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Tightened1D/3Dcarbonheterostructure infiltratingphase change materials for solar-thermoelectric energy harvesting:Faster and better

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Carbon Energy 2023年第6期5卷 104-117页

作者： Zhaodi Tang Piao Cheng Panpan Liu Yan Gao Xiao Chen Ge Wang Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory of Function Materials for Molecule&Structure ConstructionSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijingPR China Institute of Advanced Materials Beijing Normal UniversityBeijingPR China Aerospace Institute of Advanced Material and Processing Technology BeijingPR China Shunde Graduate School University of Science and Technology BeijingShundePR China

Extensive use of thermal energy in daily life is ideal for reducing carbon emissions to achieve carbon neutrality;however,the effective collection of thermal energy is a major ***(TE)conversion technology based on the Seebeck effect and thermal energy storage technology based on phase change materials(PCMs)represent smart,feasible,and research-worthy approaches to overcome this ***,the integration of multiple thermal energy sources freely existing in the environment for storage and output of thermal and electrical energy simultaneously still remains a huge ***,three-dimensional(3D)nanostructured metal-organic frameworks(MOFs)are in situ nucleated and grown onto carbon nanotubes(CNTs)via coordination *** calcination,the prepared core-shell structural CNTs@MOFs are transformed into tightened 1D/3D carbon heterostructure loading Co nanoparticles for efficient solar-thermoelectric energy ***,the corresponding composite PCMs show a record-breaking solar-thermal conversion efficiency of 98.1%due to the tightened carbon heterostructure and the local surface plasmon resonance effect of Co ***,our designed all-in-one composite PCMs are also capable of creating an electrical potential of 0.5 mV based on the Seebeck effect without a TE *** promising approach can store thermal and electrical energy simultaneously,providing a new direction in the design of advanced all-in-one multifunctional PCMs for thermal energy storage and utilization.

关键词： carbon neutrality metal-organic framework phase change materials solar-thermoelectric conversion thermal energy storage

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