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Predicting diamond-like Co-based chalcogenides as unconventional high temperature superconductors

Science Bulletin 2018年第20期63卷 1338-1344页

作者： Jiangping Hu Yuhao Gu Congcong Le Beijing National Laboratory for Condensed Matter Physics and Institute of PhysicsChinese Academy of SciencesBeijing 100190China Kavli Institute of Theoretical Sciences University of Chinese Academy of SciencesBeijing 1O0190China Collaborative Innovation Center of Quantum Matter Beijing 100049China Beijing National Laboratory for Molecular Sciences State Key Laboratory of Rare Earth Materials Chemistry and ApplicationsInstitute of Theoretical and Computational ChemistryCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

We predict Co-based chalcogenides with a diamond-like structure can host unconventional high temperature superconductivity(high-Tc). The essential electronic physics in these materials stems from the Co layers with each layer being formed by vertex-shared CoA_4(A=S, Se, Te) tetrahedra complexes, a material genome proposed recently by us to host potential unconventional high-Tcclose to a d7 filling configuration in 3 d transition metal compounds. We calculate the magnetic ground states of different transition metal compounds with this structure. It is found that(Mn, Fe, Co)-based compounds all have a G-type antiferromagnetic(AFM) insulating ground state while Ni-based compounds are paramagnetic *** AFM interaction is the largest in the Co-based compounds as the three t2 gorbitals all strongly participate in AFM superexchange interactions. The abrupt quenching of the magnetism from the Co to Ni-based compounds is very similar to those from Fe to Co-based pnictides in which a C-type AFM state appears in the Fe-based ones but vanishes in the Co-based ones. This behavior can be considered as an electronic signature of the high-Tcgene. Upon doping, as we predicted before, this family of Co-based compounds favor a strong d-wave pairing superconducting state.

关键词： Iron-based superconductors Cuprates Cobalt chalcogenides d-wave pairing symmetry

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High-magnetic-field induced charge order in high-T_c cuprate superconductors

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Chinese Physics B 2019年第11期28卷 25-42页

作者： L X Zheng J Li T WU Hefei National Laboratory for Physical Science at Microscale University of Science and Technology of ChinaHefei 230026China Key Laboratory of Strongly-coupled Quantum Matter Physics University of Science and Technology of ChinaChinese Academy of SciencesHefei 230026China CAS Center for Excellence in Superconducting Electronics(CENSE) Shanghai 200050China CAS Center for Excellence in Quantum Information and Quantum Physics Hefei 230026China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

In the last few years, charge order and its entanglement with superconductivity are under hot debate in high-Tc community due to the new progress on charge order in high-Tc cuprate superconductors YBa2Cu3O6+x. Here, we will briefly introduce the experimental status of this field and mainly focus on the experimental progress of high-field nuclear magnetic resonance(NMR) study on charge order in YBa2Cu3O6+x. The pioneering high-field NMR work in YBa2Cu3O6+x sets a new stage for studying charge order which has become a ubiquitous phenomenon in high-Tc cuprate superconductors.

关键词： charge order cuprates nuclear magnetic resonance YBa2Cu3O6+x superconductors competing order

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Topological vortex phase transitions in iron-based superconductors

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Science Bulletin 2019年第17期64卷 1207-1214页

作者： Shengshan Qin Lunhui Hu Xianxin Wu Xia Dai Chen Fang Fu-Chun Zhang Jiangping Hu Kavli Institute of Theoretical Sciences University o f Chinese Academy of Sciences Beijing 100049 China Beijing National Research Center for Condensed Matter Physics and Institute o f Physics Chinese Academy of Sciences Beijing 100190 China Department of Physics University of California San Diego CA 92093 USA Institute for Theoretical Physics and Astrophysics Julius-Maximilians University o f Wurzburg Am Hubland D-97074 Wurzburg Germany CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences Beijing 100049 China Collaborative Innovation Center of Quantum Matter Beijing 100049 China

We study topological vortex phases in iron-based superconductors. Besides the previously known vortex end Majorana zero modes(MZMs) phase stemming from the existence of a three dimensional(3 D) strong topological insulator state, we show that there is another topologically nontrivial phase as iron-based superconductors can be doped superconducting 3 D weak topological insulators(WTIs). The vortex bound states in a superconducting 3 D WTI exhibit two different types of quantum states, a robust nodal superconducting phase with pairs of bulk MZMs and a full-gap topologically nontrivial superconducting phase which has single vortex end MZM in a certain range of doping level. Moreover, we predict and summarize various topological phases in iron-based superconductors, and find that carrier doping and interlayer coupling can drive systems to have phase transitions between these different topological phases.

关键词： Weak topological insulators Vortex bound states Majorana modes Iron-based superconductors

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NMR Evidence for Universal Pseudogap Behavior in Quasi-Two-Dimensional FeSe-Based superconductors

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Chinese Physics Letters 2022年第12期39卷 71-76页

作者： B.L.Kang M.Z.Shi D.Zhao S.J.Li J.Li L.X.Zheng D.W.Song L.P.Nie T.Wu X.H.Chen Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China Key Laboratory of Strongly coupled Quantum Matter Physics Department of PhysicsUniversity of Science and Technology of ChinaHefei 230026China CAS Center for Excellence in Superconducting Electronics(CENSE) Shanghai 200050China 4Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China Hefei National Laboratory University of Science and Technology of ChinaHefei 230088China

Recently,by intercalating organic ions into bulk FeSe superconductors,two kinds of layered FeSe-based superconductors[(TBA)xFeSe and(CTA)xFeSe]with superconducting transition temperatures(Tc)above 40 K have been *** to the large interlayer distance(~15A),these new layered superconductors have a large resistivity anisotropy analogous to bismuth-based cuprate ***,remarkable pseudogap behavior well above Tcis revealed by nuclear magnetic resonance(NMR)measurements on77Se nuclei,suggesting a preformed pairing scenario similar to that of ***,we report another new kind of organic-ion-intercalated FeSe superconductor,(PY)xFeSe,with a reduced interlayer distance(~10A)compared to(TBA)xFeSe and(CTA)*** performing77Se NMR and transport measurements,we observe a similar pseudogap behavior well above Tcof~40 K and a large resistivity anisotropy of~10~4 in(PY)*** these facts strongly support a universal pseudogap behavior in these layered FeSe-based superconductors with quasi-two-dimensional electronic structures.

关键词： NMR superconductors layered

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MODELLING AND NUMERICAL SOLUTIONS OF A GAUGE PERIODIC TIME DEPENDENT GINZBURG-LANDAU MODEL FOR TYPE-Ⅱ superconductors

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Journal of Computational Mathematics 1997年第4期15卷 365-384页

作者： Zhi-ming Chen (Institute of Mathematics, Chinese Academy of Sciences, Beijing, China) 中科院数学所北京

In this paper we seek the solutions of the time dependent Ginzburg-Landau model for type-Ⅱ superconductors such that the associated physical observables are spatially periodic with respect to some lattice whose basic lattice cell is not necessarily rectangular. After appropriately foring the gange, the model can be formulated as a system of nonlinear parabolic partial differential equations with quasi-periodic boundary conditions. We first give some results concerning the existence, uniqueness and regularity of solutions and then we propose a semiimplicit finite element scheme solving the system of nonlinear partial dmerential equations and show the optimal error estimates both in the L2 and energy *** also report on some numerical results at the end of the paper.

关键词： Math QT MODELLING AND NUMERICAL SOLUTIONS OF A GAUGE PERIODIC TIME DEPENDENT GINZBURG-LANDAU MODEL FOR TYPE superconductors

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A brief review on/μSR studies of unconventional Fe-and Cr-based superconductors

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Science China(Physics,Mechanics & Astronomy) 2018年第12期61卷 3-24页

作者： A.Bhattacharyya D.T.Adroja M.Smidman V.K.Anand ISIS Facility Rutherford Appleton LaboratoryChiltonDidcot OxonOX11OQXUK Department of Physics Ramakrishna Mission Vivekananda Educational and Research InstituteHowrah 711202India Highly Correlated Matter Research Group Physics DepartmentUniversity of JohannesburgAuckland Park 2006South Africa Center for Correlated Matter and Department of Physics Zhejiang UniversityHangzhou 310058China Helmholtz-Zentrum Berlin fur Materialien und Energie GmbH Berlin D-14109Germany

Muon spin relaxation/rotation(μSR) is a vital technique for probing the superconducting gap structure, pairing symmetry and time reversal symmetry breaking, enabling an understanding of the mechanisms behind the unconventional superconductivity of cuprates and Fe-based high-temperature superconductors, which remain a puzzle. Very recently double layered Fe-based superconductors having quasi-2 D crystal structures and Cr-based superconductors with a quasi-1D structure have drawn considerable attention. Here we present a brief review of the characteristics of a few selected Fe-and Cr-based superconducting materials and highlight some of the major outstanding problems, with an emphasis on the superconducting pairing symmetries of these materials. We focus on μSR studies of the newly discovered superconductors ACa_2Fe_4As_4F_2(A = K, Rb, and Cs), ThFeAsN, and A_2Cr_3As_3(A = K, Cs), which were used to determine the superconducting gap structures, the presence of spin fluctuations, and to search for time reversal symmetry breaking in the superconducting states. We also briefly discuss the results of μSR investigations of the superconductivity in hole and electron doped BaFe_2As_2.

关键词： unconventional superconductors iron-based superconductors Cr-based superconductors superconducting pairing symmetry time reversal symmetry muon spin rotation/relaxation

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Evolution of Superconducting-Transition Temperature with Superfluid Density and Conductivity in Pressurized Cuprate superconductors

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Chinese Physics Letters 2024年第4期41卷 110-117页

作者：赵金瑜蔡树陈逸雯顾根大闫宏涛郭静韩金宇王鹏玉周亚洲李延春李晓东任治安吴奇周兴江丁阳向涛毛河光孙力玲 Institute of Physics Chinese Academy of SciencesBeijing 100190China Center for High Pressure Science&Technology Advanced Research Beijing 100094China Condensed Matter Physics&Materials Science Department Brookhaven National LaboratoryNY 11973-5000USA University of Chinese Academy of Sciences Beijing 100190China Institute of High Energy Physics Chinese Academy of ScienceBeijing 100049China Beijing Academy of Quantum Information Sciences Beijing 100193China

What factors fundamentally determine the value of superconducting transition temperature Tc in high temperature superconductors has been the subject of intense *** the establishment of an empirical law known as Homes'law,there is a growing consensus in the community that the Tc value of the cuprate superconductors is closely linked to the superfluid density(ρ_(s))of its ground state and the conductivity(σ)of its normal ***,all the data supporting this empirical law(ρ_(s)=AσT_(c))have been obtained from the ambientpressure *** this study,we present the first high-pressure results about the connection of the quantities of ρ_(s) and σ with T_(c),through the studies on the Bi_(1.74)Pb_(0.38)Sr_(1.88)CuO_(6+δ)and Bi_(2)Sr_(2)CaCu_(2)O_(8+δ),in which the value of their high-pressure resistivity(ρ=1/σ)is achieved by adopting our newly established method,while the quantity ofρs is extracted using Homes'*** highlight that the Tc values are strongly linked to the joint response factors of magnetic field and electric field,i.e.,ρ_(s) and σ,respectively,implying that the physics determining T_(c) is governed by the intrinsic electromagnetic fields of the system.

关键词： superconductors Transition Conductivity

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The role of CALYPSO in the discovery of high-T_c hydrogen-rich superconductors

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Chinese Physics B 2019年第10期28卷 56-61页

作者： Wenwen Cui Yinwei Li Laboratory of Quantum Materials Design and Application School of Physics and Electronic EngineeringJiangsu Normal University

Hydrogen-rich compounds are promising candidates for high-Tc or even room-temperature superconductors. The search for high-Tc hydrides poses a major experimental challenge because there are many known hydrides and even more unknown hydrides with unusual stoichiometries under high pressure. The combination of crystal structure prediction and first-principles calculations has played an important role in the search for high-Tc hydrides, especially in guiding experimental synthesis. Crystal structure AnaLYsis by Particle Swarm Optimization(CALYPSO) is one of the most efficient methods for predicting stable or metastable structures from the chemical composition alone. This review summarizes the superconducting hydrides predicted using CALYPSO. We focus on two breakthroughs toward room-temperature superconductors initiated by CALYPSO: the prediction of high-Tc superconductivity in compressed hydrogen sulfide and lanthanum hydrides, both of which have been confirmed experimentally and have set new record Tc values. We also address the challenges and outlook in this field.

关键词： CALYPSO structure prediction hydrogen-rich superconductors

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Magnetism in Quasi-One-Dimensional A2Cr3As3（A=K,Rb） superconductors

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Chinese Physics Letters 2015年第5期32卷 119-123页

作者：吴贤新勒聪聪袁静范桁胡江平 Institute of Physics Chinese Academy of Sciences Beijing 100190 Collaborative Innovation Center of Quantum Matter Beijing 100190 Department of Physics Purdue University West Lafayette 47907 USA

We predict that the recently discovered quasi-one-dimensional superconductors, A2 Cr3As3 （A=K, Rb）, possess strong frustrated magnetic fluctuations and are nearby a novel in-out co-planar magnetic ground state. The frustrated magnetism is very sensitive to the c-axis lattice constant and can thus be suppressed by increasing pressure. Our results qualitatively explain strong non-Fermi liquid behaviors observed in the normal state of the superconductors as the intertwining between the magnetism and superconductivity can create a large quantum critical region in quasi-one-dimensional systems and also suggest that the materials share similar phase diagrams and superconducting mechanism with other unconventional superconductors, such as cuprates and iron-based superconductors.

关键词： As A=K,Rb superconductors Magnetism in Quasi-One-Dimensional A2Cr3As3 Cr

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Nonlinear Flux Diffusion and ac Susceptibility in High-T_(c) superconductors

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Chinese Physics Letters 1998年第9期15卷 668-670页

作者： BAI Wei-ping CHEN Han-dong YIN Dao-le LI Gang LI Chuan-yi CHEN Kai-xuan LU Guo Department of Physics Peking UniversityBeijing 100871

It is shown that the flux motion in high-T_(c) superconductors can be well consistently analysed by a unified materials *** different models of U(J)so far suggested can be shown as specific forms or limits of this unified materials *** scaling law of flux pinning derived from this equation agrees with recent experimental observations on high-Jc NdBa2Gu3O7-δsingle *** amplitude dependence of ac susceptibility derived from this equation is compared with several experimental results of high-T_(c) superconductors and a general power law is found.

关键词： equation. unified superconductors

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