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Dual strategy of modulating growth temperature and inserting ultrathin barrier to enhance the wave function overlap in type-Ⅱ superlattices

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Nano Research 2022年第6期15卷 5626-5632页

作者： Yuyang Wu Yahui Zhang Yi Zhang Yunhao Zhao Yu Zhang Yingqiang Xu Chongyun Liang Zhichuan Niu Yi Shi Renchao Che Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438China State Key Laboratory for superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China National Laboratory of Solid-State Microstructures School of Electronic Science and Engineering and CollaborativeInnovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China Joint-Research Center for Computational Materials Zhejiang LaboratoryHangzhou 311100China

Maximizing wave function overlap(WFO)within type-ii superlattices(T2SL)is demonstrated to be important for improving their photoelectric properties,such as optical transition strength and quantum efficiency,which,however,remains a great challenge for ***,the dual strategy of modulating growth temperature and inserting ultrathin AlAs barrier into the AlSb layers is presented to enhance the WFO in InAs/AlSb *** charge distributions and strain states indicate that moderate growth temperature of 470°C promotes the As-Sb exchange at AlSb-on-InAs(AOI)interfaces,which would introduce skew of energy band structure towards InAs-on-AlSb(IOA)*** band structure could drive electrons and holes to the IOA interfaces simultaneously,thus resulting in the enhanced *** this basis,insertion of relatively thick(0.3 nm)AlAs layers is found to squeeze more holes towards adjacent interfaces,boosting the WFO *** InAs/AlSb superlattices with optimized WFO reveal better optical performance,where the peak intensity shows 50%improvement in the PL spectra than the original ***,a dual-miniband radiative transition mechanism appears in the InAs/AlSb superlattice with relatively thick AlAs intercalation,which helps broaden the wavelength range of the superlattice.

关键词： wave function overlap type-ii superlattices photoelectric properties charge distribution energy band alignment

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