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Activation of 2D MoS_(2) electrodes induced by high-rate lithiation processes

Journal of Energy Chemistry 2023年第3期78卷 56-70,I0003页

作者： Tianzhu Liu Georgian Melinte Oleksandr Dolotko Michael Knapp Beatriz Mendoza-Sánchez Institute for Applied Materials-Energy Storage Systems(IAM-ESS) Karlsruhe Institute of Technology(KIT)Eggenstein-Leopoldshafen D-76344Germany Karlsruhe Nano Micro Facility(KNMF) Karlsruhe Institute of Technology(KIT)Eggenstein-Leopoldshafen D-76344Germany Helmholtz-Institute Ulm for Electrochemical Energy Storage(HIU) Ulm 89081Germany

MoS_(2) is a highly promising material for application in lithium-ion battery anodes due to its high theoretical capacity and low ***,problems with a fast capacity decay over cycling,especially at the first cycles,and poor rate performance have deterred its practical ***,electrodes comprised solely of few-layers 2D MoS_(2) nanosheets have been manufactured by scalable liquid-phase exfoliation and spray deposition *** long-standing controversy questioning the reversibility of conversion processes of MoS_(2)-based electrodes was *** studies revealed that,in 2D MoS_(2) electrodes,conversion processes are indeed reversible,where nanostructure played a key *** of the electrodes at high current rates revealed an intriguing phenomenon consisting of a continuously increasing capacity after ca.100-200 *** phenomenon was comprehensively addressed by a variety of electrochemical and microscopy methods that revealed underlying physical activation mechanisms that involved a range of profound electrode structural *** mechanisms delivered a capacitive electrode of a superior rate performance and cycling stability,as compared to the corresponding pristine electrodes,and to MoS_(2) electrodes previously ***,we have devised a methodology to overcome the problem of cycling stability of 2D MoS_(2) ***,activation of electrodes constitutes a methodology that could be applied to enhance the energy storage performance of electrodes based on other 2D nanomaterials,or combinations thereof,strategically combining chemistries to engineer electrodes of superior energy storage properties.

关键词： 2D MoS_(2) Liquid-phase exfoliation spray-deposition Conversion processes Activation mechanisms Energy storage mechanisms

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A new composite:spray-deposited M2 high speed steel reinforced by WC particles

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International Journal of Minerals,Metallurgy and Materials 1997年第3期11卷 14-17页

作者： ZHANG Liying TIAN Haige HUANG Thuo WU Chengyi (Material Science and Engineering School, University of Science and Technology Beijing, Beijing 100083, China) Univ of Science and Technology Beijing Beijing China

The fabrication of the high speed steel matrix composites reinforced by WC particles utilizing the ultrasonicgas atomization and spray-deposition was studied. The change of microstware and mechanical Properties of thecomposites added WC Particles were investigated and analyzed as well. As some results, the WC particles exhibit tWomorphologies (spherical and angular) with different content of WC particles; and with the increase of content of WCparticles, the hardness of the composites increases, yet the bending strength appears a trend of decreasing.

关键词： spray-deposition high speed steel composite

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