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Recent Advance on Torrefaction Valorization and Application of Biochar from Agricultural Waste for soil remediation

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Journal of Renewable Materials 2022年第2期10卷 247-261页

作者： Kai Su Qirui Qin Jingyu Yang Linxiao Li and Shaoqi Deng Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu611756China

With the increase of global proportion of soil pollution and the number of areas at risk,researchers have sought to develop various pathways to repair or relieve the pollutants in *** them,biochar represents one multi-dimensional soil amendment which has got great deal of attention on its physicochemical properties towards the removal or mitigation of contaminants in soil.A variety of agricultural wastes like straw and manure prepared from different torrefaction process have been employed as feedstock for the production of biochar,which can be applied to the contaminated soil to facilitate the growing environment for crops,and to improve soil fertility and microbial *** addition,the utilization of biochar for soil remediation is also considered as a pro-cess of carbon *** purpose of this review is to summarize the latest research progress in torrefac-tion processes and mechanism of agricultural waste,the effects of different torrefaction methods on the formation and properties of biochar were explained,coupled with the effects of process ***,the conver-sion and mechanisms of biochar prepared from agricultural wastes composed mainly with lignocellulosic material were discussed,and the characteristics of biochar prepared for improving soil physical and chemical character-istics,microbial community characteristics,nutrients,and the stability and relief of soil pollutants,especially heavy metals,are ***,this work discussed the application and future technical challenges of soil remediation based on agricultural waste derived biochar.

关键词： Torrefaction biochar soil remediation agricultural waste

Synthesis,characterization,safety design,and application of NPs@BC for contaminated soil remediation and sustainable agriculture

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Biochar 2023年第1期5卷 71-101页

作者： Tong Zheng Shaohu Ouyang Qixing Zhou Carbon Neutrality Interdisciplinary Science Center Nankai UniversityTianjin 300350China Key Laboratory of Pollution Processes and Environmental Criteria(Ministry ofEducation) College of Environmental Science and EngineeringNankai UniversityTianjin 300350China

Biochar(BC)and nanoparticle-decorated biochar(NPs@BC)have emerged as potential high-performance function materials to facilitate simultaneous soil remediation and agricultural ***,there is an urgent need to incorporate environmental sustainability and human health targets into BC and NPs@BC selection and design *** contrast to extensive research on the preparation,modification,and environmental application of BC to soil ecosystems,reports about the adapted framework and material selection strategy of NPs@BC under environmental and human health considerations are still ***,few studies systematically explored the impact of NPs@BC on soil ecosystems,including soil biota,geochemical properties,and nutrient cycles,which are critical for largescale utilization as a multifunctional *** main objective of this systematic literature review is to show the high degrees of contaminant removal for different heavy metals and organic pollutants,and to quantify the economic,environmental,and toxicological outcomes of NPs@BC in the context of sustainable *** address this need,in this review,we summarized synthesis techniques and characterization,and highlighted a linkage between the evolution of NPs@BC properties with the framework for sustainable NPs@BC selection and design based on environmental effects,hazards,and economic ***,research advances in contaminant remediation for heavy metals and organic pollutants of NPs@BC are minutely ***,NPs@BC positively acts on sustainable agriculture,which is *** the meantime,evaluating from the perspective of plant growth,soil characterizations as well as carbon and nitrogen cycle was conducted,which is critical for comprehending the NPs@BC environmental *** work may develop a potential framework that can inform decision-making for the use of NPs@BC to facilitate promising environmental applications and prevent unintended conseq

关键词： Biochar Nanotechnology Safety design framework soil remediation Environment sustainability

Overestimate of remediation efficiency due to residual sodium persulfate in PAHs contaminated soil and a solution

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Journal of Environmental Sciences 2022年第3期34卷 242-250页

作者： Liping He Jianhao Tong Yuanqiang Yang Jianxun Wu Linqian Li Zhonghua Wei Wei Long Jingli Pang Jiyan Shi Yunnan Research Academy of Eco-environmental Sciences Kunming 650034China Department of Environmental Engineering College of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China Beijing Construction Engineering Group Environmental remediation Co.Ltd. Beijing 100015China

Oxidation remediation is a commonly used technology for PAHs contaminated soil presently,but the overestimate of efficiency due to ongoing remediation by residual oxidants during extraction and testing has not been paid enough *** this study,persulfate was activated by Fe(Ⅱ)to investigate the effects of residual oxidants on PAHs removal during detection process and the elimination effects of adding Na_(2)SO_(3) and extending sampling time on residual *** verified that the residual oxidants removed PAHs in extraction process,making the results lower than the actual values:the detection recovery rate η of ΣPAHs and 3-6 ring PAHs ranged from 24.3%(25%Na_(2)S_(2)O_(8)treatment)to 87.4%(5%Na_(2)S_(2)O_(8)+4/4Fe^(2+) treatment),20.1%-99.0%,28.9%-87.9%,20.8%-89.4%,and 1.8.6%-76.9%,*** adding Na_(2)SO_(3),the accuracy of detection results increased significantly:the η of ΣPAHs and 3-6 ring PAHs increased to 64.1%-96.5%,58.8%-95.5%,73.8%-114.4%,60.6%-95.6%,and 45.4%-77.1%,*** 49 days of adding oxidants,residual oxidants had no considerable effect on the detection of PAHs,indicating it was appropriate to start soil remediation verification sampling49 days after the remediation was *** observed results will help scientific evaluation of the remediation effects of chemical oxidation on or-ganic contaminated soil.

关键词： Persulfate activation soil remediation Polycyclic aromatic hydrocarbons Residual oxidant removal

Mechanistic insights into the synergetic remediation and amendment effects of zeolite/biochar composite on heavy metal-polluted red soil

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Frontiers of Environmental Science & Engineering 2024年第9期18卷 105-114页

作者： Jing Li Dazhong Yang Wensong Zou Xuezhen Feng Ranhao Wang Renji Zheng Siyuan Luo Zheting Chu Hong Chen State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution ControlSchool of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China

Red soil,the most critical soil resource in tropical/subtropical regions worldwide,faces tremendous threats,including nutrient deficiency,acidification,and heavy metal *** is a great demand for multifunctional eco-materials capable of modifying this ***,we used widely distributed soil and biomass to develop a zeolite/biochar composite for synergistic red soil remediation and *** the composite material,the Pb^(2+) and Cd^(2+) remediation efficiencies reached 92.8%and 92.9%,respectively,in stems under optimal ***,the acidity and nutrient deficiency conditions of red soil significantly *** atomic-scale interaction mechanism during the remediation and amendment process was elucidated with complementary characterization methods,which revealed that in the zeolite/biochar composite material,zeolite contributes to longterm heavy metal remediation ***,biochar is responsible for soil quality amendment and short-term heavy metal ***,for the first time,single-atom heavy metal ions were observed on biochar during the remediation process,indicating the broad distribution of single atoms in the natural environment.

关键词： Red soil Heavy metal pollution Zeolite/biochar composite soil remediation soil amendment

Enhanced remediation of chlorpyrifos-contaminated soil by immobilized strain Bacillus H27

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Journal of Environmental Sciences 2024年第10期144卷 172-184页

作者： Changrui Liu Shengfang Wen Shuhan Li Yu Tian Lanjun Wang Lusheng Zhu Jun Wang Young Mo Kim Jinhua Wang National Engineering Research Center for Efficient Utilization of soil and Fertilizer Resources Key Laboratory of Agricultural Environment in Universities of ShandongCollege of Resources and EnvironmentShandong Agricultural UniversityTaian 271018China Department of Civil and Environmental Engineering Hanyang UniversitySeongdong-guSeoul 04763Korea

Chlorpyrifos is a pesticide widely used in agricultural production with a relatively long residual half-life in *** the problem of residual chlorpyrifos is of universal *** this study,rice hull biochar was used as an immobilized carrier to prepare the immobilized strain H27 for the remediation of chlorpyrifos-contamination *** microorganisms after remediation were investigated by ecotoxicological *** immobilized strain H27 had the highest removal rate of chlorpyrifos when 10%bacterial solution was added to the liquid medium containing 0.075-0.109 mm diameter biochar cultured for 22 *** study on the removal of chlorpyrifos by immobilized strain H27 showed that the initial concentration of chlorpyrifos in solution was 25mg/L,and the removal rate reached 97.4%after 7 days of *** the soil,the removal rate of the immobilized bacteria group increased throughout the experiment,which was significantly higher than that of the free bacteria and biochar treatment *** Biolog-ECO test,T-RFLP and RT-RCR were used to study the effects of the soil microbial community and nitrogen cycling functional genes during chlorpyrifos *** was found that ICP group had the highest diversity index among the four treatment *** microflora of segment containing 114 bp was the dominant bacterial community,and the dominant microflora of the immobilized bacteria group was more evenly *** influence of each treatment group on ammonia-oxidizing bacteria(AOB)was greater than on ammonia-oxidizing archaea(AOA).This study offers a sound scientific basis for the practical application of immobilized bacteria to reduce residual soil pesticides.

关键词： Chlorpyrifos Immobilized microorganisms soil remediation soil microorganism

remediation performance and mechanisms of Cu and Cd contaminated water and soil using Mn/Al-layered double oxide-loaded biochar

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Journal of Environmental Sciences 2023年第3期125卷 593-602页

作者： Pengcheng Lin Hang Liu Hua Yin Minghan Zhu Haoyu Luo Zhi Dang School of Environment and Energy South China University of TechnologyGuangzhou 510006China Key Laboratory of Ministry of Education on Pollution Control and Ecosystem Restoration in Industry Clusters Guangzhou 510006China Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and Recycling Guangzhou 510006China

The combined pollution of heavy metals is ubiquitous ***/Al-layered double oxide-loaded crab shells biochar (LDO/BC) was prepared,so as to remediate the combined pollution of Cd and Cu in soil and *** pristine and used LDO/BC were characterized and the results revealed that the layered double oxide was successfully loaded on crab shells biochar (BC) and metal element Ca in crab shells was beneficial to the formation of more regular layered and flake *** maximal adsorption capacity (Qm) of LDO/BC for aqueous Cu^(2+)and Cd^(2+)was 66.23 and 73.47 mg/g,***/BC and BC were used to remediate e-waste-contaminated soil for the first time and exhibited highly efficient *** extraction amount of Cu and Cd in the contaminated soil by diethylene triamine penta-acetic acid (DTPA) after treating with 5% LDO/BC was significantly reduced from 819.84 to 205.95 mg/kg (with passivation rate 74.8%) and 8.46 to 4.16 mg/kg(with passivation rate 50.8%),respectively,inferring that the bioavailability of heavy metals declined *** experimental result also suggested that after remediation by LDO/BC the exchangeable and weak acid soluble Cu and Cd in soil translated to reducible,residual and oxidizable fraction which are more stable ***,complexation and ion exchange were proposed as the possible mechanisms for Cd and Cu *** general,these experiment results indicate that LDO/BC can be a potentially effective reagent for remediation of heavy metal contaminated water and soil.

关键词： Mn/Al-layered double oxide Biochar Cd and Cu combined pollution Adsorption soil remediation

remediation of soil and groundwater contaminated with organic chemicals using stabilized nanoparticles: Lessons from the past two decades

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Frontiers of Environmental Science & Engineering 2020年第5期14卷 83-102页

作者： Zhengqing Cai Xiao Zhao Jun Duan Dongye Zhao Zhi Dang Zhang Lin National Engineering Lab for High-concentration Refractory Organic Wastewater East China University of Science and TechnologyShanghai 200237China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China College of Water Resources&Civil Engineering China Agricultural UniversityBeijing 100083China Environmental Engineering Program Department of Civil EngineeringAuburn UniversityAuburnAL 36849USA School of Environment and Energy South China University of TechnologyGuangzhou 510006China

Due to improved soil deliverability and high reactivity,stabilized nanoparticles have been studied for nearly two decades for in situ remediation of soil and groundwater contaminated with organic *** large amounts of bench-and field-scale experimental data have demonstrated the potential of the innovative technology,extensive research results have also unveiled various merits and constraints associated different soil characteristics,types of nanoparticles and particle stabilization ***,this work aims to critically overview the fundamental principles on particle stabilization,and the evolution and some recent developments of stabilized nanoparticles for degradation of organic contaminants in soil and *** specific objectives are to:1)overview fundamental mechanisms in nanoparticle stabilization;2)summarize key applications of stabilized nanoparticles for in situ remediation of soil and groundwater contaminated by legacy and emerging organic chemicals;3)update the latest knowledge on the transport and fate of stabilized nanoparticles;4)examine the merits and constraints of stabilized nanoparticles in environmental remediation applications;and 5)identify the knowledge gaps and furore research needs pertaining to stabilized nanoparticles for remediation of contaminated soil and *** instructions of this invited special issue,this review is focused on contributions from our group(one of the pioneers in the subject field),which,however,is supplemented by important relevant works by *** knowledge gained is expected to further advance the science and technology in the environmental applications of stabilized nanoparticles.

关键词： Stabilized nanoparticle In-situ remediation Organic contaminant soil remediation Groundwater Fate and transport

remediation of Cu and As contaminated water and soil utilizing biochar supported layered double hydroxide:Mechanisms and soil environment altering

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Journal of Environmental Sciences 2023年第4期126卷 275-286页

作者： Pengling Shao Hua Yin Yingchao Li Yuhao Cai Caiya Yan Yibo Yuan Zhi Dang School of Environment and Energy South China University of TechnologyGuangzhou 510006China Key Laboratory of Ministry of Education on Pollution Control and Ecosystem Restoration in Industry Clusters Guangzhou 510006China Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and Recycling Guangzhou 510006China

Preparing materials for simultaneous remediation of anionic and cationic heavy metals contamination has always been the focus of research. Herein a biochar supported FeMnMg layered double hydroxide(LDH) composites(LB) for simultaneous remediation of copper and arsenic contamination in water and soil has been assembled by a facile co-precipitation approach. Both adsorption isotherm and kinetics studies of heavy metals removal by LB were applied to look into the adsorption performance of adsorbents in water. Moreover, the adsorption mechanisms of Cu and As by LB were investigated, showing that Cu in aqueous solution was removed by the isomorphic substitution, precipitation and electrostatic adsorption while As was removed by complexation. In addition, the availability of Cu and As in the soil incubation experiments was reduced by 35.54%–63.00% and 8.39%–29.04%, respectively by using LB. Meanwhile, the addition of LB increased the activities of urease and sucrase by 93.78%–374.35% and 84.35%–520.04%, respectively, of which 1% of the dosage was the best. A phenomenon was found that the richness and structure of microbial community became vigorous within 1% dosage of LB, which indirectly enhanced the passivation and stabilization of heavy metals. These results indicated that the soil environment was significantly improved by LB. This research demonstrates that LB would be an imaginably forceful material for the remediation of anionic and cationic heavy metals in contaminated water and soil.

关键词： Heavy metal Biochar supported layered double hydroxide composite Adsorption mechanism soil remediation Microbial community

Combination of steam-enhanced extraction and electrical resistance heating for efficient remediation of perchloroethylene-contaminated soil:Coupling merits and energy consumption

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Frontiers of Environmental Science & Engineering 2022年第11期16卷 249-260页

作者： Rui Yue Zhikang Chen Liujun Liu Lipu Yin Yicheng Qiu Xianhui Wang Zhicheng Wang Xuhui Mao School of Resource and Environmental Sciences Wuhan UniversityWuhan 430079China China State Science Dingshi Environmental Engineering Company Beijing 100020China

In situ thermal desorption(ISTD)technology effectively remediates soil contaminated by dense nonaqueous phase liquids(DNAPLs).However,more efforts are required to minimize the energy consumption of ISTD *** study developed a laboratory-scale experimental device to explore the coupling merits of two traditional desorption technologies:steam-enhanced extraction(SEE)and electrical resistance heating(ERH).The results showed that injecting high-density steam(>1 g/min)into loam or clay with relatively high moisture content(>13.3%)could fracture the soil matrix and lead to the occurrence of the preferential flow of *** ERH alone,the electrical resistance and soil moisture loss were critical factors influencing heating *** ERH and SEE were combined,preheating soil by ERH could increase soil permeability,effectively alleviating the problem of preferential flow of ***,steam injection heated the soil and provided moisture for maintaining soil electrical conductivity,thereby ensuring power stability in the ERH *** with ERH alone(8 V/cm)and SEE alone(1 g/min steam),the energy consumption of combined method in remediating perchloroethylene-contaminated soil was reduced by 39.3%and 52.9%,*** findings indicate that the combined method is more favorable than ERH or SEE alone for remediating DNAPL-contaminated subsurfaces when considering ISTD technology.

关键词： Steam-enhanced extraction Electrical resistance heating Dense nonaqueous phase liquid soil remediation Energy consumption