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thermodynamics calculation on the oxidation and sulfur removal abilities of slag in EAF dust pellet reduction process

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Journal of Central South University of Technology 2001年第1期8卷 64-68页

作者： PENG Bing 1,PENG Ji 1,ZHANG Chuan fu 1,Jonathan Lobel 2,Janusz A. Kozinski 2 (1 Department of Metallurgical Science and Engineering, Central South University, Changsha 410083, China 2 Department of Metallurgical Engineering, McGill University Department of Metallurgical Science and Engineering Central South University Changsha China Department of Metallurgical Engineering McGill University Montreal Canada

The valuable metals in the dust can be recycled by mixing it with reducing agent carbon and lignosulfonate as the binder to make pellets, then returning the pellets to electric arc furnace (EAF) and adding ferro silicon. Part of valuable metals in the dust is reduced by carbon and part of them reduced by ferro silicon for the economical consideration. The reduced metals get into the steel in the stainless steel or special steel production. But the sulfur in the lignosulfonate may affect the quality of produced steel, which is dependent on the status of the smelting slag. The experiments were conducted in the way of changing the ratio of start iron, pellets, ferro silicon and lime. The content of the slag was checked by XRF for the calculation thermodynamics study. The active concentrations of materials in the slag, the slag abilities of oxidation and sulfur removal in EAF dust reduction process were determined by thermodynamics calculation study on CaO MgO FeO Fe 2O 3 SiO 2 S slag at 1 550 ℃. The oxidation ability of slag can be expressed as N (FetO)= N (FeO)+6 N (Fe 2O 3)+8 N (Fe 3O 4). The sulfur removal ability is dependent on the amount of added ferro silicon and the basicity of the slag. The calculation thermodynamics model was set up and it could be applied to the practical production.

关键词： thermodynamics calculation slag electric arc furnace dust

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Phase relationship of complex multi-component system in chromate cleaner production

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Progress in Natural Science:Materials International 2007年第7期17卷 845-850页

作者： Ge Xinlei~1 Wang Xidong~(1,3**) Zheng Shili~2 Zhang Mei~1 Zhang Yi~2 (1.Department of Physical Chemistry,University of Science and Technology Beijing,Beijing 100083,China 2.Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100080,China 3.College of Engineering,Peking University,Beijing 100871,China) Department of Physical Chemistry University of Science and Technology Beijing Beijing 100083 China College of Engineering Peking University Beijing 100871 China Institute of Process Engineering Chinese Academy of Sciences Beijing 100080 China

The phase relationships of the complex multi-component systems in the liquid-phase oxidization and separation process related with the chromate cleaner production are investigated theoretically and *** phase diagram of main system Fe- Cr2O4-KOH-O2of oxidization process and the relationship of its standard Gibbs free energy change with temperature are calculated.A se- ries of phase diagrams of the separation process at different temperatures,such as K（Na）OH-K（Na）2CrO4-H2O,KOH-KAlO2-H2O, K（Na）OH-K（Na）2CO3-H2O,K（Na）OH-K（Na）HCO3-H2O and K（Na）HCO3-K（Na）2CrO4-H2O have also been *** ex- periments are carried out to verify the calculated *** results showed that the sub-molten salt media are suitable for the oxidization and separation processes;FeCr2O4can be oxidized across a wide range of temperature;K（Na）2CrO4can be separated from K（Na）AlO2system at appropriate temperature and proper concentration;the crystallization of carbonate is easier than that of K（Na）2CrO4.

关键词： chromite chromate system thermodynamics calculation phase diagram

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