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Metal-organic framework nanosheets and their composites for heterogeneous thermal catalysis:Recent progresses and challenges

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Chinese Chemical Letters 2021年第11期32卷 3307-3321页

作者： Chengqian Cui Guodong Li Zhiyong Tang CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China

Metal-organic framework nanosheets(MONs)as the emerging materials have been attracting great interest because the nanosheets possess a range of fascinating attributes including high surface areas and sufficient accessible active sites,and their nanoscale thicknesses are favorable for mass diffusion and transfer of substrates and products with respect to bulk metal-organic frameworks(MOFs).This review first summarizes the synthetic methods of various MONs from top-down and bottom-up methods as well as their diverse composites with different ***,the catalytic applications of MON based nanocatalysts are discussed and the relationships among the composition,structure and catalytic performances are ***,the challenges and future outlook about the synthesis of diverse MONs and their composites for heterogeneous catalysis are prospected.

关键词： Metal-organic framework nanosheet top-down synthesis Bottom-up synthesis Composite structure Heterogeneous catalysis

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Synthetic Strategies for Constructing Two-Dimensional Metal-Organic Layers （MOLs）： A Tutorial Review

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Chinese Journal of Chemistry 2018年第8期36卷 754-764页

作者： Lingyun Cao Tingting Wang Cheng Wang Collaborative Innovation Center of Chemistry for Energy Materials State Key Laboratory of Physical Chemistry of Solid Surfaces Department of Chemistry College of Chemistry and Chemical Engineering Xiamen University Xiamen Fujian 361005 China

Two-dimensional （2D） metal-organic layers （MOLs） are the 2D version of metal-organic frameworks （MOFs） with nanometer thickness in one dimension. MOLs are also known as 2D-MOFs, 2D coordination polymers, ultrathin MOF nanosheets （UMOFNs） or coordination nanosheets in literature. This new category of 2D materials has attracted a lot of interests because of the opportunity in combining molecular chemistry, surface/interface chemistry and material chemistry of low dimensional materials in these systems. Several synthetic strategies have been developed for the construction of 2D MOLs, but the general synthesis of MOLs still presents a challenge. This tutorial level review summarizes the recent progress in the fabrication of novel 2D MOLs and aims to highlight challenges in this field.

关键词： metal-organic layers metal-organic frameworks 2D materials bottom-up synthesis top-down synthesis

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