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Remarkable carbon dioxide catalytic capture (CDCC) leading to solid-form carbon material via a new CVD integrated process (CVD-IP): An alternative route for CO_2 sequestration

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Journal of Energy Chemistry 2013年第1期22卷 136-144页

作者： Wei Chu Maofei Ran Xu Zhang Ning Wang Yufei Wang Heping Xie Xiusong Zhao Key Laboratory Green Chemistry & Technology of Ministry of Education (MOE) College of Chemical Engineering Sichuan University SABIC Technology Center Riyadh State Key Laboratory of Hydraulics and Mountain River Engineering Sichuan University Department of Chemical and Biomolecular Engineering National University of Singapore University Queensland School Chemical Engineering

Through our newly-developed ＂chemical vapor deposition integrated process （ISVD-IP）＇＂ using carbon OlOXlae （t..u2） as me raw matenal and only carbon source introduced, CO2 could be catalytically activated and converted to a new solid-form product, i.e., carbon nanotubes （CO2-derived） at a quite high yield （the single-pass carbon yield in the solid-form carbon-product produced from CO2 catalytic capture and conversion was more than 30% at a single-pass carbon-base）. For comparison, when only pure carbon dioxide was introduced using the conventional CVD method without integrated process, no solid-form carbon-material product could be formed. In the addition of saturated steam at room temperature in the feed for CVD, there were much more end-opening carbon nano-tubes produced, at a slightly higher carbon yield. These inspiring works opened a remarkable and alternative new approach for carbon dioxide catalytic capture to solid-form product, comparing with that of CO2 sequestration （CCS） or CO2 mineralization （solidification）, etc. As a result, there was much less body volume and almost no greenhouse effect for this solid-form carbon-material than those of primitive carbon dioxide.

关键词： carbon dioxide catalytic capture (CDCC) carbon nanotubes (CNTs) chemical vapor deposition integrated process (CVD-IP) solid-formcarbon material debating greenhouse gases (GHG) effects

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