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Visualization of atomic scale reaction dynamics of supported nanocatalysts during oxidation and ammonia synthesis using in-situ environmental(scanning) transmission electron microscopy

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Journal of Energy Chemistry 2021年第6期30卷 281-290,I0007页

作者： Michael R.Ward Robert W.Mitchell Edward D.Boyes Pratibha L.Gai The York Nanocentre University of YorkYork YO105DDUK Department of Physics University of YorkYork YO105DDUK Department of electronic Engineering University of YorkYork YO105DDUK Department of Chemistry University of YorkYork YO105DDUK

Reaction dynamics in gases at operating temperatures at the atomic level are the basis of heterogeneous gas-solid catalyst reactions and are crucial to the catalyst *** noble metal nanocatalysts such as platinum are of interest in fuel cells and as diesel oxidation catalysts for pollution control,and practical ruthenium nanocatalysts are explored for ammonia *** and graphitic carbons are of interest as supports for the *** considerable literature on the catalytic processes on graphite and graphitic supports,reaction dynamics of the nanocatalysts on the supports in different reactive gas environments and operating temperatures at the single atom level are not well *** we present real time in-situ observations and analyses of reaction dynamics of Pt in oxidation,and practical Ru nanocatalysts in ammonia synthesis,on graphite and related supports under controlled reaction environments using a novel in-situ environmental(scanning) transmission electron microscope with single atom *** recording snapshots of the reaction dynamics,the behaviour of the catalysts is *** images reveal single metal atoms,clusters of a few atoms on the graphitic supports and the support *** all play key roles in the mobility,sintering and growth of the *** experimental findings provide new structural insights into atomic scale reaction dynamics,morphology and stability of the nanocatalysts.

关键词： In-situ visualization Atomic scale reaction dynamics In-situ environmental scanning transmission electron microscopy with single atom resolution Supported nanoparticles Ammonia synthesis Oxidation reactions

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