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Temperature-sensitive and solvent-resistance hydrogel sensor for ambulatory signal acquisition in“moist/hot environment”

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Nano Research 2023年第7期16卷 10348-10357页

作者： Xinyu Qu Hanjun Sun Xiaolong Kan Bing Lei Jinjun Shao Qian Wang Wenjun Wang Zhenhua Ni Xiaochen Dong Key Laboratory of Flexible Electronics(KLOFE)&Institute of Advanced Materials(IAM) School of Physical and Mathematical SciencesNanjing Tech University(NanjingTech)Nanjing 211816China School of Physical Science and Information Technology Liaocheng UniversityLiaocheng 252059China School of Physics and Key Laboratory of MEMS of the Ministry of Education Southeast UniversityNanjing 211189China School of Chemistry&Materials Science Jiangsu Normal UniversityXuzhou 221116China

To realize continuously and stably work in a“moist/hot environment”,flexible electronics with excellent humid resistance,antiswelling,and detection sensitivity are ***,a solvent-resistant and temperature-ultrasensitive hydrogel sensor was prepared by combining MXene and quaternized chitosan(QCS)with the binary polymer *** strong electrostatic interaction between the QCS chain and the poly(acrylic acid)(PAA)network endows the hydrogel stability against solvent erosion,high temperature,and high *** strong dynamic interaction between MXene and polymer matrix significantly improves the mechanical properties and sensing(strain and temperature)sensitivity of the *** hydrogel strain sensor exhibits a high gauge factor(5.53),temperature/humidity tolerance(equilibrium swelling ratio of 2.5%at 80℃),and excellent cycle stability,which could achieve a remote and accurate perception of complex human motion and environment fluctuation under aquatic ***,the hydrogel sensor exhibits impressive thermal response sensitivity(-3.183%/℃),ultrashort response time(<2.53 s),and a low detection limit(<0.5℃)in a wide temperature range,which is applied as an indicator of the body surface and ambient *** short,this study broadens the application scenarios of hydrogels in persistent extreme thermal and wet environments.

关键词： flexible electronics hydrogel sensor solvent-resistance underwater application

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CHARACTERIZATION OF REGENERATED CELLULOSE MEMBRANES HYDROLYZED FROM CELLULOSE ACETATE

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Chinese Journal of Polymer Science 2002年第4期20卷 369-375页

作者： Yun Chen Xiao-peng Xiong Guang Yang Li-na Zhang Sen-lin Lei Hui Liang Electron Microscope Lab of Medical School, Wuhan University Wuhan 430072, China College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, China Wuhan Univ Coll Chem & Mol Sci Wuhan 430072 Peoples R China Wuhan Univ Sch Med Electron Microscope Lab Wuhan 430072 Peoples R China

A series of cellulose acetate membranes were prepared by using formamide as additive, and then were hydrolyzed in 4 wt% aqueous NaOH solution for 8 h to obtain regenerated cellulose membranes. The dependence of degree of substitution, structure, porous properties, solubility and thermal stability on hydrolysis time was studied by chemical titration, Fourier transform infrared spectroscopy, scanning electron microscopy, wide-angle X-ray diffraction, and differential scanning calorimetry, respectively. The results indicated that the pore size of the regenerated cellulose membranes was slightly smaller than that of cellulose acetate membrane, while solvent-resistance, crystallinity and thermostability were significantly improved. This work provides a simple way to prepare the porous cellulose membranes, which not only kept the good pore characteristics of cellulose acetate membranes, but also possessed solvent-resistance, high crystallinity and thermostability. Therefore, the application range of cellulose acetate membranes can be expanded.

关键词： hydrolysis cellulose acetate thermal stability regenerated cellulose membrane pore size solvent-resistance SEM

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High-performance all-solution-processed inverted quantum dot light-emitting diodes enabled by water treatment

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Nano Research 2023年第7期16卷 10215-10221页

作者： Qianqing Hu Junjie Si Desui Chen Xiaoming Hao Rui Xu Yihang Du Zhuopeng Du Xinquan Gong Hong Zhao Peiqing Cai Qi Ai Xin Yao Yu Yan Zenan Zhang Muzhi Cai Wei Liu Yongyin Kang Zugang Liu College of Optical and Electronic Technology China Jiliang UniversityHangzhou 310018China Key Laboratory of Excited-State Materials of Zhejiang Province State Key Laboratory of Silicon MaterialsDepartment of ChemistryZhejiang UniversityHangzhou 310027China Institute of Flexible Electronics Technology of THU ZhejiangJiaxing Key Laboratory of Flexible Electronics based Intelligent Sensing and Advanced Manufacturing TechnologyJiaxing 314000China Zhejiang Najing Technology Co. Ltd.Quzhou 324004China Najing Technology Corporation Ltd. Hangzhou 310052China

All-solution-processed inverted quantum dot(QD)light-emitting diodes(QLEDs)with transparent bottom cathodes can be directly connected to the n-type thin-film transistors,offering a feasible solution for low-cost active matrix-driven QD ***,the subsequent solution-deposition of the hole-transporting layer destroys the underneath QD films,resulting in largely deteriorated device *** strategies have been implemented to prevent QD film from dissolution,but all at a heavy cost of device performance suffering from either reduced efficiency or increased driving ***,a facile and effective water-treatment approach for QD film to fabricate inverted QLEDs through all solution processing is *** water treatment substitutes the long-chain oleate ligands with hydroxyl groups,resulting in significantly improved non-polar solvent resistance of the QD ***,the QD films reserve their excellent photoluminescence efficiency after water *** the water-treated QD film as the emissive layer,all-solution-processed inverted red QLED with a peak external quantum efficiency of 19.6%,a turn-on voltage of 1.8 V,and a T50 operational lifetime of 150,000 h at 100 cd·m^(-2) was ***,efficient and low-voltage-driven green and blue QLEDs can also be prepared with this *** work provides a feasible strategy for the fabrication of high-performance all-solution-processed inverted QLEDs,paving the way toward achieving QLEDs by all ink-jet printing.

关键词： solvent-resistance quantum dots inverted electroluminescence all solution processing

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