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Surface-functionalized hole-selective monolayer for high efficiency single-junction wide-bandgap and monolithic tandem perovskite solar cells

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Journal of Energy Chemistry 2024年第1期88卷 317-326,I0008页

作者： Devthade Vidyasagar Yeonghun Yun Jae Yu Cho Hyemin Lee Kyung Won Kim Yong Tae Kim Sung Woong Yang Jina Jung Won Chang Choi Seonu Kim Rajendra Kumar Gunasekaran Seok Beom Kang Kwang Heo Dong Hoe Kim Jaeyeong Heo Sangwook Lee School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Department of Materials Science and Engineering and Optoelectronics Convergence Research CenterChonnam National UniversityGwangju 61186Republic of Korea Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea Department of Nanotechnology and Advanced Materials Engineering Sejong UniversitySeoul 05006Republic of Korea

Carbazole moiety-based 2PACz([2-(9H-carbazol-9-yl)ethyl]phosphonic acid)self-assembled monolayers(SAMs)are excellent hole-selective contact(HSC)materials with abilities to excel the charge-transferdynamics of perovskite solar cells(PSCs).Herein,we report a facile but powerful method to functionalize the surface of 2PACz-SAM,by which reproducible,highly stable,high-efficiency wide-bandgap PSCs can be obtained.The 2PACz surface treatment with various donor number solvents improves assembly of 2PACz-SAM and leave residual surface-bound solvent molecules on 2PACz-SAM,which increases perovskite grain size,retards halide segregation,and accelerates hole extraction.The surface functionalization achieves a high power conversion efficiency(PCE)of 17.62%for a single-junction wide-bandgap(~1.77 e V)PSC.We also demonstrate a monolithic all-perovskite tandem solar cell using surfaceengineered HSC,showing high PCE of 24.66%with large open-circuit voltage of 2.008 V and high fillfactor of 81.45%.Our results suggest this simple approach can further improve the tandem device,when coupled with a high-performance narrow-bandgap sub-cell.

关键词： Perovskite solar cells 2PACz Monolithic tandem solar cells wide bandgap

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High performance wide bandgap perovskite solar cell with low V_(OC) deficit less than 0.4 V

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Journal of Energy Chemistry 2024年第4期91卷 313-322页

作者： Haikuo Guo Fuhua Hou Xuli Ning Xiaoqi Ren Haoran Yang Rui Liu Tiantian Li Chengjun Zhu Ying Zhao Wei Li Xiaodan Zhang School of Physical Science and Technology Key Laboratory of Semiconductor Photovoltaic Technology and Energy Materials at Universities of Inner Mongolia Autonomous RegionInner Mongolia UniversityHohhot 010021Inner MongoliaChina Institute of Photoelectronic Thin Film Devices and Technology of Nankai University Key Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinSolar Energy Research Center of Nankai UniversityTianjin 300350China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430000HubeiChina

wide bandgap perovskite solar cells(PSCs)have attracted significant attention because they can be applied to the top cells of tandem solar cells.However,high open-circuit voltage(V_(OC))deficit(>0.4 V)result from poor crystallization and high non-radiative recombination losses become a serious limitation in the pursuit of high performance.Here,the relevance between different Pbl_(2)proportions and performance parameters are revealed through analysis of surface morphology,residual stress,and photostability.The increase of Pbl_(2)proportion promotes crystal growth and reduces the work function of the perovskite film surface and promotes the energy level alignment with the carrier transport layer,which decreased the V_(OC)deficit.However,residual PbI_(2)exacerbated the stress level of perovskite film,and the resulting lattice disorder deteriorated the photostability of the device.Ultimately,after the synergistic passivation of residual PbI_(2)and PEAI,the V_(OC)achieves 1.266 V and V_(OC)deficit is less than 0.4 V,the record value in wide bandgap PSCs.

关键词： Pb management Perovskite solar cell Strain wide bandgap Stability

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Antimony Potassium Tartrate Stabilizes wide-bandgap Perovskites for Inverted 4-T All-Perovskite Tandem Solar Cells with Efficiencies over 26%

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Nano-Micro Letters 2023年第7期15卷 204-217页

作者： Xuzhi Hu Jiashuai Li Chen Wang Hongsen Cui Yongjie Liu Shun Zhou Hongling Guan Weijun Ke Chen Tao Guojia Fang Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education School of Physics and TechnologyWuhan UniversityWuhan 430072People’s Republic of China

wide-bandgap(WBG)perovskites have been attracting much attention because of their immense potential as a front light-absorber for tandem solar cells.However,WBG perovskite solar cells(PSCs)generally exhibit undesired large open-circuit voltage(VOC)loss due to light-induced phase segregation and severe non-radiative recombination loss.Herein,antimony potassium tartrate(APTA)is added to perovskite precursor as a multifunctional additive that not only coordinates with unbonded lead but also inhibits the migration of halogen in perovskite,which results in suppressed non-radiative recombination,inhibited phase segregation and better band energy alignment.Therefore,a APTA auxiliary WBG PSC with a champion photoelectric conversion efficiency of 20.35%and less hysteresis is presented.They maintain 80%of their initial efficiencies under 100 mW cm^(-2)white light illumination in nitrogen after 1,000 h.Furthermore,by combining a semi-transparent WBG perovskite front cell with a narrow-bandgap tin–lead PSC,a perovskite/perovskite four-terminal tandem solar cell with an efficiency over 26%is achieved.Our work provides a feasible approach for the fabrication of efficient tandem solar cells.

关键词： Perovskite solar cell Tandem wide bandgap Multifunctional additive

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High-performance self-powered color filter-free blue photodetector based on wide-bandgap halide perovskites

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Journal of Materials Science & Technology 2023年第21期152卷 100-108页

作者： Yeonghun Yun Hanbyeol Cho Jina Jung Sung Woong Yang Devthade Vidyasagar Rajendra Kumar Gunasekaran Sangwook Lee School of Materials Science and Engineering Kyungpook National University(KNU)Daegu 41566South Korea KNU Advanced Material Research Institute Kyungpook National UniversityDaegu 41566South Korea Institute of Microstructure Technology&Light Technology Institute Karlsruhe Institute of TechnologyKarlsruhe 76131Federal Republic of Germany

Blue photodetectors(PDs)are attracting great attention for various applications.Commercial blue PDs based on inorganic GaP or InGaN absorbers are limited by their expensive,complex,and high-temperature fabrication techniques.Organic absorber-based blue PDs still have much lower photode-tecting properties than inorganic blue PDs.In this study,a high-performance self-powered blue PD is developed using methylammonium lead halide(MAPbX_(3);X=I,Br,and Cl)perovskites based on the eco-nomic and facile solution process at low temperatures.Optimal composition is obtained through halide-composition engineering.Our best-performing device exhibits an average external quantum efficiency and an average detectivity of 42.7%and 8.65×10^(11) Jones,respectively,within the blue region.The peak responsivity of the proposed PD is 0.174 A W^(−1) at 455 nm,which is comparable to that of commercial gallium phosphide blue PD(0.180 A W^(−1) at 470 nm).Moreover,the proposed device exhibits excellent environmental stability under ambient air conditions.These findings will act as a basis for next-generation image sensor technologies,such as vertically stacked red/green/blue PDs.

关键词： Perovskites Photodetectors Blue Composition engineering Self-powered wide bandgap

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Chlorinated phthalimide polymer donor as ultra-wide bandgap and deep HOMO guest for achieving highly efficient polymer solar cells

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Chinese Chemical Letters 2023年第4期34卷 501-506页

作者： Weichao Zhang Jianhua Huang Xiaoyu Lv Ming Zhang Wanru Liu Tianzi Xu Jun Ning Alata Hexig Feng Liu Aiju Xu Chuanlang Zhan Inner Mongolia Autonomous University Key Laboratory of Advanced Materials Chemistry and Devices(AMC&DLab) Inner Mongolia Key Laboratory of Green CatalysisCollege of Chemistry and Environmental ScienceInner Mongolia Normal UniversityHuhhot 010022China College of Materials Science and Engineering Huaqiao UniversityXiamen 361021China Inner Mongolia Key Laboratory of Functional Materials Physics and Chemistry College of Physics and Electronic InformationInner Mongolia Normal UniversityHohhot 010022China School of Chemistry and Chemical Engineering Center for Advanced Electronic Materials and DevicesShanghai Jiao Tong UniversityShanghai 200240China

Quaternary approach has been receiving more and more attention due to its effectiveness in improving solar cell performance, while synthesis/selection of the fourth component is yet a key issue. Herein, we report a chlorinated phthalimide based donor polymer(namely Ph I-Cl) having an ultra-wide bandgap(2.10 e V) and a deep HOMO(-5.58 e V) level. Addition of Ph I-Cl as the third component of PM6:Y6 and the fourth of PM6:Y6:PC71BM increases both hole and electron mobilities and gives rise to more balanced charge carriers mobilities. Both the short-circuit current-density and fill-factor are increased and open-circuit voltage is well maintained, delivering 17.0% and 18.1% efficiencies, respectively. These results demonstrate that chlorination on the side thiophene of phthalimide-based donor polymer is a way to make deep HOMO and ultra-wide bandgap donor polymer guest used for highly efficient ternary and quaternary strategies.

关键词： Phthalimide polymer donor Quaternary strategy Polymer solar cell wide bandgap Fullerene-free

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Blue-Light Emission from Undoped and Rare Earth-Doped wide bandgap Oxides

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Journal of Rare Earths 2006年第6期24卷 728-731页

作者：郝建华何国庚黄雄武吴锐 Department of Optoelectronic Engineering Huazhong University of Science and TechnologyWuhan 430074China School of Energy and Power Engineering Huazhong University of Science and TechnologyWuhan 430074China

Rare earth-doped oxide thin-film phosphors may emerge as an alternate choice for the blue phosphor, due to their chemical and thermal stability in high vacuum and absence of corrosive gas emission under electron bombardment. The blue phosphors in this study were activated in air at temperatures suitable for glass substrates, which have been used in a number of applications. The effects of rare earth ions and oxide hosts on the blue-light-emitting properties of phosphors are discussed. In addition, novel blue-light emission was observed in certain typical undoped wide bandgap oxides. The luminescence of the oxides depends on the growth and annealing conditions under different atmospheres, suggesting that it is associated with the presence of oxygen vacancies. Radiative processes related to oxygen vacancies were also presented.

关键词： wide bandgap luminescence rare earths oxide blue light rare earths

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Surfactant-assisted doctor-blading-printed FAPbBr3 films for efficient semitransparent perovskite solar cells

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Frontiers of Optoelectronics 2020年第3期13卷 272-281页

作者： Hangkai YING Yifan LIU Yuxi DOU Jibo ZHANG Zhenli WU Qi ZHANG Yi-Bing CHENG Jie ZHONG State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China School of Aerospace Transport and ManufacturingCranfield UniversityCranfieldBedfordshireMK430ALUK Department of Materials Science and Engineering Monash UniversityVIC 3800Australia

Organic-inorganic hybrid perovskite solar cells have generated wide interest due to the rapid development of their photovoltaic conversion effciencies.However,the majority of the reported devices have been fabricated via spin coating with a device areaofwide-bandgap formamidi-nium lead bromide(FAPbBr3)film using a cost-effective,high-yielding doctor-blade-coating process.The effects of different surfactants,such as I-α-phosphatidylcholine,polyoxyethylene sorbitan monooleate,sodium lauryl sulfonate,and hexadecyl trimethyl ammonium bromide,were studied during the printing process.Accompanying the optimization of the blading temperature,crystal sizes of over 10μm and large-area perovskite films of5cm×5 cm were obtained using this method.The printed FAPbBr3 solar cells exhibited a short-circuit current density of 8.22 mA/cm2,an open-circuit voltage of 1.175 V,and an efficiency of 7.29%.Subsequently,we replaced the gold with silver nanowires as the top electrode to prepare a semitransparent perovskite solar cell with an average transmittance(400-800 nm)of 25.42%,achieving a high-power efficiency of 5.11%.This study demonstrates efficient doctor-blading printing for preparing large-area FAPbBr3 films that possess high potential for applications in building integrated photovoltaics.

关键词： semitransparent printing perovskite solar cell(PSC) doctor blading wide bandgap

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Magneto-Optical Properties of wider Gap Semiconductors ZnMnTe and ZnMnSe Films Prepared by MBE

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Journal of Electronic Science and Technology 2020年第3期18卷 201-211页

作者： Masaaki Imamura Daisuke Tashima Jiro Kitagawa Hironori Asada Department of Electrical Engineering Fukuoka Institute of TechnologyFukuoka 811-0295 Graduate School of Sciences and Technology of Innovation Yamaguchi UniversityUbe 755-8611

TheⅡ-Ⅵbased magnetic semiconductors with a direct and wide optical bandgap are expected to show high potential for optical applications utilizing short wavelength laser diodes(LDs),such as 532-nm green and475-nm blue LDs.We have confirmed that the Faraday rotationθ_F in the ZnMnTe and ZnMnSe films deposited on quartz glass(QG)and sapphire(SA)substrates by using molecular beam epitaxy(MBE)is large near the absorption edge.This paper reports the magneto-optical properties of ZnMnTe and ZnMnSe films synthesized on the QG and SA substrates,and shows the result of a direct Faraday rotation observation successfully made for the ZnMnTe films under 1.28-kHz alternating magnetic fields.The optical absorption characteristics of the ZnMnTe films grown on the SA substrates by MBE are discussed by comparing them with the optical absorption properties and photoluminescence spectra of theⅡ-ⅥZnTe parent single crystals.

关键词： Magnetic semiconductors magneto-optical effects wide bandgap ZnMnTe and ZnMnSe films

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Growth properties of gallium oxide on sapphire substrate by plasma-assisted pulsed laser deposition

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Journal of Semiconductors 2019年第12期40卷 121-125页

作者： Congyu Hu Katsuhiko Saito Tooru Tanaka Qixin Guo Department of Electrical and Electronic Engineering Synchrotron Light Application Center Saga University

Gallium oxide was deposited on a c-plane sapphire substrate by oxygen plasma-assisted pulsed laser deposition(PLD).An oxygen radical was generated by an inductive coupled plasma source and the effect of radio frequency(RF)power on growth rate was investigated.A film grown with plasma assistance showed 2.7 times faster growth rate.X-ray diffraction and Raman spectroscopy analysis showedβ-Ga2 O3 films grown with plasma assistance at 500℃.The roughness of the films decreased when the RF power of plasma treatment increased.Transmittance of these films was at least 80%and showed sharp absorption edge at 250 nm which was consistent with data previously reported.

关键词： wide bandgap gallium oxide oxygen radical pulsed laser deposition plasma

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