinghua UniversityBeijing 100084China State Key Laboratory of Advanced Welding and Joining and School of Materials Science and EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055GuangdongChina

Aqueous zinc-ion batteries(ZIB) are attracting immense attention because of their merits of excellent safety and quite cheap properties compared with lithium-ion batteries(LIB).Manganese oxide is one of the most important cathode materials of *** this paper,α-Mn2O3 used as cathode of ZIB is synthesized via Metal-Organic Framework(MOF)-derived method,which delivers a high specific capacity of225 mAh g^(-1) at 0.05 A g^(-1) and 92.7 mAh g^(-1) after 1700 cycles at 2 A g^(-1).The charge storage mechanism of α-Mn2O3 cathode is found to greatly depend on the discharge current *** lower current density discharging,the H+ and Zn2+ are successively intercalated into the α-Mn2O3 before and after the "turning point" of discharge voltage and their discharging products present obviously different morphologies changing from flower-like to large plate-like *** a higher current density,the low-voltage plateau after the turning point disappears due to the decrease of amount of Zn2+ intercalation and the H+intercalation is dominated in α-Mn2 *** study provides significant understanding for future design and research of high-performance Mn-based cathodes of ZIB.

关键词： zinc ion batteries α-Mn2O3 Metal-organic framework(MOF) Charge storage mechanism

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Molecular crowding electrolytes for stabilizing Zn metal anode in rechargeable aqueous batteries

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Chinese Chemical Letters 2024年第7期35卷 445-451页

作者： Li Lin Song-Lin Tian Zhen-Yu Hu Yu Zhang Li-Min Chang Jia-Jun Wang Wan-Qiang Liu Qing-Shuang Wang Fang Wang School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China School of Life Science and Technology Changchun University of Science and TechnologyChangchun 130022China Key Laboratory of Preparation and Applications of Environmental Friendly Materials of the Ministry of Education Jilin Normal UniversityChangchun 130103China Zhongshan Institute of Changchun University of Science and Technology Zhongshan 528437China

A solid electrolyte interphase(SEI)with a robust mechanical property and a high ionic conductivity is imperative for high-performance zinc metal ***,it is difficult to form such a SEI directly from an *** this work,a molecular crowding effect is based on the introduction of Zn(OTF)_(2)and Zn(ClO_(4))_(2)to 2 mol/L ZnSO_(4)*** and experiments indicate that the Zn(OTF)_(2)and Zn(ClO_(4))_(2)not only create a molecularly crowded electrolyte environment to promote the interaction of Zn^(2+)and OTF^(-),but also participate in the reduction to construct a robust and high ionic-conductive SEI,thus promoting metal zinc deposition to the(002)crystal *** this molecular crowding electrolyte,a high current density of 1 mA/cm^(2)can be obtained by assembling symmetric batteries with Zn as the anode for over 1000 *** in a temperature environment of-10℃,a current density of 1 mA/cm^(2)can be obtained by assembling symmetric batteries with Zn for over 200 ***//Bi_(2)S_(3)/VS4@C cells achieve a CE rate of up to 99.81%over 1000 ***,the utilization of a molecular crowding electrolyte is deemed a highly effective approach to fabricating a sophisticated SEI for a zinc anode.

关键词： zinc ion batteries Anode Electrolyte Solid electrolyte interphase Molecular crowding effect

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Dynamic reconstruction of Ni-Zn alloy solid-electrolyte interface for highly stable Zn anode

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Nano Research 2023年第9期16卷 11604-11611页

作者： Qian Zhang Yuhang Dai Kangning Zhao Chengyi Zhang Ruihu Lu Jinghao Li Shuhan Jin Lei Zhang Qinyou An Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Department of Physical Science and Technology School of ScienceWuhan University of TechnologyWuhan 430070China Hainan Institute Wuhan University of TechnologySanya 572000China

Aqueous zinc ion batteries(AZIBs)are ideal candidates for large-scale battery storage,with a high theoretical specific capacity,ecological friendliness,and extremely low cost but are strongly hindered by zinc dendrite ***,Ni-Zn alloy is artificially constructed as a solid-electrolyte interface(SEI)for Zn anodes by electrodeposition and *** Ni-Zn alloy layer acts as a dynamic shield at the electrode/electrolyte ***,the zinc atoms migrate out of the electrode body during zinc stripping while merging into the electrode body during the *** this way,the Ni-Zn alloy is able to guide the zinc deposition in the horizontal direction,thereby suppressing the formation of *** from those,the Ni-Zn alloy symmetric cell shows a greatly improved cycle life and is able to operate stably for 1,900 h at a current density of 0.5 mA·cm^(−2).The present study is a strategy for negative electrode protection of AZIBs.

关键词： zinc ion batteries Zn anodes Ni-Zn alloy migration mechanism

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